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1. 发明申请

WO0074827A3 COMPOSITES AND COMPOSITE MEMBRANES 审中-公开
标题翻译：复合膜和复合膜
公开(公告)号：WO0074827A3
公开(公告)日：2001-03-29
申请号：PCT/EP0003910
申请日：2000-05-02
申请人： UNIV STUTTGART INST FUER CHEMI , KERRES JOCHEN , HAERING THOMAS , ULLRICH ANDREAS
发明人： KERRES JOCHEN , HAERING THOMAS , ULLRICH ANDREAS
IPC分类号： B01D53/22 , B01D61/02 , B01D61/14 , B01D61/24 , B01D61/36 , B01D69/12 , B01D69/14 , B01D71/00 , B01D71/02 , B01D71/62 , B01D71/66 , B01D71/68 , B01J21/16 , B01J31/06 , B01J31/10 , B01J35/06 , C01B33/38 , C01B33/44 , C08J5/20 , C08J5/22 , C08K3/34 , C08L101/02 , H01M8/02 , H01M8/10
CPC分类号： B01D67/0041 , B01D69/141 , B01D71/00 , B01D71/024 , B01D71/62 , B01D71/68 , B01D2325/18 , B01D2325/26 , B01J21/16 , B01J31/10 , B01J31/1633 , B01J35/065 , C08J5/2275 , C08J2383/02 , H01M8/0289 , H01M8/1023 , H01M8/103 , H01M8/1032 , H01M8/1051 , H01M8/1081 , Y02E60/523 , Y02P70/56 , Y10T428/249953 , Y10T428/249969
摘要： The invention relates to a composite or a composite membrane consisting of an ionomer and of an inorganic optionally functionalized phyllosilicate. The isomer can be: (a) a cation exchanger polymer; (b) an anion exchanger polymer; (c) a polymer containing both anion exchanger groupings as well as cation exchanger groupings on the polymer chain; (d) a blend consisting of (a) and (b), whereby the mixture ratio can range from 100 % (a) to 100 % (b). The blend can be ionically and even covalently cross-linked. The inorganic constituents can be selected from the group of the phyllosilicates or tectosilicates. The use of bentonites and zeolites are generally preferred in special montomorillonite. The mixture ratio isomer:bentonite ranges from 99:1 to 30:70. The invention also relates to the application of the composites/composite membranes: as proton conductors in membrane fuel cells (H2 fuel cells PEFC, direct methanol fuel cells DMFC) at temperatures greater than 100 DEG C; in (electro)membrane separation methods such as dialysis, diffusion dialysis, gas separation, pervaporation, perstraction and in microfiltration and ultrafiltration, particularly due to their antifouling properties, and; as catalytic membranes in catalytic membrane reactors.
摘要翻译：本发明是一种复合材料或离子交联聚合物的复合膜和无机任选地官能层状硅酸盐。在此，离聚物可以是：（a）一种阳离子交换聚合物; （B）阴离子交换聚合物; （C）含有聚合物链上的两个阴离子交换剂和Kationenaustauschergruppierungen的聚合物; （D）的范围可以的共混物（a）和（b）中，其特征在于，100％的混合比（A）100％（B）。该共混物可以是离子，甚至共价交联。选自片岩或框架硅酸盐的无机组分可以是。一般而言，膨润土和沸石，优选特别是蒙脱石。混合比离聚物/膨润土的范围为99/1至30/70。此外，本发明的主题，复合材料/复合膜的应用：如在膜燃料电池中的温度范围高于100℃的质子导体（H2-燃料PEFC，直接甲醇燃料电池DMFC）; 在因为它们的防污性的（电）的膜分离过程，例如透析，扩散渗析，气体分离，全蒸发，渗透萃取和在微滤和超滤，特别; 如在催化膜反应器的催化膜。

