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1. 发明申请

WO2008070059A2 SEPARATION OF ELECTROLYTES 审中-公开
标题翻译：电解质的分离
公开(公告)号：WO2008070059A2
公开(公告)日：2008-06-12
申请号：PCT/US2007024805
申请日：2007-12-04
申请人： SION POWER CORP , MIKHAYLIK YURIY V , BURGESS CATHIE , KOVALEV IGOR , SCORDILIS-KELLEY CHARICLEA
发明人： MIKHAYLIK YURIY V , BURGESS CATHIE , KOVALEV IGOR , SCORDILIS-KELLEY CHARICLEA
IPC分类号： H01M2/16 , H01M4/02 , H01M4/134 , H01M4/136 , H01M4/1395 , H01M10/0565 , H01M10/0566
CPC分类号： H01M10/0569 , H01M2/1653 , H01M4/134 , H01M4/136 , H01M4/1395 , H01M10/0525 , H01M10/0565 , H01M10/0566 , H01M2300/0085 , H01M2300/0094 , H02J7/0068 , Y10T29/49115
摘要： Methods and articles relating to separation of electrolyte compositions within lithium batteries are provided. The lithium batteries described herein may include an anode having lithium as the active anode species and a cathode having sulfur as the active cathode species. Suitable electrolytes for the lithium batteries can comprise a heterogeneous electrolyte including a first electrolyte solvent (e.g., dioxolane (DOL)) that partitions towards the anode and is favorable towards the anode (referred to herein as an "anode-side electrolyte solvent") and a second electrolyte solvent (e.g., 1,2 - dimethoxyethane (DME)) that partitions towards the cathode and is favorable towards the cathode (and referred to herein as an "cathode-side electrolyte solvent"). By separating the electrolyte solvents during operation of the battery such that the anode- side electrolyte solvent is present disproportionately at the anode and the cathode-side electrolyte solvent is present disproportionately at the cathode, the battery can benefit from desirable characteristics of both electrolyte solvents (e.g., relatively low lithium reactivity of the anode-side electrolyte solvent and relatively high polysulfide solubility of the cathode-side electrolyte solvent).
摘要翻译：提供了关于在锂电池中分离电解质组合物的方法和制品。本文所述的锂电池可以包括具有锂作为活性阳极物质的阳极和具有硫作为活性阴极物质的阴极。用于锂电池的合适电解质可以包括非均相电解质，其包括朝向阳极分隔并且有利于阳极（在本文中称为“阳极侧电解质溶剂”）的第一电解质溶剂（例如，二氧戊环（DOL）），以及第二电解质溶剂（例如，1,2-二甲氧基乙烷（DME）），其分隔成阴极并且有利于阴极（并且在本文中称为“阴极侧电解质溶剂”）。通过在电池操作期间分离电解质溶剂使得阳极侧电解质溶剂在阳极处不成比例地存在，并且阴极侧电解质溶剂在阴极处不成比例地存在，电池可以受益于两种电解质溶剂的期望特性（例如阳极侧电解质溶剂的锂反应性相对较低，阴极侧电解质溶剂的多硫化物溶解度相对较高）。

