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21. 发明授权

US09040905B2 Analysis device and analysis method 有权
公开(公告)号：US09040905B2
公开(公告)日：2015-05-26
申请号：US13884755
申请日：2011-11-08
申请人： Hisashi Nagano , Yasutaka Suzuki , Hideo Kashima , Yuichiro Hashimoto , Masuyuki Sugiyama , Masakazu Sugaya , Yasunori Doi , Koichi Terada
发明人： Hisashi Nagano , Yasutaka Suzuki , Hideo Kashima , Yuichiro Hashimoto , Masuyuki Sugiyama , Masakazu Sugaya , Yasunori Doi , Koichi Terada
IPC分类号： H01J49/04 , G01N1/22 , G01N1/02 , H01J49/00 , G01N33/00
CPC分类号： H01J49/0422 , G01N1/2211 , G01N1/2214 , G01N33/0057 , G01N2001/028 , H01J49/00 , H01J49/0036 , H01J49/04 , H01J49/0459 , H01J49/0468 , Y02A50/25
摘要： Provided is a technique of analyzing particles in real time while collecting and condensing the particles continuously. Gas and/or particles as a detection target substance that are attached to an authentication target 2 are removed by air flow from a blowing region 5. The removed sample is sucked and is condensed and sampled at a sampling region 10, and ions of the sample are generated at an ion source 21 and are then subjected to mass analysis at a mass analysis region 23. Determination of the obtained mass spectrum is made as to the presence or not of a mass spectrum derived from the detection target substance, and a monitor 27 displays a result thereof. Thereby, the detection target substance attached to the authentication target 2 can be detected continuously in real time, promptly and with a less error rate.

22. 发明授权

US08973606B2 Gas concentration controller system 有权
公开(公告)号：US08973606B2
公开(公告)日：2015-03-10
申请号：US13327678
申请日：2011-12-15
申请人： Yuichiro Hashimoto , Junichi Miyaji
发明人： Yuichiro Hashimoto , Junichi Miyaji
IPC分类号： F17D3/00 , G05D11/13 , G01N33/00
摘要： The present invention is one that prevents standard gas from remaining in a standard gas line to prevent a concentration of standard gas from being reduced due to adsorption, modification, or the like, and has: a diluent gas line provided with a diluent gas flow rate controlling mechanism; a standard gas line provided with a standard gas flow rate controlling mechanism; an output gas line joined by the diluent gas line and standard gas line and outputs the standard gas having a predetermined concentration; an exhaust gas line connected to an upstream side of the standard gas flow rate controlling mechanism in the standard gas line and provided with an on/off valve and a flow rate control part; and a control part that, depending on a flow rate of the standard gas flowing through the standard gas line or the type of the standard gas, switches on/off the on/off valve.

23. 发明授权

US08710430B2 Mass spectrometry method 有权
标题翻译：质谱法
公开(公告)号：US08710430B2
公开(公告)日：2014-04-29
申请号：US13527619
申请日：2012-06-20
申请人： Masuyuki Sugiyama , Yuichiro Hashimoto , Shun Kumano , Yohei Kawaguchi , Hidetoshi Morokuma
发明人： Masuyuki Sugiyama , Yuichiro Hashimoto , Shun Kumano , Yohei Kawaguchi , Hidetoshi Morokuma
IPC分类号： H01J49/42 , H01J49/26 , H01J49/00
CPC分类号： H01J49/4265 , H01J49/0009 , H01J49/0036
摘要： A mass spectrometry method that corrects the effects from space charge and that achieves both sensitivity and a dynamic range. The mass axis of the mass spectrum is corrected based on the counts of ions accumulated within the ion trap at the point in time each ion was extracted.
摘要翻译：一种校正空间电荷效应并实现灵敏度和动态范围的质谱法。基于在每个离子被提取的时间点内积聚在离子阱内的离子的计数校正质谱的质量轴。

24. 发明申请

US20130334416A1 MASS SPECTROMETER AND ION SOURCE USED THEREFOR 有权
标题翻译：质谱仪及其使用的离子源
公开(公告)号：US20130334416A1
公开(公告)日：2013-12-19
申请号：US14001711
申请日：2012-01-27
申请人： Hiroyuki Satake , Hideki Hasegawa , Masuyuki Sugiyama , Yuichiro Hashimoto
发明人： Hiroyuki Satake , Hideki Hasegawa , Masuyuki Sugiyama , Yuichiro Hashimoto
IPC分类号： H01J49/10
CPC分类号： H01J49/10 , H01J49/0431 , H01J49/165
摘要： The quantitative accuracy of analysis is improved without reducing the dynamic range for measurement of concentrations by performing stable ionization through electrospray or the like which repeats sampling and ionization using a movable probe electrode.A voltage is applied from a high-voltage power source 4 to a sample transport electrode 7 having a plurality of probe electrodes 1 and a driving section 3 drives the sample transport electrode 7 to rotate. The plurality of probe electrodes 1, to which a sample solution 5 is adhered, are sequentially transported to an inlet 21 of a mass spectrometer 20, thus electrospray ionization is continuously performed.
摘要翻译：通过使用可移动探针电极重复取样和电离的电喷雾等进行稳定的电离，可以提高分析的定量精度，而不降低浓度测定的动态范围。从高电压电源4向具有多个探针电极1的检体输送电极7施加电压，驱动部3驱动检体输送电极7旋转。将附着有样品溶液5的多个探针电极1依次输送到质谱仪20的入口21，从而连续进行电喷雾离子化。

