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1. 发明申请

WO2006104884A3 CONVERSION OF ALKYLHALIDES INTO ALCOHOL ALKOXYLATES 审中-公开
公开(公告)号：WO2006104884A3
公开(公告)日：2006-10-05
申请号：PCT/US2006/010769
申请日：2006-03-24
申请人： SHELL OIL COMPANY , FONG, Howard, Lam-Ho , JOHNSON, Thomas, Howard , SEMPLE, Thomas, Carl
发明人： FONG, Howard, Lam-Ho , JOHNSON, Thomas, Howard , SEMPLE, Thomas, Carl
IPC分类号： C07C41/01 , A61K8/33
摘要： A process for converting alkyl halides to alkyl alcohol alkoxylates is described. This is a direct alkoxylation because the alkyl alcohol alkoxylates are made without going through an alkyl alcohol intermediate. The process comprises direct alkoxylation coupling of alkyl halides with a nucleophilic material in the presence of a homogeneous catalyst system to produce alkyl alcohol alkoxylates, wherein the homogeneous catalyst system comprises at least one metal or metal compound which has the ability to form metal-halogen bonds. A process for converting alkanes (paraffins) to alkyl alcohol alkoxylates is also described. This method comprises a) halogenation of at least one alkane to produce at least one alkyl halide; and b) direct alkoxylation coupling of at least a portion of the alkyl halide with a nucleophilic material in the presence of a homogeneous catalyst system to produce alkyl alcohol alkoxylates, wherein the homogeneous catalyst system comprises at least one metal or metal compound which has the ability to form metal-halogen bonds.

2. 发明申请

WO2010042440A1 AN INTEGRATED PROCESS TO COPRODUCE AROMATIC HYDROCARBONS AND ETHYLENE AND PROPYLENE 审中-公开
标题翻译：一体化芳香烃和乙烯和丙烯共聚物
公开(公告)号：WO2010042440A1
公开(公告)日：2010-04-15
申请号：PCT/US2009/059538
申请日：2009-10-05
申请人： SHELL OIL COMPANY , SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , FONG, Howard Lam Ho , SWAIN, Richard Dale
发明人： FONG, Howard Lam Ho , SWAIN, Richard Dale
IPC分类号： C07C4/02 , C10G3/00 , C07C1/26
CPC分类号： C10G50/00 , C07C1/26 , C07C2/66 , C07C4/02 , C07C4/18 , C07C5/2729 , C07C5/333 , C07C6/126 , Y02P20/125 , Y02P30/20 , C07C15/06 , C07C15/08 , C07C15/04 , C07C15/073 , C07C15/085 , C07C11/04 , C07C11/06 , C07C15/02 , C07C15/46
摘要： An integrated process for producing aromatic hydrocarbons and ethylene and/or propylene and optionally other lower olefins from low molecular weight hydrocarbons, preferably methane, which comprises: (a) contacting at least one low molecular weight alkane, preferably methane, with a halogen, preferably bromine. under process conditions sufficient to produce a monohaloalkane, preferably monobromomethane, (b) reacting the monohaloalkane in the presence of a coupling catalyst to produce aromatic hydrocarbons and C 2 + alkanes, (c) separating the aromatic hydrocarbons from the product mixture of step (b) to produce aromatic hydrocarbons, and (d) cracking at least part of the C 2 + alkanes in an alkane cracking system to produce ethylene and/or propylene and optionally other lower olefins.
摘要翻译：一种用于从低分子量烃（优选甲烷）生产芳烃和乙烯和/或丙烯和任选的其它低级烯烃的综合方法，其包括：（a）使至少一种低分子量烷烃，优选甲烷与卤素溴。（b）在偶联催化剂存在下使单卤烷反应生成芳族烃和C 2 +烷烃，（c）将芳烃从步骤（b）的产物混合物中分离成产生芳族烃，和（d）在烷烃裂解体系中裂化至少部分C 2 +烷烃以产生乙烯和/或丙烯和任选的其它低级烯烃。