2. 发明申请

WO03022892A2 OLIGOMERS AND POLYMERS CONTAINING SULFONITE GROUPS AND METHOD FOR THE PRODUCTION THEREOF 审中-公开
标题翻译：亚磺酸酯的低聚物和含聚合物及其制造方法
公开(公告)号：WO03022892A2
公开(公告)日：2003-03-20
申请号：PCT/DE0203260
申请日：2002-09-02
申请人： UNIV STUTTGART INST FUER CHEMI , HAERING THOMAS , KERRES JOCHEN , ZHANG WEI
发明人： HAERING THOMAS , KERRES JOCHEN , ZHANG WEI
IPC分类号： B01D53/22 , B01D61/36 , B01D71/82 , C08C19/02 , C08F8/04 , C08G85/00 , C08J5/22 , H01B1/06 , H01B13/00 , H01M6/18 , H01M8/02 , H01M8/10 , H01M10/40
CPC分类号： H01M6/181 , C08C19/02 , C08F8/04 , C08J5/2243 , C08J2381/00 , H01M8/1023 , H01M8/1025 , H01M8/1027 , H01M8/103 , H01M8/1032 , H01M8/1039 , H01M8/1072 , Y02P70/56
摘要： The invention relates to novel polymers or oligomers containing at least sulfonite groups (P-(SO2)nX, X=1-(n=1), 2-(n=2) or 3-(n=3) valent metal cation or H or ammonium ion NR4 where R=alkyl, aryl, H), which are obtained by completely or partially reducing polymers or oligomers containing at least SO2Y-groups (Y=F, C1, Br, I, OR, NR2 (R=alkyl and/or aryl and/or H), N-imidazolyl, N-pyrazolyl) by means of suitable reducing agents in a suspension or in a solution form. The invention also relates to polymers and polymer(blend) membranes which are obtained by further reacting the obtained sulfinated polymers, especially by alkylation of the sulfinate groups with mono- di- or oligo functional electrophiles. The invention further relates to methods for producing the sulfinated polymers and for further reacting the sulfinated polymers with electrophiles by S-alkylation.
摘要翻译：本发明包括新颖的（亚磺酸酯与至少P-（SO 2）N X，X = 1-（N = 1），2-（N = 2）或3（N = 3）价的金属阳离子或H <+>或铵离子NR4 <+> R =烷基，含有聚合物或它们获得的低聚物（由完全或部分减少至少SO2Y基团Y = F，C1，溴，I，OR，NR 2（R =烷基和芳基，H）/ 或芳基和/或H），N-咪唑，N-吡唑基）通过在悬浮液中或在溶液中适当的还原剂是指含有聚合物或低聚物。和聚合物和聚合物（共混物）的要求保护的隔膜，其由所得到的亚磺酸化的聚合物的进一步的反应通过烷基化与单 - ，二 - 或寡官能的亲电试剂的亚磺酸酯基团获得的，特别是。以及用于制备聚合物和亚磺酸化，用于通过S-烷基化亚磺化亲电的聚合物的进一步的反应方法要求保护。