2. 发明申请

WO2011031297A3 ELECTROCHEMICAL CELLS COMPRISING POROUS STRUCTURES COMPRISING SULFUR 审中-公开
标题翻译：包含硫的多孔结构的电化学电池
公开(公告)号：WO2011031297A3
公开(公告)日：2011-07-21
申请号：PCT/US2010002329
申请日：2010-08-24
申请人： SION POWER CORP , SCORDILIS-KELLEY CHARICLEA , MIKHAYLIK YURIY V , KOVALEV IGOR , OLESHKO VLADIMIR , CAMPBELL CHRISTOPHER T S , AFFINITO JOHN D , WILKENING WILLIAM F , BURNSIDE SAVANNAH V
发明人： SCORDILIS-KELLEY CHARICLEA , MIKHAYLIK YURIY V , KOVALEV IGOR , OLESHKO VLADIMIR , CAMPBELL CHRISTOPHER T S , AFFINITO JOHN D , WILKENING WILLIAM F , BURNSIDE SAVANNAH V
IPC分类号： H01M4/02 , H01B1/00 , H01M4/58 , H01M4/62 , H01M10/05
CPC分类号： H01M4/364 , H01G11/06 , H01M4/0402 , H01M4/136 , H01M4/38 , H01M4/5815 , H01M4/583 , H01M4/60 , H01M4/602 , H01M4/64 , H01M4/668 , H01M4/80 , H01M2004/021 , H01M2010/4292 , Y02E60/122 , Y02E60/13 , Y02P70/54 , Y02T10/7022 , Y10T29/49108 , Y10T29/49115
摘要： The present invention relates to the use of porous structures comprising sulfur in electrochemical cells. Such materials may be useful, for example, in forming one or more electrodes in an electrochemical cell. For example, the systems and methods described herein may comprise the use of an electrode comprising a conductive porous support structure and a plurality of particles comprising sulfur (e.g., as an active species) substantially contained within the pores of the support structure. The inventors have unexpectedly discovered that, in some embodiments, the sizes of the pores within the porous support structure and/or the sizes of the particles within the pores can be tailored such that the contact between the electrolyte and the sulfur is enhanced, while the electrical conductivity and structural integrity of the electrode are maintained at sufficiently high levels to allow for effective operation of the cell. Also, the sizes of the pores within the porous support structures and/or the sizes of the particles within the pores can be selected such that any suitable ratio of sulfur to support material can be achieved while maintaining mechanical stability in the electrode. The inventors have also unexpectedly discovered that the use of porous support structures comprising certain materials (e.g., metals such as nickel) can lead to relatively large increases in cell performance. In some embodiments, methods for forming sulfur particles within pores of a porous support structure allow for a desired relationship between the particle size and pore size. The sizes of the pores within the porous support structure and/or the sizes of the particles within the pores can also be tailored such that the resulting electrode is able to withstand the application of an anisotropic force, while maintaining the structural integrity of the electrode.
摘要翻译：本发明涉及在电化学电池中使用包含硫的多孔结构。例如，这种材料可用于在电化学电池中形成一个或多个电极。例如，本文所述的系统和方法可以包括使用包含导电多孔支撑结构和基本上包含在支撑结构的孔内的包含硫（例如作为活性物质）的多个粒子的电极。本发明人出乎意料地发现，在一些实施方案中，多孔载体结构内的孔的尺寸和/或孔内颗粒的尺寸可以被调整，使得电解质和硫之间的接触增强，而电极的电导率和结构完整性保持在足够高的水平以允许电池的有效操作。而且，可以选择多孔载体结构内的孔的尺寸和/或孔内颗粒的尺寸，使得可以实现硫与载体材料的任何合适的比例，同时维持电极中的机械稳定性。发明人还出乎意料地发现，使用包含某些材料（例如，诸如镍的金属）的多孔载体结构可以导致电池性能的相对较大的增加。在一些实施方案中，用于在多孔载体结构的孔内形成硫颗粒的方法允许颗粒尺寸和孔尺寸之间的期望关系。多孔载体结构内孔的尺寸和/或孔内颗粒的尺寸也可以定制，使得所得电极能够承受施加各向异性力，同时保持电极的结构完整性。

3. 发明申请

WO2009042071A2 ELECTROLYTE ADDITIVES FOR LITHIUM BATTERIES AND RELATED METHODS 审中-公开
标题翻译：锂电池用电解液添加剂及相关方法
公开(公告)号：WO2009042071A2
公开(公告)日：2009-04-02
申请号：PCT/US2008010894
申请日：2008-09-19
申请人： SION POWER CORP , MIKHAYLIK YURIY V , KOVALEV IGOR
发明人： MIKHAYLIK YURIY V , KOVALEV IGOR
IPC分类号： H01M4/134 , H01M4/58 , H01M6/14 , H01M10/052 , H01M10/0567 , H01M10/0568
CPC分类号： H01M10/0567 , H01M4/134 , H01M4/581 , H01M10/052 , H01M10/0568 , H01M10/44 , H01M2010/4292 , Y10T29/49108
摘要： The present invention relates generally to electrochemical cells, and more specifically, to additives for electrochemical cells which may enhance the performance of the cell. In some cases, the additive may advantageously reduce or prevent formation of impurities and/or depletion of active components of the cell during operation, to increase the efficiency and/or lifetime of the cell. The incorporation of certain additives within the electrolyte of the cell may improve the cycling lifetime and/or performance of the cell.
摘要翻译：本发明一般涉及电化学电池，并且更具体地涉及可以提高电池性能的电化学电池添加剂。在一些情况下，添加剂可有利地减少或防止操作期间电池的杂质的形成和/或电池的活性组分的耗尽，以提高电池的效率和/或寿命。在电池的电解质中掺入某些添加剂可以改善电池的循环寿命和/或性能。

