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81. 发明申请

WO2020186641A1 一种微界面强化蜡油加氢反应系统及方法审中-公开
公开(公告)号：WO2020186641A1
公开(公告)日：2020-09-24
申请号：PCT/CN2019/090316
申请日：2019-06-06
申请人：南京延长反应技术研究院有限公司
发明人：张志炳 , 周政 , 张锋 , 李磊 , 王宝荣 , 杨高东 , 罗华勋 , 孟为民 , 杨国强 , 田洪舟 , 曹宇
IPC分类号： C10G65/04 , C10G45/00
摘要：本发明涉及一种微界面强化蜡油加氢反应系统及方法，包括：液相进料单元、气相进料单元、微界面发生器、固定床反应器和分离罐。与传统的固定床反应器相比，本发明通过破碎气体使其形成微米尺度的微气泡，使微气泡与蜡油混合形成乳化液，以增大气液两相的相间面积，并达到在较低预设范围内强化传质的效果，在保证反应效率的同时，能够使反应过程中的压力降低10-80％；同时，本发明通过大幅度强化传质，因此可大幅减小气液比，这不但减少了气体的物耗，同时也降低了后续气体循环压缩的能耗；且本发明所述方法工艺苛刻度低，生产安全性高，吨产品成本低，市场竞争力强。

82. 发明申请

WO2019229072A1 RENEWABLE DIESEL FUEL PRODUCTION IN RETROFITTED FOSSIL PETROLEUM REFINERY TO PRODUCE BIOFUEL AND BIO-FEEDSTOCK FOR STEAM CRACKERS 审中-公开
公开(公告)号：WO2019229072A1
公开(公告)日：2019-12-05
申请号：PCT/EP2019/063843
申请日：2019-05-28
申请人： TOTAL RESEARCH & TECHNOLOGY FELUY
发明人： VERMEIREN, Walter
IPC分类号： C10G9/36 , C10G69/06 , C10G47/00 , C10G3/00 , C10G65/04 , C10G65/12 , C10G69/14
摘要： The present invention relates to a process for the conversion of a feedstock comprising at least 50 wt % related to the total weight of the feedstock of triglycerides, fatty acid esters and/or fatty acids having at least 10 carbon atoms into hydrogen, olefins, dienes, aromatics, gasoline, diesel fuel, jet fuel, naphtha and liquefied petroleum gas comprising : a) introducing of said feedstock in a first reactor to produce linear paraffins in presence of a hydrodesulfurization catalyst and hydrogen, b) separating the effluent of said first reactor in at least three parts to produce at least a first stream comprising part of said linear paraffins and at least a second stream comprising part of said linear paraffins, and at least a third stream comprising part of said linear paraffins c) sending said first stream to a steam cracker to produce hydrogen, olefins, dienes, aromatics and gasoline, diesel fuel being further fractionated; d) introducing said second stream into a second reactor in presence of a hydrocracking or hydroisomerization catalyst to produce a mixture comprising diesel fuel, jet fuel, naphtha and liquefied petroleum gas being further fractionated e) blending said third stream with the diesel fuel obtained at said step d) wherein said feedstock of said first reactor is diluted in order to limit the temperature increase within said first reactor; and wherein before entering the first reactor said dilution is performed with a weight ratio diluent : feedstock being 1:1, and wherein said diluent comprises at least part of said paraffins obtained at step b).

