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31. 发明授权

US4435274A Process for manufacturing gasoline with upgrading of hydrocarbon oils 失效
标题翻译：用烃油改造制造汽油的方法
公开(公告)号：US4435274A
公开(公告)日：1984-03-06
申请号：US425348
申请日：1982-09-28
申请人： Bernard Juguin , Jean-Pierre Franck , Yves Jacquin , Christian Marcilly , Germain Martino
发明人： Bernard Juguin , Jean-Pierre Franck , Yves Jacquin , Christian Marcilly , Germain Martino
IPC分类号： C10G1/06 , C10G1/00 , C10G65/12 , C10G69/00 , C10L1/06 , C10G45/02 , C10G35/04 , C10G65/00
CPC分类号： C10L1/06 , C10G1/002 , C10G2400/02
摘要： Residual oils from steam-cracking or catalytic cracking, oils from coal liquefaction and oils from bituminous sands and shales are converted to gasoline by a process comprising the fractionation of the feed charge to a naphtha and a middle distillate: the naphtha, admixed with a gasoline cut "E", is hydrotreated and then dehydrogenated to gasoline; the middle distillate is hydrotreated and fractionated to gasoline and a heavier fraction, the heavier fraction is hydrocracked and fractionated, thus producing a gasoline cut which constitutes the above cut "E".
摘要翻译：来自蒸汽裂解或催化裂化的残余油，来自煤液化的油和来自沥青砂和页岩的油通过包括将进料装料分馏成石脑油和中间馏分的方法转化为汽油：石脑油与汽油混合切“E”，加氢处理后脱氢至汽油; 将中间馏分加氢处理并分馏成汽油和较重的馏分，将较重的馏分进行加氢裂化和分馏，从而产生构成上述馏分“E”的汽油馏分。

32. 发明授权

US4217205A Catalysts for hydrocarbon conversion 失效
标题翻译：用于烃转化的催化剂
公开(公告)号：US4217205A
公开(公告)日：1980-08-12
申请号：US936966
申请日：1978-08-25
申请人： Christian Marcilly , Jean-Francois Le Page , Germain Martino , Jean Miquel
发明人： Christian Marcilly , Jean-Francois Le Page , Germain Martino , Jean Miquel
IPC分类号： B01J23/652 , B01J27/13 , C10G35/09 , C10G35/08
CPC分类号： B01J23/6527 , C10G35/09
摘要： Catalyst, particularly useful in catalytic reforming and for producing highly pure aromatic hydrocarbons, comprising an alumina carrier and containing, expressed in proportion of the weight of the alumina carrier:0.005 to 1% of platinum0.01 to 4% of gallium, indium or thallium0.01 to 2% of tungsten, and0.1 to 10% of halogen.
摘要翻译：催化剂，特别适用于催化重整和生产高纯度芳族烃，包含氧化铝载体并含有以氧化铝载体重量比例表示的：0.005至1％的铂，0.01至4％的镓，铟或铊0.01 至2％的钨和0.1至10％的卤素。

