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11. 发明授权

US5939597A Fluid bed process for para-xylene production 失效
标题翻译：对二甲苯生产的流化床工艺
公开(公告)号：US5939597A
公开(公告)日：1999-08-17
申请号：US954787
申请日：1997-10-21
申请人： Ralph M. Dessau , David H. Olson , Robert A. Ware , Sadi Mizrahi
发明人： Ralph M. Dessau , David H. Olson , Robert A. Ware , Sadi Mizrahi
IPC分类号： C07C2/86 , C07C2/66
CPC分类号： C07C2/865 , C07C2/861 , C07C2/864 , C07C2/868 , C07C2521/06 , C07C2521/08 , C07C2521/10 , C07C2521/12 , C07C2521/14 , C07C2521/16 , C07C2523/12 , C07C2529/40
摘要： Para-xylene is produced by toluene methylation by charging toluene and a methylating agent to a fluidized bed of catalyst at a rate sufficient to maintain the fluidized bed in a turbulent sub-transport flow regime, reacting the toluene with the methylating agent, and recovering para-xylene from the fluidized bed. The fluidizable catalyst is a microporous material having a Constraint Index of about 1 to about 12. The relative concentration of the catalyst particles having a major dimension of less than 40 microns is controlled at between about 5 and 35 weight percent. The catalyst particles have an apparent particle density of about 0.9 to 1.6 grams per cubic centimeter, a size range of about 1 to 150 microns, and average particle size of about 20 to 100 microns.
摘要翻译：通过将甲苯和甲基化剂以足以将流化床保持在湍流亚运输流动状态的速率将甲苯和甲基化剂装载到催化剂的流化床中，通过甲苯甲基化反应，使甲苯与甲基化剂反应，并回收对数 - 二甲苯。可流化催化剂是具有约1至约12的约束指数的微孔材料。主要尺寸小于40微米的催化剂颗粒的相对浓度控制在约5至35重量％之间。催化剂颗粒具有约0.9至1.6克/立方厘米的表观颗粒密度，约1至150微米的尺寸范围和约20至100微米的平均粒度。

12. 发明授权

US5219814A Catalyst for light cycle oil upgrading 失效
标题翻译：催化剂用于轻循环油升级
公开(公告)号：US5219814A
公开(公告)日：1993-06-15
申请号：US629952
申请日：1990-12-19
申请人： Garry W. Kirker , Michael E. Landis , Daria N. Lissy , Sadi Mizrahi , Michael S. Sarli , Stuart S. Shih
发明人： Garry W. Kirker , Michael E. Landis , Daria N. Lissy , Sadi Mizrahi , Michael S. Sarli , Stuart S. Shih
IPC分类号： B01J29/16 , C10G47/20
CPC分类号： C10G47/20 , B01J29/166
摘要： A moderate pressure hydrocracking process in which a highly aromatic, substantially dealkylated feedstock is processed to high octane gasoline and low sulfur distillate by hydrocracking over a catalyst, preferably comprising ultrastable Y and a Group VIII metal and a Group VI metal, in which the amount of the Group VIII metal content is incorporated at specified proportion into the framework aluminum content of the ultrastable Y component. The feedstock which is preferably a light cycle oil has an aromatic content of at least 50, usually at least 60 percent, and an API gravity not more than 25. The hydrocracking typically operates at 400-1000 psig at moderate to high conversion levels to maximize the production of monocyclic aromatics which provide the requisite octane value to the product gasoline. The distillate products from the hydrocracker are reduced in their sulfur content.
摘要翻译：中等压力加氢裂化方法，其中高度芳香的，基本上脱烷基化的原料通过催化剂上的加氢裂化加工成高辛烷值汽油和低硫馏分，优选包括超稳定Y和VIII族金属和第VI族金属，其中第VIII族金属含量以规定比例掺入超稳Y组分的骨架铝含量中。优选轻循环油的原料具有至少50，通常至少60％的芳烃含量，API重力不超过25.加氢裂化通常在中等至高转化率的400-1000psig下操作，以使生产提供产品汽油必需辛烷值的单环芳烃。来自加氢裂化器的馏出物的硫含量降低。

