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1. 发明授权

US6133191A Heteroaromatic diphosphines as chiral ligands 失效
标题翻译：杂芳基二膦作为手性配体
公开(公告)号：US6133191A
公开(公告)日：2000-10-17
申请号：US286582
申请日：1999-04-05
申请人： Patrizia Antognazza , Tiziana Benincori , Elisabetta Brenna , Edoardo Cesarotti , Francesco Sannicolo' , Licia Trimarco
发明人： Patrizia Antognazza , Tiziana Benincori , Elisabetta Brenna , Edoardo Cesarotti , Francesco Sannicolo' , Licia Trimarco
IPC分类号： B01J31/22 , B01J31/24 , C07C67/303 , C07C67/31 , C07F9/572 , C07F9/6506 , C07F9/6539 , C07F9/655 , C07F9/6553 , C07F9/6558 , C07F15/00 , B01J23/40 , C07F9/28
CPC分类号： C07F15/008 , B01J31/1865 , B01J31/2409 , B01J31/2452 , C07C67/303 , C07C67/31 , C07F15/0053 , C07F15/0073 , C07F9/5728 , C07F9/65515 , C07F9/65517 , C07F9/655345 , C07F9/655354 , B01J2231/645 , B01J2531/0266 , B01J2531/52 , B01J2531/82 , B01J2531/821 , B01J2531/822 , B01J31/2295
摘要： Chiral diphosphines constituted by an aromatic pentatomic biheterocyclic system, suitable to act as chiral ligands, complexes between said diphosophines and transition metals, and their utilization as chiral catalysts in stereocontrolled reactions, such as diastereo- and enantioselective reduction reactions. Process for the preparation of said chiral diphosophines and process for the preparation of said complexes and for their utilization as chiral catalysts in stereocontrolled reactions.
摘要翻译：由芳族五原子双杂环系统构成的手性二膦系，其适合作为手性配体，所述二磷酸和过渡金属之间的复合物，以及它们作为立体控制反应中的手性催化剂的用途，例如非对映选择性还原反应。用于制备所述手性二硫辛酸的方法和用于制备所述复合物的方法及其用作立体控制反应中的手性催化剂。

2. 发明授权

US06297387B1 Heteroaromatic diphosphines as chiral ligands 失效
标题翻译：杂芳基二膦作为手性配体
公开(公告)号：US06297387B1
公开(公告)日：2001-10-02
申请号：US09286583
申请日：1999-04-05
申请人： Patrizia Antognazza , Tiziana Benincori , Elisabetta Brenna , Edoardo Cesarotti , Francesco Sannicolo , Licia Trimarco
发明人： Patrizia Antognazza , Tiziana Benincori , Elisabetta Brenna , Edoardo Cesarotti , Francesco Sannicolo , Licia Trimarco
IPC分类号： C07F950
CPC分类号： C07F15/008 , B01J31/1865 , B01J31/2295 , B01J31/2409 , B01J31/2452 , B01J2231/645 , B01J2531/0266 , B01J2531/52 , B01J2531/82 , B01J2531/821 , B01J2531/822 , C07C67/303 , C07C67/31 , C07F9/5728 , C07F9/65515 , C07F9/65517 , C07F9/655345 , C07F9/655354 , C07F15/0053 , C07F15/0073 , C07C69/675 , C07C69/732
摘要： Chiral diphosphines constituted by an aromatic pentatomic biheterocyclic system, suitable to act as chiral ligands, complexes between said diphosophines and transition metals, and their utilization as chiral catalysts in stereocontrolled reactions, such as diastereo- and enantioselective reduction reactions. Process for the preparation of said chiral diphosophines and process for the preparation of said complexes and for their utilization as chiral catalysts in stereocontrolled reaction.
摘要翻译：由芳族五原子双杂环系统构成的手性二膦系，其适合作为手性配体，所述二磷酸和过渡金属之间的复合物，以及它们作为立体控制反应中的手性催化剂的用途，例如非对映选择性还原反应。用于制备所述手性二硫辛酸的方法和制备所述复合物的方法，并用于其作为立体控制反应中的手性催化剂。

