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1. 发明申请

WO2023069896A1 PROTON-EXCHANGE MEMBRANES FOR ELECTROCHEMICAL REACTIONS 审中-公开
公开(公告)号：WO2023069896A1
公开(公告)日：2023-04-27
申请号：PCT/US2022/078207
申请日：2022-10-17
申请人： UOP LLC
发明人： LIU, Chunqing , BA, Chaoyi , KARNS, Nicole , DONG, Xueliang
IPC分类号： C08G61/12 , C08G61/02 , C08J5/22 , C25B13/08 , C25B9/23 , C25B1/04
摘要： A proton-conducting polymer comprises a plurality of repeating units of formula (I) for electrochemical reactions. The polymer may be synthesized from a super acid catalyzed polyhydroxyalkylation reaction of monomers Ar1', Ar2', and X1 (I) followed by a nucleophilic substitution reaction or a grafting reaction, and optionally an acidification reaction. Proton-exchange membranes and membrane electrode assemblies made from the polymer are also described.

2. 发明申请

WO2021025856A1 HIGH SELECTIVITY MEMBRANES FOR HYDROGEN SULFIDE AND CARBON DIOXIDE REMOVAL FROM NATURAL GAS 审中-公开
公开(公告)号：WO2021025856A1
公开(公告)日：2021-02-11
申请号：PCT/US2020/042842
申请日：2020-07-21
申请人： UOP LLC
发明人： DONG, Xueliang , LIU, Chunqing , TRAN, Howie
IPC分类号： B01D53/22 , B01D71/80 , B01D69/08
摘要： A thin film composite gas separation membrane comprising a polyether block amide copolymer coating layer and a nanoporous asymmetric support membrane with nanopores on the skin layer surface of the support membrane and gelatin polymers inside the nanopores on the skin layer surface of the support membrane. A method for making the thin film composite gas separation membrane is provided as well as the use of the membrane for a variety of separations such as separations of hydrogen sulfide and carbon dioxide from natural gas, carbon dioxide removal from flue gas, fuel gas conditioning, hydrogen/methane, polar molecules, and ammonia mixtures with methane, nitrogen or hydrogen and other light gases separations, but also for natural gas liquids recovery and hydrogen sulfide and carbon dioxide removal from natural gas in a single step.

3. 发明申请

WO2018183057A1 RUBBERY POLYMERIC MEMBRANES FOR SEPARATION 审中-公开
公开(公告)号：WO2018183057A1
公开(公告)日：2018-10-04
申请号：PCT/US2018/023522
申请日：2018-03-21
申请人： UOP LLC
发明人： LIU, Chunqing , KARNS, Nicole K.
IPC分类号： B01D67/00 , B01D69/12 , B01D71/70 , C08J7/04 , C10L3/10
摘要： A super high permeance and high selectivity dual layer rubbery polymeric membrane comprising a thin selective layer of a fumed silica reinforced, cross-linked polyorganosiloxane on top of a porous glassy polymer support membrane and a thin selective layer of a chemically cross-linked polyorganosiloxane rubbery polymer on top of the thin selective layer of a fumed silica reinforced, cross-linked polyorganosiloxane, and a porous glassy polymer support membrane that is formed from a glassy polymer and the processes of making these membranes and using these membranes in separating mixtures of two or more gases or liquids.

