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1. 发明授权

US06861550B2 Polyhydroxyalkanoate containing 3-hydroxybenzoylalkanoic acid as monomer unit, and method for producing the same 失效
标题翻译：含有3-羟基苯甲酰基链烷酸作为单体单元的聚羟基链烷酸酯及其制造方法
公开(公告)号：US06861550B2
公开(公告)日：2005-03-01
申请号：US09791610
申请日：2001-02-26
申请人： Tsutomu Honma , Etsuko Sugawa , Tetsuya Yano , Shin Kobayashi , Takeshi Imamura , Takashi Kenmoku
发明人： Tsutomu Honma , Etsuko Sugawa , Tetsuya Yano , Shin Kobayashi , Takeshi Imamura , Takashi Kenmoku
IPC分类号： C12P7/42 , C08G63/06 , C12P7/62 , C07C69/73
CPC分类号： C12P7/625 , C08G63/06
摘要： Microorganisms capable of producing novel polyalkanoates having 3-hydroxybenzoylalkanoic acids as monomer units by utilizing benzoylalkanoic acids as starting materials are cultured in media containing benzoylalkanoic acids and saccharides, and the polyhydroxyalkanoates produced in the culture cells are extracted and recovered.
摘要翻译：在含有苯甲酰基链烷酸和糖类的培养基中培养能够以苯甲酰基链烷酸为起始原料，以具有3-羟基苯甲酰基链烷酸作为单体单元生产新型聚链烷酸的微生物，提取并回收培养细胞中产生的聚羟基链烷酸酯。

2. 发明授权

US06908720B2 Polyhydroxyalkanoate, its production method, charge control agent containing the polyhydroxyalkanoate, toner binder and toner, and image forming method and image forming apparatus using the toner 失效
标题翻译：聚羟基链烷酸酯，其制备方法，含有聚羟基链烷酸酯的电荷控制剂，调色剂粘合剂和调色剂，以及使用该调色剂的图像形成方法和图像形成装置
公开(公告)号：US06908720B2
公开(公告)日：2005-06-21
申请号：US10133576
申请日：2002-04-29
申请人： Takashi Kenmoku , Toyoko Kobayashi , Etsuko Sugawa , Tetsuya Yano , Shin Kobayashi , Takeshi Imamura , Tsutomu Honma
发明人： Takashi Kenmoku , Toyoko Kobayashi , Etsuko Sugawa , Tetsuya Yano , Shin Kobayashi , Takeshi Imamura , Tsutomu Honma
IPC分类号： C08G63/688 , C12P7/62 , C12P11/00 , G03G9/087 , G03G9/097 , C08G13/06 , C08F20/00
CPC分类号： G03G9/08771 , C08G63/6882 , C12P7/625 , C12P11/00 , G03G9/08728 , G03G9/0874 , G03G9/08768 , G03G9/08773 , G03G9/08791 , G03G9/08795 , G03G9/08797 , G03G9/09733 , G03G9/09775
摘要： The present invention provides a novel PHA comprising a unit containing thioether with high reactivity, and its production method. The present invention also provides polyhydroxyalkanoate (PHA) comprising units having defined chemical formulas (1) and (2), and at least one of four units having defined chemical formulas (3), (4), (5) and (6); its production method; a charge control agent containing the PHA; a toner binder containing the charge control agent; an electrostatic latent image developing toner; and an image forming method and an image forming apparatus using the electrostatic latent image developing toner.
摘要翻译：本发明提供了包含含有高反应性的硫醚的单元的新型PHA及其制造方法。本发明还提供了包含具有确定的化学式（1）和（2）的单元和具有确定的化学式（3），（4），（5）和（6）的四个单元中的至少一个的聚羟基链烷酸酯（PHA）其生产方式; 含有PHA的电荷控制剂; 含有电荷控制剂的调色剂粘合剂; 静电潜像显影调色剂; 以及使用静电潜像显影用调色剂的图像形成方法和图像形成装置。

