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1. 发明授权

US4414138A Fluid catalytic cracking catalyst 失效
标题翻译：流化催化裂化催化剂
公开(公告)号：US4414138A
公开(公告)日：1983-11-08
申请号：US384422
申请日：1982-06-02
申请人： Randall H. Petty , Burton H. Bartley
发明人： Randall H. Petty , Burton H. Bartley
IPC分类号： B01D53/86 , B01J29/076 , C10G11/04 , C10G11/18 , B01J29/16 , B01J21/04 , B01J23/18
CPC分类号： B01J29/076 , B01D53/8609 , C10G11/04 , C10G11/18 , B01J2229/20 , B01J2229/42
摘要： An active alumina composite and a cracking catalyst comprising the composite useful in hydrocarbon conversion processes. The composite and catalyst are particularly useful in fluid catalytic cracking processes, wherein sulfur-containing feedstock is subjected to catalytic conversion at a temperature in the range of about 800.degree. F. to about 1300.degree. F. in the presence of the catalyst which becomes sulfided during the conversion reaction and thereafter the catalyst is subjected to regeneration by burning sulfur-containing coke from the catalyst with an oxygen-containing gas at a temperature within the range of about 800.degree. to 1500.degree. F. The novel catalyst composition comprises 90 to 99 weight percent cracking catalyst and 1 to 10 weight percent of a composite of alumina and bismuth oxides containing 0.05 to 25 weight percent bismuth, calculated as the metal. This catalyst composition has the ability to remove sulfur oxides from gases to a greater extent than catalyst compositions comprising cracking catalyst and active alumina. The composition may comprise also platinum or a platinum group metal as a carbon monoxide combustion promoter.
摘要翻译：活性氧化铝复合材料和裂解催化剂，其包含可用于烃转化方法的复合材料。复合材料和催化剂在流化催化裂化方法中特别有用，其中含硫原料在约800°F至约1300°F范围内的温度下进行催化转化。在转化反应期间，然后通过在约800-1500℃的温度范围内用含氧气体从催化剂中燃烧含硫焦炭来使催化剂再生。新型催化剂组合物包含90至99 重量百分比的裂化催化剂和1至10重量％的含有0.05至25重量％铋的氧化铝和氧化铋的复合材料，以金属计算。该催化剂组合物具有比包含裂化催化剂和活性氧化铝的催化剂组合物更大程度地从气体中除去硫氧化物的能力。组合物还可以包含铂或铂族金属作为一氧化碳燃烧促进剂。

2. 发明授权

US4344926A Fluid catalytic cracking 失效
标题翻译：流体催化裂化
公开(公告)号：US4344926A
公开(公告)日：1982-08-17
申请号：US180357
申请日：1980-08-22
申请人： Randall H. Petty , Burton H. Bartley
发明人： Randall H. Petty , Burton H. Bartley
IPC分类号： B01D53/50 , B01D53/81 , B01D53/86 , B01J20/08 , B01J29/076 , C10G11/05 , C10G11/18 , B01D53/34
CPC分类号： B01J29/076 , B01D53/8609 , C10G11/05 , C10G11/18 , B01J2229/20 , B01J2229/42
摘要： Gaseous sulfur compounds are removed from a sulfur-containing gas mixture by reacting sulfur oxides in the gas mixture with alumina in association with bismuth.The process is particularly useful in fluid catalytic cracking of sulfur-containing petroleum charge stocks wherein sulfur is contained in coke deposited on the fluidized cracking catalyst. By the process of this invention, sulfur oxides may be removed from regenerator off-gases from a fluidized catalytic cracking unit by incorporating particulate alumina impregnated with bismuth in particulate cracking catalyst whereby sulfur oxides generated in the regeneration of the catalyst are reacted with bismuth-impregnated alumina. Sulfur oxides produced during regeneration of the catalyst by burning the coke with air are captured and converted to hydrogen sulfide in the cracking reactor. The hydrogen sulfide so produced is readily separated from petroleum products of the catalytic cracking reaction process.
摘要翻译：通过将气体混合物中的氧化硫与铋相关联的氧化铝反应，从含硫气体混合物中除去气态硫化合物。该方法在含硫石油电荷原料的流化催化裂化中特别有用，其中硫在沉积在流化裂化催化剂上的焦炭中含有。通过本发明的方法，硫化氢可以从流化催化裂化装置的再生器废气中除去，其中通过将在铋中浸渍的颗粒氧化铝掺入颗粒裂化催化剂中，由此在催化剂再生中产生的硫氧化物与铋浸渍氧化铝。在空气中燃烧焦炭催化剂再生过程中产生的硫氧化物在裂解反应器中被捕获并转化成硫化氢。所生成的硫化氢容易与催化裂化反应过程的石油产物分离。