3. 发明申请

WO2007101415A3 PHOSPHONIC ACID-CONTAINING BLENDS AND PHOSPHONIC ACID-CONTAINING POLYMERS 审中-公开
标题翻译：含膦酸的共混物和含膦酸的聚合物
公开(公告)号：WO2007101415A3
公开(公告)日：2007-12-21
申请号：PCT/DE2007000260
申请日：2007-02-05
申请人： UNIV STUTTGART INST FUER CHEMI , HAERING THOMAS , KERRES JOCHEN , SCHOENBERGER FRANK , HEIN MARTIN
发明人： HAERING THOMAS , KERRES JOCHEN , SCHOENBERGER FRANK , HEIN MARTIN
IPC分类号： C08J5/00 , C08G61/00 , C08G65/00 , C08G75/00 , C08G79/00 , C08J5/20 , C08J5/22 , C08L61/00 , C08L71/00 , H01M8/00 , H01M8/10
CPC分类号： H01M8/1034 , B01J39/20 , C08G61/02 , C08G61/122 , C08J5/2287 , C08J2341/00 , H01M8/1011 , H01M8/1023 , H01M8/1025 , H01M8/1027 , H01M8/103 , H01M8/1032 , H01M8/1039 , H01M8/1044 , H01M8/1048 , H01M8/1072 , H01M2008/1095 , H01M2300/0082 , Y02E60/522 , Y02E60/523 , Y02P70/56
摘要： The invention relates to blends and blend membranes from low-molecular hydroxymethylene-oligo-phosphonic acids R-C(PO 3 H 2 ) x (OH) y and polymers, the group R representing any organic group and the polymers containing the following functional groups: cation exchanger groups or their nonionic precursors of the type SO 2 X, X = HaI, OH, OMe, NR 1 R 2 , OR 1 with Me = any metal cation or ammonium cation, R 1 , R 2 = H or any aryl- or alkyl group, POX 2 , COX and/or basic groups such as primary, secondary or tertiary amino groups, imidazole groups, pyridine groups, pyrazole groups etc. and/or OH groups. Low molecular hydroxymethylene-oligo-phosphonic acids R-C(PO 3 H 2 ) x (OH) y are preferred in which x = 2 and y = 1. The invention also relates to low-molecular hydroxymethylene-oligo-phosphonic acids R-C(PO 3 H 2 ) 2 (OH) 1 and polymers, wherein the group R of the hydroxymethylene-oligophosphonic acid contains an aliphatic or aromatic basic group which ionically interacts with the acidic groups of the polymer or of the polymer mixture. The invention further relates to blends and blend membranes from low-molecular hydroxymethylene-oligo-phosphonic acids R-C(PO 3 H 2 ) 2 (OH) 1 and polymers, wherein the OH groups of the low-molecular hydroxymethylene-1,1-bisphosphonic acid are covalently cross-linked with each other or optionally with OH groups of the polymer. The invention also relates to polymers that are modified with the 1-hydroxymethylene-1,1-bisphosphonic acid group. The polymers are produced by reacting polymers which contain carboxylic acid groups or carboxylic halide groups -COHal (Hal=F, Cl, Br, I) with phosphite compounds or by reacting polymeric aldehydes or polymeric keto compounds with phosphite esters while carrying out an amine catalysis, an oxidation of the intermediary hydroxyphosphonic acid with MnO 2 or any other oxidant. The invention finally relates to methods for producing the aforementioned materials and to the use of membranes of the aforementioned materials in membrane processes and especially in fuel cells, even at temperatures of >100°C.
摘要翻译：在本发明中，将以下材料都声称：1.共混物和共混物的低分子量的羟基亚甲基的膜低聚膦酸RC（PO _{3 ħ_{2 ）×（OH）_{ÿ< / SUB>和的聚合物，其中R是任何有机基团和所述聚合物包含以下的官能团：阳离子交换基团或类型的它们的非离子母体SO _{2 X，X =哈尔，OH，OME，NO _{1 - [R _{2 或_{1 我=任何金属阳离子或铵阳离子，R _{1 ，R _{2 = H或任何的芳基或烷基，POX _{2 ，COX和/或碱性基团，例如伯，仲或叔氨基，咪唑基，吡啶基，吡唑等，和/或OH基团，这里将低分子量羟基亚低聚膦酸RC（PO _{3 ħ_{2 ）×（OH）_{ý是优选的，其中x = 2和y = 1。 2.共混物和共混物的低分子量的羟基亚甲基的膜低聚膦酸RC（PO _{3 ħ_{2 ）_{2 （OH）_{1 和聚合物，其中所述羟基亚甲基的基团ROligophosphonsäure包含其经历与聚合物或聚合物共混物的酸性基团的离子相互作用的脂族或芳族碱性部分。 3.共混物和共混物的低分子量的羟基亚甲基的膜低聚膦酸RC（PO _{3 ħ_{2 ）_{2 （OH）_{1 和聚合物，其中，低分子1-羟基亚甲基-1,1-二膦酸的OH基团被交联彼此并任选地与该聚合物的OH基团共价结合。 4.用1-羟基亚甲基-1,1-二膦酸改性的聚合物，它们是由含羧酸基团或羧酸卤基团-COHal（HAL = F，氯，溴，I）的聚合物的反应制备，其中亚磷酸酯化合物或通过反应聚合醛或与下胺催化亚磷酸，中间Hydroxyphosphonsäure的氧化与MnO的_{2 或其他氧化剂聚合酮基化合物。还要求保护的方法用于上述材料的制备和使用上述材料中的膜分离过程的膜，特别是在燃料电池中，甚至在> 100℃的温度下}}}}}}}}}}}}}}}}}}}}}}

