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1. 发明申请

WO2010100203A3 PROCESS FOR THE PREPARATION OF AN ISOMORPHOUSLY SUBSTITUTED SILICATE 审中-公开
标题翻译：制备同分异构取代的硅酸盐的方法
公开(公告)号：WO2010100203A3
公开(公告)日：2010-11-18
申请号：PCT/EP2010052713
申请日：2010-03-03
申请人： BASF SE , TOKYO INST TECH , YILMAZ BILGE , MUELLER ULRICH , PFAFF MEIKE , XIAO FENG-SHOU , GIES HERMANN , DE VOS DIRK , BAO XINHE , ZHANG WEIPING , TATSUMI TAKASHI
发明人： YILMAZ BILGE , MUELLER ULRICH , PFAFF MEIKE , XIAO FENG-SHOU , GIES HERMANN , DE VOS DIRK , BAO XINHE , ZHANG WEIPING , TATSUMI TAKASHI
IPC分类号： B01J29/06 , C01B33/38 , C01B39/04
CPC分类号： C01B33/20 , B01J21/16 , B01J29/061 , B01J29/70 , B01J35/002 , C01B33/38 , C01B37/00 , C01B39/02 , C01B39/04 , C07C1/20 , C07C209/16 , C07C2521/06 , C07C2521/08 , C07C2521/12 , C07C211/04
摘要： A process for the preparation of an isomorphously substituted layered silicate comprising (1) providing a mixture containing silica or a precursor thereof, at least one structure directing agent (SDA) allowing for the crystallization of the layered silicate, and water; (2) heating the mixture obtained according to (1) under hydrothermal conditions; (3) adding at least one source at least one element suitable for isomorphous substitution; (4) heating the mixture obtained according to (3) under hydrothermal conditions.
摘要翻译：一种制备同形取代的层状硅酸盐的方法，该方法包括（1）提供含二氧化硅或其前体，至少一种允许层状硅酸盐结晶的结构导向剂（SDA）和水的混合物; （2）在水热条件下加热根据（1）得到的混合物; （3）向至少一个源添加至少一个适于同晶取代的元素; （4）在水热条件下加热根据（3）得到的混合物。

