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21. 发明授权

US07361797B2 Hydrocarbon conversion using nanocrystalline zeolite Y 有权
标题翻译：使用纳米晶体沸石Y进行烃转化
公开(公告)号：US07361797B2
公开(公告)日：2008-04-22
申请号：US10774774
申请日：2004-02-09
申请人： Xingtao Gao , Johannes Hendrik Koegler , Lawrence L. Murrell , Philip J. Angevine
发明人： Xingtao Gao , Johannes Hendrik Koegler , Lawrence L. Murrell , Philip J. Angevine
IPC分类号： C07C2/68
CPC分类号： B01J29/088 , B01J29/084 , B01J35/023 , B01J37/08 , B01J2229/40 , B01J2229/42 , B01J2229/64 , C01B39/04 , C01B39/24 , C07C2/58 , C07C2/66 , C07C6/126 , C07C2521/04 , C07C2521/06 , C07C2521/08 , C07C2521/12 , C07C2529/08 , C07C2529/12 , C07C2529/14 , C07C2529/16 , C10G29/205 , C10G2300/1081 , C10G2300/1088 , C10G2300/1096 , C10G2300/305 , C10G2300/4018 , C10G2400/02 , C10G2400/30 , Y02P20/52 , C07C9/14 , C07C15/073 , C07C15/085
摘要： A process for alkylation of a hydrocarbon compound includes providing a catalyst including a zeolite Y having a crystal size of no more than 100 nm, and reacting an alkylatable hydrocarbon with an alkylating agent in the presence of the catalyst under alkylation reaction conditions to provide a gasoline product having a Research Octane Number of over 99.5.
摘要翻译：烃化合物的烷基化方法包括提供包含结晶尺寸不超过100nm的沸石Y的催化剂，并且在烷基化反应条件下在催化剂存在下使烷基化烃与烷基化剂反应以提供汽油研究辛烷值超过99.5的产品。

22. 发明授权

US07304199B2 Solid acid catalyst and method of using same 有权
标题翻译：固体酸催化剂及其使用方法
公开(公告)号：US07304199B2
公开(公告)日：2007-12-04
申请号：US10824390
申请日：2004-04-14
申请人： Jinsuo Xu , Chuen Y. Yeh , Philip J. Angevine
发明人： Jinsuo Xu , Chuen Y. Yeh , Philip J. Angevine
IPC分类号： C07C5/22 , C07C6/08 , C07C2/58 , C01G11/00 , B01J27/053
CPC分类号： B01J23/6527 , B01J21/063 , B01J21/066 , B01J23/24 , B01J23/30 , B01J23/652 , B01J27/053 , B01J27/057 , B01J37/0009 , B01J37/08 , C07C5/2772 , C07C2523/652 , C10G45/60 , C10G45/62 , C10G47/02 , C10G49/04 , C10G2300/1081 , C10G2300/4018 , C07C9/00
摘要： A catalyst composition includes an oxygen compound of an element selected from Group IVB or Group IVA of the Periodic Table of the Elements; an oxygen compound of an element selected from Group VIB or Group VIA of the Periodic Table of the Elements; and at least about 1% by weight based upon total catalyst weight of fumed silica particles. The catalyst composition is advantageously employed in hydrocarbon conversion processes such as isomerization.
摘要翻译：催化剂组合物包括选自元素周期表的IVB族或IVA族元素的元素的氧化合物; 选自元素周期表的VIB族或VIA族的元素的氧化合物; 和基于热解二氧化硅颗粒的总催化剂重量的至少约1重量％。催化剂组合物有利地用于烃转化过程如异构化。