3. 发明授权

US6077958A Heteroaromatic diphosphines as chiral ligands 失效
标题翻译：杂芳基二膦作为手性配体
公开(公告)号：US6077958A
公开(公告)日：2000-06-20
申请号：US300531
申请日：1999-04-27
申请人： Patrizia Antognazza , Tiziana Benincori , Elisabetta Brenna , Edoardo Cesarotti , Francesco Sannicolo' , Licia Trimarco
发明人： Patrizia Antognazza , Tiziana Benincori , Elisabetta Brenna , Edoardo Cesarotti , Francesco Sannicolo' , Licia Trimarco
IPC分类号： B01J31/22 , B01J31/24 , C07C67/303 , C07C67/31 , C07F9/572 , C07F9/6506 , C07F9/6539 , C07F9/655 , C07F9/6553 , C07F9/6558 , C07F15/00
CPC分类号： C07F15/008 , B01J31/1865 , B01J31/2409 , B01J31/2452 , C07C67/303 , C07C67/31 , C07F15/0053 , C07F15/0073 , C07F9/5728 , C07F9/65515 , C07F9/65517 , C07F9/655345 , C07F9/655354 , B01J2231/645 , B01J2531/0266 , B01J2531/52 , B01J2531/82 , B01J2531/821 , B01J2531/822 , B01J31/2295
摘要： Chiral diphosphines are constituted by an aromatic pentatomic biheterocyclic system, suitable to act as chiral ligands and complexes between the diphosphines and transition metals. They may be utilized as chiral catalysts in stereocontrolled reactions, such as diastereo- and enantioselective reduction reactions. Process is for the preparation of these chiral diphosphines; and process is for the preparation of these complexes and for their utilization as chiral catalysts in stereocontrolled reactions.
摘要翻译：手性二膦由芳族五原子双杂环系统构成，适合作为二膦和过渡金属之间的手性配体和络合物。它们可以用作立体控制反应中的手性催化剂，例如非对映选择性还原反应。方法是制备这些手性二膦; 并且方法是用于制备这些络合物并用于其作为立体控制反应中的手性催化剂。

4. 发明授权

US06586357B1 Heteroaromatic diphosphines as chiral ligands 失效
标题翻译：杂芳基二膦作为手性配体
公开(公告)号：US06586357B1
公开(公告)日：2003-07-01
申请号：US09938354
申请日：2001-08-24
申请人： Patrizia Antognazza , Tiziana Benincori , Elisabetta Brenna , Edoardo Cesarotti , Francesco Sannicolo′ , Licia Trimarco
发明人： Patrizia Antognazza , Tiziana Benincori , Elisabetta Brenna , Edoardo Cesarotti , Francesco Sannicolo′ , Licia Trimarco
IPC分类号： B01J3124
CPC分类号： C07F15/008 , B01J31/1865 , B01J31/2295 , B01J31/2409 , B01J31/2452 , B01J2231/645 , B01J2531/0266 , B01J2531/52 , B01J2531/82 , B01J2531/821 , B01J2531/822 , C07C67/303 , C07C67/31 , C07F9/5728 , C07F9/65515 , C07F9/65517 , C07F9/655345 , C07F9/655354 , C07F15/0053 , C07F15/0073 , C07C69/675 , C07C69/732
摘要： Chiral diphosphines constituted by an aromatic pentatomic biheterocyclic system, suitable to act as chiral ligands, complexes between said diphosophines and transition metals, and their utilization as chiral catalysts in sterocontrolled reactions, such as diastereo- and enantioselective reduction reactions. Process for the preparation of said chiral diphosophines and process for the preparation of said complexes and for their utilization as chiral catalysts in sterocontrolled reactions.
摘要翻译：由芳族五原子双杂环系统构成的手性二膦系，其适合作为手性配体，所述二磷酸和过渡金属之间的复合物，以及它们作为异步反应中的手性催化剂的用途，例如非对映选择性还原反应。用于制备所述手性二硫辛酸的方法和制备所述复合物的方法及其作为在sterocontrolled反应中的手性催化剂的使用。