3. 发明授权

US06872788B2 Production method of polyester containing epoxy group in side chain and production method of crosslinked polymer 失效
标题翻译：侧链中含有环氧基的聚酯的生产方法和交联聚合物的制备方法
公开(公告)号：US06872788B2
公开(公告)日：2005-03-29
申请号：US10427919
申请日：2003-05-02
申请人： Takeshi Imamura , Etsuko Sugawa , Tetsuya Yano , Shin Kobayashi , Tsutomu Honma , Takashi Kenmoku
发明人： Takeshi Imamura , Etsuko Sugawa , Tetsuya Yano , Shin Kobayashi , Tsutomu Honma , Takashi Kenmoku
IPC分类号： C12N1/28 , C12P7/62 , C08F20/00
CPC分类号： C12P7/625 , C12N1/28 , Y10S435/874
摘要： A method is provided which biosynthesizes a PHA having an epoxy group on a side chain with improved physicochemical properties. Specifically, a method of producing a polyester containing an epoxy group in a side chain thereof using alkene as a raw material is provided which comprises the steps of bringing alkene into contact with a microorganism having an ability to uptake alkene and convert it to a polyester and allowing the microorganism to convert the alkene into a polyester containing an epoxy group in a side chain thereof. Further, a method of producing a crosslinked polymer is provided which comprises reacting the polyester obtained by the above mentioned method with a diamine compound.
摘要翻译：提供一种方法，其生物合成具有改善的物理化学性质的侧链上具有环氧基的PHA。具体地说，提供了使用烯烃作为原料在其侧链中制备含有环氧基的聚酯的方法，其包括使烯与具有吸收烯烃的能力并将其转化为聚酯的微生物接触的步骤，以及允许微生物将烯烃转化成其侧链中含有环氧基的聚酯。此外，提供了一种制备交联聚合物的方法，其包括使通过上述方法获得的聚酯与二胺化合物反应。

4. 发明授权

US07078200B2 Method for manufacturing a polyhydroxyalkanoate 失效
标题翻译：聚羟基链烷酸酯的制造方法
公开(公告)号：US07078200B2
公开(公告)日：2006-07-18
申请号：US10603996
申请日：2003-06-26
申请人： Tsutomu Honma , Etsuko Sugawa , Tetsuya Yano , Takeshi Imamura , Takashi Kenmoku
发明人： Tsutomu Honma , Etsuko Sugawa , Tetsuya Yano , Takeshi Imamura , Takashi Kenmoku
IPC分类号： C12P7/62 , C08G63/06 , C08G63/78
CPC分类号： C12P7/625 , C08G63/06 , C08G63/6822 , C08G63/6852
摘要： A method for producing a polyhydroxyalkanoate using a microorganism capable of substantially reducing unintended monomer units and obtaining the polyhydroxyalkanoate in a high yield. A microorganism capable of synthesizing a novel polyhydroxyalkanoate having 3-hydroxy-substituted benzoylalkanoic acid as a monomer unit, using a substituted benzoylalkanoic acid as a material, is cultured in a medium containing a substituted benzoylalkanoic acid. Then, the polyhydroxyalkanoate produced in the cultured bacteria is extracted and recovered.
摘要翻译：使用能够显着降低非预期的单体单元并以高产率获得聚羟基链烷酸酯的微生物制备聚羟基链烷酸酯的方法。在含有取代的苯甲酰基链烷酸的培养基中培养能够以取代的苯甲酰基链烷酸为原料合成具有3-羟基取代的苯甲酰基链烷酸作为单体单元的新型聚羟基链烷酸酯的微生物。然后，提取并回收在培养细菌中产生的聚羟基链烷酸酯。

5. 发明授权

US06635782B2 Polyhydroxyalkanoate and manufacturing method thereof 失效
标题翻译：聚羟基链烷酸酯及其制造方法
公开(公告)号：US06635782B2
公开(公告)日：2003-10-21
申请号：US09951720
申请日：2001-09-14
申请人： Tsutomu Honma , Etsuko Sugawa , Tetsuya Yano , Takeshi Imamura , Takashi Kenmoku
发明人： Tsutomu Honma , Etsuko Sugawa , Tetsuya Yano , Takeshi Imamura , Takashi Kenmoku
IPC分类号： C07C6976
CPC分类号： C12P7/625 , C08G63/06 , C08G63/6822 , C08G63/6852
摘要： To provide a novel polyhydroxyalkanoate and a manufacturing method by a microorganism capable of substantially reducing unintended monomer units and obtaining the polyhydroxyalkanoate in a high yield. A microorganism capable of synthesizing a novel polyhydroxyalkanoate having 3-hydroxy-substituted benzoylalkanoic acid as a monomer unit using a substituted benzoylalkanoic acid as a material is cultured in the medium containing a substituted benzoylalkanoic acid, then the polyhydroxyalkanoate produced in the cultured bacteria is extracted and recovered.
摘要翻译：提供一种新型的聚羟基链烷酸酯及其制造方法，该微生物能够基本上减少非预期的单体单元并以高产率获得聚羟基链烷酸酯。在含有取代的苯甲酰基链烷酸的培养基中培养能够使用取代的苯甲酰基链烷酸合成具有3-羟基取代的苯甲酰基链烷酸作为单体单元的新型聚羟基链烷酸酯的微生物，然后提取培养细菌中产生的聚羟基链烷酸酯，恢复。