83. 发明申请

WO2019229049A1 PROCESS FOR DESULFURIZATION OF HYDROCARBONS 审中-公开
公开(公告)号：WO2019229049A1
公开(公告)日：2019-12-05
申请号：PCT/EP2019/063794
申请日：2019-05-28
申请人： HALDOR TOPSØE A/S
发明人： STREBEL, Christian Ejersbo
IPC分类号： C10G45/08 , C10G65/04 , C10G45/32 , C10G65/06 , B01J23/882
摘要： The present disclosure relates to a process for hydrodesulfurizing an olefinic naphtha feedstock while retaining a substantial amount of the olefins, which feedstock has a T 95 boiling point below 250°C and contains at least 50 ppmw of organically bound sulfur and from 5% to 60% olefins, said process comprising hydrodesulfurizing the feedstock in a sulfur removal stage in the presence of a gas comprising hydrogen and a hydrodesulfurization catalyst, at hydrodesulfurization reaction conditions including a tem- perature from 200°C to 350°C, a pressure of 2 barg or 5 barg to 10 barg, 15 barg, 25 barg or 35 barg, and gas to oil ratio of 500 Nm 3 /m 3 , 600 Nm 3 /m 3 , 700 Nm3/m3 or 750 10 Nm 3 /m 3 to 900 Nm 3 /m 3 or 1000 Nm 3 /m 3 , to convert at least 60 % of the organically bound sulfur to hydrogen sulfide and to produce a desulfurized product stream, with the associated benefit of such a process providing a lower octane loss at all severities above 60% HDS, compared to a process with similar conversion of organic sulfur with a lower gas to oil ratio, as measured by the selectivity slope, while avoiding excessive increase of equipment size by limiting gas to oil ratio.

84. 发明申请

WO2019138002A1 PROCESS FOR UPGRADING OXYGEN CONTAINING RENEWABLE OIL 审中-公开
公开(公告)号：WO2019138002A1
公开(公告)日：2019-07-18
申请号：PCT/EP2019/050554
申请日：2019-01-10
申请人： STEEPER ENERGY APS
发明人： IVERSEN, Steen B. , JENSEN, Claus Uhrenholt , RODRIGUEZ GUERRERO, Julie Katerine
IPC分类号： C10G65/04 , C01B3/38 , C10G3/00 , C10G1/00
摘要： The invention relates to a process for producing an upgraded renewable oil from renewable carbonaceous material(-s) comprising providing an oxygen containing renewable crude oil having an oxygen content in the range of 3.0 to 20 % by weight, a water content of less than 1.5 wt. %, a total acid number in the range from 5 to 80 mg KOH/g, a fraction of the oil having a boiling point below than 350 °C of less than 70 % by weight, and a residue fraction having a boiling point of more than 450 °C of at least 10 %by weight, pressurisingthe oxygen containing renewable crude oil to an operational pressure in the range 60 to 200 bar; adding and mixing hydrogen to the pressurized oxygen containing renewable crude oil,contacting the pressurized mixture with at least one heterogeneous catalyst contained in a first reaction zone at a temperature of 260 to 350 °C having a weight based hourly space velocity (WHSV) in the range 0.1 to 1 h -1 so as to produce a partially hydrogenated and deoxygenated oil,separating water, gas and optionally a low boiling fraction from the partially hydrogenated and deoxygenatedoil from the first reaction zone, heating the partially hydrogenated and deoxygenated oil from the first reaction zone to a temperature in the range 350 to 400 °C,contacting the partially hydrogenated and deoxygenated oil with at least one heterogeneous catalysts in a second reaction zone at a temperature of 350 to 400 °C at weight based hourly space velocity (WHSV) in the range 0.1 to 1.5 h -1 , separating the product from the second reaction zone into a at least a gas fraction, a water fraction, a low boiling point renewable liquid hydrocarbon fraction and a high boiling point renewable liquid hydrocarbon fraction, contacting the low boiling point fraction from the second reaction zone with hydrogen and one or more heterogeneous catalysts at a temperature in the range 350 to 390 °C in a third reaction zone having a weight based space velocity in the range 0.1 to 1 h -1 , thereby producing a first product stream and contacting the high boiling point oil fraction with hydrogen and one or more heterogeneous catalysts at a temperature in the range 360-420 °C in a fourth reaction zone having a weight based space velocity in the range 0.1 to 1 h -1 , thereby producing a second product stream.