3. 发明授权

US4941964A Hydrotreatment process employing catalyst with specified pore size distribution 失效
标题翻译：使用具有规定孔径分布的催化剂的加氢处理方法
公开(公告)号：US4941964A
公开(公告)日：1990-07-17
申请号：US168095
申请日：1988-03-14
申请人： Pei-Shing E. Dai , David E. Sherwood, Jr. , Burton H. Bartley , Randall H. Petty
发明人： Pei-Shing E. Dai , David E. Sherwood, Jr. , Burton H. Bartley , Randall H. Petty
IPC分类号： B01J35/10 , C10G45/08
CPC分类号： C10G45/08 , B01J35/1019 , B01J35/1042 , B01J35/1061 , B01J35/108
摘要： A process for the hydrotreatment of a sulfur and metal-containing hydrocarbon feed comprises contacting said feed with hydrogen and a catalyst in a manner such that the catalyst is maintained at isothermal conditions and is exposed to a uniform quality of feed, where said catalyst has a composition comprising 3.0-5.0 wt. % of an oxide of a Group VIII metal, 14.5-24.0 wt. % of an oxide of a Group VIB metal and 0-2.0 wt. % of an oxide of phosphorus supported on a porous alumina support, and said catalyst is further characterized by having a total surface area of 150-210 m.sup.2 /g and a total pore volume of 0.50-0.75 cc/g with a pore diameter distribution such that micropores having diameters of 100-160A constitute 70-85% of the total pore volume of said catalyst and macropores having diameters of greater than 250A constitute 5.5-22.0% of the total pore volume of said catalyst. The process of the instant invention is particularly effective in achieving desired levels of hydrodesulfurization in the fraction of hydrotreated/hydrocracked petroleum resid product having a boiling point greater than 1000.degree. F.
摘要翻译：用于加氢处理含硫和含金属的烃进料的方法包括使所述进料与氢气和催化剂以使得催化剂保持在等温条件并暴露于均匀质量的进料的方式接触，其中所述催化剂具有组合物包含3.0-5.0重量％％的VIII族金属的氧化物，14.5-24.0wt。％VIB族金属的氧化物和0-2.0wt。负载在多孔氧化铝载体上的磷氧化物的％，并且所述催化剂的特征还在于总表面积为150-210m 2 / g，总孔体积为0.50-0.75cc / g，孔直径分布如直径为100-160A的微孔构成所述催化剂的总孔体积的70-85％，直径大于250A的大孔构成所述催化剂总孔体积的5.5-22.0％。本发明的方法在沸点大于1000°F的加氢处理/加氢裂化石油渣产物馏分中达到所需加氢脱硫水平特别有效。