3. 发明申请

WO2005110953A1 DERIVATIVES OF ALCOHOLS AND OLEFINS 审中-公开
标题翻译：酒精和油脂的衍生物
公开(公告)号：WO2005110953A1
公开(公告)日：2005-11-24
申请号：PCT/US2005/014526
申请日：2005-04-27
申请人： SHELL OIL COMPANY , CANO, Manuel Luis , FONG, Howard Lam-Ho , MURRAY, Brendan Dermot , THOMASON, Terry Blane , TREVINO, Lizbeth Olivia Cisneros
发明人： CANO, Manuel Luis , FONG, Howard Lam-Ho , MURRAY, Brendan Dermot , THOMASON, Terry Blane , TREVINO, Lizbeth Olivia Cisneros
IPC分类号： C07C17/10
CPC分类号： C07C1/30 , C07C29/124 , C07C31/20 , C07C11/02
摘要： Derivatives of branched or linear olefins and alcohols made by halogenation of branched or n-alkanes of the same carbon number, preferably to make primary mono-haloalkanes, which may then be oxidized with metal oxides. The derivatives of primary alcohols of this invention include alcohol ethoxylates, alcohol sulfates, alcohol sulfated ethoxylates, surfactants, including those made with these ethoxylates and/or sulfated ethoxylates, detergents made with these surfactants, oxyalkylated alcohols, oxyalkylated alcohol sulfates, polymethacrylate esters, alkyl amines and their derivatives, linear phthalates, linear adipates, alcohol ether amines, alkyl glycerol ether sulfonates, thioproprionate esters, alkyl polyglucosides, alcohol phosphates, alcohol ether phosphates, esters of fatty acids, alcohol phosphites, and benzophenones. Secondary alcohol derivatives include secondary alcohol ethoxylates, secondary alcohol sulfates, secondary alcohol sulfated ethoxylates, surfactants, including those made with these ethoxylates and/or sulfated ethoxylates, and detergents made with these surfactants. Internal olefins derivatives included within the scope of this invention include alkylbenzene, alkylxylene, detergent alcohols, plasticizer alcohols, alkenyl succinates, ether secondary alcohols, and diols and polyols produced by catalytic dihydroxylation of internal olefins with the use of hydrogen peroxide. Alpha olefin derivatives included within the scope of this invention include internal olefins, alkylbenzene, alkylxylene, alkylphenol, alkylnaphthalene, detergent alcohols, plasticizer alcohols, alkylates of phenylbenzo compounds, alkyl ammonium salts of unsaturated fatty acids, alkyl amines and their derivatives, alpha olefin sulfonates, alkenyl succinates, polyalphaolefins, linear mercaptans, synthetic acids such as based on 1-butene, 1-hexene, or 1-octene, chlorinated alpha olefins, aluminum alkyls, alkyl diphenylether disulfonates, fatty acids, lubricant additives, and ether primary alcohols.
摘要翻译：支链或直链烯烃的衍生物和通过卤化相同碳数的支链或正烷烃制备的醇，优选制备主要的单卤代烷烃，然后可以用金属氧化物氧化。本发明的伯醇的衍生物包括醇乙氧基化物，醇硫酸盐，醇硫酸化乙氧基化物，表面活性剂，包括由这些乙氧基化物和/或硫酸化乙氧基化物制成的表面活性剂，用这些表面活性剂制备的洗涤剂，烷氧基化醇，烷氧基化醇硫酸盐，聚甲基丙烯酸酯，胺及其衍生物，直链邻苯二甲酸酯，直链己二酸酯，醇醚胺，烷基甘油醚磺酸酯，硫代丙酸酯，烷基聚葡糖苷，醇磷酸酯，醇醚磷酸酯，脂肪酸酯，醇亚磷酸酯和二苯甲酮。仲醇衍生物包括仲醇乙氧基化物，仲醇硫酸盐，仲醇硫酸化乙氧基化物，表面活性剂，包括用这些乙氧基化物和/或硫酸化乙氧基化物制备的那些，以及用这些表面活性剂制成的洗涤剂。包括在本发明范围内的内烯烃衍生物包括烷基苯，烷基二甲苯，洗涤剂醇，增塑剂醇，烯基琥珀酸酯，醚仲醇，以及通过使用过氧化氢催化二烯化内烯烃的二醇和多元醇。包括在本发明范围内的α-烯烃衍生物包括内烯烃，烷基苯，烷基二甲苯，烷基酚，烷基萘，洗涤剂醇，增塑剂醇，苯基苯并化合物的烷基化物，不饱和脂肪酸的烷基铵盐，烷基胺及其衍生物，α-烯烃磺酸盐，烯基琥珀酸酯，聚α-烯烃，线性硫醇，合成酸，例如基于1-丁烯，1-己烯或1-辛烯，氯化α-烯烃，烷基铝，烷基二苯基醚二磺酸酯，脂肪酸，润滑剂添加剂和醚伯醇。

