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1. 发明申请

WO2008071291A2 PROCESS FOR THE SYNTHESIS OF HYDROCARBON CONSTITUENTS OF GASOLINE 审中-公开
标题翻译：汽油组合物合成方法
公开(公告)号：WO2008071291A2
公开(公告)日：2008-06-19
申请号：PCT/EP2007010017
申请日：2007-11-20
申请人： TOPSOE HALDOR AS , JOENSEN FINN , NIELSEN POUL ERIK HOEJLUND , SCHIOEDT NIELS CHRISTIAN , JANSSENS TON V W , VOSS BODIL
发明人： JOENSEN FINN , NIELSEN POUL ERIK HOEJLUND , SCHIOEDT NIELS CHRISTIAN , JANSSENS TON V W , VOSS BODIL
CPC分类号： C10G3/49 , C10G2300/1011 , C10G2300/1022 , C10G2300/805 , C10G2400/02 , C10G2400/20 , Y02P30/20
摘要： Process for the synthesis of hydrocarbon constituents of gasoline comprising catalytic conversion in a gasoline synthesis step of an oxygenate-containing feed comprising methanol and/or dimethyl ether and a mixture of at least on a total oxygenate basis 0.05 wt% C 3+ higher alcohols and/or their oxygenate equivalents to hydrocarbon constituents of gasoline.
摘要翻译：在包含甲醇和/或二甲醚的含氧化合物进料的汽油合成步骤和至少在总含氧化合物基础上的混合物为0.05重量％C 3+的合成步骤中合成含汽油的烃组分的方法包括催化转化，高级醇和/或它们的含氧化合物等同于汽油的烃成分。

2. 发明申请

WO2010149339A1 PROCESS FOR THE PREPARATION OF HYDROCARBONS 审中-公开
标题翻译：制备油料的方法
公开(公告)号：WO2010149339A1
公开(公告)日：2010-12-29
申请号：PCT/EP2010/003755
申请日：2010-06-22
申请人： HALDOR TOPSOE A/S , NIELSEN, Poul, Erik, Højlund , JOENSEN, Finn , SØRENSEN, Esben, Lauge
发明人： NIELSEN, Poul, Erik, Højlund , JOENSEN, Finn , SØRENSEN, Esben, Lauge
IPC分类号： C10G1/00 , C10G2/00 , C10G3/00 , C07C1/04 , C10J3/00 , C07C29/151 , C07C41/01
CPC分类号： C10G1/00 , C07C29/1518 , C07C41/01 , C10G2/33 , C10G3/42 , C10G3/49 , C10G2300/1011 , C10G2300/1022 , C10G2400/02 , C10J2300/0956 , C10J2300/1659 , C10J2300/1665 , Y02E50/18 , Y02P30/20 , C07C31/04 , C07C43/04
摘要： The application relates to a process for preparation of hydrocarbons from a synthesis gas, in particular a synthesis gas obtained from gasification of a solid biomass. The synthesis gas comprises carbon monoxide, hydrogen and more than 20 mole % of inert gases and methane. The process comprises catalyticall the synthesis gas to an oxygenate mixture comprising methanol, dimethyl ether and/or higher alcohols; withdrawing the entire mixture and transferring said entire mixture to a catalytic oxygenate conversion step; catalytically converting methanol, dimethyl ether and/or higher alcohols to obtain a liquid phase comprising hydrocarbons and a gaseous phase comprising inert gases and methane; generating power from said inert gases and methane; pocessing said liquid phase comprising hydrocarbons into gasoline.
摘要翻译：本申请涉及从合成气制备烃的方法，特别是从固体生物质气化得到的合成气。合成气包括一氧化碳，氢气和大于20摩尔％的惰性气体和甲烷。该方法包括将合成气催化成包含甲醇，二甲醚和/或更高级醇的含氧混合物; 抽出整个混合物并将所述整个混合物转移到催化氧化合物转化步骤; 催化转化甲醇，二甲醚和/或更高级醇以获得包含烃和包含惰性气体和甲烷的气相的液相; 从所述惰性气体和甲烷产生动力; 将包含烃的所述液相加工成汽油。