4. 发明授权

US4446010A Fluid catalytic cracking 失效
标题翻译：流体催化裂化
公开(公告)号：US4446010A
公开(公告)日：1984-05-01
申请号：US403096
申请日：1982-07-29
申请人： Randall H. Petty , Burton H. Bartley
发明人： Randall H. Petty , Burton H. Bartley
IPC分类号： B01D53/86 , B01J29/076 , C10G11/18 , C10G25/09
CPC分类号： C10G11/18 , B01D53/8609 , B01J29/076 , B01J2229/20 , B01J2229/42
摘要： A fluid catalytic cracking process for sulfur-containing petroleum charge stocks wherein sulfur contained in coke deposited on the fluidized cracking catalyst in the reactor is converted to sulfur oxides in the regenerator and removed from regenerator off-gases by incorporating a composite of alumina and bismuth oxides in a particulate cracking catalyst. Sulfur oxides produced during regeneration of the catalyst by burning the coke with air in the regenerator are captured by the alumina-bismuth oxides composite and converted to hydrogen sulfide in the cracking reactor. The hydrogen sulfide so produced is readily separated from petroleum products of the catalytic cracking reaction process.
摘要翻译：用于含硫石油电荷原料的流化催化裂化方法，其中沉积在反应器中的流化裂化催化剂上的焦炭中所含的硫转化为再生器中的硫氧化物，并通过掺入氧化铝和氧化铋的复合物从再生器废气中除去在颗粒裂化催化剂中。在再生器中用空气燃烧焦炭在催化剂再生期间产生的硫氧化物被氧化铝 - 氧化铋复合物捕获并在裂化反应器中转化成硫化氢。所生成的硫化氢容易与催化裂化反应过程的石油产物分离。

5. 发明授权

US5047142A Catalyst composition and method for hydroprocessing petroleum feedstocks 失效
标题翻译：用于加氢处理石油原料的催化剂组合物和方法
公开(公告)号：US5047142A
公开(公告)日：1991-09-10
申请号：US194379
申请日：1988-05-13
申请人： David E. Sherwood, Jr. , Burton H. Bartley , Laurence D. Neff , Pei-Shing E. Dai
发明人： David E. Sherwood, Jr. , Burton H. Bartley , Laurence D. Neff , Pei-Shing E. Dai
IPC分类号： B01J23/85 , B01J35/10 , C10G45/08
CPC分类号： C10G45/08 , B01J23/85 , B01J35/002 , B01J35/1019 , B01J35/1042 , B01J35/1061 , B01J35/108
摘要： A catalyst composition useful in the hydroprocessing of a sulfur- and metal-containing hydrocarbon feedstock comprises 1.0-5.0 weight percent of an oxide of nickel or cobalt and 10.0-25.0 weight percent of an oxide of molybdenum, all supported on a porous alumina support in such a manner that the molybdenum gradient of the catalyst has a value of less than 6.0 and 15-30% of the nickel or cobalt contained in the catalyst is in an acid extractable form. The catalyst is further characterized by having a total surface area of 150-210 m.sup.2 /g, a total more volume of 0.50-0.75 cc/g, and a pore size distribution such that pores having diameters of less than 100A constitute less than 25.0%, pores having diameters of 100-160A constitute 70.0-85.0% and pores having diameters of greater than 250A constitutes 1.0-15.0% of the total pore volume of the catalyst. A method for the hydroprocessing of a sulfur- and metal-containing hydrocarbon feedstock comprises contacting the feedstock with the abovedescribed catalyst and hydrogen in a maner such that the catalyst is maintained at isothermal conditions and is exposed to a uniform quality of feed. The method is particularly effective in achieving desired levels of hydrodesulfurization in vacuum residual feedstocks.
摘要翻译：用于含硫和金属的烃原料的加氢处理的催化剂组合物包含1.0-5.0重量％的镍或钴的氧化物和10.0-25.0重量％的钼的氧化物，所有这些都负载在多孔氧化铝载体上催化剂的钼梯度的值小于6.0，催化剂中所含的镍或钴的15-30％为酸可萃取形式。催化剂的特征还在于总表面积为150-210m2 / g，总体积为0.50-0.75cc / g，孔径分布使直径小于100A的孔隙小于25.0％直径为100-160A的孔构成70.0-85.0％，直径大于250A的孔构成催化剂总孔体积的1.0-15.0％。用于加氢处理含硫和金属的烃原料的方法包括使原料与上述催化剂和加氢器中的氢接触，使得催化剂保持在等温条件下并暴露于均匀的进料质量。该方法在真空残留原料中达到期望水平的加氢脱硫特别有效。