25. 发明申请

US20130240726A1 MASS SPECTROMETER 有权
标题翻译：质谱仪
公开(公告)号：US20130240726A1
公开(公告)日：2013-09-19
申请号：US13877717
申请日：2011-10-03
申请人： Hideki Hasegawa , Masuyuki Sugiyama , Hiroyuki Satake , Yuichiro Hashimoto
发明人： Hideki Hasegawa , Masuyuki Sugiyama , Hiroyuki Satake , Yuichiro Hashimoto
IPC分类号： H01J49/06
CPC分类号： H01J49/063 , H01J49/005 , H01J49/068 , H01J49/4255
摘要： This mass spectrometer is provided with an ion guide (37) having a multipole rod electrode (1), a power source unit (5) for applying voltage to the multipole rod electrode, and a control unit for controlling the power source unit, said mass spectrometer being characterised by the multipole rod electrode having a rod electrode divided into a plurality of segmented rods (2A-1, 2A-2, 2B-1, 2B-2, 2C-1, 2C-2, 2D-1, 2D-2) at mutually different positions in the axial direction. Thus enabled is low-cost, high-throughput analysis.
摘要翻译：该质谱仪设置有具有多极杆电极（1）的离子引导件（37），用于向多极杆电极施加电压的电源单元（5），以及用于控制电源单元的控制单元，所述质量光谱仪的特征在于多极杆电极具有分为多个分段杆（2A-1,2A-2,2B-1,2B-2,2C-1,2C-2，2D-1，2D- 2）在轴向上相互不同的位置。因此启用了低成本，高通量分析。

26. 发明授权

US08368013B2 Analyzer, ionization apparatus and analyzing method 有权
标题翻译：分析仪，电离装置及分析方法
公开(公告)号：US08368013B2
公开(公告)日：2013-02-05
申请号：US13084930
申请日：2011-04-12
申请人： Masako Ishimaru , Yuichiro Hashimoto , Hideki Hasegawa , Masuyoshi Yamada , Masuyuki Sugiyama , Hidetoshi Morokuma
发明人： Masako Ishimaru , Yuichiro Hashimoto , Hideki Hasegawa , Masuyoshi Yamada , Masuyuki Sugiyama , Hidetoshi Morokuma
IPC分类号： B01D59/44 , H01J49/00
CPC分类号： H01J49/145
摘要： An analyzer performs dielectric barrier discharge and ionization of a sample by a reaction between the sample and excited molecules or ions generated by the dielectric barrier discharge at a pressure lower than an atmospheric pressure.
摘要翻译：分析仪通过在低于大气压的压力下通过介电阻挡放电产生的样品和激发的分子或离子之间的反应来进行介电阻挡放电和样品的离子化。

27. 发明申请

US20120326022A1 MASS SPECTROMETER AND MASS ANALYZING METHOD 有权
标题翻译：质谱仪和质谱分析方法
公开(公告)号：US20120326022A1
公开(公告)日：2012-12-27
申请号：US13527627
申请日：2012-06-20
申请人： Shun KUMANO , Masuyuki Sugiyama , Yuichiro Hashimoto , Hideki Hasegawa , Masuyoshi Yamada , Hidetoshi Morokuma , Shuhei Hashiba
发明人： Shun KUMANO , Masuyuki Sugiyama , Yuichiro Hashimoto , Hideki Hasegawa , Masuyoshi Yamada , Hidetoshi Morokuma , Shuhei Hashiba
IPC分类号： H01J49/04
CPC分类号： H01J49/0409 , H01J49/0495
摘要： A mass spectrometer including a sample attaching member of attaching a sample, an ionizing chamber including an introductory port of the sample attaching member and an ionization source of generating a sample ion, a vacuumed chamber having a mass analyzer of analyzing the sample ion, and an opening/closing mechanism provided between the ionizing chamber and the vacuumed chamber, in which the opening/closing mechanism is controlled from a closed state to an open state after introducing the sample attaching member into the ionizing chamber to thereby enable to perform ionization with inconsiderable fragmentation at a high sensitivity with a high throughput
摘要翻译：一种质谱仪，包括附着样品的样品附着构件，包括样品附着构件的入口的电离室和产生样品离子的离子源，具有分析样品离子的质量分析器的真空室，以及设置在离子化室和真空室之间的开/关机构，其中将样品附着构件引入电离室之后，将开/关机构从关闭状态控制到打开状态，从而能够以不可分割的碎片进行电离灵敏度高，吞吐量高

