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1. 发明授权

US07641972B2 Surface-modified nanoparticles comprising polysiloxane modifier, their preparation and use 有权
标题翻译：包含聚硅氧烷改性剂的表面改性纳米粒子，其制备和应用
公开(公告)号：US07641972B2
公开(公告)日：2010-01-05
申请号：US11354338
申请日：2006-02-14
申请人： Ulrich Nolte , Alfred Bubat , Karlheinz Haubennestel , Thomas Sawitowski
发明人： Ulrich Nolte , Alfred Bubat , Karlheinz Haubennestel , Thomas Sawitowski
IPC分类号： B32B5/16 , B05D7/00
CPC分类号： C09C1/3684 , B82Y30/00 , C01P2004/64 , C08G18/3893 , C08G18/4277 , C08G18/807 , C08K3/22 , C08K3/36 , C08K9/06 , C09C1/3081 , C09C1/407 , C09C3/12 , C09D7/62 , C09D7/67 , C09D7/68 , C09D175/04 , Y10T428/2991 , Y10T428/2995 , Y10T428/31663 , C08L2666/54
摘要： The invention relates to surface-modified nanoparticles composed of metal or semimetal oxides or hydroxides and having been reacted on their surface with a modifier, with formation of covalent bonds. The modifier is a polysiloxane. The invention also relates to a process for preparing the nanoparticles, to their use as fillers in coating materials, plastics, foams and nail varnishes, and to dispersions which comprise the nanoparticles.
摘要翻译：本发明涉及由金属或半金属氧化物或氢氧化物组成的表面改性纳米颗粒，并且在其表面上与改性剂反应形成共价键。改性剂是聚硅氧烷。本发明还涉及一种制备纳米颗粒的方法，其用作涂料，塑料，泡沫和指甲油中的填料，以及包含纳米颗粒的分散体。

2. 发明申请

US20060204528A1 Surface-modified nanoparticles, their preparation and use 有权
标题翻译：表面改性纳米粒子，其制备和应用
公开(公告)号：US20060204528A1
公开(公告)日：2006-09-14
申请号：US11354338
申请日：2006-02-14
申请人： Ulrich Nolte , Alfred Bubat , Karlheinz Haubennestel , Thomas Sawitowski
发明人： Ulrich Nolte , Alfred Bubat , Karlheinz Haubennestel , Thomas Sawitowski
IPC分类号： A61K8/02
CPC分类号： C09C1/3684 , B82Y30/00 , C01P2004/64 , C08G18/3893 , C08G18/4277 , C08G18/807 , C08K3/22 , C08K3/36 , C08K9/06 , C09C1/3081 , C09C1/407 , C09C3/12 , C09D7/62 , C09D7/67 , C09D7/68 , C09D175/04 , Y10T428/2991 , Y10T428/2995 , Y10T428/31663 , C08L2666/54
摘要： The invention relates to surface-modified nanoparticles composed of metal or semimetal oxides or hydroxides and having been reacted on their surface with a modifier, with formation of covalent bonds. The modifier is a polysiloxane. The invention also relates to a process for preparing the nanoparticles, to their use as fillers in coating materials, plastics, foams and nail varnishes, and to dispersions which comprise the nanoparticles.
摘要翻译：本发明涉及由金属或半金属氧化物或氢氧化物组成的表面改性纳米颗粒，并且在其表面上与改性剂反应形成共价键。改性剂是聚硅氧烷。本发明还涉及一种制备纳米颗粒的方法，其用作涂料，塑料，泡沫和指甲油中的填料，以及包含纳米颗粒的分散体。

3. 发明授权

US08530048B2 Surface-modified particles and production method 有权
标题翻译：表面改性颗粒及其制备方法
公开(公告)号：US08530048B2
公开(公告)日：2013-09-10
申请号：US12376519
申请日：2007-07-16
申请人： Ulrich Nolte , Alfred Bubat , Karlheinz Haubennestel , Thomas Sawitowski
发明人： Ulrich Nolte , Alfred Bubat , Karlheinz Haubennestel , Thomas Sawitowski
IPC分类号： B32B5/16 , B32B1/00 , B05D7/00
CPC分类号： C09C3/12 , B82Y30/00 , C01P2004/62 , C01P2004/64 , C08K3/22 , C08K9/06 , C09C1/407 , C09D7/62 , C09D7/67 , C09D7/68 , Y10T428/2991 , Y10T428/2995
摘要： The invention relates to surface-modified particles, more particularly inorganic-based particles having reactive surfaces, more particularly surfaces containing silane-reactive and/or siloxane-reactive groups, preferably hydroxyl-containing surfaces and/or particles comprising or consisting of metal and/or semi-metal oxides and/or hydroxides, preferably nanoparticles, which on their surface have a polysiloxane-based modifier having more particularly been reacted on their surface with a polysiloxane-based modifier, preferably with the formation of chemical bonds, more particularly covalent bonds, and also to a method of producing these surface-modified particles.
摘要翻译：本发明涉及具有反应性表面的表面改性颗粒，更特别是含有反应性表面的无机基颗粒，更具体地说，含有硅烷反应性和/或硅氧烷反应性基团，优选含羟基的表面和/或包含金属和/ 或半金属氧化物和/或氢氧化物，优选纳米颗粒，其在其表面上具有聚硅氧烷基改性剂，其更特别地在其表面上与基于聚硅氧烷的改性剂反应，优选形成化学键，更特别是共价键，以及这些表面改性粒子的制造方法。

