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1. 发明申请

US20110198216A1 REMOVAL OF IMPURITY PHASES FROM ELECTROCHEMICAL DEVICES 有权
标题翻译：从电化学设备中去除污染物相
公开(公告)号：US20110198216A1
公开(公告)日：2011-08-18
申请号：US12674943
申请日：2008-08-29
申请人： Peter Halvor Larsen , Mogens Mogensen , Peter Vang Hendriksen , Søren Linderoth , Ming Chen
发明人： Peter Halvor Larsen , Mogens Mogensen , Peter Vang Hendriksen , Søren Linderoth , Ming Chen
IPC分类号： C25B9/00 , H01M8/10 , B05D3/02
CPC分类号： H01M8/1213 , H01M4/8663 , H01M4/8889 , H01M2008/1293 , Y02E60/521 , Y02E60/525
摘要： The present invention provides a solid oxide cell comprising a support layer, a first electrode layer, an electrolyte layer, and a second cathode layer, wherein at least one of the electrode layers comprises electrolyte material, a catalyst and agglomerated particles selected from the group consisting of alkali oxides, earth alkali oxides and transition metal oxides.
摘要翻译：本发明提供了一种固体氧化物电池，其包括支撑层，第一电极层，电解质层和第二阴极层，其中至少一个电极层包括电解质材料，催化剂和附聚粒子的碱金属氧化物，碱土金属氧化物和过渡金属氧化物。

2. 发明授权

US09077021B2 Removal of impurity phases from electrochemical devices 有权
标题翻译：从电化学装置去除杂质相
公开(公告)号：US09077021B2
公开(公告)日：2015-07-07
申请号：US12674943
申请日：2008-08-29
申请人： Peter Halvor Larsen , Mogens Mogensen , Peter Vang Hendriksen , Søren Linderoth , Ming Chen
发明人： Peter Halvor Larsen , Mogens Mogensen , Peter Vang Hendriksen , Søren Linderoth , Ming Chen
IPC分类号： H01M4/90 , H01M8/06 , H01M8/12 , H01M4/86 , H01M4/88
CPC分类号： H01M8/1213 , H01M4/8663 , H01M4/8889 , H01M2008/1293 , Y02E60/521 , Y02E60/525
摘要： The present invention provides a solid oxide cell comprising a support layer, a first electrode layer, an electrolyte layer, and a second cathode layer, wherein at least one of the electrode layers comprises electrolyte material, a catalyst and agglomerated particles selected from the group consisting of alkali oxides, earth alkali oxides and transition metal oxides.
摘要翻译：本发明提供了一种固体氧化物电池，其包括支撑层，第一电极层，电解质层和第二阴极层，其中至少一个电极层包括电解质材料，催化剂和附聚粒子的碱金属氧化物，碱土金属氧化物和过渡金属氧化物。

3. 发明申请

US20100015473A1 MULTI-LAYER COATING 有权
标题翻译：多层涂料
公开(公告)号：US20100015473A1
公开(公告)日：2010-01-21
申请号：US12298458
申请日：2007-04-24
申请人： Peter Vang Hendriksen , Lars Mikkelsen , Peter Halvor Larsen , Soeren Linderoth , Mogens Mogensen
发明人： Peter Vang Hendriksen , Lars Mikkelsen , Peter Halvor Larsen , Soeren Linderoth , Mogens Mogensen
IPC分类号： H01M8/02 , B32B7/02 , B32B9/00 , B05D3/14 , B05D1/36 , C23C16/40 , C23C14/34 , H01M6/42 , C23C16/513
CPC分类号： H01M8/0228 , C25B9/04 , C25B9/18 , H01M4/9033 , H01M8/0206 , H01M8/0215 , H01M8/0217 , H01M8/0232 , H01M8/0236 , H01M8/0245 , H01M8/12 , H01M8/1286 , H01M8/2425 , H01M2008/1293 , Y02E60/521 , Y02E60/525 , Y10T428/24942
摘要： A multi-layer coating for protection of metals and alloys against oxidation at high temperatures in general is provided. The invention utilizes a multi-layer ceramic coating on metals or alloys for increased oxidation-resistance, comprising at least two layers, wherein the first layer (3) which faces the metal containing surface and the second layer facing the surrounding atmosphere (4) both comprise an oxide, and wherein the first layer (3) has a tracer diffusion coefficient for cations Mm+, where M is the scale forming element of the alloy, and the second layer (4) has a tracer diffusion coefficient for oxygen ions O2− satisfying the following formula: wherein p(O2)m is the oxygen partial pressure in equilibrium between the metallic sub-strate and MaOb, p(O2)ex is the oxygen partial pressure in the reaction atmosphere, DM is the tracer diffusion coefficient of the metal cations Mm+ in the first layer (3), and Do is O tracer diffusion coefficient in the second layer (4). The coating may be used in high temperature devices, particularly for coating interconnect materials in solid oxide electrolytic devices, including solid oxide fuel cells (SOFCs) and solid oxide electrolysis cells (SOECs).
摘要翻译：提供了用于在高温下保护金属和合金免于氧化的多层涂层。本发明利用金属或合金上的多层陶瓷涂层来提高抗氧化性，包括至少两层，其中面对金属容纳表面的第一层（3）和面向周围大气的第二层（4）都是包括氧化物，并且其中所述第一层（3）具有用于阳离子Mm +的示踪剂扩散系数，其中M是所述合金的氧化皮形成元素，并且所述第二层（4）具有氧离子的示踪扩散系数O2-满足其中p（O2）m是金属底层与MaOb之间平衡的氧分压，p（O2）ex是反应气氛中的氧分压，DM是金属的示踪剂扩散系数阳离子Mm +在第一层（3）中，Do是第二层（4）中的O示踪剂扩散系数。该涂层可用于高温装置中，特别是用于在固体氧化物电解装置（包括固体氧化物燃料电池（SOFC））和固体氧化物电解槽（SOEC）中涂覆互连材料。

