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1. 发明申请

US20140162113A1 ALL-SOLID-STATE LITHIUM SECONDARY BATTERY AND METHOD FOR PRODUCING THE SAME 审中-公开
标题翻译：全固态锂二次电池及其制造方法
公开(公告)号：US20140162113A1
公开(公告)日：2014-06-12
申请号：US14127825
申请日：2012-06-20
申请人： Shingo Ohta , Mitsuru Asai , Takahiko Asaoka
发明人： Shingo Ohta , Mitsuru Asai , Takahiko Asaoka
IPC分类号： H01M10/0585 , H01M10/04
CPC分类号： H01M10/0585 , H01B1/08 , H01M4/0471 , H01M4/131 , H01M4/1391 , H01M10/04 , H01M10/0525 , H01M10/0562 , H01M2300/0071
摘要： An all-solid-state lithium secondary battery includes a positive electrode; a negative electrode; and a solid electrolyte arranged between the positive and negative electrodes, to conduct lithium ions. In the all-solid-state lithium secondary battery, a mixed layer is in close contact with a surface of the solid electrolyte adjacent to the positive electrode, the mixed layer containing the positive-electrode active material and (Lix(1−α), Mxα/β)γ+(B1−y, Ay)z+O2−δ (wherein in the formula, M and A each represent at least one or more elements selected from C, Al, Si, Ga, Ge, In, and Sn, α satisfies 0≦α
摘要翻译：全固态锂二次电池包括正电极; 负极; 以及设置在正极和负极之间的固体电解质，以进行锂离子。在全固态锂二次电池中，混合层与正极相邻的固体电解质的表面紧密接触，含有正极活性物质的混合层和（Lix（1-α），（式中，M和A各自表示选自C，Al，Si，Ga，Ge，In中的至少一种以上的元素，并且Sn，α满足0＆nlE;α<1，＆bgr;表示M的化合价，γ表示（Li + x（1-α），Mα）的平均化合价，y满足0＆nlE; y <1，z表示平均（B1-y，Ay）和x，α，＆bgr，γ，z和γ的化合价满足用作矩阵的关系式（x（1-α）+xα/＆bgr;）γ+ z =2δ）。

2. 发明申请

US20110244337A1 GARNET-TYPE LITHIUM ION-CONDUCTING OXIDE AND ALL-SOLID-STATE LITHIUM ION SECONDARY BATTERY CONTAINING THE SAME 有权
标题翻译： GARNET型锂离子导电氧化物和全固体锂离子二次电池
公开(公告)号：US20110244337A1
公开(公告)日：2011-10-06
申请号：US13132795
申请日：2010-02-02
申请人： Shingo Ohta , Tetsuro Kobayashi , Takahiko Asaoka , Mitsuru Asai
发明人： Shingo Ohta , Tetsuro Kobayashi , Takahiko Asaoka , Mitsuru Asai
IPC分类号： H01M10/052 , H01M10/056
CPC分类号： H01M10/0562 , C04B35/481 , C04B35/486 , C04B35/4885 , C04B35/495 , C04B35/6262 , C04B35/62685 , C04B2235/3203 , C04B2235/3217 , C04B2235/3224 , C04B2235/3225 , C04B2235/3227 , C04B2235/3232 , C04B2235/3239 , C04B2235/3244 , C04B2235/3251 , C04B2235/3286 , C04B2235/3287 , C04B2235/3293 , C04B2235/3418 , C04B2235/761 , C04B2235/764 , C04B2235/77 , C04B2235/79 , C04B2235/81 , H01M10/052 , H01M2300/0071 , Y02E60/122
摘要： An all-solid-state lithium ion secondary battery containing a novel garnet-type oxide serving as a solid electrolyte. The garnet-type lithium ion-conducting oxide is one represented by the formula Li5+XLa3(ZrX, A2-X)O12, wherein A is at least one selected from the group consisting of Sc, Ti, V, Y, Nb, Hf, Ta, Al, Si, Ga, Ge, and Sn and X satisfies the inequality 1.4≦X
摘要翻译：包含新型石榴石型氧化物作为固体电解质的全固态锂离子二次电池。石榴石型锂离子传导氧化物是由式Li5 + XLa3（ZrX，A2-X）O12表示的锂离子传导氧化物，其中A为选自Sc，Ti，V，Y，Nb，Hf中的至少一种，Ta，Al，Si，Ga，Ge，Sn和X满足不等式1.4＆nlE; X <2，或者是通过将具有与Zr的离子半径不同的元素替代为石榴石型的Zr部位而获得的元素由式Li7La3Zr2O12表示的锂离子传导性氧化物，其中基于衍射峰的强度归一化的具有衍射峰的X射线衍射（XRD）图案的归一化强度为9.2以上。