85. 发明申请

WO2018217505A1 PROCESS FOR MAXIMIZING XYLENES PRODUCTION FROM HEAVY AROMATICS FOR USE THEREIN 审中-公开
公开(公告)号：WO2018217505A1
公开(公告)日：2018-11-29
申请号：PCT/US2018/032874
申请日：2018-05-16
申请人： SAUDI ARABIAN OIL COMPANY , ARAMCO SERVICES COMPANY
发明人： XU, Qi , ABUDAWOUD, Raed , JAZZAR, Ahmad, A. , ZHANG, Zhonglin
IPC分类号： C07C6/12 , C07C4/18 , C10G47/00 , C07C15/06 , C07C15/04 , C07C15/08 , C10G65/04
摘要： A method for producing xylenes from a heavy reformate feed includes the steps of introducing the heavy reformate feed and a hydrogen feed to a dealkylation reactor, reacting the heavy reformate feed with the hydrogen gas in the presence of the dealkylation catalyst in the dealkylation reactor to produce a dealkylation effluent, introducing the dealkylation effluent to a splitter unit, separating the dealkylation effluent into a light gas stream, a toluene stream, a benzene stream, a C9 aromatics stream, a C10+ aromatics stream, and a mixed xylene stream in the splitter unit, introducing the toluene stream, the C9 aromatics stream, and a hydrogen stream into a transalkylation reactor, reacting the toluene stream and the C9 aromatics stream in the presence of the transalkylation catalyst to produce a transalkylation effluent, introducing the transalkylation effluent to the splitter unit, and separating the transalkylation effluent in the splitter unit.

86. 发明申请

WO2018005094A1 NOBLE METAL HYDROGENATION CATALYSTS AND AROMATIC SATURATION METHODS 审中-公开
标题翻译：贵金属加氢催化剂和芳烃饱和方法
公开(公告)号：WO2018005094A1
公开(公告)日：2018-01-04
申请号：PCT/US2017/037416
申请日：2017-06-14
申请人： EXXONMOBIL RESEARCH AND ENGINEERING COMPANY
发明人： LANCI, Michael, P. , SOLED, Stuart, L. , GUZMAN, Javier , MISEO, Sabato , GREEN, Thomas, E. , BAUMGARTNER, Joseph, E. , ZHANG, Lei , KLIEWER, Christine, E. , KOZIOL, Lukasz , MAO, Kanmi , OWENS, Tracie, L. , SCHLEICHER, Gary, P.
IPC分类号： C10G65/04 , B01J23/40 , C10G65/12
摘要： Methods are provided for modifying hydrogenation catalysts having silica supports (or other non-alumina supports) with additional alumina, and using such catalysts to achieve unexpectedly superior hydrogenation of feedstocks. The modified hydrogenation catalysts can have a relatively low cracking activity while providing an increased activity for hydrogenation.
摘要翻译：提供了用于改性具有二氧化硅载体（或其他非氧化铝载体）和另外的氧化铝的氢化催化剂的方法，并且使用这样的催化剂来实现出乎意料地优异的原料氢化。改性的氢化催化剂可以具有相对低的裂化活性，同时提供增加的氢化活性。

87. 发明申请

WO2017186484A1 PROCÉDÉ DE CONVERSION COMPRENANT DES LITS DE GARDE PERMUTABLES D'HYDRODEMETALLATION, UNE ETAPE D'HYDROTRAITEMENT EN LIT FIXE ET UNE ETAPE D'HYDROCRAQUAGE EN REACTEURS PERMUTABLES 审中-公开
标题翻译：转换过程，包括床GUARD SWAP加氢，固定床了一步加氢处理和加氢反应堆加氢裂化SWAP一步
公开(公告)号：WO2017186484A1
公开(公告)日：2017-11-02
申请号：PCT/EP2017/058686
申请日：2017-04-11
申请人： IFP ENERGIES NOUVELLES
发明人： WEISS, Wilfried , TELLIER, Elodie , CHATRON-MICHAUD, Pascal
IPC分类号： C10G65/04 , C10G65/12 , C10G45/08 , C10G47/12 , C10G7/06 , C10G21/14 , C10G27/12 , C10G31/10 , C10G31/09 , C10G32/02
摘要： L'invention concerne un procédé de traitement d'une charge hydrocarbonée permettant d'obtenir une fraction hydrocarbonée lourde à basse teneur en soufre, ledit procédé comprenant les étapes suivantes : a) une étape d'hydrodémétallation en réacteurs permutables b) une étape d'hydrotraitement en lit fixe de l'effluent issu de l'étape a), c) une étape d'hydrocraquage en réacteurs permutables de l'effluent issu de l'étape b), d) une étape de séparation de l'effluent issu de l'étape c), e) une étape de précipitation des sédiments, f) une étape de séparation physique desdits sédiments de la fraction liquide lourde issue de l'étape d), g) une étape de récupération de la coupe de distillât utilisée dans l'étape e).
摘要翻译：
本发明涉及一种方法处理烃原料以获得重质烃馏分; 低硫含量的工艺包括以下步骤：a）在反应性反应器中的加氢处理步骤b）来自步骤a）的流出物的固定床加氢处理步骤，（c）来自步骤（b）的流出物的可置换反应器中的加氢裂化步骤，（d）将来自步骤（c），（e）沉淀物沉淀过程，（f）从（d），（g）物理分离重质液体部分的所述组分的过程，回收步骤e）中使用的酒厂切割的步骤。