4. 发明申请

WO2012027457A3 ELECTRICALLY NON-CONDUCTIVE MATERIALS FOR ELECTROCHEMICAL CELLS 审中-公开
标题翻译：用于电化学电池的电导电材料
公开(公告)号：WO2012027457A3
公开(公告)日：2012-05-24
申请号：PCT/US2011048944
申请日：2011-08-24
申请人： SION POWER CORP , MIKHAYLIK YURIY V , AFFINITO JOHN D , KOVALEV IGOR , SCHOCK RILEY OAKS
发明人： MIKHAYLIK YURIY V , AFFINITO JOHN D , KOVALEV IGOR , SCHOCK RILEY OAKS
IPC分类号： H01M2/10 , H01M2/26
CPC分类号： H01M10/0583 , H01M2/14 , H01M2/145 , H01M4/13 , H01M4/139 , H01M10/052 , Y10T29/49117
摘要： Articles, systems, and methods related to the configuration of electrically non- conductive materials and related components in electrochemical cells are generally described. Some inventive electrochemical cell configurations include an electrically non-conductive material (e.g., as part of the electrolyte) that is configured to wrap around the edge of an electrode to prevent short circuiting of the electrochemical cell. In some embodiments, the electrically non-conductive material layer can be arranged such that it includes first and second portions (one on either side of an electrode) as well as a third portion adjacent the edge of the electrode that directly connects (and, in some cases, is substantially continuous with) the first and second portions. The electrically non- conductive material layer can be relatively thin while maintaining relatively high electrical insulation between the anode and the cathode, allowing one to produce an electrochemical cell with a relatively low mass and/or volume. The arrangements described above can be formed, for example, by forming a multi-layer structure comprising an electrode and an electrically non-conductive material layer (e.g., as a coating), and folding the multi-layer structure such that the electrically non-conductive material covers the convex surface portion of the resulting crease.
摘要翻译：通常描述与电化学电池中的非导电材料和相关组分的配置相关的制品，系统和方法。一些本发明的电化学电池构造包括被配置为围绕电极的边缘缠绕的非导电材料（例如，作为电解质的一部分），以防止电化学电池的短路。在一些实施例中，非导电材料层可以被布置成使得其包括第一和第二部分（一个在电极的任一侧上）以及与电极的边缘相邻的第三部分，其直接连接（和，一些情况，基本上连续）第一和第二部分。电非导电材料层可以相对较薄，同时在阳极和阴极之间保持相对较高的电绝缘，从而允许产生具有相对较低质量和/或体积的电化学电池。上述布置可以例如通过形成包括电极和非导电材料层（例如，作为涂层）的多层结构而形成，并且折叠多层结构，导电材料覆盖所产生的折痕的凸表面部分。

5. 发明申请

WO2009042071A3 ELECTROLYTE ADDITIVES FOR LITHIUM BATTERIES AND RELATED METHODS 审中-公开
标题翻译：锂电池用电解质添加剂及相关方法
公开(公告)号：WO2009042071A3
公开(公告)日：2009-05-14
申请号：PCT/US2008010894
申请日：2008-09-19
申请人： SION POWER CORP , MIKHAYLIK YURIY V , KOVALEV IGOR
发明人： MIKHAYLIK YURIY V , KOVALEV IGOR
IPC分类号： H01M4/134 , H01M4/58 , H01M6/14 , H01M10/052 , H01M10/0567 , H01M10/0568
CPC分类号： H01M10/0567 , H01M4/134 , H01M4/581 , H01M10/052 , H01M10/0568 , H01M10/44 , H01M2010/4292 , Y10T29/49108
摘要： The present invention relates generally to electrochemical cells, and more specifically, to additives for electrochemical cells which may enhance the performance of the cell. In some cases, the additive may advantageously reduce or prevent formation of impurities and/or depletion of active components of the cell during operation, to increase the efficiency and/or lifetime of the cell. The incorporation of certain additives within the electrolyte of the cell may improve the cycling lifetime and/or performance of the cell.
摘要翻译：本发明一般涉及电化学电池，更具体地说，涉及可增强电池性能的电化学电池用添加剂。在一些情况下，添加剂可以有利地在操作期间减少或阻止杂质的形成和/或细胞活性成分的消耗，以增加细胞的效率和/或寿命。某些添加剂在电池的电解质中的引入可以改善电池的循环寿命和/或性能。