3. 发明授权

US10530015B2 All-solid-state lithium secondary battery and method for producing the same 有权
公开(公告)号：US10530015B2
公开(公告)日：2020-01-07
申请号：US14127825
申请日：2012-06-20
申请人： Shingo Ohta , Mitsuru Asai , Takahiko Asaoka
发明人： Shingo Ohta , Mitsuru Asai , Takahiko Asaoka
IPC分类号： H01M10/0562 , H01M10/0585 , H01M10/04
摘要： An all-solid-state lithium secondary battery includes a positive electrode; a negative electrode; and a solid electrolyte arranged between the positive and negative electrodes, to conduct lithium ions. In the all-solid-state lithium secondary battery, a mixed layer is in close contact with a surface of the solid electrolyte adjacent to the positive electrode, the mixed layer containing the positive-electrode active material and (Lix(1−α), Mxα/β)γ+(B1−y, Ay)z+O2−δ (wherein in the formula, M and A each represent at least one or more elements selected from C, Al, Si, Ga, Ge, In, and Sn, α satisfies 0≤α

4. 发明授权

US08986895B2 Garnet-type lithium ion-conducting oxide and all-solid-state lithium ion secondary battery containing the same 有权
标题翻译：石榴石型锂离子传导性氧化物和含有其的全固态锂离子二次电池
公开(公告)号：US08986895B2
公开(公告)日：2015-03-24
申请号：US13132795
申请日：2010-02-02
申请人： Shingo Ohta , Tetsuro Kobayashi , Takahiko Asaoka , Mitsuru Asai
发明人： Shingo Ohta , Tetsuro Kobayashi , Takahiko Asaoka , Mitsuru Asai
IPC分类号： H01M6/18 , H01M10/0562 , C04B35/48 , C04B35/486 , C04B35/488 , C04B35/495 , C04B35/626 , H01M10/052
CPC分类号： H01M10/0562 , C04B35/481 , C04B35/486 , C04B35/4885 , C04B35/495 , C04B35/6262 , C04B35/62685 , C04B2235/3203 , C04B2235/3217 , C04B2235/3224 , C04B2235/3225 , C04B2235/3227 , C04B2235/3232 , C04B2235/3239 , C04B2235/3244 , C04B2235/3251 , C04B2235/3286 , C04B2235/3287 , C04B2235/3293 , C04B2235/3418 , C04B2235/761 , C04B2235/764 , C04B2235/77 , C04B2235/79 , C04B2235/81 , H01M10/052 , H01M2300/0071 , Y02E60/122
摘要： An all-solid-state lithium ion secondary battery containing a novel garnet-type oxide serving as a solid electrolyte. The garnet-type lithium ion-conducting oxide is one represented by the formula Li5+XLa3(ZrX, A2-X)O12, wherein A is at least one selected from the group consisting of Sc, Ti, V, Y, Nb, Hf, Ta, Al, Si, Ga, Ge, and Sn and X satisfies the inequality 1.4≦X
摘要翻译：包含新型石榴石型氧化物作为固体电解质的全固态锂离子二次电池。石榴石型锂离子传导氧化物是由式Li5 + XLa3（ZrX，A2-X）O12表示的锂离子传导氧化物，其中A为选自Sc，Ti，V，Y，Nb，Hf中的至少一种，Ta，Al，Si，Ga，Ge，Sn和X满足不等式1.4＆nlE; X <2，或者是通过将具有与Zr的离子半径不同的元素替代为石榴石型的Zr部位而获得的元素由式Li7La3Zr2O12表示的锂离子传导性氧化物，其中基于衍射峰的强度归一化的具有衍射峰的X射线衍射（XRD）图案的归一化强度为9.2以上。

5. 发明授权

US06864011B2 Fuel-cell electrode and method of manufacturing the fuel-cell electrode 失效
标题翻译：燃料电池用电极及燃料电池用电极的制造方法
公开(公告)号：US06864011B2
公开(公告)日：2005-03-08
申请号：US10242409
申请日：2002-09-13
申请人： Tatsuya Kawahara , Seiji Mizuno , Takahiko Asaoka , Yu Morimoto , Kazuo Kawahara
发明人： Tatsuya Kawahara , Seiji Mizuno , Takahiko Asaoka , Yu Morimoto , Kazuo Kawahara
IPC分类号： H01M4/90 , H01M4/86 , H01M4/88 , H01M4/92 , H01M8/10 , C25D3/50 , C25D3/56 , H01M4/96
CPC分类号： H01M8/1004 , H01M4/8605 , H01M4/8807 , H01M4/8828 , H01M4/8853 , H01M4/92 , H01M4/926 , Y02P70/56
摘要： A fuel-cell electrode and a method of manufacturing the fuel-cell electrode achieves a high catalyst utilization ratio and makes it possible to obtain higher output characteristics with a smaller amount of catalyst. The fuel-cell electrode includes a catalytic layer composed of an ion conductive substance, an electron conductive substance and catalytic activation substances. The catalytic activation substances are electrolytically deposited on the electron conductive substance.
摘要翻译：燃料电池用电极和燃料电池用电极的制造方法能够实现高的催化剂利用率，能够以较少量的催化剂获得更高的输出特性。燃料电池电极包括由离子导电物质，电子传导物质和催化活化物质组成的催化剂层。催化活化物质电解沉积在电子传导物质上。