4. 发明申请

WO2006104909A2 CATALYTIC DISTILLATION PROCESS FOR PRIMARY HALOALKANES 审中-公开
标题翻译：催化蒸馏工艺
公开(公告)号：WO2006104909A2
公开(公告)日：2006-10-05
申请号：PCT/US2006/010848
申请日：2006-03-24
申请人： SHELL OIL COMPANY , FONG, Howard Lam-Ho , MURRAY, Brendan Dermot , SEMPLE, Thomas Carl
发明人： FONG, Howard Lam-Ho , MURRAY, Brendan Dermot , SEMPLE, Thomas Carl
CPC分类号： C07C17/23 , A61K8/20 , A61Q17/04 , C07C17/10 , C07C17/358 , C07C17/383 , C07C41/16 , C11D1/72 , C11D11/0082 , Y02P20/127 , C07C19/075 , C07C43/04
摘要： A process for making primary haloalkanes by catalytic distillation of internal haloalkanes which comprises a) introducing an internal haloalkane feed into a catalytic distillation column; b) isomerizing at least a portion of the internal haloalkane feed in the presence of an internal haloalkane isomerization catalyst at a temperature at or above the boiling point of the internal haloalkanes and below the temperature and pressure at which hydrogen halide is formed to form primary haloalkanes; and removing the primary haloalkanes from the catalytic distillation column.
摘要翻译：通过内部卤代烷烃的催化蒸馏制备主要卤代烷烃的方法，其包括：a）将内部卤代烷烃进料引入催化蒸馏塔; b）在内部卤代烷烃异构化催化剂的存在下，在内部卤代烷烃的沸点或高于内部卤代烷的沸点的温度和低于形成卤化氢的温度和压力下形成主要的卤代烷烃，异构化内部卤代烷烃进料的至少一部分 ; 并从催化蒸馏塔中除去主卤代烷烃。

5. 发明申请

WO2006104883A1 FORMATION OF HETEROATOM CONTAINING DERIVATIVES OF PARAFFINS 审中-公开
标题翻译：形成含有PARAFFINS的衍生物的杂交体
公开(公告)号：WO2006104883A1
公开(公告)日：2006-10-05
申请号：PCT/US2006/010768
申请日：2006-03-24
申请人： SHELL OIL COMPANY , FONG, Howard Lam-Ho , JOHNSON, Thomas, Haward , SEMPLE, Thomas, Carl
发明人： FONG, Howard Lam-Ho , JOHNSON, Thomas, Haward , SEMPLE, Thomas, Carl
IPC分类号： C07C41/30
CPC分类号： C07C41/16 , C07C17/23 , C07C17/38 , C07C19/075 , C07C43/11 , C07C43/15
摘要： A process by which alkyl halides may be reacted (coupled) with nucleophilic materials in the presence of a homogeneous catalyst system. The process comprises reacting (coupling) alkyl halides with a nucleophilic material in the presence of a homogeneous catalyst system to produce derivatives of alkyl halides, wherein the homogeneous catalyst system comprises at least one metal or metal compound which has the ability to form metal-halogen bonds.
摘要翻译：在均相催化剂体系存在下，烷基卤化物可与亲核材料反应（偶联）的方法。该方法包括在均相催化剂体系的存在下使烷基卤与亲核材料反应（偶合）以产生烷基卤化物的衍生物，其中均相催化剂体系包含至少一种具有形成金属卤素的能力的金属或金属化合物债券。