6. 发明申请

WO2007111901A3 ELECTRODE PROTECTION IN BOTH AQUEOUS AND NON-AQUEOUS ELECTROCHEMICAL CELLS, INCLUDING RECHARGEABLE LITHIUM BATTERIES 审中-公开
标题翻译：两电池和非水电解质电池中的电极保护，包括可充电锂电池
公开(公告)号：WO2007111901A3
公开(公告)日：2007-11-29
申请号：PCT/US2007007005
申请日：2007-03-21
申请人： SION POWER CORP , AFFINITO JOHN D , MIKHAYLIK YURIY V , GERONOV YORDAN M , SHEEHAN CHRISTOPHER J
发明人： AFFINITO JOHN D , MIKHAYLIK YURIY V , GERONOV YORDAN M , SHEEHAN CHRISTOPHER J
IPC分类号： H01M10/44 , H01M4/04 , H01M4/134 , H01M10/052 , H01M10/36
CPC分类号： H01M10/44 , H01M4/0402 , H01M4/0407 , H01M4/134 , H01M4/24 , H01M4/366 , H01M4/382 , H01M4/387 , H01M4/40 , H01M10/052 , H01M10/24
摘要： Electrode protection in electrochemical cells in both aqueous and non-aqueous electrochemical cells, including rechargeable lithium batteries, are presented. In one embodiment, an electrochemical cell includes an anode comprising lithium and a multi-layered structure positioned between the anode and an electrolyte of the cell. A multi-layered structure can include at least a first single-ion conductive material layer (e.g., a lithiated metal layer), and at least a first polymeric layer positioned between the anode and the single-ion conductive material. The electrode comprises e.g. : a first layer comprising the active electrode species; a second layer comprising the active electrode species; and a single-ion conductive layer separating the first layer from the second layer and substantially preventing electronic communication between the first and second layers across the layer, is also disclosed. The invention also can provide an electrode stabilization layer positioned within the electrode, i.e., between one portion and another portion of an electrode, to control depletion and re-plating of electrode material upon charge and discharge of a battery.
摘要翻译：介绍了电化学电池在水性和非水电化学电池（包括可再充电锂电池）中的电极保护。在一个实施例中，电化学电池包括包含锂的阳极和位于电池的阳极和电解质之间的多层结构。多层结构可以包括至少第一单离子导电材料层（例如，锂化金属层）和至少第一聚合物层，其位于阳极和单离子导电材料之间。电极包括例如：包含活性电极种类的第一层; 包含所述活性电极种类的第二层; 并且还公开了将第一层与第二层分开并且基本上防止穿过该层的第一层和第二层之间的电子连通的单离子传导层。本发明还可以提供一种位于电极内，即电极的一部分与另一部分之间的电极稳定层，以在电池充电和放电时控制电极材料的耗尽和再镀层。