28. 发明申请

US20120152364A1 GAS CONCENTRATION CONTROLLER SYSTEM 有权
标题翻译：气体浓度控制系统
公开(公告)号：US20120152364A1
公开(公告)日：2012-06-21
申请号：US13327678
申请日：2011-12-15
申请人： Yuichiro Hashimoto , Junichi Miyaji
发明人： Yuichiro Hashimoto , Junichi Miyaji
IPC分类号： F15D1/00
CPC分类号： G05D11/132 , G01N33/0006 , Y10T137/0318 , Y10T137/7759 , Y10T137/7761 , Y10T137/87249 , Y10T137/8729 , Y10T137/87314 , Y10T137/87676
摘要： The present invention is one that prevents standard gas from remaining in a standard gas line to prevent a concentration of standard gas from being reduced due to adsorption, modification, or the like, and has: a diluent gas line provided with a diluent gas flow rate controlling mechanism; a standard gas line provided with a standard gas flow rate controlling mechanism; an output gas line joined by the diluent gas line and standard gas line and outputs the standard gas having a predetermined concentration; an exhaust gas line connected to an upstream side of the standard gas flow rate controlling mechanism in the standard gas line and provided with an on/off valve and a flow rate control part; and a control part that, depending on a flow rate of the standard gas flowing through the standard gas line or the type of the standard gas, switches on/off the on/off valve.
摘要翻译：本发明是防止标准气体残留在标准气体管线中，以防止标准气体由于吸附，改性等而降低的浓度，并具有：具有稀释气体流量的稀释气体管线控制机制; 设有标准气体流量控制机构的标准气体管线; 通过稀释气体管线和标准气体管路连接的输出气体管线，输出具有预定浓度的标准气体; 与标准气体流量控制机构的标准气体流量控制机构的上游侧连接并配置有开关阀和流量控制部的排气管路，以及控制部，其根据流过标准气体管路的标准气体的流量或标准气体的类型来开/关开闭阀。

29. 发明申请

US20120112059A1 MASS SPECTROMETER AND MASS SPECTROMETRY METHOD 有权
标题翻译：质谱仪和质谱方法
公开(公告)号：US20120112059A1
公开(公告)日：2012-05-10
申请号：US13383371
申请日：2010-07-09
申请人： Masuyuki Sugiyama , Yuichiro Hashimoto , Hisashi Nagano , Hideki Hasegawa , Yasuaki Takada , Masuyoshi Yamada
发明人： Masuyuki Sugiyama , Yuichiro Hashimoto , Hisashi Nagano , Hideki Hasegawa , Yasuaki Takada , Masuyoshi Yamada
IPC分类号： H01J49/26
CPC分类号： H01J49/004
摘要： An object is to measure both cations and anions with high duty cycle. In a mass spectrometer comprising an ion source (1), an ion guide part (31), and an ion trap (32), while ions are being mass-selectively ejected from the ion trap, ions having a polarity reverse to that of the ions trapped in the ion trap are introduced into the ion guide part.
摘要翻译：一个目标是测量阳离子和阴离子高占空比。在离子源（1），离子引导部（31）和离子阱（32）的质谱仪中，离子从离子阱中质量选择性地喷出时，具有与捕获在离子阱中的离子被引入离子引导部。

30. 发明授权

US07820961B2 Mass spectrometer and method of mass spectrometry 有权
标题翻译：质谱仪和质谱法
公开(公告)号：US07820961B2
公开(公告)日：2010-10-26
申请号：US11745516
申请日：2007-05-08
申请人： Yuichiro Hashimoto , Hideki Hasegawa , Izumi Waki , Masuyuki Sugiyama
发明人： Yuichiro Hashimoto , Hideki Hasegawa , Izumi Waki , Masuyuki Sugiyama
IPC分类号： B01D59/44 , H01J49/00
CPC分类号： H01J49/4225 , H01J49/429
摘要： A linear trap having high ejection efficiency and low ejection energy is realized. In a mass spectrometer in which ions generated by an ion source are introduced to a quadrupole rod structure applied with RF voltage and ejected from the quadrupole rod structure so as to be detected by a detection mechanism, a mass dependent potential is formed in the axial direction of the quadrupole rod structure and ions are ejected mass selectively from the vicinity of a minimum point of the potential, the mass dependent potential being formed by applying electrostatic voltage and RF voltage to an insertion electrode inserted in the quadrupole rods.
摘要翻译：实现了具有高喷射效率和低喷射能量的线性阱。在其中由离子源产生的离子被引入施加有RF电压并从四极杆结构喷射以便通过检测机构检测的四极杆结构的质谱仪中，在轴向上形成质量依赖电位的四极杆结构和离子从电位的最小点附近选择性地排出，质量依赖电位通过将静电电压和RF电压施加到插入四极棒中的插入电极而形成。

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