4. 发明授权

US09263758B2 Reversible solid oxide fuel cell stack and method for preparing same 有权
标题翻译：可逆固体氧化物燃料电池堆及其制备方法
公开(公告)号：US09263758B2
公开(公告)日：2016-02-16
申请号：US12065357
申请日：2006-08-31
申请人： Peter Halvor Larsen , Anders Smith , Mogens Mogensen , Soeren Linderoth , Peter Vang Hendriksen
发明人： Peter Halvor Larsen , Anders Smith , Mogens Mogensen , Soeren Linderoth , Peter Vang Hendriksen
IPC分类号： H01M8/24 , H01M4/86 , H01M4/88 , H01M4/90 , H01M8/02 , H01M8/12
CPC分类号： H01M8/243 , H01M4/861 , H01M4/8885 , H01M4/9033 , H01M4/905 , H01M8/0276 , H01M8/2404 , H01M8/2435 , H01M8/2483 , H01M8/2484 , H01M2008/1293 , Y02E60/50 , Y02E60/525 , Y02P70/56
摘要： A reversible SOFC monolithic stack is provided which comprises: 1) a first component which comprises at least one porous metal containing layer (1) with a combined electrolyte and sealing layer on the porous metal containing layer (1); wherein the at least one porous metal containing layer (1) hosts an electrode; 2) a second component comprising at least one porous metal containing layer (1) with a combined interconnect and sealing layer on the porous metal containing layer; wherein the at least one porous metal containing layers hosts an electrode. Further provided is a method for preparing a reversible solid oxide fuel cell stack. The obtained solid oxide fuel cell stack has improved mechanical stability and high electrical performance, while the process for obtaining same is cost effective.
摘要翻译：提供了可逆的SOFC单片堆叠，其包括：1）包含至少一个多孔金属含层（1）的第一组分与多孔金属含有层（1）上的组合电解质和密封层; 其中所述至少一个含多孔金属的层（1）承载电极; 2）第二组分，其包括在多孔金属含有层上具有组合的互连和密封层的至少一个含多孔金属的层（1）; 其中所述至少一个含多孔金属的层承载电极。还提供了制备可逆固体氧化物燃料电池堆的方法。所获得的固体氧化物燃料电池堆具有改进的机械稳定性和高的电性能，而获得固体氧化物燃料电池堆的方法是成本有效的。