4. 发明申请

WO2016148988A1 HIGH SELECTIVITY EPOXYSILICONE-CROSS-LINKED POLYIMIDE MEMBRANES FOR GAS SEPARATIONS 审中-公开
标题翻译：用于气体分离的高选择性环氧硅氧烷 - 交联的聚酰亚胺膜
公开(公告)号：WO2016148988A1
公开(公告)日：2016-09-22
申请号：PCT/US2016/021439
申请日：2016-03-09
申请人： UOP LLC
发明人： LIU, Chunqing , TRAN, Howie Q.
IPC分类号： B01D71/78 , B01D71/52 , B01D71/82 , B01D53/22
CPC分类号： B01D69/125 , B01D53/228 , B01D69/02 , B01D69/088 , B01D69/12 , B01D71/64 , B01D71/68 , B01D71/70 , B01D2053/224 , B01D2256/10 , B01D2256/12 , B01D2256/16 , B01D2256/18 , B01D2256/24 , B01D2257/108 , B01D2257/11 , B01D2257/304 , B01D2257/504 , B01D2257/702 , B01D2257/708 , B01D2257/80 , B01D2323/30 , Y02C10/10
摘要： The present invention provides a high selectivity epoxysilicone-cross-linked polyimide membrane comprising a polyimide polymer with hydroxyl functional groups cross-linked with epoxy functional groups on epoxysilicone polymer. The present invention also provides a process for separating at least one gas from a mixture of gases using the high selectivity epoxysilicone-cross-linked polyimide membrane. The process comprises providing the high selectivity epoxysilicone-cross-linked polyimide membrane which is permeable to the at least one gas; contacting the mixture on one side of the membrane to cause the at least one gas to permeate the membrane; and removing from the opposite side of the membrane a permeate gas composition comprising a portion of the at least one gas which permeated the high selectivity epoxysilicone-cross-linked polyimide membrane.
摘要翻译：本发明提供一种高选择性环氧硅氧烷 - 交联聚酰亚胺膜，其包含在环氧硅氧烷聚合物上与环氧官能团交联的羟基官能团的聚酰亚胺聚合物。本发明还提供了使用高选择性环氧硅氧烷 - 交联聚酰亚胺膜从气体混合物中分离至少一种气体的方法。该方法包括提供对至少一种气体是可渗透的高选择性环氧硅氧烷 - 交联聚酰亚胺膜; 使所述混合物在所述膜的一侧上接触以引起所述至少一种气体渗透所述膜; 并且从所述膜的相对侧移除包含渗透所述高选择性环氧硅氧烷交联的聚酰亚胺膜的所述至少一种气体的一部分的渗透气体组合物。

5. 发明申请

WO2016053765A2 HIGH SELECTIVITY POLYIMIDE MEMBRANE FOR NATURAL GAS UPGRADING AND HYDROGEN PURIFICATION 审中-公开
标题翻译：用于天然气升级和氢气净化的高选择性聚酰亚胺膜
公开(公告)号：WO2016053765A2
公开(公告)日：2016-04-07
申请号：PCT/US2015/052091
申请日：2015-09-25
申请人： UOP LLC
发明人： LIU, Chunqing , TRAN, Howie Q.
CPC分类号： B01D53/228 , B01D67/0006 , B01D71/64 , B01D2256/16 , B01D2325/14 , Y02C10/10 , Y02C20/20
摘要： A polyimide polymer having hydroxyl and acetoxy function groups is provided together with a membrane made from the polymer. Also provided is a process for separating at least one gas from a mixture of gases using a polyimide membrane comprising a polyimide polymer with hydroxyl and acetoxy functional the process comprising: (a) providing the polyimide membrane comprising the polyimide polymer with hydroxyl and acetoxy functional groups which is permeable to the at least one gas; (b) contacting the mixture on one side of the polyimide membrane to cause said at least one gas to permeate the membrane; and (c) removing from the opposite side of the membrane a permeate gas composition comprising a portion of said at least one gas which permeated the polyimide membrane.
摘要翻译：具有羟基和乙酰氧基官能团的聚酰亚胺聚合物与由聚合物制成的膜一起提供。还提供了使用包含具有羟基和乙酰氧基官能团的聚酰亚胺聚合物的聚酰亚胺膜从气体混合物中分离至少一种气体的方法，该方法包括：（a）提供包含聚酰亚胺聚合物的聚酰亚胺膜，其具有羟基和乙酰氧基官能团其对所述至少一种气体是可渗透的; （b）使所述混合物在所述聚酰亚胺膜的一侧上接触以使所述至少一种气体渗透所述膜; 和（c）从所述膜的相对侧去除渗透气体组合物，所述渗透气体组合物包含透过所述聚酰亚胺膜的所述至少一种气体的一部分。