4. 发明申请

US20100048809A1 SURFACE-MODIFIED PARTICLES AND PRODUCTION METHOD 有权
标题翻译：表面改性颗粒和生产方法
公开(公告)号：US20100048809A1
公开(公告)日：2010-02-25
申请号：US12376519
申请日：2007-07-16
申请人： Ulrich Nolte , Alfred Bubat , Karlheinz Haubennestel , Thomas Sawitowski
发明人： Ulrich Nolte , Alfred Bubat , Karlheinz Haubennestel , Thomas Sawitowski
IPC分类号： C08L83/04 , B32B1/00
CPC分类号： C09C3/12 , B82Y30/00 , C01P2004/62 , C01P2004/64 , C08K3/22 , C08K9/06 , C09C1/407 , C09D7/62 , C09D7/67 , C09D7/68 , Y10T428/2991 , Y10T428/2995
摘要： The invention relates to surface-modified particles, more particularly inorganic-based particles having reactive surfaces, more particularly surfaces containing silane-reactive and/or siloxane-reactive groups, preferably hydroxyl-containing surfaces and/or particles comprising or consisting of metal and/or semi-metal oxides and/or hydroxides, preferably nanoparticles, which on their surface have a polysiloxane-based modifier having more particularly been reacted on their surface with a polysiloxane-based modifier, preferably with the formation of chemical bonds, more particularly covalent bonds, and also to a method of producing these surface-modified particles.
摘要翻译：本发明涉及具有反应性表面的表面改性颗粒，更特别是含有反应性表面的无机基颗粒，更具体地说，含有硅烷反应性和/或硅氧烷反应性基团，优选含羟基的表面和/或包含金属和/ 或半金属氧化物和/或氢氧化物，优选纳米颗粒，其在其表面上具有聚硅氧烷基改性剂，其更特别地在其表面上与基于聚硅氧烷的改性剂反应，优选形成化学键，更特别是共价键，以及这些表面改性粒子的制造方法。

5. 发明申请

US20060009555A1 Polyester-modified polysiloxanes and their use as additives for thermoplastics, moulding compounds and coating materials 有权
公开(公告)号：US20060009555A1
公开(公告)日：2006-01-12
申请号：US11178231
申请日：2005-07-08
申请人： Karlheinz Haubennestel , Alfred Bubat , Hans-Willi Boegershausen , Wolfgang Griesel , Ulrich Nolte
发明人： Karlheinz Haubennestel , Alfred Bubat , Hans-Willi Boegershausen , Wolfgang Griesel , Ulrich Nolte
IPC分类号： C08K5/24
CPC分类号： C08G77/445 , C08L83/10 , C08L101/00 , C09D7/47 , C09D183/10 , D01F1/10 , C08L2666/02 , C08L83/00
摘要： The invention relates to polyester-modified poly-siloxanes of the general formula (I) where A is an alkyl group having 1 to 8 carbon atoms, Z is an aliphatic group having 1 to 14 carbon atoms, R is an aliphatic and/or cycloaliphatic and/or aromatic poly-ester group containing at least 3 and having a weight-average molecular weight of 200 to 4000 g/mol, with no Zerewitinoff hydrogen atoms, Q is a group which contains no Zerewitinoff hydrogen atoms and is free from reactive carbon-carbon multiple bonds, m is 3 to 200 and o+n=2, with both o and n being other than zero. The invention further relates to the use of the compounds of the invention in thermoplastics, moulding compounds and coating materials.