5. 发明授权

US08859116B2 Multi-layer coating 有权
标题翻译：多层涂层
公开(公告)号：US08859116B2
公开(公告)日：2014-10-14
申请号：US12298458
申请日：2007-04-24
申请人： Peter Vang Hendriksen , Lars Mikkelsen , Peter Halvor Larsen , Soeren Linderoth , Mogens Mogensen
发明人： Peter Vang Hendriksen , Lars Mikkelsen , Peter Halvor Larsen , Soeren Linderoth , Mogens Mogensen
IPC分类号： H01M8/02 , H01M6/42 , B32B7/02 , B32B9/00 , B05D3/14 , B05D1/36 , C23C16/40 , C23C14/34 , H01M8/12 , H01M4/90
CPC分类号： H01M8/0228 , C25B9/04 , C25B9/18 , H01M4/9033 , H01M8/0206 , H01M8/0215 , H01M8/0217 , H01M8/0232 , H01M8/0236 , H01M8/0245 , H01M8/12 , H01M8/1286 , H01M8/2425 , H01M2008/1293 , Y02E60/521 , Y02E60/525 , Y10T428/24942
摘要： A multi-layer coating for protection of metals and alloys against oxidation at high temperatures is provided. The invention utilizes a multi-layer ceramic coating on metals or alloys for increased oxidation-resistance, comprising at least two layers, wherein the first layer (3) and the second layer (4) both comprise an oxide, and wherein the first layer (3) has a tracer diffusion coefficient for cations Mm+, where M is the scale forming element of the alloy, and the second layer (4) has a tracer diffusion coefficient for oxygen ions O2− satisfying the following formula: ∫ ln ⁢ ⁢ p ⁡ ( O 2 ) in ln ⁢ ⁢ p ⁡ ( O 2 ) ex ⁢ ( D O + m 2 ⁢ D M ) ⁢ ⁢ ⅆ ln ⁢ ⁢ p ⁡ ( O 2 )
摘要翻译：提供了用于保护金属和合金在高温下抵抗氧化的多层涂层。本发明利用金属或合金上的多层陶瓷涂层来提高耐氧化性，包括至少两层，其中第一层（3）和第二层（2）均包含氧化物，并且其中第一层（ 3）具有阳离子Mm +的示踪剂扩散系数，其中M是合金的氧化皮形成元素，第二层（4）具有氧离子O 2的示踪剂扩散系数，满足以下公式：∫ln⁢p⁡ （O 2）ex（DO + m 2 DM）························（2）其中p （O 2）in，p（O 2）ex，DM和DO如本文所定义。该涂层可用于高温装置中，特别是用于在固体氧化物电解装置（包括固体氧化物燃料电池（SOFC））和固体氧化物电解槽（SOEC）中涂覆互连材料。

6. 发明申请

US20130025292A1 REVERSIBLE SOLID OXIDE FUEL CELL STACK AND METHOD FOR PREPARING SAME 审中-公开
标题翻译：可逆的固体氧化物燃料电池堆和其制备方法
公开(公告)号：US20130025292A1
公开(公告)日：2013-01-31
申请号：US13559937
申请日：2012-07-27
申请人： Peter Halvor Larsen , Anders Smith , Mogens Mogensen , Soeren Linderoth , Peter Vang Hendriksen
发明人： Peter Halvor Larsen , Anders Smith , Mogens Mogensen , Soeren Linderoth , Peter Vang Hendriksen
IPC分类号： F02C1/00 , C25B9/18 , H01M8/10 , H01M8/24
CPC分类号： H01M8/243 , H01M4/861 , H01M4/8885 , H01M4/9033 , H01M4/905 , H01M8/0276 , H01M8/2404 , H01M8/2435 , H01M8/2483 , H01M8/2484 , H01M2008/1293 , Y02P70/56
摘要： A reversible SOFC monolithic stack is provided which comprises: 1) a first component which comprises at least one porous metal containing layer (1) with a combined electrolyte and sealing layer on the porous metal containing layer (1); wherein the at least one porous metal containing layer (1) hosts an electrode; 2) a second component comprising at least one porous metal containing layer (1) with a combined interconnect and sealing layer on the porous metal containing layer; wherein the at least one porous metal containing layers hosts an electrode. Further provided is a method for preparing a reversible solid oxide fuel cell stack. The obtained solid oxide fuel cell stack has improved mechanical stability and high electrical performance, while the process for obtaining same is cost effective.
摘要翻译：提供了可逆的SOFC单片堆叠，其包括：1）包含至少一个多孔金属含层（1）的第一组分与多孔金属含有层（1）上的组合电解质和密封层; 其中所述至少一个含多孔金属的层（1）承载电极; 2）第二组分，其包括在多孔金属含有层上具有组合的互连和密封层的至少一个含多孔金属的层（1）; 其中所述至少一个含多孔金属的层承载电极。还提供了制备可逆固体氧化物燃料电池堆的方法。所获得的固体氧化物燃料电池堆具有改进的机械稳定性和高的电性能，而获得固体氧化物燃料电池堆的方法是成本有效的