23. 发明授权

US06676829B1 Process for removing sulfur from a hydrocarbon feed 失效
标题翻译：从烃进料中除去硫的方法
公开(公告)号：US06676829B1
公开(公告)日：2004-01-13
申请号：US09456851
申请日：1999-12-08
申请人： Philip J. Angevine , Anna B. Gorshteyn , Larry A. Green , Yuk Mui Louie , David A. Pappal , Peter J. Owens , Richard J. Quann , Jolie A. Rhinehart
发明人： Philip J. Angevine , Anna B. Gorshteyn , Larry A. Green , Yuk Mui Louie , David A. Pappal , Peter J. Owens , Richard J. Quann , Jolie A. Rhinehart
IPC分类号： C10G4504
CPC分类号： C10G45/52 , C10G65/04 , C10G65/08
摘要： A method is provided for removing sulfur from an effluent produced by hydrotreating a hydrocarbon feed, said effluent having a heavy fraction containing polyaromatic sulfur compounds and a lighter fraction, said method comprising contacting the effluent with a noble metal containing hydrodearomatization catalyst on a support under super-atmospheric hydrogen pressure and reaction conditions sufficient to hydrogenate at least one ring of said polyaromatic sulfur compounds and thereby produce a product with a reduced sulfur content.
摘要翻译：提供一种从通过加氢处理烃进料产生的流出物中除去硫的方法，所述流出物具有含有多芳族硫化合物的重馏分和较轻馏分，所述方法包括将流出物与含有脱氢脱氢催化剂的贵金属接触， - 大气压力和足以氢化所述多芳族硫化合物的至少一个环的反应条件，从而产生具有降低的硫含量的产物。

24. 发明授权

US06652735B2 Process for isomerization dewaxing of hydrocarbon streams 有权
标题翻译：烃流异构化脱蜡方法
公开(公告)号：US06652735B2
公开(公告)日：2003-11-25
申请号：US09843125
申请日：2001-04-26
申请人： Thomas F. Degnan , Philip J. Angevine
发明人： Thomas F. Degnan , Philip J. Angevine
IPC分类号： C10G7338
CPC分类号： C10G45/62 , B01J29/74 , B01J29/7415 , B01J29/80 , B01J2229/20 , B01J2229/42 , C10G45/64 , C10G65/043
摘要： A process for isomerization dewaxing of a hydrocarbon feed which includes contacting the hydrocarbon feed with a large pore size, small crystal size, crystalline molecular sieve and an intermediate pore size, small crystal size, crystalline molecular sieve to produce a dewaxed product with a reduced pour point and a reduced cloud point. In a preferred embodiment, the feed is contacted with the molecular sieves sequentially, first with the large pore sieve followed by the intermediate pore sieve.
摘要翻译：烃原料异构化脱蜡的方法，其包括使烃进料与大孔径，小结晶尺寸，结晶分子筛和中等孔径，小晶体尺寸，结晶分子筛接触以产生具有降低的倾倒的脱蜡产物点和减少的浊点。在一个优选的实施方案中，进料与分子筛依次接触，首先用大孔筛，然后是中间孔筛。

25. 发明授权

US06500329B2 Selective ring opening process for producing diesel fuel with increased cetane number 有权
标题翻译：用于生产具有增加的十六烷值的柴油的选择性开环过程
公开(公告)号：US06500329B2
公开(公告)日：2002-12-31
申请号：US09981575
申请日：2001-10-16
申请人： Ying-Yen P. Tsao , Tracy J. Huang , Philip J. Angevine
发明人： Ying-Yen P. Tsao , Tracy J. Huang , Philip J. Angevine
IPC分类号： C10G6502
CPC分类号： C10G45/54 , C10G2400/04
摘要： A two stage process useful for cetane upgrading of diesel fuels. More particularly, the invention relates to a process for selective naphthenic ring-opening utilizing an extremely low acidic distillate selective catalyst having highly dispersed Pt. The process is a two stage process wherein the first stage is a hydrotreating stage for removing sulfur from the feed and the second stage is the selective ring-opening stage.
摘要翻译：用于柴油燃料十六烷值升级的两阶段过程。更具体地说，本发明涉及利用具有高度分散的Pt的极低酸性馏出物选择性催化剂的选择性环烷开环方法。该方法是两阶段方法，其中第一阶段是用于从进料中除去硫的加氢处理阶段，第二阶段是选择性开环阶段。