13. 发明授权

US5078751A Process for upgrading olefinic gasoline by etherification wherein asymmetrical dialkyl ethers are produced 失效
标题翻译：通过非对称二烷基醚生产过氧化物来提高烯烃汽油的方法
公开(公告)号：US5078751A
公开(公告)日：1992-01-07
申请号：US505094
申请日：1990-04-04
申请人： Sadi Mizrahi , Charles M. Sorensen , Samuel A. Tabak
发明人： Sadi Mizrahi , Charles M. Sorensen , Samuel A. Tabak
IPC分类号： C07C41/06 , C07C43/04 , C10G35/04 , C10L1/00 , C10L1/02 , C10L1/182
CPC分类号： C10L1/023
摘要： A process is disclosed for upgrading C.sub.5 -C.sub.8 olefin-containing gasoline to a high octane motor gasoline blending component.C.sub.3 -C.sub.4 olefins are hydrated to alcohols and then selectively removed from the aqueous hydration reactor effluent stream via liquid extraction with the gasoline feedstream. The alcohol enriched gasoline extract stream is then etherified and unreacted alcohols are extracted to yield a high octane gasoline blending component free of metal-bearing additives.

14. 发明授权

US4968406A Increasing feed volume throughput in FCC process 失效
标题翻译：在FCC工艺中增加进料量通量
公开(公告)号：US4968406A
公开(公告)日：1990-11-06
申请号：US252873
申请日：1988-10-29
申请人： Sadi Mizrahi , James C. Vartuli
发明人： Sadi Mizrahi , James C. Vartuli
IPC分类号： C10G11/05 , C10G11/18
CPC分类号： C10G11/18 , C10G11/05
摘要： A process for increasing the volume of feed throughput to the catalytic cracker by decreasing hydrogen and total gas volume production, under catalytic cracking conditions temperature of 950.degree. F. to about 1150.degree. F., a catalyst to feed ratio of 3:1 to 10:1 and a catalyst contact time of from about 1 to about 20 in the presence of catalyst comprising ZSM-20 and a matrix.
摘要翻译：一种通过降低氢气和总气体产量来提高催化裂化装置的进料通量的方法，催化裂化条件为950°F至1150°F，催化剂与进料比为3：1至10 ：1和在包含ZSM-20和基质的催化剂存在下，约1至约20的催化剂接触时间。

15. 发明授权

US4898662A Catalytic cracking process using high equilibrium activity additive catalyst 失效
标题翻译：催化裂化工艺采用高平衡活性添加剂催化剂
公开(公告)号：US4898662A
公开(公告)日：1990-02-06
申请号：US264577
申请日：1988-10-31
申请人： Pochen Chu , Sadi Mizrahi
发明人： Pochen Chu , Sadi Mizrahi
IPC分类号： B01J29/40 , C10G11/05
CPC分类号： B01J29/40 , C10G11/05 , B01J2229/26 , B01J2229/36 , B01J2229/42
摘要： A catalytic cracking process is disclosed in which octane improvement is attained by the addition to conventional cracking catalysts of small amounts of additive catalyst comprising a class of zeolites characterized by a silica to alumina mole ratio greater than about 12 and a Constraint Index of about 1 to 12 bound in a matrix chosen such that the matrix component forms a thermodynamically favored compound with selected cations. Sustained catalytic activity is achieved by pre-exchanging the catalyst to a high level of selected cation loading. By extending the active life of the additive catalyst, markedly lower makeup catalyst addition rates are required.
摘要翻译：公开了一种催化裂解方法，其中通过加入少量添加剂催化剂的常规裂化催化剂来实现辛烷值改进，所述催化剂包含一类沸石，其特征在于二氧化硅与氧化铝的摩尔比大于约12，约束指数为约1至 12以选定的矩阵结合，使得基质组分与选择的阳离子形成热力学上有利的化合物。通过将催化剂预交换为高水平的选择的阳离子负载来实现持续的催化活性。通过延长添加剂催化剂的活性，需要显着降低催化剂添加量。