6. 发明授权

US07056708B2 Method of producing polyhydroxyalkanoate from alkane having residue containing aromatic ring in its molecule 失效
标题翻译：从其分子中含有芳环的残基的烷烃生产聚羟基链烷酸酯的方法
公开(公告)号：US07056708B2
公开(公告)日：2006-06-06
申请号：US10410349
申请日：2003-04-10
申请人： Takashi Kenmoku , Etsuko Sugawa , Tetsuya Yano , Takeshi Imamura , Tsutomu Honma
发明人： Takashi Kenmoku , Etsuko Sugawa , Tetsuya Yano , Takeshi Imamura , Tsutomu Honma
IPC分类号： C12P11/00 , C12P7/62
CPC分类号： C08G63/6882 , C12P7/625 , C12P11/00
摘要： The present invention provides a method of effectively producing polyhydroxyalkanoate having an aromatic substituted residue in its monomer unit. In the method of producing polyhydroxyalkanoate by using microorganisms, microorganisms capable of producing polyhydroxyalkanoate are cultured in a culture medium containing at least one starting compound selected from the group consisting of substituted alkanes represented by formula (1) to produce polyhydroxyalkanoate having, in its molecule, at least one unit selected from the group consisting of 3-hydroxy-substituted alkanoate units represented by formula (2): R—(CH2)n—CH2—CH2—CH3 (1) wherein R represents a residue containing a substituted aromatic ring, and n represents any integer of 1 to 8; wherein R represents a residue containing a substituted aromatic ring, and n represents any integer of 1 to 8. In formulas (1) and (2), a residue R is as described in the specification.
摘要翻译：本发明提供了在其单体单元中有效制备具有芳族取代残基的聚羟基链烷酸酯的方法。在通过使用微生物制备聚羟基链烷酸酯的方法中，能够在含有选自由式（1）表示的取代烷烃中的至少一种起始化合物的培养基中培养能够产生聚羟基链烷酸酯的微生物，从而产生在其分子中具有的聚羟基链烷酸酯，选自由式（2）表示的3-羟基取代的链烷酸酯单元中的至少一个单元：<？in-line-formula description =“In-line Formulas”end =“lead”？> R-（CH （2）-CH 2 CH 2 CH 2 CH 2（1）其中，R表示含有取代芳环的残基，n表示1〜8的整数，n表示1〜8的整数。其中R表示含有取代芳环的残基，n表示1至8的任何整数。在式（1）和（2）中，残基R如说明书所述。

7. 发明授权

US06777153B2 POLYHYDROXYALKANOATE CONTAINING UNIT WITH THIENYL STRUCTURE IN THE SIDE CHAIN, PROCESS FOR ITS PRODUCTION, CHARGE CONTROL AGENT, TONER BINDER AND TONER WHICH CONTAIN THIS POLYHYDROXYALKANOATE, AND IMAGE-FORMING METHOD AND IMAGE-FORMING APPARATUS WHICH MAKE USE OF THE TONER 失效
标题翻译：含有三链体结构的聚羟基烷基酯单元，其链中具有三烯结构，其制备方法，充电控制剂，含有该聚羟基烷酸酯的调色剂和调色剂，以及使用该调色剂的成像方法和图像形成装置
公开(公告)号：US06777153B2
公开(公告)日：2004-08-17
申请号：US10105305
申请日：2002-03-26
申请人： Tetsuya Yano , Etsuko Sugawa , Takeshi Imamura , Tsutomu Honma , Takashi Kenmoku
发明人： Tetsuya Yano , Etsuko Sugawa , Takeshi Imamura , Tsutomu Honma , Takashi Kenmoku
IPC分类号： G03G900
CPC分类号： C08G63/6882 , C12P7/62 , G03G9/08755 , G03G9/08791 , Y10S435/874 , Y10S435/877
摘要： A polyhydroxyalkanoate characterized by having in the molecule a unit represented by Chemical Formula (1): wherein n may assume any one integral value within the range of from 1 to 8. Also disclosed are a process for producing the polyhydroxyalkanoate by the use of a microorganism having the ability to produce the polyhydroxyalkanoate and accumulate it in the bacterial body; a charge control agent, a toner binder and a toner which contain this polyhydroxyalkanoate; and an image-forming method and an image-forming apparatus which make use of the toner.
摘要翻译：特征在于在分子中具有由化学式（1）表示的单元的聚羟基链烷酸酯：其中n可以在1至8的范围内呈现任何一个整数值。还公开了通过使用微生物制备聚羟基链烷酸酯的方法具有生产聚羟基链烷酸酯并将其积聚在细菌体内的能力; 电荷控制剂，调色剂粘合剂和含有该聚羟基链烷酸酯的调色剂; 以及利用调色剂的图像形成方法和图像形成装置。