5. 发明授权

US5907045A Heteroaromatic diphosphines as chiral ligands 失效
标题翻译：杂芳基二膦作为手性配体
公开(公告)号：US5907045A
公开(公告)日：1999-05-25
申请号：US765479
申请日：1996-12-23
申请人： Patrizia Antognazza , Tiziana Benincori , Elisabetta Brenna , Edoardo Cesarotti , Francesco Sannicolo' , Licia Trimarco
发明人： Patrizia Antognazza , Tiziana Benincori , Elisabetta Brenna , Edoardo Cesarotti , Francesco Sannicolo' , Licia Trimarco
IPC分类号： B01J31/22 , B01J31/24 , C07C67/303 , C07C67/31 , C07F9/572 , C07F9/6506 , C07F9/6539 , C07F9/655 , C07F9/6553 , C07F9/6558 , C07F15/00 , C07D333/00 , C07D275/02
CPC分类号： C07F15/008 , B01J31/1865 , B01J31/2409 , B01J31/2452 , C07C67/303 , C07C67/31 , C07F15/0053 , C07F15/0073 , C07F9/5728 , C07F9/65515 , C07F9/65517 , C07F9/655345 , C07F9/655354 , B01J2231/645 , B01J2531/0266 , B01J2531/52 , B01J2531/82 , B01J2531/821 , B01J2531/822 , B01J31/2295
摘要： Chiral diphosphines constituted by an aromatic pentatomic biheterocyclic system, suitable to act as chiral ligands, complexes between said diphosophines and transition metals, and their utilization as chiral catalysts in sterocontrolled reactions, such as diastereo- and enantioselective reduction reactions. Process for the preparation of said chiral diphosophines and process for the preparation of said complexes and for their utilization as chiral catalysts in sterocontrolled reactions.
摘要翻译： PCT No.PCT / EP95 / 02647 Sec。 371日期：1996年12月23日 102（e）日期1996年12月23日PCT提交1995年7月7日PCT公布。出版物WO96 / 01831 日期1996年1月25日由适合作为手性配体的芳族五原子双杂环系统构成的手性二膦由所述二磷酸酯和过渡金属之间的复合物及其作为异步反应中的手性催化剂的利用，如非对映选择性还原反应。用于制备所述手性二硫辛酸的方法和制备所述复合物的方法及其作为在sterocontrolled反应中的手性催化剂的使用。

6. 发明授权

US08801804B2 Non-metal tanning process 有权
标题翻译：非金属鞣制工艺
公开(公告)号：US08801804B2
公开(公告)日：2014-08-12
申请号：US13879230
申请日：2011-10-05
申请人： Claus Reineking , Roberta Gamarino , Licia Trimarco , Maurizio Quaglierini , Markus Gisler , Rainer Nusser
发明人： Claus Reineking , Roberta Gamarino , Licia Trimarco , Maurizio Quaglierini , Markus Gisler , Rainer Nusser
IPC分类号： C14C3/26 , C07D237/06 , C14C3/00 , C14C3/02 , C14C3/04 , C07D237/00 , C07D247/02 , C07D239/02
CPC分类号： C14C3/00 , C07D237/00 , C07D237/06 , C07D239/02 , C07D247/02 , C14C3/02 , C14C3/04 , C14C3/26
摘要： Tanned leather, skin or pelt is produced by non-metal tanning, comprising the step of tanning a bated hide, skin or belt with a tanning agent (A) of at least a mixture of compounds of formula (I) and formula (II), wherein Hal signifies fluorine or chlorine, R1 signifies hydrogen, C1-8-alkyl or an alkyleneoxy radical of formula (III), —(—C2-3 alkylene-O—)q—H (III); R2 signifies a) phenyl, mono- or di-substituted with SO3M or COOM and optionally substituted also with hydroxyl, C1-4-alkyl C1-4-alkoxy; b) naphthyl, mono- or di- or tri-substituted with SO3M and optionally substituted also with hydroxyl; c) C1-8-alkylene, substituted with (SO3M) or (COOM); d) aradical of formula (IV), —(—C2-3 alkylene-O—)p—Y (IV) or e) a radical of formula (IVa) —(C2-3 alkylene-O)p—C2-3 alkylene-SO2CH2CH2O—Y (IVa), M signifies 1 or 2, p signifies 0 or 1, Y signifies hydrogen or —SO3M, q signifies 1 to 10, M signifies hydrogen, an alkali metal cation or an ammonium cation being aprotonated tertiary amine or a quaternary ammonium cation, R3 signifies hydrogen or chlorine. In a tanning bath having a pH of from 6 to 10 at the beginning of tanning step.
摘要翻译：鞣制的皮革，皮肤或毛皮是通过非金属鞣制生产的，其包括用至少一种式（I）和式（II）的化合物的混合物的鞣剂（A）鞣制皮肤，皮肤或皮带的步骤，其中Hal表示氟或氯，R1表示氢，C1-8 - 烷基或式（III）的亚烷基氧基， - （ - C2-3亚烷基-O-）q-H（III）; R2表示a）苯基，被SO 3 M或COOM单取代或二取代，并任选也被羟基，C 1-4 - 烷基C 1-4 - 烷氧基取代; b）萘基，被SO 3 M单取代或二取代或三取代，并任选被羟基取代; c）被（SO 3 M）或（COOM）取代的C 1-8亚烷基; （IV）， - （ - C2-3亚烷基-O-）p-Y（IV）或e）式（Ⅳa） - （C2-3亚烷基-O）p-C2-3的基团亚烷基-SO 2 CH 2 CH 2 O-Y（IVa），M表示1或2，p表示0或1，Y表示氢或-SO 3 M，q表示1至10，M表示氢，碱金属阳离子或铵阳离子为非质子化叔胺或季铵阳离子，R3表示氢或氯。在鞣制步骤开始时pH为6〜10的鞣制浴。