7. 发明授权

US08802321B2 Horizontally graded structures for electrochemical and electronic devices 有权
标题翻译：用于电化学和电子器件的水平分级结构
公开(公告)号：US08802321B2
公开(公告)日：2014-08-12
申请号：US12191568
申请日：2008-08-14
申请人： Peter Halvor Larsen , Peter Vang Hendriksen , Soren Linderoth , Mogens Mogensen
发明人： Peter Halvor Larsen , Peter Vang Hendriksen , Soren Linderoth , Mogens Mogensen
IPC分类号： H01M8/00 , H01M8/10 , H01M8/12 , B05D5/12
CPC分类号： H01M4/8857 , C23C28/042 , C23C28/044 , C23C28/048 , H01M4/861 , H01M4/8636 , H01M4/8642 , H01M4/8657 , H01M4/8835 , H01M8/1213 , H01M8/124 , H01M2004/8684 , H01M2008/1293 , H01M2300/0094 , Y02P70/56 , Y10T156/1089
摘要： The present invention provides a graded multilayer structure, comprising a support layer (1) and at least 10 layers (2, 3) forming a graded layer, wherein each of the at least 10 layers (2, 3) is at least partially in contact with the support layer (1), wherein the at least 10 layers (2, 3) differ from each other in at least one property selected from layer composition, porosity and conductivity, and wherein the at least 10 layers (2, 3) are arranged such that the layer composition, porosity and/or conductivity horizontally to the support layer (1) forms a gradient over the total layer area.
摘要翻译：本发明提供了一种分级多层结构，其包括支撑层（1）和形成梯度层的至少10层（2,3），其中所述至少10层（2,3）中的每一层至少部分地接触与所述支撑层（1）形成，其中所述至少10层（2,3）在选自层组成，孔隙率和导电性中的至少一种性质中彼此不同，并且其中所述至少10层（2,3）布置成使得水平到支撑层（1）的层组成，孔隙率和/或导电性在总层面积上形成梯度。

8. 发明申请

US20080248361A1 Reversible Solid Oxide Fuel Cell Stack and Method For Preparing Same 有权
标题翻译：可逆固体氧化物燃料电池堆及其制备方法
公开(公告)号：US20080248361A1
公开(公告)日：2008-10-09
申请号：US12065357
申请日：2006-08-31
申请人： Peter Halvor Larsen , Anders Smith , Mogens Mogensen , Soeren Linderoth , Peter Vang Hendriksen
发明人： Peter Halvor Larsen , Anders Smith , Mogens Mogensen , Soeren Linderoth , Peter Vang Hendriksen
IPC分类号： H01M8/10 , H01M8/00 , B05D5/12
CPC分类号： H01M8/243 , H01M4/861 , H01M4/8885 , H01M4/9033 , H01M4/905 , H01M8/0276 , H01M8/2404 , H01M8/2435 , H01M8/2483 , H01M8/2484 , H01M2008/1293 , Y02E60/50 , Y02E60/525 , Y02P70/56
摘要： A reversible SOFC monolithic stack is provided which comprises: 1) a first component which comprises at least one porous metal containing layer (1) with a combined electrolyte and sealing layer on the porous metal containing layer (1); wherein the at least one porous metal containing layer (1) hosts an electrode; 2) a second component comprising at least one porous metal containing layer (1) with a combined interconnect and sealing layer on the porous metal containing layer; wherein the at least one porous metal containing layers hosts an electrode. Further provided is a method for preparing a reversible solid oxide fuel cell stack. The obtained solid oxide fuel cell stack has improved mechanical stability and high electrical performance, while the process for obtaining same is cost effective.
摘要翻译：提供了一种可逆SOFC单片堆叠，其包括：1）包含至少一个多孔金属含有层（1）的第一组分与多孔金属含有层（1）上的组合电解质和密封层; 其中所述至少一个含多孔金属的层（1）承载电极; 2）第二组分，其包括在多孔金属含有层上具有组合的互连和密封层的至少一个含多孔金属的层（1）; 其中所述至少一个含多孔金属的层承载电极。还提供了制备可逆固体氧化物燃料电池堆的方法。所获得的固体氧化物燃料电池堆具有改进的机械稳定性和高的电性能，而获得固体氧化物燃料电池堆的方法是成本有效的。