6. 发明授权

US07504469B2 Polyester-modified polysiloxanes and their use as additives for thermoplastics, moulding compounds and coating materials 有权
标题翻译：聚酯改性聚硅氧烷及其作为热塑性塑料，模塑料和涂料的添加剂
公开(公告)号：US07504469B2
公开(公告)日：2009-03-17
申请号：US11178231
申请日：2005-07-08
申请人： Karlheinz Haubennestel , Alfred Bubat , Hans-Willi Boegershausen , Wolfgang Griesel , Ulrich Nolte
发明人： Karlheinz Haubennestel , Alfred Bubat , Hans-Willi Boegershausen , Wolfgang Griesel , Ulrich Nolte
IPC分类号： C08G77/04 , C07F7/08 , C07F7/00
CPC分类号： C08G77/445 , C08L83/10 , C08L101/00 , C09D7/47 , C09D183/10 , D01F1/10 , C08L2666/02 , C08L83/00
摘要： The invention relates to polyester-modified poly-siloxanes of the general formula (I) where A is an alkyl group having 1 to 8 carbon atoms, Z is an aliphatic group having 1 to 14 carbon atoms, R is an aliphatic and/or cycloaliphatic and/or aromatic poly-ester group containing at least 3 and having a weight-average molecular weight of 200 to 4000 g/mol, with no Zerewitinoff hydrogen atoms, Q is a group which contains no Zerewitinoff hydrogen atoms and is free from reactive carbon-carbon multiple bonds, m is 3 to 200 and o+n=2, with both o and n being other than zero. The invention further relates to the use of the compounds of the invention in thermoplastics, moulding compounds and coating materials.
摘要翻译：本发明涉及通式（I）的聚酯改性聚硅氧烷，其中A是具有1至8个碳原子的烷基，Z是具有1至14个碳原子的脂族基团，R是脂族和/或脂环族和/或含有至少3并且具有200至4000g / mol的重均分子量的芳族聚酯基团，没有Zerewitinoff氢原子，Q是不含Zerewitinoff氢原子且不含活性碳的基团碳多重键，m为3〜200，o + n = 2，o和n均不为0。本发明还涉及本发明化合物在热塑性塑料，模塑料和涂料中的用途。

7. 发明授权

US07230051B2 Use of polyacrylate-modified polysiloxanes as levelling agents in coating compositions 有权
标题翻译：在涂料组合物中使用聚丙烯酸酯改性的聚硅氧烷作为流平剂
公开(公告)号：US07230051B2
公开(公告)日：2007-06-12
申请号：US10465536
申请日：2003-06-19
申请人： Bernd Gobelt , Alfred Bubat , Albert Frank , Karlheinz Haubennestel
发明人： Bernd Gobelt , Alfred Bubat , Albert Frank , Karlheinz Haubennestel
IPC分类号： C08L83/02
CPC分类号： C08G77/442 , C08F293/005 , C09D7/47 , Y10S525/934
摘要： The invention relates to the use of block copolymers as leveling agents for surface coatings, having a weight-average molecular weight of from 1000 to 100000. The leveling agent is a linear or branched block copolymer composed of a polysiloxane block and one or more blocks prepared from ethylenically unsaturated monomers by controlled free-radical addition polymerization.The invention also relates to coating compositions which comprise the leveling agent.
摘要翻译：本发明涉及嵌段共聚物作为表面涂料的流平剂的用途，其重均分子量为1000-100000。流平剂是由聚硅氧烷嵌段和一个或多个嵌段制备的直链或支链嵌段共聚物通过控制的自由基加成聚合从烯属不饱和单体中获得。本发明还涉及包含流平剂的涂料组合物。

8. 发明授权

US06512058B1 Method of producing modified vinyl ether polymers 有权
标题翻译：改性乙烯基醚聚合物的制备方法
公开(公告)号：US06512058B1
公开(公告)日：2003-01-28
申请号：US09531584
申请日：2000-03-21
申请人： Karlheinz Haubennestel , Alfred Bubat
发明人： Karlheinz Haubennestel , Alfred Bubat
IPC分类号： C08F800
CPC分类号： C08F8/00 , C08F8/18 , C08F8/30 , C08F2810/30 , C08F116/18
摘要： This invention relates to a method of producing modified vinyl ether polymers, wherein vinyl ether polymers comprising recurring units of general formula (I) where R represents a C2-C4 alkyl group and x denotes an integer from 10 to 1000, are partially transetherified with compounds of general formula Y—OH, wherein Y represents aliphatic and/or cycloaliphatic hydrocarbon groups comprising 5 to 30 carbon atoms, the hydrogen atoms of which can be replaced at least in part by halogen atoms and/or aryl radicals, and/or represents aliphatic, cycloaliphatic and/or aromatic groups with a molecular weight of up to 6000 which contain at least one ether group —O— or an ester group —COO— within the molecule, in the presence of compounds of the platinum metals with the release of the corresponding C2-C4 alcohols, wherein statistically at least one R radical is replaced by a Y radical per molecule of vinyl ether polymer.
摘要翻译：本发明涉及一种制备改性乙烯基醚聚合物的方法，其中包含通式（I）的重复单元的乙烯基醚聚合物，其中R表示C 2 -C 4烷基，x表示10至1000的整数，其与化合物部分转化的通式Y-OH，其中Y表示包含5至30个碳原子的脂族和/或脂环族烃基，其氢原子可至少部分地被卤素原子和/或芳基取代，和/或表示脂族，分子量高达6000的脂环族和/或芳族基团，其在分子内含有至少一个醚基-O-或酯基-COO-，在铂金属化合物的存在下释放相应的C 2 -C 4醇，其中统计学上每个乙烯基醚聚合物每一个Y基团被Y基团代替。