7. 发明授权

US08795389B2 Non metal tanning 有权
标题翻译：非金属鞣制
公开(公告)号：US08795389B2
公开(公告)日：2014-08-05
申请号：US13879172
申请日：2011-10-05
申请人： Claus Reineking , Roberta Gamarino , Licia Trimarco , Maurizio Quaglierini , Markus Gisler , Rainer Nusser
发明人： Claus Reineking , Roberta Gamarino , Licia Trimarco , Maurizio Quaglierini , Markus Gisler , Rainer Nusser
IPC分类号： C14C3/26 , C14C3/00 , C14C3/02 , C14C3/04 , C14C3/08 , C07D253/00 , C07D253/065 , C07D253/07 , C07D253/075
CPC分类号： C14C3/00 , C07D251/44 , C07D253/00 , C07D253/065 , C07D253/07 , C07D253/075 , C14C3/02 , C14C3/04 , C14C3/08 , C14C3/26 , C14C3/28
摘要： Tanned leather, skin or pelt is produced by non-metal tanning, comprising the step of tanning a bated hide, skin or pelt with a tanning agent (A), the tanning agent (A) being at least one compound of a formula (I), wherein X signifies fluorine or chlorine, and/or (+NR3)0-1, wherein R is a substituted or unsubstituted C1 to C6 alkyl group, a substituted or unsubstituted C6 to C10 aryl or a C5 to C6heteroaryl group, R1 signifies hydrogen, C1-8-alkyl or an alkyleneoxy radical of a formula (Ia), -(—C2-3 alkylene-O—)q—H (Ia), R2 signifies hydrogen or hydroxyl, m, signifies 1, 2 or 3, q is of from 1 to 10, M signifies hydrogen or an alkali metal cation or an ammonium cation, being a protonated tertiary amine or a quaternary ammonium cation, in a tanning bath having a pH of from 6 to 10 at the beginning of tanning step.
摘要翻译：鞣制的皮革，皮肤或毛皮是通过非金属鞣制制成的，包括用鞣剂（A）鞣制皮肤，皮肤或皮肤的步骤，鞣剂（A）是至少一种式（I ），其中X表示氟或氯，和/或（+ NR3）0-1，其中R是取代或未取代的C1至C6烷基，取代或未取代的C6至C10芳基或C5至C6杂芳基，R1表示氢，C1-8烷基或式（Ia）的亚烷基氧基， - （ - C2-3亚烷基-O-）q-H（Ia），R2表示氢或羟基，m表示1,2或3 q为1〜10，M表示在鞣制开始时pH为6〜10的鞣制浴中的氢或碱金属阳离子或铵阳离子，为质子化叔胺或季铵阳离子步。