6. 发明授权

US5354452A Synthesis of zeolites 失效
标题翻译：沸石的合成
公开(公告)号：US5354452A
公开(公告)日：1994-10-11
申请号：US962549
申请日：1992-10-19
申请人： Eugene P. Dai , David E. Sherwood, Jr. , Burton H. Bartley
发明人： Eugene P. Dai , David E. Sherwood, Jr. , Burton H. Bartley
IPC分类号： B01J29/08 , C10G47/16 , C10G45/12
CPC分类号： C10G47/16 , B01J29/084
摘要： A novel zeolite characterized by a large number of secondary pores, a substantially decreased lattice constant, and a substantially decreased acid site density is attained by hydrothermal and acid-treating of an ultrastable Y-zeolite or a superultrastable Y-zeolite.
摘要翻译：通过对超稳定的Y型沸石或超级不可渗透的Y型沸石的水热和酸处理，可以获得特征在于大量二次孔，基本上降低的晶格常数和基本上降低的酸位密度的沸石。

7. 发明授权

US4065514A Preparation of methane 失效
标题翻译：甲烷的制备
公开(公告)号：US4065514A
公开(公告)日：1977-12-27
申请号：US636237
申请日：1975-11-28
申请人： Burton H. Bartley , John H. Estes
发明人： Burton H. Bartley , John H. Estes
IPC分类号： B01J23/89 , C07C4/00 , C07C9/02
CPC分类号： B01J23/89 , C07C4/00 , C07C2523/40 , C07C2523/42 , C07C2523/74 , C07C2523/745 , C07C2523/89
摘要： In accordance with certain of its aspects, this invention relates to a finely-divided, high surface area supported catalyst containing a metal of the platinum-palladium group and a metal of the iron group wherein each of said metals is substantially uniformly distributed throughout the body of said supported catalyst -- and to the use of this catalyst to prepare methane by the reaction of hydrogen and hydrocarbons.
摘要翻译：根据其某些方面，本发明涉及一种细分散的高表面积负载催化剂，其包含铂 - 钯基金属和铁基金属，其中所述金属中的每一种基本上均匀分布在整个体内的所述负载催化剂，以及使用该催化剂通过氢和烃的反应制备甲烷。

8. 发明授权

US4297245A Catalyst for the preparation of methane 失效
标题翻译：用于制备甲烷的催化剂
公开(公告)号：US4297245A
公开(公告)日：1981-10-27
申请号：US853079
申请日：1977-11-21
申请人： Burton H. Bartley , John H. Estes
发明人： Burton H. Bartley , John H. Estes
IPC分类号： B01J23/89 , C07C4/00 , B01J21/08 , B01J23/56 , B01J23/74
CPC分类号： B01J23/89 , C07C4/00 , C07C2523/40 , C07C2523/42 , C07C2523/74 , C07C2523/745 , C07C2523/89
摘要： In accordance with certain of its aspects, this invention relates to a finely-divided, high surface area supported catalyst containing a metal of the platinum-palladium group and a metal of the iron group wherein each of said metals is substantially uniformly distributed throughout the body of said supported catalyst--and to the use of this catalyst to prepare methane by the reaction of hydrogen and hydrocarbons.
摘要翻译：根据其某些方面，本发明涉及一种细分散的高表面积负载催化剂，其包含铂 - 钯基金属和铁基金属，其中所述金属中的每一种基本上均匀分布在整个体内的所述负载催化剂，以及使用该催化剂通过氢和烃的反应制备甲烷。