6. 发明申请

WO2009058654A1 PROCESS FOR PRODUCING SECONDARY ALCOHOL ALKOXY SULFATES 审中-公开
标题翻译：生产次级醇型烷基硫酸盐的方法
公开(公告)号：WO2009058654A1
公开(公告)日：2009-05-07
申请号：PCT/US2008/080918
申请日：2008-10-23
申请人： SHELL OIL COMPANY , SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , COLANTONIO, Maria Celeste , FONG, Howard Lam Ho , HORTON, Andrew David , MEURS, Jan Hermen Hendrik , SEMPLE, Thomas Carl , WIJNANS, Sanne , VAN ZON, Arie
发明人： COLANTONIO, Maria Celeste , FONG, Howard Lam Ho , HORTON, Andrew David , MEURS, Jan Hermen Hendrik , SEMPLE, Thomas Carl , WIJNANS, Sanne , VAN ZON, Arie
IPC分类号： C11D1/00
CPC分类号： C11D1/29
摘要： A process for making secondary alcohol alkoxy sulfates which comprises: (a) reacting carbon monoxide and hydrogen under Fischer-Tropsch conditions in the presence of a Fischer-Tropsch catalyst to produce a reaction mixture comprising paraffins, (b) contacting the paraffins with oxygen in the presence of an oxidation catalyst to produce secondary alcohols, (c) contacting the secondary alcohols with an alkylene oxide in the presence of a double metal cyanide catalyst to produce secondary alcohol alkoxylates, and (d) sulfating the secondary alcohol alkoxylates.
摘要翻译：制备仲醇烷氧基硫酸盐的方法，其包括：（a）在费 - 托催化剂存在下，在费 - 托条件下使一氧化碳和氢气反应，以产生包含链烷烃的反应混合物，（b）使链烷烃与氧气接触存在氧化催化剂以产生仲醇，（c）在双金属氰化物催化剂存在下使仲醇与烯化氧接触以产生仲醇烷氧基化物，和（d）将仲醇烷氧基化物硫酸化。

7. 发明申请

WO2007050745A1 INTERNAL OLEFINS PROCESS 审中-公开
标题翻译：内部过程
公开(公告)号：WO2007050745A1
公开(公告)日：2007-05-03
申请号：PCT/US2006/041767
申请日：2006-10-26
申请人： SHELL OIL COMPANY , FONG, Howard, Lam-Ho , MURRAY, Brendan, Dermot
发明人： FONG, Howard, Lam-Ho , MURRAY, Brendan, Dermot
IPC分类号： C07C5/23 , C07C5/25 , C07C2/04 , C07C2/34 , C07C11/02 , C07C11/08
CPC分类号： C07C11/02 , C07C2/08 , C07C2/34 , C07C5/2506 , C07C29/16 , C07C303/24 , C07C2521/04 , C07C2523/04 , C07C2531/22 , C11D1/146 , C11D11/0082 , C07C31/125 , C07C305/06 , C07C11/08
摘要： This invention provides a process for making internal olefins which comprises isomerizing a feed comprising one or more internal olefin(s) in the presence of an isomerization catalyst to produce alpha olefins and reacting said alpha olefins in the presence of a dimerization catalyst to produce internal olefins.
摘要翻译：本发明提供了一种制备内烯烃的方法，该方法包括在异构化催化剂存在下将包含一种或多种内烯烃的进料异构化以产生α-烯烃，并在二聚催化剂存在下使所述α-烯烃反应以产生内烯烃。

