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31. 发明授权

US07214746B2 Phosphorus bridged metallocene compounds for olefin polymerization 失效
标题翻译：用于烯烃聚合的磷桥接茂金属化合物
公开(公告)号：US07214746B2
公开(公告)日：2007-05-08
申请号：US11077741
申请日：2005-03-11
申请人： Alexander Z. Voskoboynikov , Denis N. Kazyulkin , Vyatcheslav V. Izmer , Alexey N. Ryabov , Jo Ann M. Canich
发明人： Alexander Z. Voskoboynikov , Denis N. Kazyulkin , Vyatcheslav V. Izmer , Alexey N. Ryabov , Jo Ann M. Canich
IPC分类号： C08F4/60 , C08F4/6392 , C08F210/02 , C08F210/06
CPC分类号： B01J31/2295 , B01J31/143 , B01J31/146 , B01J2531/0225 , B01J2531/0297 , B01J2531/46 , B01J2531/48 , B01J2531/49 , C07F17/00 , C08F4/65912 , C08F10/02 , C08F110/02 , C08F210/02 , C08F210/16 , Y10S526/943 , C08F4/65927 , C08F2500/03 , C08F210/14
摘要： This invention relates to metallocene compounds represented by formula: wherein M is a group 3, 4, 5 or 6 transition metal atom, or a lanthanide metal atom, or actinide metal atom; E is a substituted or unsubstituted indenyl ligand that is bonded to Y through the two position of the indenyl ring; A is bonded to Y, and is a substituted or unsubstituted cyclopentadienyl ligand, a substituted or unsubstituted heterocyclopentadienyl ligand, a substituted or unsubstituted indenyl ligand, a substituted or unsubstituted heteroindenyl ligand, a substituted or unsubstituted fluorenyl ligand, a substituted or unsubstituted heterofluorenyl ligand, or other mono-anionic ligand, or A may, independently, be defined as E; Y is a phosphorus containing group that is bonded to both E and A, and is bonded via the phosphorus atom to E; and X are, independently, univalent anionic ligands, or both X are joined and bound to the metal atom to form a metallocycle ring, or both X join to form a chelating ligand, a diene ligand, or an alkylidene ligand.
摘要翻译：本发明涉及由下式表示的茂金属化合物：其中M是3,4,5或6族过渡金属原子，或镧系元素金属原子或锕系金属原子; E是通过茚基环的两个位置与Y键合的取代或未取代的茚基配体; A与Y结合，为取代或未取代的环戊二烯基配体，取代或未取代的杂环戊二烯基配体，取代或未取代的茚基配体，取代或未取代的杂茚基配体，取代或未取代的芴基配位体，取代或未取代的杂芴基配位体，或其它单阴离子配体，或者A可以独立地定义为E; Y是与E和A键合的含磷基团，通过磷原子与E结合; X独立地为一价阴离子配体，或两者X连接并结合到金属原子以形成金属环，或两者X连接形成螯合配体，二烯配体或亚烷基配体。

32. 发明授权

US08557936B2 Catalyst compounds and use thereof 失效
公开(公告)号：US08557936B2
公开(公告)日：2013-10-15
申请号：US12908522
申请日：2010-10-20
申请人： Garth R. Giesbrecht , Timothy M. Boller , Alexander Z. Voskoboynikov , Andrey F. Asachenko , Mikhail V. Nikulin , Alexey A. Tsarev
发明人： Garth R. Giesbrecht , Timothy M. Boller , Alexander Z. Voskoboynikov , Andrey F. Asachenko , Mikhail V. Nikulin , Alexey A. Tsarev
IPC分类号： C08F4/76 , C08F4/64 , C07F7/00
CPC分类号： C07F7/00
摘要： This invention relates to Group 4 catalyst compounds containing di-anionic tridentate nitrogen/oxygen based ligands. The catalyst compounds are useful, with or without activators, to polymerize olefins, particularly α-olefins, or other unsaturated monomers. Systems and processes to oligomerize and/or polymerize one or more unsaturated monomers using the catalyst compound, as well as the oligomers and/or polymers produced therefrom are also provided.