8. 发明授权

US08790416B2 Non-metal tanning process 有权
标题翻译：非金属鞣制工艺
公开(公告)号：US08790416B2
公开(公告)日：2014-07-29
申请号：US13879207
申请日：2011-10-05
申请人： Claus Reineking , Roberta Gamarino , Licia Trimarco , Maurizio Quaglierini , Markus Gisler , Rainer Nusser
发明人： Claus Reineking , Roberta Gamarino , Licia Trimarco , Maurizio Quaglierini , Markus Gisler , Rainer Nusser
IPC分类号： C14C3/26 , C14C3/00 , C14C3/02 , C14C3/04 , C14C3/08 , C07D251/44 , C07D253/00 , C07D253/07 , C07D253/075
CPC分类号： C14C3/00 , C07D251/44 , C07D253/00 , C07D253/07 , C07D253/075 , C14C3/02 , C14C3/04 , C14C3/08 , C14C3/26 , C14C3/28
摘要： Tanned leather, skin or pelt is produced by non-metal tanning, comprising the step of tanning a bated hide, skin or pelt with a tanning agent (A), the tanning agent (A) being at least one compound of a formula (I), wherein X signifies fluorine or chlorine, and/or (+NR3)0-1, wherein R is a substituted or unsubstituted C1 to C6 alkyl group, a substituted or unsubstituted C6 to C10 aryl or a C5 to C6 heteroaryl group, R1 signifies hydrogen, C1-8-alkyl or an alkyleneoxy radical of a formula (Ia), —(—C2-3 alkylene-O—)q—H (Ia), R2 signifies hydrogen, hydroxyl, C1-4-alkyl or C1-4-alkoxy, m, signifies 1 or 2, n signifies 0 to 2, q is of from 1 to 10, M signifies hydrogen or an alkali metal cation or an ammonium cation, the ammonium cation being a protonated tertiary amine or a quaternary ammonium cation, in a tanning bath, the tanning bath having a pH of from 6 to 10 at the beginning of tanning step, wherein the bated hide or skin or pelt is subjected to tanning with (A) without previous pickling.
摘要翻译：鞣制的皮革，皮肤或毛皮是通过非金属鞣制制成的，包括用鞣剂（A）鞣制皮肤，皮肤或皮肤的步骤，鞣剂（A）是至少一种式（I ），其中X表示氟或氯，和/或（+ NR3）0-1，其中R是取代或未取代的C1至C6烷基，取代或未取代的C6至C10芳基或C5至C6杂芳基，R1 表示氢，C 1-8 - 烷基或式（Ia）的亚烷氧基， - （ - C 2-3亚烷基-O-）q -H（Ia），R 2表示氢，羟基，C 1-4 - 烷基或C 1 -4-烷氧基，m表示1或2，n表示0至2，q表示1至10，M表示氢或碱金属阳离子或铵阳离子，铵阳离子为质子化叔胺或季铵铵阳离子，在鞣制浴中，在鞣制步骤开始时，鞣制浴的pH为6至10，其中所述皮肤或皮肤或毛皮用（A）进行鞣制，不需要预先我们酸洗