4. 发明申请

WO0074827A8 COMPOSITES AND COMPOSITE MEMBRANES 审中-公开
标题翻译：复合膜和复合膜
公开(公告)号：WO0074827A8
公开(公告)日：2002-01-24
申请号：PCT/EP0003910
申请日：2000-05-02
申请人： HAERING THOMAS , HAERING RIMA , KERRES JOCHEN
发明人： HAERING THOMAS , HAERING RIMA , KERRES JOCHEN
IPC分类号： B01D53/22 , B01D61/02 , B01D61/14 , B01D61/24 , B01D61/36 , B01D69/12 , B01D69/14 , B01D71/00 , B01D71/02 , B01D71/62 , B01D71/66 , B01D71/68 , B01J21/16 , B01J31/06 , B01J31/10 , B01J35/06 , C01B33/38 , C01B33/44 , C08J5/20 , C08J5/22 , C08K3/34 , C08L101/02 , H01M8/02 , H01M8/10
CPC分类号： B01D67/0041 , B01D69/141 , B01D71/00 , B01D71/024 , B01D71/62 , B01D71/68 , B01D2325/18 , B01D2325/26 , B01J21/16 , B01J31/10 , B01J31/1633 , B01J35/065 , C08J5/2275 , C08J2383/02 , H01M8/0289 , H01M8/1023 , H01M8/103 , H01M8/1032 , H01M8/1051 , H01M8/1081 , Y02E60/523 , Y02P70/56 , Y10T428/249953 , Y10T428/249969
摘要： The invention relates to a composite or a composite membrane consisting of an ionomer and of an inorganic optionally functionalized phyllosilicate. The isomer can be: (a) a cation exchanger polymer; (b) an anion exchanger polymer; (c) a polymer containing both anion exchanger groupings as well as cation exchanger groupings on the polymer chain; (d) a blend consisting of (a) and (b), whereby the mixture ratio can range from 100 % (a) to 100 % (b). The blend can be ionically and even covalently cross-linked. The inorganic constituents can be selected from the group of the phyllosilicates or tectosilicates. The use of bentonites and zeolites are generally preferred in special montomorillonite. The mixture ratio isomer:bentonite ranges from 99:1 to 30:70. The invention also relates to the application of the composites/composite membranes: as proton conductors in membrane fuel cells (H2 fuel cells PEFC, direct methanol fuel cells DMFC) at temperatures greater than 100 DEG C; in (electro)membrane separation methods such as dialysis, diffusion dialysis, gas separation, pervaporation, perstraction and in microfiltration and ultrafiltration, particularly due to their antifouling properties, and; as catalytic membranes in catalytic membrane reactors.
摘要翻译：本发明是一种复合材料或离子交联聚合物的复合膜和无机任选地官能层状硅酸盐。在此，离聚物可以是：（a）一种阳离子交换聚合物; （B）阴离子交换聚合物; （C）含有聚合物链上的两个阴离子交换剂和Kationenaustauschergruppierungen的聚合物; （D）的范围可以的共混物（a）和（b）中，其特征在于，100％的混合比（A）100％（B）。该共混物可以是离子，甚至共价交联。选自片岩或框架硅酸盐的无机组分可以是。一般而言，膨润土和沸石，优选特别是蒙脱石。混合比离聚物/膨润土的范围为99/1至30/70。此外，本发明的主题，复合材料/复合膜的应用：如在膜燃料电池中的温度范围高于100℃的质子导体（H2-燃料PEFC，直接甲醇燃料电池DMFC）; 在因为它们的防污性的（电）的膜分离过程，例如透析，扩散渗析，气体分离，全蒸发，渗透萃取和在微滤和超滤，特别; 如在催化膜反应器的催化膜。