6. 发明申请

WO2016049274A1 ASYMMETRIC INTEGRALLY-SKINNED FLAT SHEET MEMBRANES FOR H2 PURIFICATION AND NATURAL GAS UPGRADING 审中-公开
标题翻译：用于纯化和天然气升级的非对称整体平滑薄膜
公开(公告)号：WO2016049274A1
公开(公告)日：2016-03-31
申请号：PCT/US2015/051865
申请日：2015-09-24
申请人： UOP LLC
发明人： LIU, Chunqing , TRAN, Howie Q.
IPC分类号： C07C7/144 , B01D71/64 , B01D53/22
CPC分类号： B01D53/228 , B01D67/0006 , B01D67/0093 , B01D69/02 , B01D69/06 , B01D69/125 , B01D71/64 , B01D71/68 , B01D2256/16 , B01D2256/245 , B01D2257/108 , B01D2257/504 , B01D2323/12 , B01D2323/30 , B01D2323/345 , B01D2325/022 , B01D2325/04 , Y02C10/10 , Y02C20/20
摘要： An asymmetric integrally-skinned flat sheet membrane comprising a miscible blend of an aromatic polyethersulfone (PES) polymer and an aromatic polyimide polymer is used for gas separations such as hydrogen purification, separation of hydrogen and methane and to separate other gases and liquids. UV radiation may be applied to the surface of the membrane for improved properties.
摘要翻译：包含芳族聚醚砜（PES）聚合物和芳族聚酰亚胺聚合物的可混溶共混物的不对称整体剥离的平片膜用于气体分离，例如氢气净化，氢气和甲烷的分离以及分离其它气体和液体。 UV辐射可以施加到膜的表面以获得改进的性能。

7. 发明申请

WO2015153117A1 NANOPOROUS MACROCYCLE-CONTAINING CROSS-LINKED POLYMERIC MEMBRANES FOR SEPARATIONS 审中-公开
标题翻译：用于分离的含有纳米聚合物的交联聚合物膜
公开(公告)号：WO2015153117A1
公开(公告)日：2015-10-08
申请号：PCT/US2015/021152
申请日：2015-03-18
申请人： UOP LLC
发明人： LIU, Chunqing , TRAN, Howie, Q. , KARNS, Nicole, K. , BOWEN, Travis, C.
IPC分类号： C08L67/06 , C08L71/00 , C08K5/103 , C08J5/18
CPC分类号： B01D53/228 , B01D69/125 , B01D71/54 , B01D71/58 , B01D2053/221 , B01D2256/24 , B01D2256/245 , B01D2257/504 , B01D2257/702 , B01D2257/7027 , B01D2323/30 , B01D2325/20 , C08G18/42 , C08G18/48 , C08G18/6484 , C08J9/286 , C08J9/365 , C08J2201/026 , C08J2201/0502 , C08J2375/04 , C10L3/101 , Y02C10/10 , Y02P20/152 , C08G18/10 , C08G18/64
摘要： The present invention involves a type of nanoporous macrocycle-containing cross-linked polymeric membrane, a method of making the membrane, and the use of such a novel membrane system for natural gas liquids (NGL) recovery, fuel gas conditioning, natural gas pre-treatment, sulfur removal from fluidized catalytic cracking (FCC) and other naphtha streams, as well as aromatic separations such as aromatic/paraffin separation and xylene separation. The nanoporous macrocycle-containing cross-linked polymeric membrane is prepared from a diisocyanate-terminated polyether or a diisocyanate-terminated polyester, that is crosslinked with a nanoporous macrocycle comprising hydroxyl functional groups such as α-, β-, and γ- cyclodextrins.
摘要翻译：本发明涉及一种纳米多孔大环交联聚合物膜，一种制备该膜的方法，以及使用这种新型天然气液体（NGL）回收膜系统，燃料气体调节剂，天然气预处理剂，处理，从流化催化裂化（FCC）和其他石脑油流中除去硫，以及芳族分离，如芳烃/石蜡分离和二甲苯分离。含有纳米多孔大环的交联聚合物膜由二异氰酸酯封端的聚醚或二异氰酸酯封端的聚酯制备，其与包含羟基官能团如α-，β-和γ-环糊精的纳米多孔大环交联。