88. 发明申请

WO2017112647A1 TRIM DEWAXING OF DISTILLATE FUEL 审中-公开
标题翻译： TRIM对馏分燃料进行脱蜡
公开(公告)号：WO2017112647A1
公开(公告)日：2017-06-29
申请号：PCT/US2016/067717
申请日：2016-12-20
申请人： EXXONMOBIL RESEARCH AND ENGINEERING COMPANY
发明人： PODSIADLO, Paul , MCCARTHY, Stephen, J. , BALIBAN, Richard, C. , MILLER, Amanda, K.
IPC分类号： B01J29/44 , B01J29/46 , B01J29/48 , B01J29/70 , B01J37/00 , B01J37/02 , C10G45/08 , C10G45/10 , C10G45/12 , C10G45/62 , C10G45/64 , C10G65/04
CPC分类号： C10G69/02 , B01J29/44 , B01J29/48 , B01J29/7461 , B01J29/7861 , B01J2229/186 , B01J2229/42 , C10G45/08 , C10G45/10 , C10G45/12 , C10G45/62 , C10G45/64 , C10G65/043 , C10G2300/202 , C10G2300/70 , C10G2400/04 , C10G2400/10
摘要： Methods and catalysts are provided for performing dewaxing of diesel boiling range fractions, such as trim dewaxing, that allow for production of diesel boiling range fuels with improved cold flow properties at desirable yields. In some aspects, the methods can include use of dewaxing catalysts based on an MEL framework structure (ZSM-11) to provide improved dewaxing activity. In some aspects improved dewaxing is achieved operating at lower pressures and with higher amounts of organic nitrogen slip from hydrotreatment.
摘要翻译：提供了用于进行柴油沸程馏分脱蜡的方法和催化剂，例如装饰脱蜡，其允许以期望的产率生产具有改进的冷流性质的柴油沸程燃料。在一些方面，该方法可以包括使用基于MEL骨架结构（ZSM-11）的脱蜡催化剂以提供改进的脱蜡活性。在一些方面，改进的脱蜡在较低的压力下操作并且加氢处理的有机氮逸出量较高。