26. 发明授权

US06241876B1 Selective ring opening process for producing diesel fuel with increased cetane number 有权
标题翻译：用于生产具有增加的十六烷值的柴油的选择性开环过程
公开(公告)号：US06241876B1
公开(公告)日：2001-06-05
申请号：US09330386
申请日：1999-06-11
申请人： Ying-Yen P. Tsao , Tracy J. Huang , Philip J. Angevine
发明人： Ying-Yen P. Tsao , Tracy J. Huang , Philip J. Angevine
IPC分类号： C10G3506
CPC分类号： C10G45/64 , C10G45/54 , C10G2400/04
摘要： A process, preferably in a counter-current configuration, for selectively cracking carbon-carbon bonds of naphthenic species using a low acidic catalyst, preferably having a crystalline molecular sieve component and carrying a Group VIII noble metal. The diesel fuel products are higher in cetane number and diesel yield.
摘要翻译：优选以逆流配置的方法，用于使用低酸性催化剂，优选具有结晶分子筛组分并携带第VIII族贵金属来选择性地裂解环烷烃的碳 - 碳键。柴油燃料产品的十六烷值和柴油产量较高。

27. 发明授权

US5685972A Production of benzene, toluene, and xylene (BTX) from FCC naphtha 失效
标题翻译：从FCC石脑油生产苯，甲苯和二甲苯（BTX）
公开(公告)号：US5685972A
公开(公告)日：1997-11-11
申请号：US502733
申请日：1995-07-14
申请人： Hye Kyung C. Timken , Philip J. Angevine
发明人： Hye Kyung C. Timken , Philip J. Angevine
IPC分类号： B01J29/40 , B01J29/70 , C07C7/10 , C07C15/04 , C07C15/06 , C07C15/08 , C10G35/06 , C10G45/08 , C10G69/08 , C10G45/00
CPC分类号： C10G69/08 , Y02P20/52
摘要： Cracked naphtha feeds such as FCC naphtha and coker naphtha are upgraded to produce chemical grade BTX (benzene, toluene, xylene with ethylbenzene) while co-producing a low sulfur gasoline of relatively high octane number. The cracked, sulfur-containing naphtha is processed by hydrodesulfurization followed by treatment over an acidic catalyst, preferably a zeolite such as ZSM-5 or zeolite beta with a hydrogenation component, preferably molybdenum. The treatment over the acidic catalyst in the second step restores the octane loss which takes place as a result of the hydrogenative treatment and results in a low sulfur gasoline product to permit a low sulfur gasoline of blending quality to be obtained with the BTX. The BTX can be extracted from the second stage effluent, preferably from a C.sub.6 -C.sub.8 fraction of this effluent.
摘要翻译：裂化石脑油原料如FCC石脑油和焦化石脑油被升级，以生产具有相对较高辛烷值的低硫汽油的化学级BTX（苯，甲苯，二甲苯与乙苯）。裂解的含硫石脑油通过加氢脱硫然后在酸性催化剂，优选沸石如ZSM-5或β沸石上用氢化组分，优选钼处理。在第二步骤中对酸性催化剂的处理恢复了由于氢化处理而发生的辛烷值损失，并导致低硫汽油产物，以允许用BTX获得混合质量的低硫汽油。 BTX可以从第二阶段流出物中提取，优选从该流出物的C6-C8馏分中提取。