33. 发明授权

US4180693A New preparation process of a catalyst for converting aromatic hydrocarbons 失效
标题翻译：用于转化芳烃的催化剂的新制备方法
公开(公告)号：US4180693A
公开(公告)日：1979-12-25
申请号：US965466
申请日：1978-11-30
申请人： Christian Marcilly
发明人： Christian Marcilly
IPC分类号： B01J29/20 , C07C6/12 , C07C3/62
CPC分类号： C07C6/126 , B01J29/20 , C07C6/123 , C07C2529/22
摘要： Process for manufacturing a catalyst for hydrocarbon conversion consisting of a mordenite containing less than 0.5% by weight ofsodium, having a molar ratio SiO.sub.2 /Al.sub.2 O.sub.3 from 10 to 100 and further containing at least one metal selected from cobalt, nickel, silver and palladium, wherein said metal in incorporated to a mordenite of the sodic form having a molar ratio SiO.sub.2 /Al.sub.2 O.sub.3 close to 10, the major portion of the sodium is eliminated, the resulting catalyst mass is dried from about 50.degree. to 150.degree. C. and then subjected to a first so-called dry calcination between 300.degree. and 700.degree. C., in the presence of a dry, inert or oxidizing gas containing less than 1% by volume of steam, and to a second so-called wet calcination between 250.degree. and 700.degree. C., in the presence of either steam or an inert or oxidizing gas containing at least 3% of steam.
摘要翻译：制备用于烃转化的催化剂的方法，其由包含小于0.5重量％的钠的丝光沸石组成，SiO 2 / Al 2 O 3的摩尔比为10至100，并且还含有至少一种选自钴，镍，银和钯的金属，其中所述金属掺入到SiO 2 / Al 2 O 3摩尔比接近10的钠盐形式的丝光沸石中，大部分钠被除去，所得催化剂物质从约50℃至150℃干燥，在含有少于1体积％蒸汽的干，惰性或氧化性气体的存在下，在300℃和700℃之间进行第一次所谓的干法煅烧，以及第二次所谓的在250°和 700℃，在蒸汽或含有至少3％蒸汽的惰性或氧化气体的存在下。

34. 发明授权

US06709639B1 Apparatus for purification of raw gasoline from catalytic cracking 有权
标题翻译：用于从催化裂化中净化原料汽油的装置
公开(公告)号：US06709639B1
公开(公告)日：2004-03-23
申请号：US09522179
申请日：2000-03-09
申请人： Thierry Chapus , Blaise Didillon , Christian Marcilly , Charles Cameron
发明人： Thierry Chapus , Blaise Didillon , Christian Marcilly , Charles Cameron
IPC分类号： B01J804
CPC分类号： C10G67/12 , C10G2400/02
摘要： An apparatus for the purification of catalytic cracking gasolines containing dienic and/or acetylenic impurities, and mercaptans, said apparatus comprising at least one selective hydrogenation reactor 3 containing at least one fixed catalyst bed, and having at least one line 1 for introducing a feed, at least one effluent outlet line, and a line supplying hydrogen to the reactor, said reactor being followed by at least one stabilization drum 4 connected to said effluent outlet line, the drum having at least one gas outlet line 5 and at least one stabilized effluent outlet line, and said effluent passing into at least one sweetening reactor 8 comprising at least one effluent inlet line 6 and at least one effluent outlet line, said reactor having close thereto at least one oxidizing agent supply line, said apparatus also comprising at least one drum 9 for degassing the effluent from the sweetening reactor 8, said drum 9 having at least one gas outlet line and at least one outlet line 11 for dedienized, stabilized and sweetened gasoline.
摘要翻译：一种用于纯化含有二烯和/或炔属杂质的催化裂解汽油的装置和硫醇，所述装置包括至少一个含有至少一个固定催化剂床的选择性氢化反应器3，并具有至少一条用于引入进料的管线1，至少一个流出物出口管线和向反应器供应氢气的管线，所述反应器后面连接有至少一个与所述流出物出口管线连接的稳定鼓筒，所述转鼓具有至少一个气体出口管线5和至少一个稳定的流出物出口管线，并且所述流出物进入至少一个甜味反应器8，其包含至少一个流出物入口管线6和至少一个流出物出口管线，所述反应器具有至少一个氧化剂供应管线，所述设备还包括至少一个鼓9用于对来自甜味反应器8的流出物进行脱气，所述滚筒9具有至少一个气体出口管线和至少一个出口管线11 用于发明，稳定和增甜的汽油。