89. 发明申请

WO2017112558A1 TRIM DEWAXING OF DISTILLATE FUEL 审中-公开
标题翻译： TRIM对馏分燃料进行脱蜡
公开(公告)号：WO2017112558A1
公开(公告)日：2017-06-29
申请号：PCT/US2016/067423
申请日：2016-12-19
申请人： EXXONMOBIL RESEARCH AND ENGINEERING COMPANY
发明人： MCCARTHY, Stephen, J. , PODSIADLO, Paul , BAI, Chuansheng , DOUGHERTY, Richard, C. , LAI, Wenyih, Frank , LONERGAN, William, W.
IPC分类号： B01J29/44 , B01J29/46 , B01J29/48 , B01J29/70 , B01J37/00 , B01J37/02 , C10G45/08 , C10G45/10 , C10G45/12 , C10G45/62 , C10G45/64 , C10G65/04
CPC分类号： B01J29/40 , B01J29/48 , B01J29/703 , B01J29/7861 , B01J29/80 , B01J35/002 , B01J35/1019 , B01J37/0009 , B01J37/0018 , B01J37/0203 , C10G45/08 , C10G45/10 , C10G45/12 , C10G45/62 , C10G45/64 , C10G65/043 , C10G2400/04 , C10G2400/10
摘要： Methods and catalysts are provided for performing dewaxing of diesel boiling range fractions, such as trim dewaxing, that allow for production of diesel boiling range fuels with improved cold flow properties at desirable yields. In some aspects, the methods can include use of dewaxing catalysts based on an MEL framework structure (ZSM-11) to provide improved dewaxing activity. This can provide sufficient dewaxing activity to achieve a desired level of improvement in cold flow properties at the lower hydrotreating temperatures that are generally desired near the start of operation of a hydrotreating reactor. In other aspects, the methods can include use of MEL dewaxing catalysts with reduced ratios of molecular sieve to binder so that trim dewaxing can be provided while maintaining a desirable yield under end-of-run hydrotreating conditions.
摘要翻译：提供了用于进行柴油沸程馏分脱蜡的方法和催化剂，例如装饰脱蜡，其允许以期望的产率生产具有改进的冷流性质的柴油沸程燃料。在一些方面，该方法可以包括使用基于MEL骨架结构（ZSM-11）的脱蜡催化剂以提供改进的脱蜡活性。这可以提供足够的脱蜡活性，以在加氢处理反应器开始操作附近通常期望的较低加氢处理温度下实现冷流性质的期望水平的改善。在其它方面，所述方法可包括使用MEL脱蜡催化剂，其分子筛与粘合剂的比率降低，从而可提供修饰脱蜡，同时在运行结束的加氢处理条件下保持所需产率。

90. 发明申请

WO2017112377A1 BASE METAL DEWAXING CATALYST 审中-公开
标题翻译：碱金属脱蜡催化剂
公开(公告)号：WO2017112377A1
公开(公告)日：2017-06-29
申请号：PCT/US2016/064144
申请日：2016-11-30
申请人： EXXONMOBIL RESEARCH AND ENGINEERING COMPANY
发明人： MCCARTHY, Stephen, J. , BAI, Chuansheng , LAI, Wenyih, F. , PODSIADLO, Paul , LONERGAN, William, W.
IPC分类号： C10G45/62 , C10G45/64 , C10G45/10 , C10G45/12 , B01J29/44 , B01J29/46 , B01J29/48 , B01J29/70 , B01J37/00 , B01J37/02 , B01J37/20 , C10G65/04
CPC分类号： C10G45/64 , B01J29/48 , B01J29/7861 , B01J2229/186 , B01J2229/42 , C10G45/10 , C10G45/12 , C10G45/62 , C10G65/043 , C10G2400/04 , C10G2400/10
摘要： Methods are provided for making base metal catalysts with improved activity. After forming catalyst particles based on a support comprising a zeolitic molecular sieve, the catalyst particles can be impregnated with a solution comprising a) metal salts (or other precursors) for a plurality of base metals and b) an organic dispersion agent comprising 2 to 10 carbons. The impregnated support particles can be dried to form a base metal catalyst, and then optionally sulfided to form a sulfided base metal catalyst. The resulting (sulfided) base metal catalyst can have improved activity for cloud point reduction and/or for improved activity for heteroatom removal, relative to a base metal dewaxing catalyst prepared without the use of a dispersion agent.
摘要翻译：提供了用于制备具有改善的活性的贱金属催化剂的方法。在形成基于包含沸石分子筛的载体的催化剂颗粒之后，可以用包含a）用于多种贱金属的金属盐（或其他前体）和b）包含2至10 碳。浸渍的载体颗粒可以被干燥以形成贱金属催化剂，然后任选地被硫化以形成硫化的贱金属催化剂。与不使用分散剂制备的贱金属脱蜡催化剂相比，所得（硫化）贱金属催化剂可降低浊点降低活性和/或提高杂原子去除活性。

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