2. 发明申请

WO2013038372A3 PROCESS FOR THE PRODUCTION OF A CORE/SHELL ZEOLITIC MATERIAL HAVING A CHA FRAMEWORK STRUCTURE 审中-公开
标题翻译：生产具有CHA框架结构的核心/壳体热塑性材料的工艺
公开(公告)号：WO2013038372A3
公开(公告)日：2013-05-10
申请号：PCT/IB2012054800
申请日：2012-09-14
申请人： BASF SE , TOKYO INST TECH , BASF CHINA CO LTD , YILMAZ BILGE , MUELLER ULRICH , XIAO FENG-SHOU , TATSUMI TAKASHI , DE VOS DIRK , BAO XINHE , ZHANG WEIPING , GIES HERMANN , IMAI HIROYUKI , TIJSEBAERT BART , REN LIMIN , YANG CHENGGUAN
发明人： YILMAZ BILGE , MUELLER ULRICH , XIAO FENG-SHOU , TATSUMI TAKASHI , DE VOS DIRK , BAO XINHE , ZHANG WEIPING , GIES HERMANN , IMAI HIROYUKI , TIJSEBAERT BART , REN LIMIN , YANG CHENGGUAN
IPC分类号： C01B39/54 , B01J29/06 , B01J29/85
CPC分类号： C01B39/00 , B01D53/02 , B01D53/9418 , B01D2255/2025 , B01D2255/20707 , B01D2255/20715 , B01D2255/2092 , B01D2255/2094 , B01D2255/50 , B01J29/005 , B01J29/7015 , B01J29/83 , B01J29/84 , B01J29/85 , B01J35/002 , B01J35/023 , B01J35/1019 , B01J35/1023 , B01J35/1066 , B01J37/02 , B01J37/0221 , B01J37/023 , B01J2229/62 , C01B37/08 , C01B39/48 , C01B39/54 , C01P2002/72 , C01P2004/03 , C01P2006/12 , C07C1/20 , C07C2529/85 , C10G3/49 , C10G11/18 , Y02P20/52 , Y02P30/20 , C07C11/02
摘要： The present invention relates to a process for the preparation of a zeolitic material having a CHA framework structure, said zeolitic material comprising zeolite crystals having a core-shell structure, wherein said process comprises the steps of (1) providing a mixture comprising one or more sources for Z2O5, one or more sources for X2O3, optionally one or more structure directing agents, and seed crystals having a CHA framework structure, wherein the CHA framework structure of the seed crystals comprises Y02, X2O3, and optionally Z2O5, and wherein the seed crystals have a diameter of 450 nm or greater; (2) crystallizing the mixture provided in (1) to afford zeolite crystals comprising a core of seed crystal provided in step (1 ) and a shell crystallized on the seed crystal; wherein Z is a pentavalent element, Y is a tetravalent element, and X is a trivalent element, and wherein preferably one or more sources for YO2 are further provided in step (1 ).
摘要翻译：本发明涉及一种制备具有CHA骨架结构的沸石材料的方法，所述沸石材料包含具有核 - 壳结构的沸石晶体，其中所述方法包括以下步骤：（1）提供包含一种或多种 Z2O5的来源，X2O3的一种或多种来源，任选的一种或多种结构导向剂，以及具有CHA骨架结构的晶种，其中晶种的CHA骨架结构包含Y02，X2O3和任选的Z2O5，并且其中种子晶体的直径为450nm以上; （2）使（1）中提供的混合物结晶，得到包含步骤（1）中提供的晶种核心的沸石晶体和在晶种上结晶的壳; 其中Z是五价元素，Y是四价元素，X是三价元素，并且其中优选在步骤（1）中进一步提供一种或多种YO2源。

3. 发明申请

WO2010100205A3 PROCESS FOR THE PREPARATION OF LAYERED SILICATES 审中-公开
标题翻译：制备层状硅酸盐的方法
公开(公告)号：WO2010100205A3
公开(公告)日：2010-11-18
申请号：PCT/EP2010052716
申请日：2010-03-03
申请人： BASF SE , TOKYO INST TECH , YILMAZ BILGE , MUELLER ULRICH , PFAFF MEIKE , GIES HERMANN , XIAO FENG-SHOU , TATSUMI TAKASHI , DE VOS DIRK , BAO XINHE , ZHANG WEIPING
发明人： YILMAZ BILGE , MUELLER ULRICH , PFAFF MEIKE , GIES HERMANN , XIAO FENG-SHOU , TATSUMI TAKASHI , DE VOS DIRK , BAO XINHE , ZHANG WEIPING
IPC分类号： C01B33/38 , C01B37/00 , C01B37/02
CPC分类号： C01B33/20 , B01J20/10 , B01J20/30 , B01J21/16 , B01J29/049 , C01B33/38 , C01B37/00 , C01B37/02 , C01B39/02 , C01B39/04
摘要： The present invention relates to a process for the preparation of a layered silicate containing at least silicon and oxygen, comprising (1) providing a mixture containing silica and/or at least one silica precursor, water, at least one tetraalkylammonium compound selected from the group consisting of diethyldimethylammonium compound, a triethylmethylammonium compound, and a mixture of a diethyldimethylammonium and a triethylmethylammonium compound, and at least one base, and optionally at least one suitable seeding material; and (2) heating of the mixture obtained according to (1) under autogenous pressure (hydrothermal conditions) to a temperature in the range of from to 120 to 160 °C for a period in the range of from 5 to 10 days to give a suspension containing the layered silicate.
摘要翻译：本发明涉及一种制备至少含有硅和氧的层状硅酸盐的方法，其包括（1）提供含有二氧化硅和/或至少一种二氧化硅前体的混合物，水，至少一种选自以下的四烷基铵化合物：由二乙基二甲基铵化合物，三乙基甲基铵化合物和二乙基二甲基铵和三乙基甲基铵化合物的混合物组成，以及至少一种碱和任选的至少一种合适的接种材料; 和（2）根据（1）得到的混合物在自生压力（水热条件）下加热至120至160℃的温度范围为5至10天，得到含有层状硅酸盐的悬浮液。