16. 发明授权

US08222459B2 Process for producing cyclohexanone 有权
标题翻译：环己酮生产工艺
公开(公告)号：US08222459B2
公开(公告)日：2012-07-17
申请号：US12933700
申请日：2009-02-19
申请人： Jihad M. Dakka , John S. Buchanan , James R. Lattner , Sadi Mizrahi
发明人： Jihad M. Dakka , John S. Buchanan , James R. Lattner , Sadi Mizrahi
IPC分类号： C07C45/00
CPC分类号： C07C407/00 , C07C37/07 , C07C37/08 , C07C45/006 , C07C45/53 , C07C2601/14 , C07C39/04 , C07C49/403 , C07C409/14
摘要： In a process for producing cyclohexanone, cyclohexylbenzene is oxidized to produce cyclohexylbenzene hydroperoxide and then the resultant cyclohexylbenzene hydroperoxide is cleaved to produce an effluent stream comprising phenol and cyclohexanone. At least a portion of the effluent stream is then fed to at least one hydrogenation reaction zone, where the effluent stream portion is contacted with hydrogen in the presence of a hydrogenation catalyst under conditions effective to convert at least part of the phenol in the effluent portion into cyclohexanone.
摘要翻译：在制备环己酮的方法中，环己基苯被氧化以产生环己基苯氢过氧化物，然后将所得环己基苯氢过氧化物切割以产生包含苯酚和环己酮的流出物流。然后将至少一部分流出物流送入至少一个氢化反应区，在氢化催化剂存在下，在有效地将至少部分苯酚在流出物部分中转化的条件下，流出料流部分与氢气接触加入环己酮。

17. 发明授权

US5000839A Hydrocracking process for producing a high density jet fuel 失效
标题翻译：用于生产高密度喷气燃料的加氢裂化工艺
公开(公告)号：US5000839A
公开(公告)日：1991-03-19
申请号：US479789
申请日：1990-02-14
申请人： Garry W. Kirker , Sadi Mizrahi , Stuart S. Shih
发明人： Garry W. Kirker , Sadi Mizrahi , Stuart S. Shih
IPC分类号： B01J29/14 , B01J29/16 , B01J29/70 , B01J29/74 , B01J29/80 , C10G65/10 , C10G65/12
CPC分类号： B01J29/7038 , B01J29/146 , B01J29/166 , B01J29/7088 , B01J29/7415 , B01J29/7476 , B01J29/80 , C10G65/10 , C10G65/12 , B01J2229/16 , B01J2229/26 , B01J2229/42
摘要： A two-stage hydrocracking process for producing high density jet fuel from an aromatic feedstock using a synthetic zeolite catalyst. The feedstock is hydrotreated in the first stage to convert heteroatoms. After removal of sulfur and nitrogen compounds, the feed is directed to a hydrocracker where it contacted with MCM-22 zeolite.
摘要翻译：使用合成沸石催化剂从芳族原料生产高密度喷气燃料的两阶段加氢裂化方法。原料在第一阶段加氢处理以转化杂原子。在除去硫和氮化合物之后，将进料引导至与MCM-22沸石接触的加氢裂化器。

18. 发明授权

US5942651A Process for converting C.sub.9 + aromatic hydrocarbons to lighter aromatic products by transalkylation in the prescence of two zeolite-containing catalysts 失效
标题翻译：在两种含沸石的催化剂的情况下，通过烷基转移将C9 +芳族烃转化成较轻的芳香族产物的方法
公开(公告)号：US5942651A
公开(公告)日：1999-08-24
申请号：US874875
申请日：1997-06-13
申请人： James H. Beech, Jr. , Stuart Damon Hellring , Terry Eugene Helton , Timothy Frederick Kinn , Sadi Mizrahi , Norman J. Rouleau
发明人： James H. Beech, Jr. , Stuart Damon Hellring , Terry Eugene Helton , Timothy Frederick Kinn , Sadi Mizrahi , Norman J. Rouleau
IPC分类号： C07C4/18 , C07B61/00 , C07C6/12 , C07C15/02 , C07C15/04 , C10G11/05 , C07C5/22
CPC分类号： C07C6/126 , C07C2529/06 , C07C2529/70 , Y02P20/52
摘要： A process for converting a heavy aromatics feed to lighter aromatic products, such as benzene and xylene, by reacting C.sub.9+ aromatic hydrocarbons and toluene or benzene under transalkylation reaction conditions, over a first catalyst composition including a zeolite having a constraint index ranging from 0.5 to 3 and a hydrogenation component and a second catalyst composition including an intermediate pore size zeolite having a constraint index ranging from 3 to 12 and a silica to alumina ratio of at least about 5, to produce a transalkylation reaction product containing benzene or toluene and xylene. The benzene or toluene from the reaction product can then be distilled to obtain a benzene or toluene product.
摘要翻译：通过在烷基转移反应条件下使C9 +芳族烃和甲苯或苯反应，在包含约0.5到3的约束指数的沸石的第一种催化剂组合物上，将重质芳族化合物进料转化成较轻的芳香族产物如苯和二甲苯的方法以及氢化组分和第二催化剂组合物，其包含约3至12的约束指数和至少约5的二氧化硅与氧化铝的中等孔径的沸石，以产生含有苯或甲苯和二甲苯的烷基转移反应产物。然后可以将来自反应产物的苯或甲苯蒸馏得到苯或甲苯产物。