6. 发明授权

US5097358A Electrochromic element 失效
标题翻译：电致变色元件
公开(公告)号：US5097358A
公开(公告)日：1992-03-17
申请号：US514225
申请日：1990-04-25
申请人： Toshiyasu Ito , Takaaki Mori , Mamoru Kato , Masanobu Senda , Takahiko Asaoka
发明人： Toshiyasu Ito , Takaaki Mori , Mamoru Kato , Masanobu Senda , Takahiko Asaoka
IPC分类号： G02F1/15
CPC分类号： G02F1/1523
摘要： An electrochromic element comprising a pair of electrode films, at least one of which is a transparent electrode film, a color forming film laminated between both the electrode films and an electrolyte. The color forming film is formed on the electrode film by depositing thereon a conductive metal oxide such as indium oxide and tungsten oxide. The depositing ratio of tungsten oxide and indium oxide preferably is within the range of 10:1 to 3:1 by weight ratio.
摘要翻译：一种电致变色元件，包括一对电极膜，其中至少一个是透明电极膜，层压在两个电极膜和电解质之间的成色膜。通过在其上沉积诸如氧化铟和氧化钨的导电金属氧化物，在电极膜上形成彩色形成膜。氧化钨和氧化铟的沉积比优选在10:1至3:1的重量比范围内。

7. 发明申请

US20070196659A1 Carbon gel composite material 审中-公开
标题翻译：碳凝胶复合材料
公开(公告)号：US20070196659A1
公开(公告)日：2007-08-23
申请号：US11218285
申请日：2005-08-31
申请人： Norihiko Setoyama , Tsutomu Kajino , Hideki Takagi , Takahiko Asaoka , Yoshiaki Fukushima
发明人： Norihiko Setoyama , Tsutomu Kajino , Hideki Takagi , Takahiko Asaoka , Yoshiaki Fukushima
IPC分类号： B32B9/00 , C01B31/08
CPC分类号： H01M4/926 , C01B32/00 , H01M4/90 , H01M4/9083 , Y10T428/30
摘要： A carbon gel composite material including: a carbon gel which is composed of primary particles with an average particle diameter of 2 to 50 nm, where no x-ray diffraction peaks are observed over a scan angle (2θ) range of 0.5 to 10° (CuK60 radiation) and where in a pore size distribution calculated from an adsorption/desorption isotherm, if a pore diameter corresponding to the peak of the pore size distribution is not smaller than 1 nm and is smaller than 10 nm (pore diameter (d)), pores accounting for 60% or more of the total pore volume have a pore diameter within plus or minus 2 nm of the pore diameter (d), and if a pore diameter corresponding to the peak of the pore size distribution is in a range of 10 to 50 nm (pore diameter (D)), pores accounting for 60% or more of the total pore volume have a pore diameter in a range of (0.75×D) to (1.25×D); and at least one adsorbed component selected from the group consisting of proteins, metal complexes and metals, which is adsorbed on the carbon gel.
摘要翻译：一种碳凝胶复合材料，包括：由平均粒径为2〜50nm的一次粒子构成的碳凝胶，在0.5〜10°的扫描角（2θ）范围内不观察到x射线衍射峰（CuK <60>辐射），并且在由吸附/解吸等温线计算的孔径分布中，如果对应于孔径分布的峰值的孔径不小于1nm并且小于 10nm（孔径（d）），占孔体积的60％以上的孔的孔径（d）的孔径在±2nm以内，如果孔径对应于孔径分布在10〜50nm的范围（孔径（D）），占孔体积的60％以上的孔的孔径在（0.75×D）〜（1.25×D）的范围内， ; 以及吸附在碳凝胶上的至少一种选自蛋白质，金属络合物和金属的吸附组分。