4. 发明申请

WO2010100191A3 PROCESS FOR THE PREPARATION OF PILLARED SILICATES 审中-公开
标题翻译：制备支柱硅酸盐的方法
公开(公告)号：WO2010100191A3
公开(公告)日：2011-05-12
申请号：PCT/EP2010052695
申请日：2010-03-03
申请人： BASF SE , TOKYO INST TECH , YILMAZ BILGE , MUELLER ULRICH , XIAO FENG-SHOU , GIES HERMANN , TATSUMI TAKASHI , DE VOS DIRK , BAO XINHE , ZHANG WEIPING
发明人： YILMAZ BILGE , MUELLER ULRICH , XIAO FENG-SHOU , GIES HERMANN , TATSUMI TAKASHI , DE VOS DIRK , BAO XINHE , ZHANG WEIPING
IPC分类号： C01B37/00 , C01B33/38 , C01B33/40 , C01B33/42 , C01B37/02 , C01B39/46 , C01B39/48
CPC分类号： C01B37/005 , C01B32/05 , C01B37/02 , C01B39/026 , C01B39/46 , C01B39/48 , C04B35/16 , C04B2235/3201 , C04B2235/3222 , C04B2235/3427 , C04B2235/5409
摘要： The present invention relates to a process for the preparation of a silicate compound, comprising (1) providing at least one layered silicate; and (2) mixing said layered silicate with water and at least one silicon containing compound according to formula R4-mSi[-(SiR2)n-R]m wherein at least one residue R is a leaving group and none of the residues R contains Si; m is 0, 1, 2, 3, or 4; and n is an integer greater than or equal to 0.
摘要翻译：本发明涉及一种制备硅酸盐化合物的方法，包括（1）提供至少一种层状硅酸盐; 和（2）将所述层状硅酸盐与水和至少一种根据式R 4-m Si [ - （SiR 2）n -R] m的含硅化合物混合，其中至少一个残基R是离去基团，并且残基R都不含有Si; m为0,1,2,3或4; 并且n是大于或等于0的整数。

5. 发明申请

WO2010100193A3 ISOMORPHOUSLY SUBSTITUTED SILICATE 审中-公开
标题翻译：异构取代的硅酸盐
公开(公告)号：WO2010100193A3
公开(公告)日：2010-11-18
申请号：PCT/EP2010052699
申请日：2010-03-03
申请人： BASF SE , TOKYO INST TECH , YILMAZ BILGE , MUELLER ULRICH , XIAO FENG-SHOU , GIES HERMANN , BAO XINHE , DE VOS DIRK , TATSUMI TAKASHI , ZHANG WEIPING
发明人： YILMAZ BILGE , MUELLER ULRICH , XIAO FENG-SHOU , GIES HERMANN , BAO XINHE , DE VOS DIRK , TATSUMI TAKASHI , ZHANG WEIPING
IPC分类号： C01B33/38 , C01B37/00 , C01B37/02
CPC分类号： C01B37/005 , C01B37/02 , C04B35/16 , C04B2235/3217 , C04B2235/3232 , C04B2235/3239 , C04B2235/3244 , C04B2235/3251 , C04B2235/3272 , C04B2235/3286 , C04B2235/3287 , C04B2235/3293 , C04B2235/3409 , C04B2235/3427 , C04B2235/441 , C04B2235/5409 , C04B2235/602 , C04B2235/6021
摘要： The present invention relates to a process for the preparation of an isomorphously substituted RUB-36 silicate comprising (1) providing a mixture containing silica, preferably amorphous silica, and/or at least one silica precursor, water, at least one suitable structure directing agent, (2) heating the mixture obtained according to (1) under hydrothermal conditions to give a suspension containing an RUB-36 silicate, (3) separating the RUB-36 silicate, wherein (a) either the mixture according to (1) contains at least one element suitable for isomorphous substitution and/or (b) the separated RUB-36 silicate according to (3) is subjected to isomorphous substitution.
摘要翻译：本发明涉及制备同晶取代的RUB-36硅酸盐的方法，其包括（1）提供含有二氧化硅，优选无定形二氧化硅和/或至少一种二氧化硅前体，水，至少一种合适的结构导向剂，（2）在水热条件下加热根据（1）获得的混合物，得到含有RUB-36硅酸盐的悬浮液，（3）分离RUB-36硅酸盐，其中（a）根据（1）的混合物含有适于同晶取代的至少一种元素和/或（b）根据（3）的分离的RUB-36硅酸盐进行同晶取代。