9. 发明授权

US08790415B2 Non metal tanning 有权
标题翻译：非金属鞣制
公开(公告)号：US08790415B2
公开(公告)日：2014-07-29
申请号：US13879152
申请日：2011-10-05
申请人： Claus Reineking , Roberta Gamarino , Licia Trimarco , Maurizio Quaglierini , Markus Gisler , Rainer Nusser
发明人： Claus Reineking , Roberta Gamarino , Licia Trimarco , Maurizio Quaglierini , Markus Gisler , Rainer Nusser
IPC分类号： C14C3/26
CPC分类号： C14C3/26 , C07D251/44 , C14C3/28
摘要： Tanned leather, skin or pelt is produced by non-metal tanning, comprising the step of tanning a bated hide, skin or pelt with a tanning agent (A), the tanning agent (A) being at least one compound of a formula (I), wherein X signifies fluorine or chlorine, and/or (+NR3)0-1, wherein R is a substituted or unsubstituted C1 to C6 alkyl group, a substituted or unsubstituted C6 to C10 aryl group or a C5 to C6 heteroaryl group, R1 signifies hydrogen, C1-8-alkyl or an alkyleneoxy radical of a formula (Ia), —(—C2-3 alkylene-O—)q—H (Ia), R2 signifies substituted or unsubstituted C2 to C8 alkylenesulphonic acid, substituted or unsubstituted C2 to C8 alkylenecarboxylic acid or an alkyleneoxy radical of formula (Ib), —(—C2-3 alkylene-O—)m—Y (Ib) or an alkylene sulfonyl alkyleneoxy radical of formula (Ic), —(—C2-3 alkylene-O—)p—C2-3 alkylene- SO2CH2O—Y (Ic), m signifies 1 or 2, p signifies 0 or 1, q is of from 1 to 10, Y signifies hydrogen or —SO3M, M signifies hydrogen or an alkali metal cation or an ammonium cation, the ammonium cation being a protonated tertiary amine or a quaternary ammonium cation, in a tanning bath, the tanning bath having a pH of from 6 to 10 at the beginning of tanning step.
摘要翻译：鞣制的皮革，皮肤或毛皮是通过非金属鞣制制成的，包括用鞣剂（A）鞣制皮肤，皮肤或皮肤的步骤，鞣剂（A）是至少一种式（I ），其中X表示氟或氯，和/或（+ NR3）0-1，其中R是取代或未取代的C1至C6烷基，取代或未取代的C6至C10芳基或C5至C6杂芳基， R1表示氢，C1-8 - 烷基或式（Ia）的亚烷基氧基， - （ - C2-3亚烷基-O-）q-H（Ia），R2表示取代或未取代的C2至C8亚烷基磺酸，取代或（C 1 -C 6）的 - （ - C 2-3亚烷基-O-）m-Y（Ib）或亚烷基磺酰基亚烷基氧基， - （ - C2 -3亚烷基-O-）对-C2-3亚烷基-SO2CH2O-Y（Ic），m表示1或2，p表示0或1，q表示1至10，Y表示氢或-SO3M，M表示氢气碱金属阳离子或铵阳离子，铵阳离子是质子化叔胺或季铵阳离子，在鞣制浴中，鞣制浴在鞣制步骤开始时的pH为6至10。

10. 发明申请

US20130227799A1 Non Metal Tanning 有权
标题翻译：非金属鞣制
公开(公告)号：US20130227799A1
公开(公告)日：2013-09-05
申请号：US13884799
申请日：2011-10-25
申请人： Claus Reineking , Roberta Gamarino , Licia Trimarco , Maurizio Quaglierini , Markus Gisler , Rainer Nusser
发明人： Claus Reineking , Roberta Gamarino , Licia Trimarco , Maurizio Quaglierini , Markus Gisler , Rainer Nusser
IPC分类号： C14C3/26
CPC分类号： C14C3/26
摘要： Tanned leather, skin or pelt is produced by non-metal tanning, comprising the step of tanning a bated hide, skin or pelt with a tanning agent (A), the tanning agent (A) being at least one compound of formula (I), R—NH—Y—SO2—Z (I), wherein R signifies a radical of formula wherein Hal signifies fluorine or chlorine, X signifies N or CR1, Y signifies an aliphatic, araliphatic or aromatic hydrocarbonic bridge which may optionally be interrupted by a heteroatom or heteroatomic group, Z signifies vinyl, β-chloroethyl, β-phosphatoethyl or β-sulphatoethyl R1 signifies hydrogen or Cl, in a tanning bath, the tanning bath having a pH of from 6 to 10 at the beginning of tanning step.
摘要翻译：鞣制的皮革，皮肤或毛皮是通过非金属鞣制制成的，包括用鞣剂（A），鞣制剂（A）为至少一种式（I）化合物鞣制皮肤，皮肤或皮肤的步骤，其中R表示下式的基团，其中Hal表示氟或氯，X表示N或CR1，Y表示脂肪族，芳脂族或芳族烃桥，其可任选地被杂原子或杂原子基团Z表示乙烯基，β-氯乙基，β-磷酸乙酯或β-硫酸乙基R1表示氢或Cl，在鞣制浴中，鞣制浴在鞣制步骤开始时pH为6至10。

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