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1. 发明授权

US5929272A Aliphatic epoxide-amine adducts with substantial side-chain, branching process for their preparation, and their use 失效
标题翻译：脂肪族环氧 - 胺加合物具有实质的侧链，其制备方法及其用途
公开(公告)号：US5929272A
公开(公告)日：1999-07-27
申请号：US641733
申请日：1996-05-02
申请人： Ulrich Epple , Manfred Marten , Uwe Kubillus , Harald Oswald
发明人： Ulrich Epple , Manfred Marten , Uwe Kubillus , Harald Oswald
IPC分类号： C08G59/02 , C08G18/32 , C08G18/64 , C08G59/00 , C08G59/14 , C08G59/18 , C08G59/40 , C08G59/64 , C08L63/00 , C09D133/00 , C09D133/04 , C09D133/06 , C09D133/08 , C09D163/00 , C09D167/00 , C09J163/00 , C09K3/10 , C07C67/18
CPC分类号： C09D133/066 , C08G18/3271 , C08G18/643 , C08G59/184 , C08G59/64 , C09D163/00 , C09D167/00 , C08L63/00
摘要： Epoxide-amine adducts having a proportion by mass of at least 20% of aliphatic epoxide or amine units which comprise at least one tertiary or quaternary carbon atom are disclosed. The adducts are employed as binders for coatings of relatively high environment-friendliness, if desired, for example, in a mixture with other hydroxy-functional binders, and as reactive component in corresponding adhesive compositions and sealing compounds.
摘要翻译：公开了具有至少20％脂肪族环氧化物或包含至少一个叔碳原子或季碳原子的胺单元的质量比的环氧胺加合物。如果需要，加合物用作具有相对高的环境友好性的涂料的粘合剂，例如与其它羟基官能粘合剂的混合物，以及作为相应的粘合剂组合物和密封化合物中的反应性组分。

2. 发明授权

US6048944A Aliphatic epoxide-amine adducts with substantial side-chain branching, process for their preparation, and their use 失效
标题翻译：具有大量侧链支化的脂族环氧胺 - 加合物，其制备方法及其用途
公开(公告)号：US6048944A
公开(公告)日：2000-04-11
申请号：US6388
申请日：1998-01-13
申请人： Ulrich Epple , Manfred Marten , Uwe Kubillus , Harald Oswald
发明人： Ulrich Epple , Manfred Marten , Uwe Kubillus , Harald Oswald
IPC分类号： C08G59/02 , C08G18/32 , C08G18/64 , C08G59/00 , C08G59/14 , C08G59/18 , C08G59/40 , C08G59/64 , C08L63/00 , C09D133/00 , C09D133/04 , C09D133/06 , C09D133/08 , C09D163/00 , C09D167/00 , C09J163/00 , C09K3/10 , C08F8/30
CPC分类号： C09D133/066 , C08G18/3271 , C08G18/643 , C08G59/184 , C08G59/64 , C09D163/00 , C09D167/00 , C08L63/00
摘要： Epoxide-amine adducts having a proportion by mass of at least 20% of aliphatic epoxide or amine units which comprise at least one tertiary or quaternary carbon atom are disclosed. The adducts are employed as binders for coatings of relatively high environment-friendliness, if desired, for example, in a mixture with other hydroxy-functional binders, and as reactive component in corresponding adhesive compositions and sealing compounds.
摘要翻译：公开了具有至少20％脂肪族环氧化物或包含至少一个叔碳原子或季碳原子的胺单元的质量比的环氧胺加合物。如果需要，加合物用作具有相对高的环境友好性的涂料的粘合剂，例如与其它羟基官能粘合剂的混合物，以及作为相应的粘合剂组合物和密封化合物中的反应性组分。

3. 发明授权

US5852122A Hydroxyl-functional copolymers of low molar mass with substantial side-chain branching, process for their preparation, and their use 失效
标题翻译：低摩尔质量的羟基官能共聚物具有大量的侧链支化，其制备方法及其用途
公开(公告)号：US5852122A
公开(公告)日：1998-12-22
申请号：US641734
申请日：1996-05-02
申请人： Ulrich Epple , Uwe Kubillus , Harald Oswald
发明人： Ulrich Epple , Uwe Kubillus , Harald Oswald
IPC分类号： C08F220/32 , C08F20/32 , C08F220/04 , C08F222/02 , C08F222/16 , C08G18/62 , C09D133/04 , C09D133/14 , C09D135/00 , C09J133/04 , C09J133/14 , C09J135/00 , C09K3/10 , C08F8/00
CPC分类号： C08G18/6258 , C08F220/04 , Y10T428/31573 , Y10T428/31576
摘要： Low molar mass copolymers which can be prepared by reacting one or more glycidyl esters of saturated aliphatic monocarboxylic acids having a tertiary or quaternary .alpha. carbon atom, and at least two unsaturated copolymerizable monomers of which at least one has at least one COOH group, under the conditions of a free-radical copolymerization, whereby the weight-average molar mass of the copolymers is below 3500 g/mol and the proportion of branched side chains in the copolymer is at least 20% by mass are disclosed. Also disclosed are methods of making these copolymers and the use thereof in binder and coating systems.
摘要翻译：低摩尔质量共聚物可以通过一种或多种具有叔或季α碳原子的饱和脂族一元羧酸缩水甘油酯与至少两种具有至少一个COOH基团的不饱和可共聚单体反应制备，自由基共聚的条件，共聚物的重均摩尔质量低于3500g / mol，共聚物中支链侧链的比例为20质量％以上。还公开了制备这些共聚物的方法及其在粘合剂和涂料体系中的应用。