6. 发明申请

WO2008122579A3 METHOD FOR PRODUCING A SILICATE CONTAINING A HETEROATOM 审中-公开
标题翻译：用于生产杂原子含硅酸盐
公开(公告)号：WO2008122579A3
公开(公告)日：2009-05-28
申请号：PCT/EP2008054046
申请日：2008-04-03
申请人： BASF SE , RUBITEC GESELLSCHAFT FUER INNOVATION & TECHNOLOGIE RUHR UNIV BOCHUM MBH , MUELLER ULRICH , TRUKHAN NATALIA , GIES HERMANN , VARSZEGI CSABA , DE VOS DIRK , TIJSEBAERT BART
发明人： MUELLER ULRICH , TRUKHAN NATALIA , GIES HERMANN , VARSZEGI CSABA , DE VOS DIRK , TIJSEBAERT BART
IPC分类号： C01B39/46
CPC分类号： B01J29/87 , B01J29/04 , B01J29/048 , C01B39/06 , C01B39/48 , C04B35/16 , C04B35/624 , C04B35/62655 , C04B35/62675 , C04B2235/3284 , C04B2235/3286 , C04B2235/6021 , C04B2235/612 , Y02P20/582
摘要： The invention relates to a method for producing a layered silicate containing at least Ga and/or Zn and a tectosilicate based thereon, preferably with an RRO structure, to the layered silicate and tectosilicate and to the use of silicates, in particular tectosilicate, preferably as catalysts.
摘要翻译：本发明涉及一种用于制备至少Ga和/或含Zn层状硅酸盐，并基于此，一个框架硅酸盐，优选的结构式的RRO，移位和骨架硅酸盐本身以及硅酸盐的用途，特别是网硅酸盐，优选作为催化剂，