35. 发明授权

US5591323A Process for sweetening petroleum cuts without regular addition of alkaline solution using a basic solid catalyst 失效
标题翻译：使用碱性固体催化剂不经常地加入碱性溶液来甜化石油馏分的方法
公开(公告)号：US5591323A
公开(公告)日：1997-01-07
申请号：US474766
申请日：1995-06-07
申请人： Christian Marcilly , Serge Leporq , Philippe Courty
发明人： Christian Marcilly , Serge Leporq , Philippe Courty
IPC分类号： B01J21/16 , B01J27/26 , B01J29/06 , B01J37/00 , C10G25/00 , C10G27/10 , C10G27/00 , C10G27/04
CPC分类号： B01J21/16 , B01J27/26 , C10G27/10 , B01J37/0009
摘要： A process for sweetening a petroleum cut containing mercaptans, wherein said petroleum cut is subjected to oxidation conditions by being contacted with a porous catalyst, in the presence of air said process being characterised in that said catalyst comprises 10 to 98% by weight of at least one mineral solid phase constituted of an alkaline aluminosilicate with a Si/Al atomic ratio less than or equal to 5, 1 to 60% by weight of active carbon, 0.02 to 2% by weight of at least one metal chelate and 0 to 20% by weight of at least one organic or mineral binding agent, has a basicity determined according to the 2896 ASTM standard with 20 milligrams of potash per gram and a total BET surface area of 10 m.sup.2 g.sup.-1, and contains inside its pore structure a permanent aqueous phase representing 0.1 to 40% by weight of dry catalyst.
摘要翻译：一种用于甜化含有硫醇的石油馏分的方法，其中所述石油馏分通过与多孔催化剂接触而经受氧化条件，在空气存在下，所述方法的特征在于所述催化剂至少包含10至98重量％一个矿物固相由Si / Al原子比小于或等于5,1-60重量％的活性炭，0.02-2重量％的至少一种金属螯合物和0-20重量％的碱性硅铝酸盐构成，的至少一种有机或矿物结合剂，具有根据2896 ASTM标准确定的碱度，每克20mg的钾碱和10m 2 g -1的总BET表面积，并且在其孔结构内部含有永久性水性相为干燥催化剂的0.1-40重量％。

36. 发明授权

US5008000A Cracking catalyst for hydrocarbon charges comprising an offretite, a zeolite and a matrix 失效
标题翻译：用于烃装料的裂化催化剂包括异位素，沸石和基质
公开(公告)号：US5008000A
公开(公告)日：1991-04-16
申请号：US493601
申请日：1990-03-15
申请人： Christian Marcilly , Jean-Marie Deves , Francis Raatz
发明人： Christian Marcilly , Jean-Marie Deves , Francis Raatz
IPC分类号： B01J29/06 , B01J29/08 , B01J29/18 , B01J29/40 , B01J29/50 , B01J29/80 , C10G11/04 , C10G11/05
CPC分类号： C10G11/05 , B01J29/80 , B01J2229/16 , B01J2229/26 , B01J2229/42 , B01J29/084 , B01J29/18 , B01J29/40 , B01J29/50
摘要： The cracking catalyst of the invention contains:(a) 20-95% by weight of at least one matrix, selected from the group consisting of alumina, silica, magnesia, clay, titanium oxide, zirconia, combinations of at least two of these compounds and alumina-boron oxide combinations,(b) 1-60% by weight of at least one zeolite of open structure whose main dodecagonal channels have openings of at least 7 Angstroms, said zeolite of open structure being selected from the group formed of X, Y, L, omega and beta zeolites,(c) 0.5-60% by weight of at least one offretite whose main dodecagonal channels have openings smaller than 7 Angstroms and which have a SiO.sub.2 /Al.sub.2 O.sub.3 molar ratio from about 15 to about 500, the crystalline paramaters a and c of elementary mesh ranging respectively from 1.285 to 1.315 nm for a and from 0.748 to 0.757 nm for c and have a potassium content lower than 1.5% by weight.