3. 发明申请

WO2009033542A1 COMBINED PRODUCTION OF HYDROCARBONS AND ELECTRICAL POWER 审中-公开
标题翻译：联合生产碳氢化合物和电力
公开(公告)号：WO2009033542A1
公开(公告)日：2009-03-19
申请号：PCT/EP2008/006648
申请日：2008-08-13
申请人： HALDOR TOPSØE A/S , NIELSEN, Poul Erik Højlund , ROSTRUP-NIELSEN, Thomas , VOSS, Bodil , JOENSEN, Finn
发明人： NIELSEN, Poul Erik Højlund , ROSTRUP-NIELSEN, Thomas , VOSS, Bodil , JOENSEN, Finn
IPC分类号： C10G3/00 , C07C27/06
CPC分类号： C07C29/1518 , C07C41/01 , C10G3/42 , C10G2300/1022 , C10G2400/02 , Y02E20/14 , Y02P30/20 , C07C31/04 , C07C43/043
摘要： A process for the preparation of hydrocarbon products and for the generation of power comprising the steps of (a) providing a synthesis gas having a hydrogen to carbon monoxide ratio of between 0.1 and 1; (b) contacting the synthesis gas with one or more catalysts which together catalyse a reaction of hydrogen and carbon monoxide to oxygenates comprising methanol and dimethyl ether with a dimethyl ether to methanol ratio of higher than 2 and a carbon dioxide content of above 20 mole%; (c) contacting the carbon dioxide containing oxygenate mixture at an inlet temperature of between 240 and 4000C with a catalyst being active in the conversion of oxygenate to higher hydrocarbons and a tail gas being rich in carbon dioxide; (d) combusting the carbon dioxide rich tail gas, optionally admixed with fresh carbon monoxide rich synthesis gas in a gas turbine combustion chamber to flue gas; and (e) expanding the flue gas stream through a gas turbine for the generation of power.
摘要翻译：一种用于制备烃产物和产生动力的方法，包括以下步骤：（a）提供氢与一氧化碳比为0.1至1的合成气; （b）使合成气与一种或多种催化剂接触，这些催化剂一起催化氢和一氧化碳与包含甲醇和二甲醚的含氧化合物的反应，甲醚与甲醇的比例高于2，二氧化碳含量高于20摩尔％ ; （c）在二氧化碳混合物的入口温度为240-400℃之间的二氧化碳与在含氧化合物转化为高级烃和富含二氧化碳的尾气中具有活性的催化剂接触; （d）燃烧富含二氧化碳的尾气，任选地与燃气轮机燃烧室中的新鲜的富含一氧化碳的合成气混合成烟道气; 和（e）通过用于发电的燃气轮机扩大烟气流。

4. 发明申请

WO1996023755A1 PREPARATION OF FUEL GRADE DIMETHYL ETHER 审中-公开
标题翻译：燃料级二甲醚的制备
公开(公告)号：WO1996023755A1
公开(公告)日：1996-08-08
申请号：PCT/DK1996000047
申请日：1996-01-29
申请人： HALDOR TOPSOE A/S , VOSS, Bodil , JOENSEN, Finn , HANSEN, John, Bogild
发明人： HALDOR TOPSOE A/S
IPC分类号： C07C41/01
CPC分类号： C07C41/01 , C07C43/043
摘要： A process for the preparation of fuel grade dimethyl ether from a hydrogen and carbon oxides containing synthesis gas, wherein the synthesis gas is converted to a mixed process gas of dimethyl ether, methanol and water in one or more catalytic reactors in the presence of a catalyst having activity both in synthesis of methanol and methanol dehydration; the mixed process gas is cooled to obtain a liquid process phase containing the produced methanol, dimethyl ether and water and a gaseous process phase containing unconverted synthesis gas and a part of produced dimethyl ether, which process comprises further steps of separating the gaseous phase and liquid phase; passing the liquid phase to a first distillation unit and distilling off a top product stream containing dimethyl ether and methanol and withdrawing a bottom stream containing methanol and water; passing the bottom stream to a second distillation unit and distilling off a methanol containing stream, introducing the methanol into a purge washing unit; washing the gaseous process phase with the methanol in a purge washing unit and withdrawing from the unit a washing stream of dimethyl ether and methanol; converting a part of the methanol in the washing stream to dimethyl ether and water in a catalytic dehydration reactor by contact with a dehydration catalyst; withdrawing from the dehydration reactor a product stream of dimethyl ether, water and unconverted methanol; and combining the top product stream from the first distillation unit with the product stream from the dehydration reactor to obtain a combined product stream of fuel grade dimethyl ether.
摘要翻译：一种从含有合成气的氢和碳氧化物制备燃料级二甲醚的方法，其中在一种或多种催化反应器中在催化剂存在下将合成气转化为二甲醚，甲醇和水的混合工艺气体在甲醇和甲醇脱水合成中具有活性; 将混合工艺气体冷却以获得含有所生产的甲醇，二甲醚和水的液体工艺相和含有未转化的合成气和一部分生产的二甲醚的气态工艺相，该方法包括进一步分离气相和液体相; 将液相通入第一蒸馏单元并蒸馏出含有二甲醚和甲醇的顶部产物流并且抽出含有甲醇和水的底部物流; 将塔底物流送入第二蒸馏装置并蒸除含甲醇的料流，将甲醇引入清洗洗涤装置; 用清洗洗涤单元中的甲醇洗涤气态过程相，并从该单元中取出二甲醚和甲醇的洗涤流; 通过与脱水催化剂接触将一部分洗涤流中的甲醇转化成催化脱水反应器中的二甲醚和水; 从脱水反应器中取出二甲醚，水和未转化甲醇的产物流; 并将来自第一蒸馏单元的顶部产物流与来自脱水反应器的产物流混合以获得燃料级二甲醚的组合产物流。

