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1. 发明申请

US20050221135A1 Sulfonic acid group-containing, proton-conducting polymer composition, a solid electrolyte membrane and a solid polymer fuel cell 有权
标题翻译：含磺酸基的质子导电聚合物组合物，固体电解质膜和固体聚合物燃料电池
公开(公告)号：US20050221135A1
公开(公告)日：2005-10-06
申请号：US11081077
申请日：2005-03-16
申请人： Nawalage Cooray , Fumio Takei , Norio Sawatari , Masao Tomoi
发明人： Nawalage Cooray , Fumio Takei , Norio Sawatari , Masao Tomoi
IPC分类号： C08G65/38 , B01D67/00 , B01D71/62 , B01D71/82 , C07D251/24 , C08G73/06 , C08J5/22 , H01B1/06 , H01B13/00 , H01M8/02 , H01M8/04 , H01M8/10 , H01M8/18
CPC分类号： C08J5/2256 , B01D67/009 , B01D67/0093 , B01D71/62 , B01D71/82 , B01D2323/30 , C07D251/24 , C08G73/0644 , C08J2379/06 , H01M8/04186 , H01M8/1011 , H01M8/1027 , H01M8/103 , H01M8/1032 , H01M8/1039 , H01M2250/20 , H01M2300/0082 , Y02E60/523 , Y02P70/56 , Y02T90/32
摘要： A solid electrolyte membrane for solid polymer fuel cells, or the like is provided that is chemically stable in a strong acid atmosphere, and has low methanol cross-over as well as high proton conductivity. The solid electrolyte membrane is manufactured, using an electrolyte composition comprising a sulfonic acid group-containing polymer having a specific triazine structure. This polymer can be synthesized, for example, from a sulfonic acid group-containing dihydroxy compound having a triazine structure, and a difluoride.
摘要翻译：提供了在强酸性气氛中化学稳定的固体高分子型燃料电池用固体电解质膜等，具有低的甲醇交叉以及高的质子传导性。使用包含具有特定三嗪结构的含磺酸基的聚合物的电解质组合物制造固体电解质膜。该聚合物可以由例如具有三嗪结构的含磺酸基的二羟基化合物和二氟化物合成。

2. 发明申请

US20060216565A1 Electrolyte composition, solid electrolyte membrane, solid polymer fuel cell and manufacturing method for solid electrolyte membrane 有权
标题翻译：电解质组合物，固体电解质膜，固体聚合物燃料电池及固体电解质膜的制造方法
公开(公告)号：US20060216565A1
公开(公告)日：2006-09-28
申请号：US11363942
申请日：2006-03-01
申请人： Nawalage Cooray , Fumio Takei , Masao Tomoi
发明人： Nawalage Cooray , Fumio Takei , Masao Tomoi
IPC分类号： H01M8/10 , C08J5/22
CPC分类号： C08J5/2256 , C08J2371/12 , H01M8/1011 , H01M8/1027 , H01M8/103 , H01M8/1039 , Y02E60/523 , Y02P70/56
摘要： A method for manufacturing a solid electrolyte membrane made from an electrolyte composition that shows low methanol cross-over and exhibits high proton conductivity. The method includes applying an electrolyte composition including an organic solvent and a perfluorocyclobutane-containing polymer having a specific structure onto a substrate, and then removing the solvent. High proton conductivity is provided by sulfonic acid groups connected to the benzene rings. Reduction of methanol crossover is realized by introduction of a rigid structure with aromatic rings, or a combination of a rigid structure with aromatic rings and a three-dimensional cross-linked structure.
摘要翻译：一种由电解质组合物制成的固体电解质膜的制造方法，该电解质组合物显示低甲醇交叉并且具有高质子传导性。该方法包括将包含有机溶剂的电解质组合物和具有特定结构的含全氟环丁烷的聚合物涂覆在基材上，然后除去溶剂。由苯连接的磺酸基提供高质子传导性。通过引入具有芳环的刚性结构或者具有芳环的刚性结构和三维交联结构的组合来实现甲醇交换的还原。

3. 发明授权

US07597980B2 Sulfonic acid group-containing, proton-conducting polymer composition, a solid electrolyte membrane and a solid polymer fuel cell 有权
标题翻译：含磺酸基的质子导电聚合物组合物，固体电解质膜和固体聚合物燃料电池
公开(公告)号：US07597980B2
公开(公告)日：2009-10-06
申请号：US11081077
申请日：2005-03-16
申请人： Nawalage Florence Cooray , Fumio Takei , Norio Sawatari , Masao Tomoi
发明人： Nawalage Florence Cooray , Fumio Takei , Norio Sawatari , Masao Tomoi
IPC分类号： H01M8/10 , H01M8/18 , C08G73/06
CPC分类号： C08J5/2256 , B01D67/009 , B01D67/0093 , B01D71/62 , B01D71/82 , B01D2323/30 , C07D251/24 , C08G73/0644 , C08J2379/06 , H01M8/04186 , H01M8/1011 , H01M8/1027 , H01M8/103 , H01M8/1032 , H01M8/1039 , H01M2250/20 , H01M2300/0082 , Y02E60/523 , Y02P70/56 , Y02T90/32
摘要： A solid electrolyte membrane for solid polymer fuel cells, or the like is provided that is chemically stable in a strong acid atmosphere, and has low methanol cross-over as well as high proton conductivity. The solid electrolyte membrane is manufactured, using an electrolyte composition comprising a sulfonic acid group-containing polymer having a specific triazine structure. This polymer can be synthesized, for example, from a sulfonic acid group-containing dihydroxy compound having a triazine structure, and a difluoride.
摘要翻译：提供了在强酸性气氛中化学稳定的固体高分子型燃料电池用固体电解质膜等，具有低的甲醇交叉以及高的质子传导性。使用包含具有特定三嗪结构的含磺酸基的聚合物的电解质组合物制造固体电解质膜。该聚合物可以由例如具有三嗪结构的含磺酸基的二羟基化合物和二氟化物合成。