4. 发明授权

US5608012A Copolymers, their preparation, and their use in high-solids coating compositions 失效
公开(公告)号：US5608012A
公开(公告)日：1997-03-04
申请号：US436719
申请日：1995-05-08
申请人： Ulrich Epple , Uwe Kubillus , Holger Schmidt
发明人： Ulrich Epple , Uwe Kubillus , Holger Schmidt
IPC分类号： C08F220/32 , C08F2/02 , C08F220/04 , C08F220/06 , C08F220/10 , C08F222/02 , C08G18/62 , C09D133/02 , C09D133/06 , C09D133/14 , C09D135/00 , C09D175/04 , C08F8/30 , B32B27/28 , C08F220/02
CPC分类号： C08F220/04 , C08F2/02 , Y10T428/31855
摘要： Copolymers of particularly low viscosity, which can be prepared by a polymerization in bulk, in which one component (A) is initially charged and, in the further course of the polymerization, at least two olefinically unsaturated copolymerizable monomers (B) are added, of which at least one contains at least one COOH group and at least one is sterically-hindered are usefully employed in coating compositions.

5. 发明授权

US5539022A Aqueous dispersions of acrylate copolymers 失效
标题翻译：丙烯酸酯共聚物的水分散体
公开(公告)号：US5539022A
公开(公告)日：1996-07-23
申请号：US222674
申请日：1994-04-04
申请人： Holger Schmidt , Tanja R. Brueck , Uwe Kubillus , Harald Oswald , Petra Schaub , Andrea Travers-Hemmer
发明人： Holger Schmidt , Tanja R. Brueck , Uwe Kubillus , Harald Oswald , Petra Schaub , Andrea Travers-Hemmer
IPC分类号： B05D3/02 , C08F8/44 , C08F12/00 , C08F20/10 , C08F212/06 , C08F220/04 , C08F220/06 , C08F220/18 , C08F220/28 , C08F220/32 , C08G59/02 , C08G59/32 , C08J3/07 , C08L61/28 , C09D5/00 , C09D125/00 , C09D125/02 , C09D125/14 , C09D133/02 , C09D133/04 , C09D133/06 , C09D133/10 , C09D133/14 , C09D161/20 , C09D161/28 , C09D163/00 , C08K3/20
CPC分类号： C08J3/07 , C08F220/28 , C08F220/32 , C08F8/44 , C09D125/14 , C09D133/068 , C09D133/14 , C08J2333/00 , C08L61/28
摘要： Water-dilutable dispersions of acrylate copolymers having a hydroxyl number of from 40 to 200 mg KOH/g and an acid number of from 15 to 50 mg of KOH/g, obtained by free-radical copolymerization ofa) from 5 to 40 parts by weight of at least one glycidyl ester of an .alpha.-branched aliphatic saturated monocarboxylic acid,b) from 0 to 30 parts by weight of at least one diester of an .alpha.,.beta.-olefinically unsaturated dicarboxylic acid,c) from 0 to 70 parts by weight of at least one vinyl aromatic hydrocarbon, the molar quantity of component c) always being greater than or equal to the molar quantity of component b),d) from 0 to 60 parts by weight of an alkyl ester of an .alpha.,.beta.-olefinically unsaturated carboxylic acid,e) from 2 to 40 parts by weight of at least one .alpha.,.beta.-olefinically unsaturated carboxylic acid, the molar quantity of component e) always being greater than the molar quantity of component a),f) from 5 to 40 parts by weight of at least one hydroxyalkyl ester of an .alpha.,.beta.-olefinically unsaturated carboxylic acid,the polymerization being carried out in bulk or in solution; if desired, addition of a water-dilutable solvent, neutralization and dilution with water.These dispersions are suitable as water-dilutable binders for clearcoat baking enamels or solid-color topcoat baking enamels.
摘要翻译：羟基数为40〜200mg KOH / g，酸值为15〜50mg KOH / g的丙烯酸酯共聚物的水可稀释分散体，通过a）5〜40份的自由基共聚得到，至少一种α-支链脂肪族饱和一元羧酸的缩水甘油酯的重量，b）0至30重量份的α，β-烯属不饱和二羧酸的至少一种二酯，c）0-70份至少一种乙烯基芳烃的重量，组分c）的摩尔量总是大于或等于组分b）的摩尔量，d）0至60重量份的α，β- 烯属不饱和羧酸，e）2至40重量份的至少一种α，β-烯属不饱和羧酸，组分e）的摩尔数总是大于组分a），f）的摩尔量5）至40重量份的至少一种羟基羟基的α，β-烯属不饱和羧酸的酯，该聚合体积或溶液中进行; 如果需要，加入水可稀释溶剂，中和并用水稀释。这些分散体适合作为透明涂层烘烤搪瓷或固色面漆烘烤搪瓷的水可稀释粘合剂。