5. 发明申请

WO2010149263A1 PROCESS FOR THE PREPARATION OF HYDROCARBONS FROM SYNTHESIS GAS 审中-公开
标题翻译：从合成气中制备碳氢化合物的方法
公开(公告)号：WO2010149263A1
公开(公告)日：2010-12-29
申请号：PCT/EP2010/003368
申请日：2010-06-03
申请人： HALDOR TOPSOE A/S , SØRENSEN, Esben Lauge , JOENSEN, Finn , NIELSEN, Poul Erik HØJLUND
发明人： SØRENSEN, Esben Lauge , JOENSEN, Finn , NIELSEN, Poul Erik HØJLUND
IPC分类号： C07C1/04 , C07C1/12
CPC分类号： C10G2/32 , C10G3/49 , C10G2300/4012 , C10G2300/4081 , C10G2400/02 , Y02P30/20
摘要： A process for the preparation of hydrocarbon products comprising the steps of (a) providing a synthesis gas comprising hydrogen, carbon monoxide and carbon dioxide; (b) reacting the synthesis gas to an oxygenate mixture comprising methanol and dimethyl ether in presence of one or more catalysts which together catalyse a reaction of hydrogen and carbon monoxide to oxygenates at a pressure of at least 4 MPa; (c) withdrawing from step (b) the oxygenate mixture comprising amounts of methanol, dimethyl ether, carbon dioxide and water together with unreacted synthesis gas and introducing the entire amount of the oxygenate mixture without further treatment into a catalytic oxygenate conversion step (d); (d) reacting the oxygenate mixture in presence of a catalyst being active in the conversion of oxygenates to higher hydrocarbons; (e) withdrawing an effluent from step (d) and separating the effluent into a tail gas, a liquid hydrocarbon phase containing the higher hydrocarbons produced in step.(d) and a liquid aqueous phase, wherein the pressure employed in steps (c) to (e) is substantially the same as employed in step (b).
摘要翻译：一种用于制备烃产物的方法，包括以下步骤：（a）提供包含氢气，一氧化碳和二氧化碳的合成气; （b）在一种或多种催化剂的存在下使合成气与包含甲醇和二甲醚的含氧混合物反应，所述催化剂在至少4MPa的压力下一起催化氢和一氧化碳与含氧化合物的反应; （c）从步骤（b）中取出含有甲醇，二甲醚，二氧化碳和水的含氧化合物混合物以及未反应的合成气，并将全部量的含氧化合物混合物引入催化氧化合物转化步骤（d）中， ; （d）在含氧化合物转化为高级烃的催化剂存在下使含氧化合物混合物反应; （e）从步骤（d）中取出流出物并将流出物分离成尾气，包含步骤（d）中产生的高级烃的液体烃相和液体水相，其中步骤（c）中使用的压力至（e）基本上与步骤（b）中使用的相同。