7. 发明申请

WO2007042531A2 SILICATE PRODUCING METHOD 审中-公开
标题翻译：用于生产硅酸盐
公开(公告)号：WO2007042531A2
公开(公告)日：2007-04-19
申请号：PCT/EP2006067269
申请日：2006-10-11
申请人： BASF AG , RUBITEC GESELLSCHAFT FUER INNOVATION & TECHNOLOGIE RUHR UNIV BOCHUM MBH , MUELLER ULRICH , RUETZ ROGER , GIES HERMANN
发明人： MUELLER ULRICH , RUETZ ROGER , GIES HERMANN
CPC分类号： C01B37/02 , Y02P20/582
摘要： The invention relates to producing a silicate containing at least one type of silicium and oxygen consisting (1) in mixing silicium dioxide and/or silicium dioxide precursors with an aqueous solution, which comprises at least one type of R 1 R 2 R 3 R 4 N + compound containing a tetra-acryl ammonium compound and at least one type of base, wherein R 1 and R 2 represent methyl and, at the same time, R 3 and R 4 represent n-propyl; (2) in heating the colloidal solution thus obtained with a temperature greater than a boiling temperature at a selected colloidal solution pressure up to 180 °C at a normal pressure in such a way that at least one type of silicate-containing suspension is obtained. Said invention is characterised in that the silicium and oxygen-containing silicate is added in the form of a crystallisation-assisting agent.
摘要翻译：本发明涉及一种方法，用于至少硅和硅酸盐，包括：（1）将二氧化硅和/或与水溶液含有至少一个R二氧化硅前体含氧_{1 - [R 2 - [R _{3 - [R _{4 ñ^{+ 全面四烷基铵化合物和至少一个基极，其中R _{1 且R _{2 是甲基且R _{3 和R _{4 是相同的正丙基; （2）在（1）胶体溶液，以所选择的压力在常压下沸腾的胶体溶液，以180℃的温度，以获得至少一种含硅酸盐的悬浮液下范围从大于本的温度下加热所得到的，其特征在于，作为结晶助剂至少含有硅和含氧硅酸盐（1）中的溶液。}}}}}}}}

8. 发明申请

WO2014199348A3 METAL DOPED SILICATE CATALYSTS FOR THE SELECTIVE CONVERSION OF ETHANOL TO BUTADIENE 审中-公开
标题翻译：用于乙醇选择性转化为丁二烯的金属掺杂的硅酸盐催化剂
公开(公告)号：WO2014199348A3
公开(公告)日：2015-06-25
申请号：PCT/IB2014062202
申请日：2014-06-13
申请人： BASF SE , BASF CHINA CO LTD , TOKYO INST TECH
发明人： FEYEN MATHIAS , SPANNHOFF KIRSTEN , MÜLLER ULRICH , BAO XINHE , ZHANG WEIPING , DE VOS DIRK , GIES HERMANN , TATSUMI TAKASHI , XIAO FENG-SHOU , TOSHIYUKI YOKOI , BILGE YILMAZ
IPC分类号： C07C1/20
CPC分类号： C07C1/20 , B01J29/049 , B01J29/061 , B01J29/7049 , B01J29/7057 , B01J29/76 , B01J29/7615 , B01J29/78 , B01J29/7815 , B01J29/89 , B01J29/90 , B01J37/0201 , B01J38/12 , B01J2229/183 , B01J2229/186 , C01B39/08 , C01B39/085 , C07C2529/70 , C07C2529/89 , Y02P20/584 , C07C11/167
摘要： A process for the preparation of butadiene comprising (i) providing a gas stream G-1 comprising ethanol; (ii) contacting the gas stream G-1 provided in (i) with a catalyst, thereby obtaining a gas stream G-2 comprising butadiene; wherein the catalyst comprises a crystalline material supporting one or more catalytically active metals M, as well as to the use of the crystalline material supporting one or more catalytically active metals M.
摘要翻译：一种制备丁二烯的方法，包括（i）提供包含乙醇的气流G-1; （ii）使（i）中提供的气流G-1与催化剂接触，从而获得包含丁二烯的气流G-2; 其中所述催化剂包含支撑一种或多种催化活性金属M的结晶物质，以及支持一种或多种催化活性金属M的结晶物质的用途。