33. 发明授权

US08546501B2 Catalyst compounds and use thereof 失效
公开(公告)号：US08546501B2
公开(公告)日：2013-10-01
申请号：US12908550
申请日：2010-10-20
申请人： Garth R. Giesbrecht , Timothy M. Boller , Alexander Z. Voskoboynikov , Andrey F. Asachenko , Mikhail V. Nikulin , Alexey A. Tsarev
发明人： Garth R. Giesbrecht , Timothy M. Boller , Alexander Z. Voskoboynikov , Andrey F. Asachenko , Mikhail V. Nikulin , Alexey A. Tsarev
IPC分类号： C08F4/76 , C08F4/64 , C07F7/00
CPC分类号： C07F7/00
摘要： This invention relates to Group 4 catalyst compounds containing di-anionic tridentate nitrogen/oxygen based ligands. The catalyst compounds are useful, with or without activators, to polymerize olefins, particularly α-olefins, or other unsaturated monomers. Systems and processes to oligomerize and/or polymerize one or more unsaturated monomers using the catalyst compound, as well as the oligomers and/or polymers produced therefrom are also provided.

34. 发明申请

US20110306741A1 SYNTHESIS OF SUBSTITUTED TETRAHYDROINDENYL COMPLEXES 失效
标题翻译：取代的四氢萘基二烯化合物的合成
公开(公告)号：US20110306741A1
公开(公告)日：2011-12-15
申请号：US13140455
申请日：2009-12-15
申请人： Alexander Z. Voskoboynikov , Vyatcheslav V. Izmer , Dmitry S. Kononovich , Abbas Razavi
发明人： Alexander Z. Voskoboynikov , Vyatcheslav V. Izmer , Dmitry S. Kononovich , Abbas Razavi
IPC分类号： C08F4/6592 , C07F17/00 , C08F210/06 , C08F10/02 , C08F210/14 , C08F210/08 , C07F7/08 , C08F4/76
CPC分类号： C07F7/0814 , B01J31/2295 , B01J2231/122 , B01J2531/46 , B01J2531/48 , B01J2531/49 , C07F7/081 , C07F7/0827 , C07F17/00 , C08F4/65908 , C08F4/65912 , C08F4/65925 , C08F10/02 , C08F2420/05 , C08F4/65927
摘要： This invention relates to the synthesis of substituted tetrahydroindenyls and the use of the synthesised complexes in the homo- and co-polymerisation of ethylene and alpha-olefins.
摘要翻译：本发明涉及取代的四氢茚基的合成以及合成的络合物在乙烯和α-烯烃的均聚和共聚合中的用途。

35. 发明申请

US20110098429A1 Catalyst Compounds and Use Thereof 失效
公开(公告)号：US20110098429A1
公开(公告)日：2011-04-28
申请号：US12908268
申请日：2010-10-20
申请人： Garth R. Giesbrecht , Timothy M. Boller , Alexander Z. Voskoboynikov , Andrey F. Asachenko , Mikhail V. Nikulin , Alexey A. Tsarev
发明人： Garth R. Giesbrecht , Timothy M. Boller , Alexander Z. Voskoboynikov , Andrey F. Asachenko , Mikhail V. Nikulin , Alexey A. Tsarev
IPC分类号： C08F4/76 , C07F7/00 , C07D213/30 , C07D213/38 , C07C43/23 , C07C217/80 , B01J31/12
CPC分类号： C07F7/00
摘要： This invention relates to Group 4 catalyst compounds containing di-anionic tridentate nitrogen/oxygen based ligands. The catalyst compounds are useful, with or without activators, to polymerize olefins, particularly a-olefins, or other unsaturated monomers. Systems and processes to oligomerize and/or polymerize one or more unsaturated monomers using the catalyst compound, as well as the oligomers and/or polymers produced therefrom are also provided.