6. 发明申请

WO2008071291A3 PROCESS FOR THE SYNTHESIS OF HYDROCARBON CONSTITUENTS OF GASOLINE 审中-公开
公开(公告)号：WO2008071291A3
公开(公告)日：2008-06-19
申请号：PCT/EP2007/010017
申请日：2007-11-20
申请人： HALDOR TOPSØE A/S , JOENSEN, Finn , NIELSEN, Poul, Erik, Højlund , SCHIØDT, Niels, Christian , JANSSENS, Ton V.W. , VOSS, Bodil
发明人： JOENSEN, Finn , NIELSEN, Poul, Erik, Højlund , SCHIØDT, Niels, Christian , JANSSENS, Ton V.W. , VOSS, Bodil
IPC分类号： C10G3/00
摘要： A process for the synthesis of hydrocarbon constituents of gasoline by feeding an oxygenate-containing feed to a gasoline synthesis step, wherein the oxygenate-containing feed comprises methanol and/or dimethyl ether and at least 0.05 wt % on a total oxygenate 'basis of a mixture of C 3+ higher alcohols and/or their oxygenate equivalents.

7. 发明申请

WO2007020068A1 PROCESS FOR CONVERTING DIFFICULTLY CONVERTIBLE OXYGENATES TO GASOLINE 审中-公开
标题翻译：将难以置信的氧化剂转化为汽油的方法
公开(公告)号：WO2007020068A1
公开(公告)日：2007-02-22
申请号：PCT/EP2006/008076
申请日：2006-08-16
申请人： HALDOR TOPSØE A/S , JOENSEN, Finn , VOSS, Bodil , NERLOV, Jesper
发明人： JOENSEN, Finn , VOSS, Bodil , NERLOV, Jesper
IPC分类号： C10G3/00 , C07C1/20 , C07C1/207 , C07C29/151 , C07C41/01 , C07C45/49 , C07C47/06 , C07C1/04
CPC分类号： C07C29/151 , C10G3/00 , C10G3/49 , C10G2300/1022 , C10G2300/4081 , C10G2400/02 , C10L1/06 , Y02P30/20 , C07C31/04
摘要： Process for converting oxygenate compounds to hydrocarbons comprising the steps: (a) introducing a feed stream of synthesis gas to a synthesis section for the production of easily convertible oxygenates, (b) passing the effluent stream from said synthesis section containing easily convertible oxygenates to a gasoline synthesis section, (c) passing the effluent of said gasoline synthesis section to a separator and withdrawing from said separator hydrocarbons boiling in the gasoline boiling range, (d) admixing a recycle stream from the separator containing unconverted synthesis gas volatile hydrocarbons with the feed stream of synthesis gas of step (a), (e) introducing a feed containing difficulty convertible oxygenates to the synthesis section of step (a).
摘要翻译：将含氧化合物转化为烃的方法，包括以下步骤：（a）将合成气的进料流引入合成段，以生产容易转化的含氧化合物，（b）将含有易转化含氧化合物的合成段的流出物流送至汽油合成段，（c）将所述汽油合成段的流出物通入分离器并从汽油沸程沸腾的所述分离器中取出，（d）将含有未转化的合成气挥发性烃的分离器的再循环流与进料混合步骤（a）的合成气流，（e）将含有难以转化的含氧化合物的进料引入步骤（a）的合成部分。

8. 发明申请

WO9950218B1 PROCESS FOR PRODUCTION OF ACETIC ACID 审中-公开
标题翻译：生产乙酸的方法
公开(公告)号：WO9950218B1
公开(公告)日：1999-11-18
申请号：PCT/EP9902163
申请日：1999-03-29
申请人： TOPSOE HALDOR AS , JOENSEN FINN
发明人： JOENSEN FINN
IPC分类号： C07B61/00 , C07C51/12 , C07C53/08
CPC分类号： C07C51/12 , C07C53/08
摘要： A process for producing acetic acid which comprises: charging reactants methanol or dimethyl ether or methyl acetate or any mixture thereof, into a reactor containing (1) a rhodium carbonylation catalyst, (2) an alkyl iodide or alkyl bromide and (3) a hydrogenation catalyst and contacting said reactants with carbon monoxide and hydrogen for the production.
摘要翻译：（1）铑羰基化催化剂，（2）烷基碘或烷基溴，和（3）氢化作用的反应器中，将反应物甲醇或二甲醚或乙酸甲酯或其任何混合物装入反应器中，催化剂，并将所述反应物与一氧化碳和氢气接触用于生产。

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