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    • 2. 发明申请
    • CATALYST SUPPORT MATERIALS WITH OXYGEN STORAGE CAPACITY (OSC) AND METHOD OF MAKING THEREOF
    • WO2012088373A3
    • 2012-06-28
    • PCT/US2011/066715
    • 2011-12-22
    • PACIFIC INDUSTRIAL DEVELOPMENT CORPORATIONWU, WeiLI, YunkuiLACHAPELLE, Jeffery
    • WU, WeiLI, YunkuiLACHAPELLE, Jeffery
    • B01J23/63B01J21/04B01J21/06B01J37/00
    • A new type of catalyst support with oxygen storage capacity (OSC) and methods of making the same are disclosed. The composition ratio is x(Ce 1-w Zr w 0 2 ) : yM : zL : (1 -x-y-z)AI 2 0 3 , where Ce 1-w Zr w 0 2 is the oxygen storage composition with stabilizer Zr0 2 , molar ratio (w) in the range of 0 to about 0.8, and a weight ratio (x) of about 0.05 to about 0.8; M is an interactive promoter for oxygen storage capacity with a weight ratio (y) of 0 to about 0.10; and L is a stabilizer for the support Al 2 0 3 with weight ratio (z) of from 0 to about 0.10. In some cases, M or L can act as both OSC promoter and thermal stabilizer. The weight percentage range of ceria-zirconia and other metal and rare earth oxides (x+y+z) is from about 5 to about 80% relative to total oxides. Combining platinum group metals (PGM) and adhesive with the catalyst supports, a new wash coat made therefrom is provided that comprises a mixture of catalyst support materials according to the relationship (a)RE-Ce- Zr0 2 + (3)CZMLA + (1 -a-β)RE-AI 2 0 3 , where RE-Ce-Zr0 2 is a commercial OSC material of rare earth elements stabilized ceria zirconia having a weight ratio (a) ranging from 0 to about 0.7; CZMLA is the catalyst support material of the present disclosure having a weight ratio (β) ranging from about 0.2 to about 1 such that (α+β) 2 0 3 is rare earth element stabilized alumina having a weight ratio equal to (1 -α-β). The new wash coat made therefrom exhibits a lower activation temperature compared with traditional formulation of wash coat by at least 50°C. The new wash coat made therefrom also requires less RE-Ce-Zr0 2 oxide and/or less PGM in the formulation of emission control catalyst for gasoline and diesel engines.