8. 发明授权

US07425432B2 Polyhydroxy alkanoate copolymer including within molecule unit having vinyl group or carboxyl group in side chain, and producing method therefor 有权
标题翻译：在侧链中具有乙烯基或羧基的分子单元内的聚羟基链烷酸酯共聚物及其制造方法
公开(公告)号：US07425432B2
公开(公告)日：2008-09-16
申请号：US10531689
申请日：2003-10-23
申请人： Takashi Kenmoku , Tetsuya Yano , Chieko Mihara , Shinya Kozaki , Tsutomu Honma , Tatsuki Fukui , Takeshi Imamura , Etsuko Sugawa
发明人： Takashi Kenmoku , Tetsuya Yano , Chieko Mihara , Shinya Kozaki , Tsutomu Honma , Tatsuki Fukui , Takeshi Imamura , Etsuko Sugawa
IPC分类号： C12P11/00 , C12P7/72 , C08G63/00 , C08G63/02 , C08G63/68
CPC分类号： C08G63/06 , C08G63/6882 , C12P7/625
摘要： The invention provides a PHA copolymer including at least a 3-hydroxy-ω-carboxyalkanoic acid represented by a formula (19) or (32) and simultaneously at least a unit represented by a formula (2) or a formula (3) in a molecule, a precursor PHA copolymer having a corresponding vinyl group or a corresponding alkoxycarbonyl group, a biosynthesis method thereof by microorganisms, and a method of producing a desired PHA copolymer from the precursor PHA copolymer: (wherein k, m, n are integers; R18 represents H, Na, K, R27? represents (A); R1 represents a substituent on a cyclohexyl group and represents H, CN, NO2, a halogen atom, CH3, C2H5, C3H7, CF3, C2F5, or C3F7; R includes a residue including a phenyl structure or a thienyl structure; these being independent for each unit).
摘要翻译：本发明提供一种PHA共聚物，其包含至少一种由式（19）或（32）表示的3-羟基-ω-羧基烷酸，同时至少由式（2）或式（3）表示的单元在分子，具有相应的乙烯基或相应的烷氧基羰基的前体PHA共聚物，微生物的生物合成方法以及由前体PHA共聚物制备所需PHA共聚物的方法（其中k，m，n为整数; R ＆lt; 18＆gt;＆gt;代表H，Na，K，R 27？表示（A）; R 1表示环己基上的取代基，代表H，CN ，NO 2 2，卤素原子，CH 3，C 2 H 5，C 3， H 3，CF 3，C 2 H 5，或C 3 H 3， R> R包括残基inc 提出苯基结构或噻吩基结构; 这些对于每个单元是独立的）。