6. 发明授权

US5663265A Copolymers containing hydroxyl and carboxyl groups by reacting glycidyl esters and carboxyl monomers 失效
标题翻译：含有羟基和羧基的共聚物通过缩水甘油酯和羧基单体反应
公开(公告)号：US5663265A
公开(公告)日：1997-09-02
申请号：US424081
申请日：1995-04-19
申请人： Ulrich Epple , Uwe Kubillus , Holger Schmidt
发明人： Ulrich Epple , Uwe Kubillus , Holger Schmidt
IPC分类号： C08F2/00 , C08F8/30 , C08F20/26 , C08F220/04 , C08F220/10 , C08F220/28 , C08F220/32 , C08F222/02 , C08F222/20 , C09D5/03 , C09D5/46 , C09D133/00 , C09D133/04 , C09D133/14 , C09D135/02 , C09D175/04 , C08F220/06
CPC分类号： C08F220/32 , C08F220/04 , C08F8/30
摘要： Low-viscosity copolymers useful in coating compositions, containing hydroxyl and carboxyl groups are obtained by free-radical polymerization of A) from 3 to 50% by weight of one or more glycidyl esters of aliphatic saturated monocarboxylic acids having a tertiary or quaternary .alpha. carbon atom, and B) from 97 to 50% by weight of at least two olefinically unsaturated copolymerizable monomers of which at least one contains at least one COOH group and at least one is sterically hindered, the quantity of COOH groups in component B exceeding the quantity of epoxy groups in component A to such an extent that the resulting copolymer has an acid number of at least 15 mg of KOH/g.
摘要翻译：可用于含有羟基和羧基的涂料组合物中的低粘度共聚物通过自由基聚合得到A）3至50重量％的一种或多种具有叔或季α碳原子的脂肪族饱和一元羧酸的缩水甘油酯和B）97〜50重量％的至少两种烯属不饱和可共聚单体，其至少一种含有至少一个COOH基团并且至少一个是空间位阻的，组分B中的COOH基团的量超过组分A中的环氧基团达到所得共聚物的酸值至少为15mg KOH / g的程度。

7. 发明授权

US5596057A Copolymers, their preparation, and their use in high-solids coating compositions 失效
标题翻译：共聚物，它们的制备及其在高固含量涂料组合物中的用途
公开(公告)号：US5596057A
公开(公告)日：1997-01-21
申请号：US611550
申请日：1996-03-06
申请人： Ulrich Epple , Uwe Kubillus , Holger Schmidt
发明人： Ulrich Epple , Uwe Kubillus , Holger Schmidt
IPC分类号： C08F220/32 , C08F2/02 , C08F220/04 , C08F220/06 , C08F220/10 , C08F222/02 , C08G18/62 , C09D133/02 , C09D133/06 , C09D133/14 , C09D135/00 , C09D175/04 , C08F224/00
CPC分类号： C08F220/04 , C08F2/02 , Y10T428/31855
摘要： Copolymers of particularly low viscosity, which can be prepared by a polymerization in bulk, in which one component (A) is initially charged and, in the further course of the polymerization, at least two olefinically unsaturated copolymerizable monomers (B) are added, of which at least one contains at least one COOH group and at least one is sterically-hindered are usefully employed in coating compositions.
摘要翻译：首先加入一种组分（A）并在聚合过程中至少两种烯属不饱和可共聚的单体（B）可以通过本体聚合制备的特别低粘度的共聚物，其中至少一个含有至少一个COOH基团并且至少一个被空间位阻的物质用于涂料组合物中。