8. 发明授权

US06500573B1 Humidifer device for fuel cells and operating system thereof 失效
标题翻译：用于燃料电池的加湿器装置及其操作系统
公开(公告)号：US06500573B1
公开(公告)日：2002-12-31
申请号：US09391617
申请日：1999-09-07
申请人： Takashi Simazu , Hiroshi Aoki , Tomohisa Wakasugi , Takahiko Asaoka , Kazutaka Hiroshima , Yutaka Ohya , Katsuhito Yamada
发明人： Takashi Simazu , Hiroshi Aoki , Tomohisa Wakasugi , Takahiko Asaoka , Kazutaka Hiroshima , Yutaka Ohya , Katsuhito Yamada
IPC分类号： H01M804
CPC分类号： H01M8/04835 , H01M8/04119 , H01M8/04126 , H01M8/04365 , H01M8/04559 , H01M8/04589 , H01M8/04649 , H01M8/0618
摘要： A humidifier device for use in fuel cells comprising a mist humidifier unit for adding mists to process gas supplied to an electrolyte equipped in a fuel cell and a humidifier unit control device for intermittently operating the mist humidifier unit in accordance with operating condition of the fuel cell.
摘要翻译：一种用于燃料电池的加湿装置，包括：雾化加湿器单元，用于将加入雾化的工艺气体提供给装配在燃料电池中的电解质中;以及加湿器单元控制装置，用于根据燃料电池的运行状态间歇地操作雾化加湿器单元。

9. 发明申请

US20080090128A1 Electrode Catalyst for Fuel Cell and Fuel Cell 审中-公开
标题翻译：燃料电池和燃料电池用电极催化剂
公开(公告)号：US20080090128A1
公开(公告)日：2008-04-17
申请号：US11793309
申请日：2005-12-22
申请人： Katsushi Saito , Hiroaki Takahashi , Hideyasu Kawai , Toshiharu Tabata , Takahiro Nagata , Tomoaki Terada , Yosuke Horiuchi , Norihiko Setoyama , Takahiko Asaoka
发明人： Katsushi Saito , Hiroaki Takahashi , Hideyasu Kawai , Toshiharu Tabata , Takahiro Nagata , Tomoaki Terada , Yosuke Horiuchi , Norihiko Setoyama , Takahiko Asaoka
IPC分类号： B01J23/42 , H01M8/10
CPC分类号： B01J23/89 , B01J21/18 , B01J23/58 , B01J35/0013 , B01J35/006 , H01M4/86 , H01M4/921 , H01M4/926 , H01M2008/1095
摘要： A flooding phenomenon is suppressed in a high current density loading region so as to attempt the improvement of cell performance of fuel cells. An electrode catalyst for fuel cells, in which a catalyst comprising an alloy catalyst composed of a noble metal and one or more transition metals and having surface characteristics such that it shows a pH value in water of 6.0 or more is supported on conductive carriers, and a fuel cell using such electrode catalyst for fuel cells, are provided.
摘要翻译：在高电流密度加载区域中抑制了泛洪现象，从而试图提高燃料电池的电池性能。一种燃料电池用电极催化剂，其中，包含由贵金属和一种或多种过渡金属组成的合金催化剂，具有使其在水中的pH值为6.0以上的表面特性的催化剂负载在导电性载体上，提供了使用这种燃料电池用电极催化剂的燃料电池。

10. 发明授权

US07060385B2 Noble metal-base metal alloy catalyst, evaluation of such catalyst, and method of producing such catalyst 失效
公开(公告)号：US07060385B2
公开(公告)日：2006-06-13
申请号：US10206036
申请日：2002-07-29
申请人： Hisao Kato , Takahiko Asaoka , Kazutaka Hiroshima
发明人： Hisao Kato , Takahiko Asaoka , Kazutaka Hiroshima
IPC分类号： H01M4/96 , B01J23/89
CPC分类号： H01M4/881 , H01M4/8605 , H01M4/92 , H01M4/926 , H01M8/1004 , Y02P70/56
摘要： The technique of the present invention attains simple and accurate evaluation of the performance of a fuel cell and enables produce of a high-performance electrode catalyst and a high-performance fuel cell. The procedure makes platinum, a noble metal, and iron, a base metal, carried on carbon having a large specific surface area, and heats up the carbon with platinum and iron to a specific temperature to reduce iron. A resulting platinum-iron alloy electrode catalyst exerts excellent catalytic functions. A fuel cell using this electrode catalyst has a high IR compensation voltage. The quantity of carbon monoxide adsorbed by this novel electrode catalyst is not less than 14 Ncc per one gram of platinum. The atomic number ratio of iron (Fe) to platinum (Pt) in the catalyst is not lower than 0.14 by EDX analysis, and the ratio of the binding number of Pt atom with Fe atom to the total binding number relating to Pt atom is not lower than 0.10 by EXAFS analysis. Each electrode catalyst produced is evaluated by measurement of these data. The fuel cell including the electrode catalyst having the favorable result of evaluation ensures the desired performances.

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