8. 发明申请

WO2015088844A1 GAS SEPARATION MEMBRANES FROM CHEMICALLY AND UV TREATED POLYMERS OF INTRINSIC MICROPOROSITY 审中-公开
标题翻译：内在微生物化学和紫外线处理聚合物气体分离膜
公开(公告)号：WO2015088844A1
公开(公告)日：2015-06-18
申请号：PCT/US2014/068261
申请日：2014-12-03
申请人： UOP LLC
发明人： LISKEY, Carl W. , HAMOY, Michael B. , LIU, Chunqing
IPC分类号： B01D71/00
CPC分类号： B01D67/0006 , B01D53/228 , B01D71/52 , B01D71/82 , B01D2256/245 , B01D2257/504 , B01D2323/30 , B01D2323/345 , B01D2323/36 , B01D2325/02 , Y02C10/10
摘要： The invention is a process of making a chemically and UV treated polymer of intrinsic microporosity membrane comprising preparing a polymer of intrinsic microporosity, chemically cross-linking said polymer of intrinsic microporosity with a cross-linking compound to produce a chemically cross-linked polymer of intrinsic microporosity and then treating said chemically cross-linked polymer with UV radiation for a period of time sufficient to provide a product membrane. This product membrane is useful in the separation of C3 and higher hydrocarbons, as well as CO 2 , from natural gas and other gas streams.
摘要翻译：本发明是制备本征微孔膜的化学和UV处理的聚合物的方法，包括制备本征微孔的聚合物，与所述交联化合物化学交联所述本征微孔的聚合物以产生本征的化学交联聚合物微孔，然后用UV辐射处理所述化学交联的聚合物足以提供产物膜的时间。该产品膜可用于从天然气和其他气体流中分离C3和更高级烃以及二氧化碳。

9. 发明申请

WO2014014627A1 METHODS AND APPARATUSES FOR GENERATING NITROGEN 审中-公开
标题翻译：用于产生氮的方法和装置
公开(公告)号：WO2014014627A1
公开(公告)日：2014-01-23
申请号：PCT/US2013/047574
申请日：2013-06-25
申请人： UOP LLC
发明人： ZHOU, Lubo , LIU, Chunqing , SCHOTT, Mark E. , GREER, David W.
IPC分类号： B01D53/74 , B01D53/54
CPC分类号： B01D53/265 , B01D53/229 , B01D2256/10 , B01D2257/504 , B01D2257/80 , B01D2258/0283 , Y02C10/10
摘要： Embodiments of methods and apparatuses for generating nitrogen are provided. In one example, a method comprises the steps of contacting at least a portion of a flue gas stream with a CO 2 /N 2 separation membrane at conditions effective to form a N 2 -rich retentate stream and a CO 2 -rich permeate stream. Liquid hydrocarbons are covered with the N2-rich retentate stream to form a blanket of nitrogen.
摘要翻译：提供了用于产生氮气的方法和装置的实施例。在一个实例中，方法包括以下步骤：在有效形成富N2的滞留物流和富二氧化碳的渗透物流的条件下使至少一部分烟道气流与CO 2 / N 2分离膜接触。用富氮的滞留物流覆盖液体烃以形成氮气覆盖层。

10. 发明申请

WO2012082537A2 MEMBRANE SYSTEM FOR NATURAL GAS UPGRADING 审中-公开
标题翻译：用于天然气升级的膜系统
公开(公告)号：WO2012082537A2
公开(公告)日：2012-06-21
申请号：PCT/US2011/064084
申请日：2011-12-09
申请人： UOP LLC , LIU, Chunqing , FAHEEM, Syed A. , MINKOV, Raisa
发明人： LIU, Chunqing , FAHEEM, Syed A. , MINKOV, Raisa
IPC分类号： B01D53/62 , B01D71/06 , C10L3/12
CPC分类号： C10L3/104 , B01D53/22 , B01D2256/245 , B01D2257/504 , C10L3/101 , Y02C10/04 , Y02C10/10
摘要： The present invention involves the use of a novel membrane system for natural gas upgrading. This membrane system includes a first-stage membrane such as a membrane prepared from the polymer of intrinsic microporosity (PIM) to selectively remove hydrocarbons from C 3 to C 35 to control the dew point of natural gas, and a second-stage membrane such as a polybenzoxazole (PBO) or crosslinked PBO membrane to selectively remove CO 2 from natural gas. The new membrane system described in the current invention eliminates the use of high cost and high footprint membrane pretreatment. Therefore, the membrane system can significantly reduce the footprint and cost for natural gas upgrading compared to the current commercially available membrane systems that include a non-membrane-related pretreatment system.
摘要翻译：本发明涉及使用用于天然气升级的新型膜系统。该膜系统包括第一阶段膜，例如由固有微孔性聚合物（PIM）制备的膜，以选择性地从C35到C35去除烃以控制天然气的露点，以及第二阶段膜如聚苯并恶唑（PBO）或交联的PBO膜以选择性地从天然气中除去CO 2。本发明中描述的新膜系统消除了使用高成本和高占位面积的膜预处理。因此，与包括非膜相关预处理系统的当前市售膜系统相比，膜系统可以显着减少天然气提质的占地面积和成本。

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