36. 发明申请

US20090186995A1 Production of Propylene-Based Polymers 有权
标题翻译：丙烯基聚合物的生产
公开(公告)号：US20090186995A1
公开(公告)日：2009-07-23
申请号：US12016346
申请日：2008-01-18
申请人： Jo Ann Canich , Peijun Jiang , Gary L. Casty , Gabor Kiss , Alexander Z. Voskoboynikov
发明人： Jo Ann Canich , Peijun Jiang , Gary L. Casty , Gabor Kiss , Alexander Z. Voskoboynikov
IPC分类号： C08F2/00
CPC分类号： C08F10/06 , C08F4/65908 , C08F4/65912 , C08F210/06 , Y02P20/544 , Y10S526/943 , C08F4/65927 , C08F210/16 , C08F2500/03 , C08F2500/17 , C08F2500/20
摘要： In a process for producing a propylene-based olefin homopolymer or copolymer, a monomer composition comprising propylene is contacted with a polymerization catalyst system under homogeneous polymerization conditions (such as solution, supersolution or supercritical conditions), wherein the polymerization catalyst system includes an activator and a bridged bis-indenyl transition metal (group 4) compound substituted with a carbazole (unsubstituted or substituted) at the 4 position.
摘要翻译：在制备丙烯类烯烃均聚物或共聚物的方法中，包含丙烯的单体组合物在均相聚合条件（例如溶液，超溶剂或超临界条件）下与聚合催化剂体系接触，其中聚合催化剂体系包括活化剂和在4位被咔唑（未取代或取代的）取代的桥连双茚基过渡金属（4族）化合物。

37. 发明授权

US07446216B2 Halogen substituted metallocene compounds for olefin polymerization 有权
公开(公告)号：US07446216B2
公开(公告)日：2008-11-04
申请号：US11300054
申请日：2005-12-14
申请人： Alexander Z. Voskoboynikov , Alexey N. Ryahov , Mikhail V. Nikulin , Alexander V. Lygin , Vyatcheslav V. Izmer , Andrey F. Asachenko , Catalina L. Coker , Jo Ann M. Canich
发明人： Alexander Z. Voskoboynikov , Alexey N. Ryahov , Mikhail V. Nikulin , Alexander V. Lygin , Vyatcheslav V. Izmer , Andrey F. Asachenko , Catalina L. Coker , Jo Ann M. Canich
IPC分类号： C08F4/6392 , C08F4/6592
CPC分类号： C07F17/00 , C08F4/65908 , C08F4/65912 , C08F4/6592 , C08F10/00 , C08F210/16 , Y10S526/941 , Y10S526/943 , C08F4/65927 , C08F4/65925 , C08F210/14 , C08F2500/03 , C08F2500/01 , C08F2500/20 , C08F210/06
摘要： A metallocene compound is represented by the formula (1): A2YyMXn-2 wherein: M is a transition metal atom having a coordination number of n selected from Group 3, 4, 5 or 6 of the Periodic Table of Elements, or a lanthanide metal atom, or actinide metal atom; each A is independently a substituted polycyclic arenyl ligand pi-bonded to M, each A ligand includes at least one halogen substituent directly bonded to an sp2 carbon at a bondable ring position and, when each A is a substituted indenyl ligand and y is equal to one and the ligand includes at least one chloro, bromo or iodo substituent at the 4, 5, or 6 position of the indenyl ligand, then A also includes at least one other substituent in the indenyl ligand selected from hydrocarbyl, substituted hydrocarbyl, halogen, halocarbyl, substituted halocarbyl, silylcarbyl, substituted silylcarbyl, germylcarbyl, substituted germylcarbyl, or other heteroatom substituents wherein the heteroatom is bonded directly to a ring carbon of the ring structure ligand and is boron, a Group 15 atom, or a Group 16 atom, preferably boron, nitrogen, oxygen, phosphorus, or sulfur; Y is an optional bridging group containing at least one Group 13, 14, 15, or 16 element and is bonded to any single position of the ring structure of A, y is zero or 1, indicating the absence (y=0) or presence (y=1) of Y; and the or each X is a univalent anionic ligand, or two X are joined and bound to the metal atom to form a metallocycle ring, or two X are joined to form a chelating ligand, a diene ligand, or an alkylidene ligand; provided that when y is equal to 1, then A is not 5,6-dichloroindenyl or an indenyl group having a fluoro- or chloro substituent at the 7 position and a hydrocarbyl or substituted hydrocarbyl substituent at the 4 position, and provided further that when y is equal to 0, then A is not 5,6-difluoroindenyl.