8. 发明申请

WO2005105709A1 PROCESS TO CONVERT LINEAR ALKANES INTO ALPHA OLEFINS 审中-公开
标题翻译：将线性烷烃转化成ALPHA油脂的方法
公开(公告)号：WO2005105709A1
公开(公告)日：2005-11-10
申请号：PCT/US2005/013493
申请日：2005-04-20
申请人： SHELL OIL COMPANY , CANO, Manuel, Luis , FONG, Howard, Lam-Ho , MURRAY, Brendan, Dermont , TREVINO, Lizbeth, Olivia, Cisneros
发明人： CANO, Manuel, Luis , FONG, Howard, Lam-Ho , MURRAY, Brendan, Dermont , TREVINO, Lizbeth, Olivia, Cisneros
IPC分类号： C07C1/30
CPC分类号： C07C29/124 , C07C1/30 , C07C11/02 , C07C17/10 , C07C17/358 , C07C17/37 , C07C2521/10 , C07C2521/14 , C07C2523/14 , C07C2523/44 , C07C2523/745 , C07C2523/78 , C07C19/075 , C07C19/01 , C07C31/125
摘要： This invention provides for a process to convert branched or linear alkanes to branched or linear alpha olefins (AO) of the same carbon number. The process comprises the steps of: a) halogenating linear alkanes, branched alkanes, or a mixture of linear and branched alkane to produce a mixture containing primary mono-haloalkanes and hydrogen halide; b) separating the hydrogen halide from the mixture and optionally neutralizing it with a metal oxide to produce a partially halogenated metal oxide and/or metal halide which may be regenerated; c) separating the primary mono-haloalkanes from the mixture; d) reacting the separated primary mono-haloalkanes with a metal oxide to produce a mixture of products that contains alpha olefins, unconverted primary mono-haloalkanes, possibly other reaction products, and a partially halogenated metal oxide and/or metal halide which may be regenerated; e) regenerating the partially halogenated metal oxide and/or metal halide to halogen and/or acid and a metal oxide (such as Cl2) for recycle by reaction with air or oxygen ; and f) removing the unreacted primary mono-haloalkane from the reaction mixture and then purifying the alpha olefin.
摘要翻译：本发明提供将支链或直链烷烃转化为相同碳数的支链或直链α-烯烃（AO）的方法。该方法包括以下步骤：a）将直链烷烃，支链烷烃或直链和支链烷烃的混合物卤化以产生含有主要单卤代烷烃和卤化氢的混合物; b）从混合物中分离卤化氢并任选地用金属氧化物中和，以产生可再生的部分卤化的金属氧化物和/或金属卤化物; c）从混合物中分离初级单卤代烷烃; d）使分离的初级单卤代烷烃与金属氧化物反应以产生含有α-烯烃，未转化的初级单卤代烷烃，可能的其它反应产物和可再生的部分卤化的金属氧化物和/或金属卤化物的产物的混合物 ; e）将部分卤化的金属氧化物和/或金属卤化物再生成卤素和/或酸和金属氧化物（例如Cl 2），以通过与空气或氧气反应再循环; 和f）从反应混合物中除去未反应的主要单卤代烷烃，然后纯化α-烯烃。