28. 发明授权

US5395940A Synthesis of pyridine and 3-alkylpyridine 失效
标题翻译：吡啶和3-烷基吡啶的合成
公开(公告)号：US5395940A
公开(公告)日：1995-03-07
申请号：US73213
申请日：1993-06-07
申请人： Philip J. Angevine , Cynthia T-W. Chu , Thomas C. Potter
发明人： Philip J. Angevine , Cynthia T-W. Chu , Thomas C. Potter
IPC分类号： C07D213/08 , C07D213/09 , C07D213/10
CPC分类号： C07D213/08 , C07D213/10
摘要： An improved process is provided for selectively synthesizing pyridine and 3-alkylpyridine in high yield by reacting ammonia and a carbonyl reactant selected from the group consisting of formaldehyde, an aldehyde containing from 2 to 4 carbon atoms, a ketone containing from 3 to 5 carbon atoms, and mixtures thereof under effective conditions in the presence of a catalyst comprising an active form of a synthetic porous crystalline MCM-49 or synthetic porous crystalline material characterized by an X-ray diffraction pattern including interplanar d-spacings at 12.36.+-.0.4, 11.03.+-.0.2, 8.83.+-.0.14, 6.18.+-.0.12, 6.00.+-.0.10, 4.06.+-.0.07, 3.91.+-.0.07, and 3.42.+-.0.06 Angstroms, e.g., MCM-22, and recovering from the resulting reaction mixture a product enriched in pyridine and 3-alkylpyridine.
摘要翻译：提供了一种改进的方法，用于通过使氨和选自甲醛，含有2至4个碳原子的醛，含3至5个碳原子的酮的羰基反应物选择性合成吡咯和3-烷基吡啶，以及它们在有效条件下的存在下的混合物，所述催化剂包含活性形式的合成多孔结晶MCM-49或合成多孔结晶材料，其特征在于包括在12.36 +/- 0.4的面间d-间距的X射线衍射图， 11.03 +/- 0.2,8.33 +/- 0.14，6.18 +/- 0.12，6.00 +/- 0.10,4.06 +/- 0.07,3.91 +/- 0.07和3.42 +/- 0.06埃，例如MCM-22，并从所得反应混合物中回收富含吡啶和3-烷基吡啶的产物。

29. 发明授权

US5001295A Process for preparing dialkylnaphthalene 失效
标题翻译：制备二烷基萘的方法
公开(公告)号：US5001295A
公开(公告)日：1991-03-19
申请号：US494203
申请日：1990-03-15
申请人： Philip J. Angevine , Thomas F. Degnan , David O. Marler
发明人： Philip J. Angevine , Thomas F. Degnan , David O. Marler
IPC分类号： B01J29/04 , C07C2/12
CPC分类号： C07C2/12 , B01J29/04 , C07C2529/70
摘要： A catalytic process is provided for the preparation of dialkylnaphthalenes by alkylating a 2-alkylnaphthalene with an alkylating agent having an aliphatic group of from one to five carbon atoms, such as methanol. The catalyst comprises a synthetic zeolite characterized by an X-ray diffraction pattern including interplanar d-spacings at 12.36.+-.0.4, 11.03.+-.0.2, 8.83.+-.0.14, 6.18.+-.0.12, 6.00.+-.0.10, 4.06.+-.0.07, 3.91.+-.0.07 and 3.42.+-.0.06 Angstroms.
摘要翻译：提供了通过用具有1至5个碳原子的脂族基团如甲醇的烷基化烷基化2-烷基萘来制备二烷基萘的催化方法。该催化剂包括合成沸石，其特征在于X射线衍射图包括在12.36 +/- 0.4,11.03 +/- 0.2,8.83±0.14,6.18±0.12,6.00±0.10， 4.06 +/- 0.07,3.91 +/- 0.07和3.42 +/- 0.06埃。

30. 发明授权

US4568448A Hydrodesulfurization process employing poison-resistant catalyst 失效
标题翻译：加氢脱硫工艺采用耐毒催化剂
公开(公告)号：US4568448A
公开(公告)日：1986-02-04
申请号：US666230
申请日：1982-06-14
申请人： Philip J. Angevine , Edward J. Rosinski
发明人： Philip J. Angevine , Edward J. Rosinski
IPC分类号： B01J23/85 , B01J33/00 , B01J37/02 , C10G45/04 , C10G25/05
CPC分类号： B01J33/00 , B01J23/85 , B01J37/024 , C10G45/04 , B01J37/0215
摘要： Metal poisoning of hydrodesulfurization catalysts is reduced by coating the catalyst surface with a hydrated clay mineral, hydrated alumina, hydrated silica, or mixtures thereof. The catalyst and process in which it is used are particularly useful for the desulfurization of residual oils to produce low-sulfur, fuel oil products.
摘要翻译：通过用水合粘土矿物，水合氧化铝，水合二氧化硅或其混合物涂覆催化剂表面，降低加氢脱硫催化剂的金属中毒。其使用的催化剂和方法特别可用于残油的脱硫以产生低硫燃料油产品。

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