5. 发明申请

WO9954407A3 ENGINEERING IONOMERIC BLENDS AND ENGINEERING IONOMERIC BLEND MEMBRANES 审中-公开
标题翻译：工程与工程离子交联聚合物共混物，IONOMERBLENDMEMBRANEN
公开(公告)号：WO9954407A3
公开(公告)日：2000-03-09
申请号：PCT/EP9902755
申请日：1999-04-16
申请人： UNIV STUTTGART , KERRES JOCHEN , ULRICH ANDREAS , HAERING THOMAS
发明人： KERRES JOCHEN , ULRICH ANDREAS , HAERING THOMAS
IPC分类号： B01D71/52 , B01D71/62 , B01D71/66 , B01D71/68 , B01D71/72 , B01D71/80 , C08G65/48 , C08G73/06 , C08J5/22 , C08L71/00 , C08L71/10 , C08L79/04 , C08L79/06 , C08L81/06 , H01M8/02 , H01M8/10
CPC分类号： H01M8/103 , B01D71/52 , B01D71/62 , B01D71/66 , B01D71/68 , C08G65/48 , C08L71/00 , C08L79/04 , H01M8/1025 , H01M8/1032 , H01M8/1044 , Y02P70/56 , C08L2666/20 , C08L2666/14
摘要： The invention relates to novel compatible binary and tertiary cation exchange polymer and anion exchange polymer acid base blend membranes.
摘要翻译：本发明涉及新的兼容二元和三元Kationenaustauscherpolymer-和阴离子交换聚合物酸基共混物膜。

6. 发明申请

WO2006018020A3 IONOMERS WITH IONOGENIC GROUPS IN THE SIDECHAIN 审中-公开
标题翻译：离聚物侧链离子型组
公开(公告)号：WO2006018020A3
公开(公告)日：2006-05-18
申请号：PCT/DE2005001504
申请日：2005-08-20
申请人： UNIV STUTTGART , HAERING THOMAS , KERRES JOCHEN , HEIN MARTIN
发明人： HAERING THOMAS , KERRES JOCHEN , HEIN MARTIN
IPC分类号： B01D71/68 , B01D71/54 , B01D71/66
CPC分类号： B01J39/185 , B01D67/0006 , B01D67/0093 , B01D71/68 , B01D71/82 , B01D2325/16 , B01J39/19 , C08G65/48 , C08G75/0286 , C08J5/2231 , C08J5/2256 , C08J2365/02 , C08J2381/06 , H01M8/0289 , H01M8/1023 , H01M8/1025 , H01M8/1027 , H01M8/103 , H01M8/1032 , H01M8/1039 , H01M8/1072 , H01M2300/0082 , Y02E60/523 , Y02P70/56
摘要： The invention relates to ionomeric membranes, comprising a non- or partly-fluorinated, non-, partly- or fully-aromatic backbone and a non- or partly-fluorinated sidechain with ionogenic groups, or the non-ionic precursors thereof and a method for production of said ionomeric membranes.
摘要翻译：要求保护的是： - 用于产生上述离子交联聚合物的过程 - 包括非或部分氟化的非的，部分或完全芳族主链和具有离子基团或它们的非离子型前体的非或部分氟化的侧链离聚物膜。