9. 发明申请

WO2010132325A1 AN INTEGRATED PROCESS TO PRODUCE HYDROCARBONS FROM NATURAL GAS CONTAINING CARBON DIOXIDE 审中-公开
标题翻译：从含有二氧化碳的天然气生产碳氢化合物的综合工艺
公开(公告)号：WO2010132325A1
公开(公告)日：2010-11-18
申请号：PCT/US2010/034174
申请日：2010-05-10
申请人： SHELL OIL COMPANY , SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , BRAVO, Jose Luis , FONG, Howard Lam Ho , SWAIN, Richard Dale
发明人： BRAVO, Jose Luis , FONG, Howard Lam Ho , SWAIN, Richard Dale
IPC分类号： C25B1/24 , C10G45/58
CPC分类号： C10G50/00
摘要： A process for producing higher hydrocarbons from methane which contains carbon dioxide which comprises: (a) contacting methane, with a halogen, preferably bromine, under process conditions sufficient to produce a monohalomethane, preferably monobromomethane, which contains unreacted carbon dioxide, (b) reacting the monohalomethane in the presence of a coupling catalyst to produce higher hydrocarbons which contain carbon dioxide, and (c) separating carbon dioxide from the higher hydrocarbons.
摘要翻译：一种从包含二氧化碳的甲烷生产高级烃的方法，包括：（a）在足以产生含有未反应的二氧化碳的单卤代甲烷，优选一溴甲烷的工艺条件下使甲烷与卤素，优选溴接触，（b）使在偶联催化剂存在下制备单卤代甲烷以产生含有二氧化碳的高级烃，和（c）从高级烃分离二氧化碳。

10. 发明申请

WO2010107696A1 AN INTEGRATED PROCESS TO COPRODUCE AROMATIC HYDROCARBONS AND ETHYLENE AND PROPYLENE 审中-公开
标题翻译：一体化芳香烃和乙烯和丙烯共聚物
公开(公告)号：WO2010107696A1
公开(公告)日：2010-09-23
申请号：PCT/US2010/027314
申请日：2010-03-15
申请人： SHELL OIL COMPANY , SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , FONG, Howard Lam Ho , SWAIN, Richard Dale
发明人： FONG, Howard Lam Ho , SWAIN, Richard Dale
IPC分类号： C07C17/00 , C07C15/00
CPC分类号： C07C37/58 , C01B3/26 , C01B7/093 , C01B2203/0277 , C07C1/26 , C07C2/64 , C07C4/14 , C07C5/327 , C07C6/126 , C07C15/46 , C07C17/10 , C07C37/02 , C07C37/04 , C07C37/08 , C07C51/265 , C07C407/00 , C07C409/10 , C10G29/26 , C10G50/00 , Y02P20/125 , C07C11/04 , C07C15/00 , C07C11/06 , C07C15/04 , C07C15/085 , C07C15/073 , C07C15/06 , C07C15/08 , C07C19/075 , C07C39/04 , C07C63/26
摘要： An integrated process for producing aromatic hydrocarbons and ethylene and/or propylene and optionally other lower olefins from low molecular weight hydrocarbons, preferably methane, which comprises: (a) contacting one or more low molecular weight alkanes, preferably methane, with a halogen, preferably bromine, under process conditions sufficient to produce a monohaloalkane, preferably monobromomethane, (b) reacting a first portion of the monohaloalkane in the presence of a coupling catalyst under process conditions sufficient to produce aromatic hydrocarbons and C2-5 alkanes, (c) separating the aromatic hydrocarbons from the product mixture of step (b) to produce aromatic hydrocarbons, (d) reacting a second portion of the monohaloalkane in the presence of a coupling catalyst under process conditions sufficient to produce ethylene and/or propylene.
摘要翻译：一种用于从低分子量烃（优选甲烷）生产芳烃和乙烯和/或丙烯和任选的其它低级烯烃的综合方法，其包括：（a）使一种或多种低分子量烷烃，优选甲烷与卤素溴，在足以产生单卤代烷烃，优选单溴甲烷的工艺条件下，（b）使偶联催化剂的第一部分在偶联催化剂存在下在足以产生芳烃和C 2-5烷烃的工艺条件下反应，（c）使来自步骤（b）的产物混合物的芳族烃生成芳族烃，（d）在足够产生乙烯和/或丙烯的工艺条件下，在偶联催化剂存在下使第二部分单卤代烷烃反应。

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