7. 发明申请

WO2010107499A3 CATHODE FOR LITHIUM BATTERY 审中-公开
标题翻译：锂电池阴极
公开(公告)号：WO2010107499A3
公开(公告)日：2011-02-24
申请号：PCT/US2010000819
申请日：2010-03-19
申请人： SION POWER CORP , MIKHAYLIK YURIY V , KUMARESAN KARTHIKEYAN
发明人： MIKHAYLIK YURIY V , KUMARESAN KARTHIKEYAN
IPC分类号： H01M4/583 , H01M4/02 , H01M4/38 , H01M10/05 , H01M10/0525
CPC分类号： H01M10/058 , H01M4/133 , H01M4/1393 , H01M4/364 , H01M4/38 , H01M4/5815 , H01M4/587 , H01M10/052 , Y10T29/49108
摘要： The present invention relates to cathodes used in electrochemical cells. A force, or forces, applied to portions of an electrochemical cell as described in this application can reduce irregularity or roughening of an electrode surface of the cell, improving performance. The cathodes described herein may possess enhanced properties that render them particularly suitable for use in electrochemical cells designed to be charged and/or discharged while a force is applied. In some embodiments, the cathode retains sufficient porosity to charge and discharge effectively when a force is applied to the cell. Cathodes described herein may also comprise relatively high electrolyte-accessible conductive material (e.g., carbon) areas. The cathode may comprise a relatively low ratio of the amount of binder and/or mass of electrolyte to cathode active material (e.g., sulfur) ratio in some instances. In some embodiments, electrochemical cells comprising the cathodes described herein may achieve relatively high specific capacities and/or relatively high discharge current densities. In addition, the cathode described herein may exhibit relatively high cathode active material (e.g., sulfur) utilization during charge and discharge. In still further cases, the electrical conductivity between conductive material in the cathode (e.g., carbon) may be enhanced during the application of the force.
摘要翻译：本发明涉及电化学电池中使用的阴极。施加到如本申请中描述的电化学电池的部分的力或力可以减小电池的电极表面的不规则性或粗糙度，从而提高性能。本文所述的阴极可以具有增强的特性，使得它们特别适用于设计成在施加力时被充电和/或放电的电化学电池中。在一些实施方案中，当将力施加到电池时，阴极保留足够的孔隙以有效地充电和放电。本文所述的阴极还可以包括相对高的电解质可接近的导电材料（例如碳）区域。在一些情况下，阴极可以包括粘合剂的量和/或电解质与阴极活性材料的质量比例（例如硫）的比例相对较低。在一些实施例中，包含本文所述的阴极的电化学电池可以实现相对较高的比容量和/或相对高的放电电流密度。此外，本文所述的阴极可以在充电和放电期间显示相对高的正极活性材料（例如硫）利用。在另外的情况下，在施加力期间可以增强阴极中导电材料（例如碳）之间的电导率。

8. 发明申请

WO2009089018A3 POROUS ELECTRODES AND ASSOCIATED METHODS 审中-公开
标题翻译：多孔电极和相关方法
公开(公告)号：WO2009089018A3
公开(公告)日：2009-10-08
申请号：PCT/US2009000090
申请日：2009-01-08
申请人： SION POWER CORP , MIKHAYLIK YURIY V , WILKENING WILLIAM F , CAMPBELL CHRISTOPHER T S , BURNSIDE SAVANNAH V
发明人： MIKHAYLIK YURIY V , WILKENING WILLIAM F , CAMPBELL CHRISTOPHER T S , BURNSIDE SAVANNAH V
IPC分类号： H01M4/04 , H01M4/139 , H01M4/62 , H01M10/052 , H01M10/40
CPC分类号： H01M4/139 , H01M4/04 , H01M4/38 , H01M4/62 , H01M4/621 , H01M4/663 , H01M4/80 , H01M10/052 , Y02E60/122 , Y02P70/54
摘要： The present invention relates to electrochemical cells, electrodes, and related methods. In some embodiments, a removable filler material may be employed during fabrication of an electrochemical cell, or component thereof, to produce electrochemical devices having improved cell performance and rate capability. Electrochemical cells may exhibit enhanced utilization of electroactive species and/or increased accessibility of electroactive species within the electrochemical cell during operation. In some cases, the invention may provide electrodes which advantageously possess both high loading of an electroactive species (e.g., greater than 1.5 mg/cm2), while also maintaining the stability and good mechanical properties of the electrode.
摘要翻译：本发明涉及电化学电池，电极和相关方法。在一些实施例中，可在制造电化学电池或其部件期间使用可移除的填充材料来制造具有改进的电池性能和倍率能力的电化学装置。在操作期间，电化学电池可以表现出电活性物质的增强的利用和/或电化学电池内的电活性物质的增加的可接近性。在一些情况下，本发明可以提供有利地同时具有高负载电活性物质（例如，大于1.5mg / cm 2）的电极，同时还保持电极的稳定性和良好的机械性能。