8. 发明授权

US5169979A Curing component, and the use thereof 失效
标题翻译：固化成分及其用途
公开(公告)号：US5169979A
公开(公告)日：1992-12-08
申请号：US620283
申请日：1990-11-30
申请人： Uwe Kubillus , Gerhard Brindopke , Helmut Plum
发明人： Uwe Kubillus , Gerhard Brindopke , Helmut Plum
IPC分类号： C08G59/40 , C08G63/91 , C08J3/24 , C08L63/10
CPC分类号： C08L63/10 , C08G59/40 , C08G63/91 , C08J3/24
摘要： The invention relates to a curing component (A) containing active CH groups, which contains at least two groups of the formula (I) ##STR1## or structural units of the formula (I') or (I") ##STR2## in which: A denotes ##STR3## X and Y are identical or different and denote ##STR4## CO.sub.2 R.sup.1, CN, NO.sub.2, CONH.sub.2, CONR.sup.1 H or CONR.sup.1 R.sup.1, where the R.sup.1 radicals may be identical or different and represent a hydrocarbon radical, preferably an alkyl radical having 1 to 12 carbon atoms, which may also be interrupted by oxygen or an N-alkyl radical, with the proviso that only one of the two radicals X and Y may represent the NO.sub.2 group;A' denotes ##STR5## X' and Y' are identical or different and denote ##STR6## Curable mixtures of (A) and a Michael acceptor (B) and, if appropriate diluents and customary additivies cure rapidly even at low temperatures and are suitable, in particular for surface-coating preparations.
摘要翻译：本发明涉及含有活性CH基团的固化组分（A），其含有至少两个式（I）的基团（I）或式（I'）或（I“）的结构单元，（I'）（I'）其中：A表示X和Y相同或不同，表示CO 2 R 1，CN，NO 2，CONH 2，CONR 1 H或CONR 1 R 1，其中R 1基团可以相同或不同，表示烃基，优选具有1至12个碳原子的烷基，其也可被氧或N-烷基中断，条件是两个基团X和Y中只有一个可以代表NO2组; A'表示 X'和Y'相同或不同，表示（IMA）>（A）和迈克尔受体（B）的可固化混合物，如果合适，稀释剂和常规添加剂即使在低温下也能快速固化，，特别是表面涂层制剂。

9. 发明授权

US5328978A Triazine/formaldehyde resin 失效
标题翻译：三嗪/甲醛树脂
公开(公告)号：US5328978A
公开(公告)日：1994-07-12
申请号：US142006
申请日：1993-10-28
申请人： Manfred Schon , Jurgen Ott , Uwe Kubillus , Elif Tas
发明人： Manfred Schon , Jurgen Ott , Uwe Kubillus , Elif Tas
IPC分类号： C08G12/30 , C09D163/00 , C09D167/00 , C09D167/08
CPC分类号： C09D167/00 , C08G12/30 , C09D163/00 , C09D167/08 , Y10T428/31942
摘要： The present invention relates to a triazine/formaldehyde resin which contains a compound of the general formula I ##STR1## wherein R.sup.1 and R.sup.2 are defined as stated in claim 1, a process for its preparation and its use as a curing agent in surface coating systems.
摘要翻译：本发明涉及三嗪/甲醛树脂，其含有通式Ⅰ的化合物，其中R 1和R 2如权利要求1中所定义，其制备方法及其用作表面涂层中的固化剂系统。

10. 发明授权

US5344897A Liquid coating agent based on transesterified, modified epoxy resins and blocked polyamines 失效
标题翻译：基于酯交换，改性环氧树脂和封端多胺的液体涂料
公开(公告)号：US5344897A
公开(公告)日：1994-09-06
申请号：US146573
申请日：1993-10-29
申请人： Gerhard Brindoepke , Uwe Kubillus , Helmut Plum
发明人： Gerhard Brindoepke , Uwe Kubillus , Helmut Plum
IPC分类号： A47K3/28 , A47K3/30 , C08G59/14 , C08G59/16 , C08G59/40 , C08G59/50 , C08G59/62 , C09D163/00
CPC分类号： C09D163/00 , C08G59/1427 , C08G59/1455 , C08G59/4042 , C08G59/50 , C08G59/625
摘要： Liquid coating agent based on a polymer containing acetoacetate groups and a polyamine in the form of the corresponding aldimine or ketimine, the polymer containing acetoacetate groups being obtained by reaction of a polyepoxide with water, an amine or a hydroxycarboxylic acid and subsequent esterification or transesterification with acetoacetic acid. These liquid coating agents are particularly suitable as binders in two-component automobile repair fillers or as two-component primers.
摘要翻译：基于含有乙酰乙酸酯基团的聚合物和相应的醛亚胺或酮亚胺形式的多胺的液体包衣剂，含有乙酰乙酸酯基团的聚合物通过聚环氧化物与水，胺或羟基羧酸的反应获得，随后酯化或酯交换与乙酰乙酸。这些液体涂覆剂特别适合作为双组分汽车修补填料中的粘合剂或作为双组分引物。

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