9. 发明授权

US07408017B2 Polyhydroxyalkanoate containing unit with phenylsulfanyl structure in the side chain, process for its production, charge control agent, toner binder and toner which contain novel polyhydroxyalkanoate, and image forming method and image-forming apparatus which make use of the toner 失效
标题翻译：在侧链中具有苯基硫烷基结构的聚羟基链烷酸酯单元，其制备方法，电荷控制剂，调色剂粘合剂和含有新型聚羟基链烷酸酯的调色剂，以及使用调色剂的成像方法和图像形成装置
公开(公告)号：US07408017B2
公开(公告)日：2008-08-05
申请号：US11155599
申请日：2005-06-20
申请人： Takeshi Imamura , Etsuko Sugawa , Tetsuya Yano , Tsuyoshi Nomoto , Tomohiro Suzuki , Tsutomu Honma , Takashi Kenmoku , Tatsuki Fukui
发明人： Takeshi Imamura , Etsuko Sugawa , Tetsuya Yano , Tsuyoshi Nomoto , Tomohiro Suzuki , Tsutomu Honma , Takashi Kenmoku , Tatsuki Fukui
IPC分类号： C08G63/688
CPC分类号： G03G9/08755 , C08G63/6882 , C12P7/625 , C12P11/00 , G03G9/08791 , G03G9/09733 , G03G9/09775
摘要： A polyhydroxyalkanoate is disclosed which has in the molecule a unit represented by Chemical Formula (1). wherein R is arbitrarily selected from a hydrogen atom, a halogen atom, CN, NO2, COOR′, SO2R″, CH3, C2H5, C3H7, C(CH3)2H and C(CH3)3; where R′ is H, Na, K, CH3 or C2H5, and R″ is OH, ONa, OK, a halogen atom, OCH3 or OC2H5; and x is an integer arbitrarily selected from 1 to 8; with the proviso that a polyhydroxyalkanoate is excluded which has a hydrogen atom as R and x in all the units is 2 or 4. Also disclosed is a process for producing the polyhydroxyalkanoate by the use of a microorganism having the ability to produce the polyhydroxyalkanoate and accumulate it in the bacterial body.
摘要翻译：公开了在分子中具有由化学式（1）表示的单元的聚羟基链烷酸酯。其中R可以任选地选自氢原子，卤原子，CN，NO 2，COOR'，SO 2 R“，CH 3 C 2 H 3，C 3 H 3，C（CH 3）3 H 3，C 3 H 3， 2）H和C（CH 3 3）3。其中R'是H，Na，K，CH 3或C 2 H 5，并且R“是OH，ONa，OK，卤素原子，OCH 3或OC 2 H 5; x是任意选自1至8的整数; 条件是排除了具有氢原子作为R的聚羟基链烷酸酯，并且所有单元中的x均为2或4.还公开了通过使用具有生产聚羟基链烷酸酯的能力的微生物来生产聚羟基链烷酸酯并累积它在细菌体内。

10. 发明申请

US20050250191A1 Novel polyhydroxyalkanoate containing unit with phenylsulfanyl structure in the side chain, process for its production, charge control agent, toner binder and toner which contain novel polyhydroxyalkanoate, and image forming method and image-forming apparatus which make use of the toner 失效
标题翻译：在侧链中具有苯基硫烷基结构的新型聚羟基链烷酸酯单元，其制备方法，电荷控制剂，调色剂粘合剂和含有新型聚羟基链烷酸酯的调色剂，以及使用调色剂的成像方法和图像形成装置
公开(公告)号：US20050250191A1
公开(公告)日：2005-11-10
申请号：US11155599
申请日：2005-06-20
申请人： Takeshi Imamura , Etsuko Sugawa , Tetsuya Yano , Tsuyoshi Nomoto , Tomohiro Suzuki , Tsutomu Honma , Takashi Kenmoku , Tatsuki Fukui
发明人： Takeshi Imamura , Etsuko Sugawa , Tetsuya Yano , Tsuyoshi Nomoto , Tomohiro Suzuki , Tsutomu Honma , Takashi Kenmoku , Tatsuki Fukui
IPC分类号： C08G63/688 , C12P7/62 , C12P11/00 , G03G9/087 , G03G9/097 , C08G63/68
CPC分类号： G03G9/08755 , C08G63/6882 , C12P7/625 , C12P11/00 , G03G9/08791 , G03G9/09733 , G03G9/09775
摘要： A polyhydroxyalkanoate is disclosed which has in the molecule a unit represented by Chemical Formula (1). wherein R is arbitrarily selected from a hydrogen atom, a halogen atom, CN, NO2, COOR′, SO2R″, CH3, C2H5, C3H7, C(CH3)2H and C(CH3)3; where R′ is H, Na, K, CH3 or C2H5, and R″ is OH, ONa, OK, a halogen atom, OCH3 or OC2H5; and x is an integer arbitrarily selected from 1 to 8; with the proviso that a polyhydroxyalkanoate is excluded which has a hydrogen atom as R and x in all the units is 2 or 4. Also disclosed is a process for producing the polyhydroxyalkanoate by the use of a microorganism having the ability to produce the polyhydroxyalkanoate and accumulate it in the bacterial body.
摘要翻译：公开了在分子中具有由化学式（1）表示的单元的聚羟基链烷酸酯。其中R可以任选地选自氢原子，卤原子，CN，NO 2，COOR'，SO 2 R“，CH 3 C 2 H 3，C 3 H 3，C（CH 3）3 H 3，C 3 H 3， 2）H和C（CH 3 3）3。其中R'是H，Na，K，CH 3或C 2 H 5，并且R“是OH，ONa，OK，卤原子，OCH 3或OC 2 H 5; x是任意选自1至8的整数; 条件是排除了具有氢原子作为R的聚羟基链烷酸酯，并且所有单元中的x均为2或4.还公开了通过使用具有生产聚羟基链烷酸酯的能力的微生物来生产聚羟基链烷酸酯并累积它在细菌体内。

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