9. 发明授权

US5534135A Synthesis of zeolites 失效
标题翻译：沸石的合成
公开(公告)号：US5534135A
公开(公告)日：1996-07-09
申请号：US206803
申请日：1994-03-07
申请人： Pei-Shing E. Dai , David E. Sherwood, Jr. , Burton H. Bartley
发明人： Pei-Shing E. Dai , David E. Sherwood, Jr. , Burton H. Bartley
IPC分类号： B01J29/08 , C10G11/05 , C10G49/08 , C10G45/00
CPC分类号： B01J29/084 , C10G11/05 , C10G49/08 , Y10S423/21
摘要： A novel zeolite characterized by a large number of secondary pores, a substantially decreased Lattice Constant of below about 24.19 .ANG., and a substantially decreased Acid Site Density is attained by hydrothermal and acid-treating of an ultrastable Y-zeolite.
摘要翻译：特征在于大量二次孔，基本上降低的晶格常数低于约24.19的新型沸石，并且通过对超稳定Y型沸石的水热和酸处理实现了显着降低的酸性位点密度。

10. 发明授权

US5094994A Catalyst composition for hydroprocessing petroleum feedstocks 失效
标题翻译：用于加氢处理石油原料的催化剂组合物
公开(公告)号：US5094994A
公开(公告)日：1992-03-10
申请号：US645772
申请日：1991-01-25
申请人： David E. Sherwood, Jr. , Burton H. Bartley , Laurence D. Neff , Pei-Shing E. Dai
发明人： David E. Sherwood, Jr. , Burton H. Bartley , Laurence D. Neff , Pei-Shing E. Dai
IPC分类号： B01J23/85 , B01J35/10 , C10G45/08
CPC分类号： C10G45/08 , B01J23/85 , B01J35/1019 , B01J35/1042 , B01J35/1061 , B01J35/108
摘要： A catalyst composition useful in the hydroprocessing of a sulfur- and metal-containing hydrocarbon feedstock comprises 1.0-5.0 weight percent of an oxide of nickel or cobalt and 10.0-25.0 weight percent of an oxide of molybdenum, all supported on a porous alumina support in such a manner that the molybdenum gradient of the catalyst has a value of less than 6.0 and 15-30% of the nickel or cobalt contained in the catalyst is in an acid extractable form. The catalyst is further characterized by having a total surface area of 150-210 m.sup.2 /g, a total pore volume of 0.50-0.75 cc/g, and a pore size distribution such that pores having diameters of less than 100A constitute less than 25.0%, pores having diameters of 100-160A constitute 70.0-85.0% and pores having diameters of greater than 250A constitute 1.0-15.0% of the total pore volume of the catalyst. A method for the hydroprocessing of a sulfur- and metal-containing hydrocarbon feedstock comprises contacting the feedstock with the abovedescribed catalyst and hydrogen in a manner such that the catalyst is maintained at isothermal conditions and is exposed to a uniform quality of feed. The method is particularly effective in achieving desired levels of hydrodesulfurization in vacuum residual feedstocks.
摘要翻译：用于含硫和金属的烃原料的加氢处理的催化剂组合物包含1.0-5.0重量％的镍或钴的氧化物和10.0-25.0重量％的钼的氧化物，所有这些都负载在多孔氧化铝载体上催化剂的钼梯度的值小于6.0，催化剂中所含的镍或钴的15-30％为酸可萃取形式。催化剂的特征还在于总表面积为150-210m2 / g，总孔体积为0.50-0.75cc / g，孔径分布使得直径小于100A的孔隙小于25.0％直径为100-160A的孔构成70.0-85.0％，直径大于250A的孔构成催化剂总孔体积的1.0-15.0％。用于含硫和金属的烃原料的加氢处理的方法包括使原料与上述催化剂和氢气以使得催化剂保持在等温条件并暴露于均匀的进料质量的方式接触。该方法在真空残留原料中达到期望水平的加氢脱硫特别有效。

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