19. 发明授权

US5763720A Transalkylation process for producing aromatic product using a treated zeolite catalyst 失效
标题翻译：使用经处理的沸石催化剂制备芳香族产物的烷基转移方法
公开(公告)号：US5763720A
公开(公告)日：1998-06-09
申请号：US937280
申请日：1997-09-15
申请人： John S. Buchanan , Arthur W. Chester , Anthony S. Fung , Timothy F. Kinn , Sadi Mizrahi
发明人： John S. Buchanan , Arthur W. Chester , Anthony S. Fung , Timothy F. Kinn , Sadi Mizrahi
IPC分类号： C07C2/66 , B01J29/74 , B01J29/76 , C07C2/64 , C07C5/52 , C07C6/12 , C07C15/02 , C07C15/04 , C07C15/06 , C07C15/067 , C07C15/08 , C10G35/095 , C10G45/64 , C10G47/16 , C10G47/18 , C10G47/20 , C10G49/02 , C10G49/08
CPC分类号： C10G47/16 , B01J29/7415 , B01J29/7469 , B01J29/7476 , C07C6/126 , C10G35/095 , B01J2229/26 , B01J2229/36 , B01J2229/42 , C07C2529/74 , Y02P20/52 , Y10S585/906
摘要： A heavy aromatics feed is converted to lighter aromatics products, such as benzene, toluene and xylenes by contacting a C.sub.9 + aromatics fraction and benzene and/or toluene over a catalyst comprising a zeolite, such as ZSM-12, and a hydrogenation component, preferably platinum. The catalyst, complete with hydrogenation component, is treated to reduce aromatics loss. Treatment includes exposure to steam and/or sulfur after incorporation of the hydrogenation component. For additional stability and aromatics retention the steamed and/or sulfur treated catalyst is sulfided by cofeeding a source of sulfur. In a further embodiment of the invention a low hydrogen partial pressure is employed to retain aromatics.
摘要翻译：通过使C9 +芳族化合物馏分和苯和/或甲苯在包含沸石的催化剂（例如ZSM-12）和氢化组分（优选铂）中接触，将重质芳烃进料转化为较轻的芳烃产物，例如苯，甲苯和二甲苯。处理具有氢化组分的催化剂，以减少芳族化合物的损失。处理包括在加入氢化组分后暴露于蒸汽和/或硫。为了进一步的稳定性和芳族化合物保留，蒸汽和/或硫处理的催化剂通过共同供给硫来硫化。在本发明的另一个实施方案中，采用低的氢分压来保留芳族化合物。

20. 发明授权

US4913797A Catalyst hydrotreating and dewaxing process 失效
标题翻译：催化剂加氢处理和脱蜡工艺
公开(公告)号：US4913797A
公开(公告)日：1990-04-03
申请号：US296929
申请日：1989-01-12
申请人： Kenneth R. Albinson , Sadi Mizrahi , Daniel J. Neuman
发明人： Kenneth R. Albinson , Sadi Mizrahi , Daniel J. Neuman
IPC分类号： C10G65/04
CPC分类号： C10G65/043
摘要： The present invention is directed to a cascade catalytic hydrotreating/dewaxing process, wherein a hydrocarbon feedstock containing waxy components is treated. The hydrotreating phase precedes the dewaxing phase in order to remove contaminants, such as nitrogen and sulfur, from the feedstock to prolong the life of the catalyst used in the subsequent dewaxing step. A conventional hydrotreating catalyst is used. The dewaxing catalyst is a Zeolite Beta catalyst. The cascade process is conducted with or without interstage gas separation. The treatment occurs in the same or in separate reactors. The ratio of hydrotreating catalyst to dewaxing catalyst is greater than 1:2. This sequence of treatments enhances distillate yields and lowers processing and capital costs.
摘要翻译：本发明涉及级联催化加氢处理/脱蜡方法，其中处理含有蜡质组分的烃原料。加氢处理阶段在脱蜡阶段之前，以从原料中除去诸如氮和硫的污染物，以延长随后脱蜡步骤中所用催化剂的寿命。使用常规的加氢处理催化剂。脱蜡催化剂是沸石β型催化剂。级联过程是在有或没有级间气体分离的情况下进行的。处理发生在相同或单独的反应器中。加氢处理催化剂与脱蜡催化剂的比例大于1：2。这种处理顺序增强了馏出物产率，降低了加工和资本成本。

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