9. 发明申请

WO2015018807A3 PROCESS FOR THE OXYGEN FREE CONVERSION OF METHANE TO ETHYLENE ON ZEOLITE CATALYSTS 审中-公开
标题翻译：甲醇在乙酸乙酯中自由转化成沸石催化剂的方法
公开(公告)号：WO2015018807A3
公开(公告)日：2015-04-23
申请号：PCT/EP2014066757
申请日：2014-08-05
申请人： BASF SE , TOKYO INST TECH
发明人： FEYEN MATHIAS , MÜLLER ULRICH , BAO XINHE , ZHANG WEIPING , DE VOS DIRK , GIES HERMANN , TATSUMI TAKASHI , XIAO FENG-SHOU , GUO XIAOGUANG
IPC分类号： B01J29/78 , B01J29/72 , B01J29/80 , B01J29/82 , B01J29/83 , B01J29/86 , B01J29/90 , B01J38/10 , C07C2/76 , C07C11/04
CPC分类号： C07C2/76 , B01J29/0358 , B01J29/061 , B01J29/48 , B01J29/72 , B01J29/78 , B01J29/7815 , B01J29/80 , B01J29/85 , B01J29/90 , B01J38/10 , B01J2229/186 , C07C2529/74 , C07C2529/76 , C07C2529/78 , C07C2529/80 , Y02P20/52 , Y02P20/582 , Y02P20/584 , Y02P20/588 , C07C11/04
摘要： The present invention relates to a process comprising the step of converting methane to ethene under non-oxidative conditions in the presence of a catalyst comprising (a) a zeolite with a largest pore opening which is larger than 8; (b) a metal whereas the metal (b) is loaded onto the zeolite (a); and whereas the zeolite (a) is selected from zeolites -with a maximum diameter of a sphere that can be included of 4.5 A or smaller and/or -with a maximum diameter of a sphere which can diffuse along a of 4.4 A or smaller and/or -with a maximum diameter of a sphere which can diffuse along b of 4.4 A or smaller and/or -with a maximum diameter of a sphere which can diffuse along c of 4.4 A or smaller. Zeolite (a) is preferably a RRO catalyst, in particular RUB-41.
摘要翻译：本发明涉及一种方法，其包括在催化剂存在下，在非氧化条件下将甲烷转化为乙烯的步骤，所述催化剂包含（a）最大孔径大于8的沸石; （b）金属，而金属（b）负载在沸石（a）上; 而沸石（a）选自具有球体的最大直径的沸石，其可以包括4.5A或更小的和/或具有可以沿4.4A或更小的扩散的球体的最大直径， /或 - 具有可以沿b扩散的球体的最大直径为4.4A或更小，和/或具有可以沿着4.4A或更小的c扩散的球体的最大直径。沸石（a）优选为RRO催化剂，特别是RUB-41。

10. 发明申请

WO2014199349A3 METAL IMPREGNATED AMORPHOUS SILICATES FOR THE SELECTIVE CONVERSION OF ETHANOL TO BUTADIENE 审中-公开
标题翻译：用于乙醇选择性转化为丁二烯的金属浸渍的无定形硅酸盐
公开(公告)号：WO2014199349A3
公开(公告)日：2015-07-02
申请号：PCT/IB2014062203
申请日：2014-06-13
申请人： BASF SE , BASF CHINA CO LTD , TOKYO INST TECH
发明人： FEYEN MATHIAS , SPANNHOFF KIRSTEN , MÜLLER ULRICH , BAO XINHE , ZHANG WEIPING , DE VOS DIRK , GIES HERMANN , TATSUMI TAKASHI , XIAO FENG-SHOU , TOSHIYUKI YOKOI , BILGE YILMAZ
IPC分类号： B01J21/06 , C07C11/167
CPC分类号： C07C1/20 , B01J23/80 , B01J23/94 , B01J38/02 , C07C2521/06 , C07C2521/14 , C07C2523/06 , C07C2523/72 , Y02P20/584 , C07C11/167
摘要： Providing a catalyst and a process for the preparation of butadiene, and the catalyst comprising Hf and two or more further catalytically active metals M1 and M2, wherein the two or more further catalytically active metals M1 and M2 are selected from the group consisting of Zr, Zn, Cu and combinations of two or more thereof, and wherein M1 is different from M2.
摘要翻译：提供催化剂和制备丁二烯的方法，以及包含Hf和两种或更多种其它催化活性金属M1和M2的催化剂，其中两种或更多种其它催化活性金属M1和M2选自Zr， Zn，Cu及其两种或更多种的组合，其中M1不同于M2。

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