38. 发明授权

US07214747B2 Phosphorus substituted metallocene compounds for olefin polymerization 失效
标题翻译：用于烯烃聚合的磷取代的茂金属化合物
公开(公告)号：US07214747B2
公开(公告)日：2007-05-08
申请号：US11078588
申请日：2005-03-11
申请人： Alexander Z. Voskoboynikov , Denis N. Kazyulkin , Vyatcheslav V. Izmer , Alexey N. Ryabov , Jo Ann M. Canich
发明人： Alexander Z. Voskoboynikov , Denis N. Kazyulkin , Vyatcheslav V. Izmer , Alexey N. Ryabov , Jo Ann M. Canich
IPC分类号： C08F4/6192 , C08F4/64 , C07F17/00
CPC分类号： B01J31/2295 , B01J31/143 , B01J31/146 , B01J31/2447 , B01J31/2457 , B01J2531/0225 , B01J2531/0297 , B01J2531/46 , B01J2531/48 , B01J2531/49 , C07F17/00 , C08F4/65908 , C08F4/65912 , C08F10/00 , C08F110/02 , C08F210/16 , C08F4/65925 , C08F2500/03 , C08F210/14
摘要： This invention relates to a metallocene compounds represented by formula: wherein M is a group 3, 4, 5 or 6 transition metal atom, or a lanthanide metal atom, or actinide metal atom; E is an indenyl ligand that is substituted with a PR2 group in the two position of the indenyl ligand, where each R is, independently a hydrocarbyl, substituted hydrocarbyl, halocarbyl, or substituted halocarbyl substituent, and additionally, E may be substituted with 0, 1, 2, 3, 4, 5 or 6 Rn where each Rn is, independently, a hydrocarbyl, substituted hydrocarbyl, halocarbyl, substituted halocarbyl, silylcarbyl, substituted silylcarbyl, germylcarbyl, or substituted germylcarbyl substituent, and optionally, two or more adjacent Rn substituents may join together to form a substituted or unsubstituted, saturated, partially unsaturated, or aromatic cyclic or polycyclic substituent; A is a substituted or unsubstituted cyclopentadienyl ligand, a substituted or unsubstituted heterocyclopentadienyl ligand, a substituted or unsubstituted indenyl ligand, a substituted or unsubstituted heteroindenyl ligand, a substituted or unsubstituted fluorenyl ligand, a substituted or unsubstituted heterofluorenyl ligand, or other mono-anionic ligand, or A may, independently, be defined as E or as X; each X is, independently, an univalent anionic ligand, or both X are joined and bound to the metal atom to form a metallocycle ring, or both X join to form a chelating ligand, a diene ligand, or an alkylidene ligand.
摘要翻译：本发明涉及由下式表示的茂金属化合物：其中M是3,4,5或6族过渡金属原子，或镧系元素金属原子或锕系金属原子; E是在茚基配体的两个位置被PR 2 N 2基团取代的茚基配体，其中每个R独立地是烃基，取代的烃基，卤代烃基或取代的卤代烃基取代基，另外 E可以被0,1,2,3,4,5或6个R n取代，其中每个R n独立地是烃基，取代的烃基，卤代烃基取代的卤代烃基，甲硅烷基，取代的甲硅烷基，甲硅烷基或取代的烯基羰基取代基，以及任选地，两个或多个相邻的R n取代基可以连接在一起以形成取代或未取代的，饱和的，部分不饱和的或芳族的环状或多环取代基; A是取代或未取代的环戊二烯基配体，取代或未取代的杂环戊二烯基配体，取代或未取代的茚基配体，取代或未取代的杂烯基配体，取代或未取代的芴基配体，取代或未取代的杂芴基配体或其它单阴离子配体，或A可以独立地定义为E或X定义; 每个X独立地是一价阴离子配体，或者两者X连接并结合到金属原子以形成金属环，或者两者X连接形成螯合配体，二烯配体或亚烷基配体。

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