7. 发明申请

WO0200773A9 POLYMERS AND POLYMER MEMBRANES COVALENTLY CROSS-LINKED BY SULPHINATE ALKYLATION 审中-公开
标题翻译：共价交联聚合物和聚合物膜材料VIA SULFINATALKYLIERUNG
公开(公告)号：WO0200773A9
公开(公告)日：2003-02-13
申请号：PCT/EP0105826
申请日：2001-05-21
申请人： UNIV STUTTGART , KERRES JOCHEN , ZHANG WEI , TANG CHY-MING , HAERING THOMAS
发明人： KERRES JOCHEN , ZHANG WEI , TANG CHY-MING , HAERING THOMAS
IPC分类号： B01D53/22 , B01D61/02 , B01D61/24 , B01D61/36 , B01D61/42 , B01D67/00 , B01D71/52 , B01D71/66 , B01D71/68 , B01D71/82 , C08G75/00 , C08G81/00 , C08J5/18 , C08L87/00 , C25B13/08 , H01M2/16 , H01M8/02 , H01M8/10 , H01M10/052 , H01M10/0565 , C08J5/22 , B01D71/06 , H01B1/12
CPC分类号： B01D67/0093 , B01D53/228 , B01D71/52 , B01D71/68 , B01D71/82 , B01D2323/30 , C08G75/00 , H01M2/1653 , H01M8/1025 , H01M8/1027 , H01M8/1032 , H01M8/1044 , H01M8/1072 , H01M8/1081 , H01M8/1086 , H01M10/052 , H01M10/0565 , H01M2300/0082 , Y02P70/56
摘要： The invention relates to a covalently cross-linked polymer or polymer membrane consisting of one or more polymers, which can bear the following functional groups (M=Hal (F, Cl, Br, I), OR, NR2; R=alkyl, hydroxyalkyl, aryl; (Me=H, Li, Na, K, Cs, or other metal cations or ammonium ions); a) precursors of cation exchange groups: SO2M and/or POM2 and/or COM b) sulphinate groups SO2Me and which can be covalently cross-linked using the following organic compounds: a) di, tri or oligofunctional haloalkanes or haloaromatics, which have been reacted with sulphinate groups SO2Me, whereby the following cross-linking bridges are present in the polymer/in the polymer blend/in the polymer membrane (Y=cross-linking bridges, X=Hal (F, Cl, Br, I), OR, Y=(CH2)x-; -arylene-; -(CH2)x-arylene-; CH2arylene-CH2-, x=3-12): polymer-SO2Y-SO2-polymer and/or b) compounds containing the following groups: Hal-(CH2)x-NHR, one side of which (Hal-) has been reacted with sulphinate groups SO2ME and the other side (-NHR) with SO2M groups, whereby the following cross-linking bridges are present in the polymer/in the polymer blend/in the polymer membrane: polymer-SO2-(CH2)x-NR-SO2-polymer and/or c) compounds containing the following groups: NHR-(CH2)x)-NHR, which have been reacted with sulphinate groups SO2Me, whereby the following cross-linking bridges are present in the polymer/in the polymer blend/in the polymer membrane: polymer-SO2-NR-(CH2)x-NR-SO2-polymer.
摘要翻译：共价交联的聚合物或共价交联的聚合物膜由一种或多种聚合物，其可以携带下列的官能团（M =哈尔（F，氯，溴，I），OR，NR 2; R =烷基，羟烷基，芳基（ME = H，锂，钠，钾，铯，或其它金属阳离子或铵离子）;一）阳离子交换基团的前体：SO 2 M和/或POM2和/或COM; b）中的亚磺酸SO2Me，并且其可通过以下的有机化合物的装置被共价交联的：1）二，三或寡官能的卤代烷烃或芳族卤素化合物，已被接触用亚磺酸盐SO2Me到反应中，其中聚合物/聚合物共混物/聚合物膜下面的交联桥本（Y =交联桥，X =哈尔（F，氯，溴，I），OR，Y = - （CH 2）x - ;亚芳基， - （CH 2）x - 亚芳基; CH2Arylen-CH 2 - ，X = 3-12）：聚合物-SO2-Y-SO 2 - 聚合物和/或b）包含以下基团的化合物：Hal-（CH 2）x-NHR，其中（在一侧Hal-）与亚磺酸盐反应SO2Me 过，并且在另一侧（-NHR）与SO 2 M基团，其是存在于聚合物/聚合物共混物/在以下的交联桥的聚合物膜：聚合物-SO 2 - （CH 2）x-NR-SO2-聚合物和/或c ）包含以下基团的化合物：NHR（CH 2）x-NHR，已被接触用SO2Me基团进行反应，由此，聚合物/在POLYM erblend /在聚合物膜的交联以下桥都存在：聚合物-SO 2 NR-（CH 2）x-NR-SO2-聚合物。