9. 发明申请

US20090061287A1 Horizontally Graded Structures for Electrochemical and Electronic Devices 有权
标题翻译：电化学和电子器件的水平分级结构
公开(公告)号：US20090061287A1
公开(公告)日：2009-03-05
申请号：US12191568
申请日：2008-08-14
申请人： Peter Halvor Larsen , Peter Vang Hendriksen , Soren Linderoth , Mogens Mogensen
发明人： Peter Halvor Larsen , Peter Vang Hendriksen , Soren Linderoth , Mogens Mogensen
IPC分类号： H01M4/06 , H01M4/08
CPC分类号： H01M4/8857 , C23C28/042 , C23C28/044 , C23C28/048 , H01M4/861 , H01M4/8636 , H01M4/8642 , H01M4/8657 , H01M4/8835 , H01M8/1213 , H01M8/124 , H01M2004/8684 , H01M2008/1293 , H01M2300/0094 , Y02P70/56 , Y10T156/1089
摘要： The present invention provides a graded multilayer structure, comprising a support layer (1) and at least 10 layers (2, 3) forming a graded layer, wherein each of the at least 10 layers (2, 3) is at least partially in contact with the support layer (1), wherein the at least 10 layers (2, 3) differ from each other in at least one property selected from layer composition, porosity and conductivity, and wherein the at least 10 layers (2, 3) are arranged such that the layer composition, porosity and/or conductivity horizontally to the support layer (1) forms a gradient over the total layer area.
摘要翻译：本发明提供了一种分级多层结构，其包括支撑层（1）和形成梯度层的至少10层（2,3），其中所述至少10层（2,3）中的每一层至少部分地接触与所述支撑层（1）形成，其中所述至少10层（2,3）在选自层组成，孔隙率和导电性中的至少一种性质中彼此不同，并且其中所述至少10层（2,3）布置成使得水平到支撑层（1）的层组成，孔隙率和/或导电性在总层面积上形成梯度。

10. 发明授权

US09496576B2 Thin solid oxide cell 有权
标题翻译：薄固体氧化物电池
公开(公告)号：US09496576B2
公开(公告)日：2016-11-15
申请号：US12515816
申请日：2007-11-23
申请人： Peter Halvor Larsen , Soeren Linderoth , Peter Vang Hendriksen
发明人： Peter Halvor Larsen , Soeren Linderoth , Peter Vang Hendriksen
IPC分类号： H01M8/12 , H01M4/90 , B01D67/00 , B01D69/12 , B01D71/02 , H01M4/86 , H01M4/88
CPC分类号： H01M8/1213 , B01D67/0041 , B01D67/0046 , B01D69/12 , B01D71/024 , B01D2323/46 , B01D2325/08 , B01D2325/10 , H01M4/8621 , H01M4/8652 , H01M4/8885 , H01M4/90 , H01M4/9016 , H01M4/9033 , H01M4/9066 , H01M8/122 , H01M2300/0094 , Y02E60/521 , Y02E60/525
摘要： The present invention relates to a thin and in principle unsupported solid oxide cell, comprising at least a porous anode layer, an electrolyte layer and a porous cathode layer, wherein the anode layer and the cathode layer comprise an electrolyte material, at least one metal and a catalyst material, and wherein the overall thickness of the thin reversible cell is about 150 μm or less, and to a method for producing same. The present invention also relates to a thin and in principle unsupported solid oxide cell, comprising at least a porous anode layer, an electrolyte layer and a porous cathode layer, wherein the anode layer and the cathode layer comprise an electrolyte material and a catalyst material, wherein the electrolyte material is doper zirconia, and wherein the overall thickness of the thin reversible cell is about 150 μm or less, and to a method for producing same. The present invention further provides a thin separation membrane, comprising at least a porous anode layer, a membrane layer comprising a mixed conducting material and a porous cathode layer, wherein the anode layer and the cathode layer comprise the mixed conducting material and a catalyst material, and wherein the overall thickness of the thin separation membrane is about 1050 μm or less.
摘要翻译：本发明涉及一种薄而且原则上未支撑的固体氧化物电池，其至少包括多孔阳极层，电解质层和多孔阴极层，其中阳极层和阴极层包括电解质材料，至少一种金属和催化剂材料，并且其中薄可逆电池的总厚度为约150μm以下，以及其制造方法。本发明还涉及一种薄而且原则上未支撑的固体氧化物电池，其至少包括多孔阳极层，电解质层和多孔阴极层，其中阳极层和阴极层包括电解质材料和催化剂材料，其中所述电解质材料是多氧化锆，并且其中所述薄可逆电池的总厚度为约150μm以下，以及其制造方法。本发明还提供一种薄分离膜，其至少包括多孔阳极层，包含混合导电材料的膜层和多孔阴极层，其中阳极层和阴极层包含混合导电材料和催化剂材料，并且其中所述薄分离膜的总厚度为约1050μm或更小。

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