9. 发明授权

US07122599B2 Coating compositions and polymeric moulding compounds having anti-adhesion and dirt repellency properties 有权
标题翻译：涂料组合物和具有防粘附性和防污性的聚合物模塑料
公开(公告)号：US07122599B2
公开(公告)日：2006-10-17
申请号：US09967504
申请日：2001-09-28
申请人： Karlheinz Haubennestel , Alfred Bubat , Albert Frank , Axel Woocker , Udo Krappe
发明人： Karlheinz Haubennestel , Alfred Bubat , Albert Frank , Axel Woocker , Udo Krappe
IPC分类号： C08L43/04
CPC分类号： C08G77/42 , C08G77/442 , C08G77/445 , C08G77/458
摘要： The invention relates to coating compositions having anti-adhesion and dirt repellency properties, these compositions being admixed as additive with from 0.1 to 10% by weight, based on the solids content of the coating composition, of a branched polymer which possesses a weight-average molecular weight of from 2000 to 200,000 and comprises a polymeric base molecule and also polydiorganosiloxane side chains which are bonded covalently to the base molecule via Si—C bonds, have a weight-average molecular weight of between 1000 and 30,000, and whose fraction of the total weight of the branched polymer is from 5 to 25% by weight. The present invention further relates to polymeric moulding compounds having anti-adhesion and dirt repellency properties, to which this branched polymer is added as additive in an amount of from 0.1 to 10% by weight, based on the total weight of the polymeric moulding compounds. The invention additionally relates to the use of the branched polymers as additives for coating compositions and polymeric moulding compounds.
摘要翻译：本发明涉及具有防粘附性和防污性的涂料组合物，这些组合物以占涂料组合物的固体含量为基准的0.1至10重量％的混合添加剂，其具有重均分子量分子量为2000至200,000，并且包含通过Si-C键与基础分子共价键合的聚合物基础分子和聚二有机硅氧烷侧链，其重均分子量为1000至30,000，并且其分子量为支链聚合物的总重量为5〜25重量％。本发明还涉及具有抗粘附性和防污性的聚合物模塑料，该支化聚合物以其占聚合物模塑料总重量的0.1至10重量％的量加入其中。本发明还涉及使用支化聚合物作为涂料组合物和聚合物模塑料的添加剂。

10. 发明申请

US20060216259A1 Organosilane-modified polysiloxanes and their use for surface modification 有权
公开(公告)号：US20060216259A1
公开(公告)日：2006-09-28
申请号：US11353856
申请日：2006-02-14
申请人： Karlheinz Haubennestel , Alfred Bubat , Daniela Betcke , Juergen Hartmann
发明人： Karlheinz Haubennestel , Alfred Bubat , Daniela Betcke , Juergen Hartmann
IPC分类号： C08G77/38 , C08F283/12 , A61K8/89
CPC分类号： C09C1/3684 , C01P2006/22 , C08G77/14 , C08L83/06 , C09B67/0013 , C09B68/41 , C09C1/028 , C09C1/407 , C09C3/12
摘要： The invention relates to organosilane-modified polysiloxanes of the following formula: where x=0 to 200, y=5 to 100, z=0 to 50 and p=1 to 25; R1, R2, R3, R4 and R5 independently of one another are saturated or unsaturated, straight-chain or branched alkyl radicals having 1 to 4 carbon atoms and/or aryl radicals having 6 to 9 carbon atoms; R6 is a straight-chain or branched alkyl radical having 6 to 22 carbon atoms; R7 is a radical —(CH2)s-M-Z, where s is 2 to 20, M is an aliphatic group containing at least one —O—CO— or —CO—O— group and optionally ether groups, and Z is hydrogen, —CO—CH3 or a straight-chain or branched alkyl radical having 1 to 4 carbon atoms; R8 is a radical —(CH2)n—Si(R11)v(R12)3-v, where v is 0, 1 or 2, n is 2 to 16, R11 is a straight-chain or branched alkyl radical having 1 to 4 carbon atoms, and R12 is a radical selected from the group OR13, O—CO—R13, halogen or haloalkyl having 1 to 6 carbon atoms, in which R13 is an aromatic radical or a straight-chain, branched or cyclic alkyl radical having 1 to 6 carbon atoms and optionally containing ether and/or thioether groups; and R9 and R10 independently of one another possess the definition of R1, R2, R3, R4, R5, R6, R7 or R8. The invention additionally relates to the use of the organo-modified polysiloxanes for surface coating, and to their preparation.

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