8. 发明申请

WO2007031076A3 ELECTROLYTE 审中-公开
标题翻译： ELEKTROLYT
公开(公告)号：WO2007031076A3
公开(公告)日：2007-07-26
申请号：PCT/DE2006001646
申请日：2006-09-14
申请人： HAERING THOMAS
发明人： HAERING THOMAS
IPC分类号： H01M8/10 , H01M8/00
CPC分类号： B01D67/0088 , B01D67/0079 , B01D69/148 , B01D71/02 , B01D71/62 , B01D2325/26 , H01M8/1027 , H01M8/103 , H01M8/1044 , H01M8/1048 , H01M8/1081 , H01M2300/0082 , H01M2300/0091 , Y02P70/56
摘要： The invention relates to membranes made from polybenzimidazole, doped with low-molecular-weight phosphonic acids and optionally with phosphoric acids. Membranes, doped with phosphoric acid and an aminophosphonic acid have an increased proton conductivity with relation to doping with only one of the components.
摘要翻译：本发明涉及用低分子量膦酸和任选磷酸掺杂的聚苯并咪唑的膜。掺杂有磷酸和氨基膦酸的膜与仅用两种组分中的一种掺杂相比具有更高的质子传导性。

9. 发明申请

WO2007082526A3 ELECTROLYTE CONTAINING PHOSPHONIC ACID 审中-公开
标题翻译： PHOSPHONSÄUREHALTIGERELEKTROLYT
公开(公告)号：WO2007082526A3
公开(公告)日：2008-01-24
申请号：PCT/DE2007000133
申请日：2007-01-23
申请人： BETWEEN LIZENZ GMBH , HAERING THOMAS
发明人： HAERING THOMAS
IPC分类号： H01M8/02 , B01D67/00 , B01D71/52 , B01D71/68 , C08J5/22 , H01M8/10
CPC分类号： H01M8/0291 , B01D71/82 , C08J3/091 , C08J5/2256 , C08J2371/10 , H01M8/0289 , H01M8/1039 , H01M8/1048 , H01M8/1072 , H01M8/1081 , Y02E60/523 , Y02P70/56
摘要： A method is disclosed for production of solutions of aminophosphonic acids and polymeric sulphonic acids in aprotic solvents. Membranes for membrane methodologies are produced from said solutions. Said membranes can also be doped with phosphoric acid.
摘要翻译：提供了一种用于碱性或低分子量膦酸和中所述的非质子溶剂的磺化聚合物溶液的制备方法。从这些解决方案，膜准备FTIR膜过程。这些膜可以另外用磷酸掺杂的爱好。