37. 发明授权

US4923593A Cracking catalyst and catalytic cracking process 失效
标题翻译：裂化催化剂和催化裂化过程
公开(公告)号：US4923593A
公开(公告)日：1990-05-08
申请号：US299167
申请日：1989-01-19
申请人： Christian Marcilly , Jean-Marie Deves , Michel Bourgogne
发明人： Christian Marcilly , Jean-Marie Deves , Michel Bourgogne
IPC分类号： B01J29/50 , B01J29/70 , B01J29/80 , C10G11/05 , C10G11/18
CPC分类号： B01J29/80 , B01J29/50 , C10G11/05 , C10G11/18 , B01J29/70
摘要： The invention concerns a fluidized bed cracking process of a hydrocarbon charge, carried out in an extended, appreciably tubular and vertical reaction zone (1), the catalyst being introduced at the lower end of this extended zone by a piper (2), and the charge being introduced by at least one pipe (3) opening into the reaction zone at a level higher than the level at which the catalyst is admitted.The invention wherein, for example, part of the gasoline or part (3a) to an intermediate point between the catalyst and charge entry points, and wherein a specially adapted catalyst is used for this operating procedure. The invention also concerns the catalyst used in this way, a zeolite-based catalyst of the erionite family.
摘要翻译：本发明涉及在延伸的，明显管状和垂直的反应区（1）中进行的烃装料的流化床裂解过程，催化剂通过吹塑（2）在该延伸区的下端引入，电荷通过至少一个开口进入反应区的管（3）引入，其高于催化剂进入的水平。本发明其中例如汽油或部分（3a）到催化剂和进料点之间的中间点，并且其中特别适用的催化剂用于该操作过程。本发明还涉及以这种方式使用的催化剂，即一种基于沸石的催化剂。

38. 发明授权

US4501656A Dewaxing process employing a catalyst with a highly dealuminated mordenite base 失效
标题翻译：脱蜡方法采用具有高度脱铝丝光沸石基质的催化剂
公开(公告)号：US4501656A
公开(公告)日：1985-02-26
申请号：US507415
申请日：1983-06-23
申请人： Pierre Dufresne , Edouard Freund , Christian Marcilly , Francis Raatz
发明人： Pierre Dufresne , Edouard Freund , Christian Marcilly , Francis Raatz
IPC分类号： B01J29/26 , C10G45/12 , C10G45/58 , C10G45/64 , C10G47/20
CPC分类号： B01J29/26 , C10G2400/06
摘要： A new catalyst with a highly dealuminated mordenite base, useful in particular in hydrotreatment processes for improving the low temperature properties and the pour point and cloud point of oil cuts contains:(1) an acidic carrier comprising(a) at least 50% (calculated as dry base) of highly dealuminated mordenite and characterized by a molar ratio SiO.sub.2 /Al.sub.2 O.sub.3 higher than 110 and a sodium content lower than or equal to 0.5% by weight, and(b) an amorphous matrix, and(2) said acid carrier containing in association at least one oxide of a metal from group VIII and at least one oxide of a metal from group VI of the periodic classification of elements.
摘要翻译：具有高脱铝丝光沸石基质的新型催化剂，尤其用于改进油料的低温性能和倾点和浊点的加氢处理方法中包含：（1）酸性载体，其包含（a）至少50％（计算值作为干碱），其特征在于SiO 2 / Al 2 O 3的摩尔比高于110，钠含量低于或等于0.5重量％，和（b）无定形基质，和（2）所述酸性载体含有关于来自第VIII族的金属的至少一种氧化物和至少一种元素的周期性分类的来自第VI族的金属的氧化物。