9. 发明申请

WO2007111988A3 METHODS OF CHARGING LITHIUM SULFUR CELLS 审中-公开
标题翻译：锂离子电池充电方法
公开(公告)号：WO2007111988A3
公开(公告)日：2008-11-06
申请号：PCT/US2007007219
申请日：2007-03-22
申请人： SION POWER CORP , MIKHAYLIK YURIY V
发明人： MIKHAYLIK YURIY V
IPC分类号： H02J7/04 , H01M4/38 , H01M4/58 , H01M4/60 , H01M10/052 , H01M10/0567 , H01M10/0569 , H01M10/36 , H01M10/44 , H02J7/00
CPC分类号： H02J7/0081 , H01M4/5815 , H01M10/052 , H01M10/0567 , H01M10/0569 , H01M10/44 , H02J7/0073 , H02J7/008
摘要： Disclosed is a method of charging a lithium-sulfur electrochemical cell wherein the lithium-sulfur cell comprises a cathode comprising an electroactive sulfur-containing material, an anode comprising lithium, and a nonaqueous electrolyte. Also disclosed are methods for determining charge termination when charging lithium-sulfur cells.
摘要翻译：公开了一种锂 - 硫电化学电池的充电方法，其中锂 - 硫电池包括含有电活性含硫材料的阴极，包含锂的阳极和非水电解质。还公开了当充电锂 - 硫电池时确定充电终止的方法。

10. 发明申请

WO2007111895A3 RECHARGEABLE LITHIUM/WATER, LITHIUM/AIR BATTERIES 审中-公开
标题翻译：可充电锂/水，锂/气电池
公开(公告)号：WO2007111895A3
公开(公告)日：2007-12-06
申请号：PCT/US2007006962
申请日：2007-03-21
申请人： SION POWER CORP , AFFINITO JOHN D , MIKHAYLIK YURIY V , GERONOV YORDAN M , SHEEHAN CHRISTOPHER J
发明人： AFFINITO JOHN D , MIKHAYLIK YURIY V , GERONOV YORDAN M , SHEEHAN CHRISTOPHER J
IPC分类号： H01M4/04 , H01M4/134 , H01M4/24 , H01M4/40 , H01M10/052 , H01M10/24 , H01M10/36 , H01M10/44
CPC分类号： H01M10/44 , H01M4/0402 , H01M4/0407 , H01M4/134 , H01M4/24 , H01M4/366 , H01M4/382 , H01M4/387 , H01M4/40 , H01M10/052 , H01M10/24
摘要： Electrochemical cells, and more specifically, rechargeable batteries comprising lithium anodes (20) for use in water and/or air environments, as well as non-aqueous and non- air environments, are presented. In one embodiment, an electrochemical cell includes an anode (20) comprising lithium and a multi-layered structure positioned between the anode and an electrolyte (60) of the cell. A multi-layered structure can include at least a first single- ion conductive material layer (e.g., a lithiated metal layer), (40,42) and at least a first polymeric layer (50,52) positioned between the anode and the single-ion conductive material. The invention also can provide an electrode stabilization layer (24) positioned within the electrode, i.e., between one portion (21) and another portion of an electrode (23), to control depletion and re-plating of electrode material upon charge and discharge of a battery. Advantageously, electrochemical cells comprising combinations of structures described herein are not only compatible with environments that are typically unsuitable for lithium, but the cells may be also capable of displaying long cycle life, high lithium cycling efficiency, and high energy density.
摘要翻译：提出了电化学电池，更具体地说，包括用于水和/或空气环境的锂阳极（20）以及非水和非空气环境的可再充电电池。在一个实施例中，电化学电池包括包含锂的阳极（20）和位于电池的阳极和电解质（60）之间的多层结构。多层结构可以包括至少第一单离子导电材料层（例如，锂化金属层），（40,42）和至少第一聚合物层（50,52），其位于阳极和单体之间导电材料。本发明还可以提供一种位于电极内的电极稳定层（24），即在一个部分（21）和一个电极（23）的另一部分之间，以控制在充电和放电时电极材料的耗尽和再镀覆一个电池有利地，包含本文所述结构的电化学电池不仅与通常不适合于锂的环境兼容，而且电池还可以显示长循环寿命，高锂循环效率和高能量密度。

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