10. 发明申请

WO03050169A3 COVALENTLY CROSS-LINKED COMPOSITE MEMBRANES 审中-公开
标题翻译：共价交联的复合膜
公开(公告)号：WO03050169A3
公开(公告)日：2003-08-21
申请号：PCT/DE0204173
申请日：2002-11-04
申请人： HAERING THOMAS
发明人： HAERING THOMAS
IPC分类号： C08J5/22 , B01D71/68 , H01M8/02 , H01M8/10
CPC分类号： C08J5/2275 , C08J2371/12 , C08J2381/06
摘要： The invention relates to a covalently cross-linked composite and a covalently cross-linked composite polymer membrane consisting of at least one polymer and tectosilicates and/or phyllosilicates. Said tectosilicates and/or phyllosilicates can be both functionalised or non-functionalised. The polymers are characterised in that they can carry the following functional groups (M=Hal (F, Cl, Br, I), OR, NR2; R=alkyl, hydroxyalkyl, aryl; (Me=H, Li, Na, K, Cs or other metal cations or ammonium ions): a) precursors of cation exchanger groups SO2M and/or POM2 and/or COM, and b) sulfinate groups SO2Me; and can be covalently cross-linked by means of the following organic compounds: a) difunctional, trifunctional or oligofunctional haloalkanes or haloaromatics which have been reacted with the sulfinate groups SO2Me, whereby the following cross-linking bridges are present in the polymer/in the polymer blend/in the polymer membrane (Y=cross-linking bridges, X=Hal (F, Cl, Br, I), OR, Y=-(CH2)x-; -arylene-; -(CH2)x-arylene-; CH2-arylene-CH2-, x=3-12): polymer-SO2-Y-SO2-polymer; and/or b) compounds containing the groups Hal-(CH2)x-NHR, one side (Hal-) thereof having been reacted with sulfinate groups SO2Me, and the other side (-NHR) having been reacted with SO2Me groups, whereby the following cross-linking bridges are present in the polymer/in the polymer mixture/in the polymer membrane: polymer-SO2-(CH2)x-NR-SO2-polymer; and/or c) compounds containing the groups NHR-(CH2)x-NHR which have been reacted with the SO2Me groups, whereby the following cross-linking bridges are present in the polymer/in the polymer mixture/in the polymer membrane: polymer-SO2-NR-(CH2)x-NR-SO2-polymer.
摘要翻译：本发明涉及共价交联的复合材料和包括一种或多种聚合物和支架共价交联的复合聚合物膜，和/或层状硅酸盐。脚手架和/或层状硅酸盐既可以官能化和本发明的非官能化。该聚合物的特征在于它们可以携带以下的官能团（M =哈尔（F，氯，溴，I），OR，NR 2; R =烷基，羟烷基，芳基（ME = H，锂，钠，钾，铯或其它金属阳离子或铵离子）：三 - 一）二 - 或寡官能的卤代烷或卤代芳族：1）阳离子交换基团的前体：SO 2 M和/或POM2和/或COM b）亚磺酸盐SO2Me，并且其可通过以下的有机化合物的装置被共价交联这已经带来了与亚磺酸盐SO2Me到反应中，从而存在于聚合物/聚合物共混物/聚合物膜下面的交联桥（Y =交联桥，X =哈尔（F，氯，溴，I），OR，Y = - （CH 2 ）×;亚芳基 - （CH 2）X - 亚芳基; CH2-CH2-亚芳基，X = 3-12）; 聚合物-SO2-Y-SO 2 - 聚合物和/或b）包含以下基团的化合物：Hal-（CH 2）x-NHR，其中（在一侧Hal-）与亚磺酸盐SO2Me到反应反应，和的另一侧（-NHR）与SO2Me基团，由此，下面的交联桥存在于聚合物/聚合物共混物/聚合物膜：聚合物-SO 2 - （CH 2）x-NR-SO2-聚合物和/或c）的化合物，以下包含基团：NHR（CH 2）x-NHR，已被接触用SO2Me基团进行反应，从而使下述的交联桥存在于聚合物/聚合物共混物/聚合物膜：聚合物-SO 2 NR-（CH 2）x NR -SO 2聚合物。

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