39. 发明授权

US4151120A Preparation process of a catalyst for converting aromatic hydrocarbons 失效
标题翻译：用于转化芳烃的催化剂的制备方法
公开(公告)号：US4151120A
公开(公告)日：1979-04-24
申请号：US842132
申请日：1977-10-14
申请人： Christian Marcilly
发明人： Christian Marcilly
IPC分类号： B01J29/20 , C07B61/00 , C07C1/00 , C07C6/12 , C07C15/02 , C07C67/00 , B01J29/06 , C07C3/00
CPC分类号： B01J29/20 , C07C6/123 , C07C6/126 , C07C2529/22
摘要： Process for manufacturing a catalyst for hydrocarbon conversion consisting of a mordenite containing less than 0.5% by weight of sodium, having a molar ratio SiO.sub.2 /Al.sub.2 O.sub.3 from 10 to 100 and further containing at least one metal selected from cobalt, nickel, silver and palladium, wherein said metal in incorporated to a mordenite of the sodic form having a molar ratio SiO.sub.2 /Al.sub.2 O.sub.3 close to 10, the major portion of the sodium is eliminated, the resulting catalyst mass is dried from about 50.degree. to 150.degree. C. and then subjected to a first so-called dry calcination between 300.degree. and 700.degree. C., in the presence of a dry, inert or oxidizing gas containing less than 1% by volume of steam, and to a second so-called wet calcination between 250.degree. and 700.degree. C., in the presence of either steam or an inert or oxidizing gas containing at least 3% of steam.
摘要翻译：制备用于烃转化的催化剂的方法，其由包含小于0.5重量％的钠的丝光沸石组成，SiO 2 / Al 2 O 3的摩尔比为10至100，并且还含有至少一种选自钴，镍，银和钯的金属，其中所述金属掺入到SiO 2 / Al 2 O 3摩尔比接近10的钠盐形式的丝光沸石中，大部分钠被除去，所得催化剂物质在约50℃至150℃下干燥，然后进行在300℃至700℃之间的第一次所谓的干煅烧，在含有少于1体积％蒸汽的干，惰性或氧化性气体存在下进行第一次所谓的干法煅烧，在第二次所谓的250℃ 和700℃，在蒸汽或含有至少3％蒸汽的惰性或氧化气体的存在下。

40. 发明授权

US06838060B1 Process and apparatus for the production of catalytic cracking gasoline with a low sulphur content 失效
标题翻译：用于生产硫含量低的催化裂化汽油的方法和装置
公开(公告)号：US06838060B1
公开(公告)日：2005-01-04
申请号：US09434282
申请日：1999-11-05
申请人： Thierry Chapus , Blaise Didillon , Christian Marcilly , Charles Cameron
发明人： Thierry Chapus , Blaise Didillon , Christian Marcilly , Charles Cameron
IPC分类号： B01J23/42 , B01J23/85 , B01J31/12 , C10G27/00 , C10G29/06 , C10G45/06 , C10G45/10 , C10G45/40 , C10G65/00 , C10G65/06 , C10G67/00 , C10G67/04 , C10G67/12 , B01J8/00 , C10G45/00
CPC分类号： C10G65/00 , C10G2400/02
摘要： An apparatus for the production of gasolines with a low sulphur content from a catalytic cracking gasoline, comprising a fractionation column (1) provided with a line (2) for introducing raw gasoline from a catalytic cracking step and comprising at least two lines, one (3) in the upper portion of the column for taking off a light cut, and the other (4) in the lower portion of the column for taking off the heavy cut; a zone (5) for hydrotreatment in the presence of hydrogen, comprising a catalytic bed, an inlet line (6) for the light gasoline cut to be treated, said line being connected either to the fractionation column (I), or to the zone (7) for treatment over a palladium catalyst, said hydrotreatment zone also comprising an outlet line (8) for hydrotreated effluent; a stripping zone (9) comprising a line for introducing light hydrotreated gasoline, a line (10) for evacuating H2S and an outlet line (11) for stripped light gasoline; and said apparatus also comprising at least one of the following sweetening zones: a sweetening zone (12) located after the stripping zone, comprising a line for introducing the stripped light gasoline and a line (14) for supplying an oxidizing agent to said zone; a treatment zone (7) located after the hydrotreatment zone and comprising a line (3) for introducing the light gasoline cut from the fractionation column, an outlet line for the treated light gasoline cut, said zone also comprising at least one catalyst bed containing 0.1-1% of palladium deposited on a support, and said apparatus further comprising a line (13) for taking the stripped and sweetened light gasoline out of the apparatus, and connected either to the zone (12) or to the zone (9).

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