4. 发明授权

US08906526B2 Electrolyte composition, solid electrolyte membrane, solid polymer fuel cell and manufacturing method for solid electrolyte membrane 有权
标题翻译：电解质组合物，固体电解质膜，固体聚合物燃料电池及固体电解质膜的制造方法
公开(公告)号：US08906526B2
公开(公告)日：2014-12-09
申请号：US12944270
申请日：2010-11-11
申请人： Nawalage Florence Cooray , Fumio Takei , Masao Tomoi
发明人： Nawalage Florence Cooray , Fumio Takei , Masao Tomoi
IPC分类号： H01M8/10
CPC分类号： C08J5/2256 , C08J2371/12 , H01M8/1011 , H01M8/1027 , H01M8/103 , H01M8/1039 , Y02E60/523 , Y02P70/56
摘要： An electrolyte composition that shows low methanol cross-over and exhibits high proton conductivity when used as a solid electrolyte for solid polymer fuel cells or the like, and a solid electrolyte membrane and a solid polymer fuel cell that use the electrolyte composition are provided. This electrolyte composition comprises a perfluorocyclobutane-containing polymer having a specific structure. High proton conductivity is provided by sulfonic acid groups connected to the benzene rings. Reduction of methanol crossover is realized by introduction of a rigid structure with aromatic rings, or a combination o a rigid structure with aromatic rings and a three-dimensional cross-linked structure.
摘要翻译：提供了当用作固体聚合物燃料电池等的固体电解质时显示低甲醇交叉并且表现出高质子传导性的电解质组合物，以及使用电解质组合物的固体电解质膜和固体聚合物燃料电池。该电解质组合物包含具有特定结构的含全氟环丁烷的聚合物。由苯连接的磺酸基提供高质子传导性。通过引入具有芳环的刚性结构或者具有芳环的刚性结构和三维交联结构来实现甲醇交换的还原。

5. 发明授权

US07037614B1 Electrolyte composition, solid electrolyte membrane, solid polymer fuel cell and manufacturing method for solid electrolyte membrane 失效
标题翻译：电解质组合物，固体电解质膜，固体聚合物燃料电池及固体电解质膜的制造方法
公开(公告)号：US07037614B1
公开(公告)日：2006-05-02
申请号：US11169143
申请日：2005-06-29
申请人： Nawalage Florence Cooray , Fumio Takei , Masao Tomoi
发明人： Nawalage Florence Cooray , Fumio Takei , Masao Tomoi
IPC分类号： H01M8/10
CPC分类号： C08J5/2256 , C08J2371/12 , H01M8/1011 , H01M8/1027 , H01M8/103 , H01M8/1039 , Y02E60/523 , Y02P70/56
摘要： An electrolyte composition that shows low methanol cross-over and exhibits high proton conductivity when used as a solid electrolyte for solid polymer fuel cells or the like, and a solid electrolyte membrane and a solid polymer fuel cell that use the electrolyte composition are provided. This electrolyte composition comprises a perfluorocyclobutane-containing polymer having a specific structure. High proton conductivity is provided by sulfonic acid groups connected to the benzene rings. Reduction of methanol crossover is realized by introduction of a rigid structure with aromatic rings, or a combination o a rigid structure with aromatic rings and a three-dimensional cross-linked structure.
摘要翻译：提供了当用作固体聚合物燃料电池等的固体电解质时显示低甲醇交叉并且表现出高质子传导性的电解质组合物，以及使用电解质组合物的固体电解质膜和固体聚合物燃料电池。该电解质组合物包含具有特定结构的含全氟环丁烷的聚合物。由苯连接的磺酸基提供高质子传导性。通过引入具有芳环的刚性结构或者具有芳环的刚性结构和三维交联结构来实现甲醇交换的还原。

6. 发明授权

US07858215B2 Electrolyte composition, solid electrolyte membrane, solid polymer fuel cell and manufacturing method for solid electrolyte membrane 有权
标题翻译：电解质组合物，固体电解质膜，固体聚合物燃料电池及固体电解质膜的制造方法
公开(公告)号：US07858215B2
公开(公告)日：2010-12-28
申请号：US11363942
申请日：2006-03-01
申请人： Nawalage Florence Cooray , Fumio Takei , Masao Tomoi
发明人： Nawalage Florence Cooray , Fumio Takei , Masao Tomoi
IPC分类号： H01M8/10
CPC分类号： C08J5/2256 , C08J2371/12 , H01M8/1011 , H01M8/1027 , H01M8/103 , H01M8/1039 , Y02E60/523 , Y02P70/56
摘要： A method for manufacturing a solid electrolyte membrane made from an electrolyte composition that shows low methanol cross-over and exhibits high proton conductivity. The method includes applying an electrolyte composition including an organic solvent and a perfluorocyclobutane-containing polymer having a specific structure onto a substrate, and then removing the solvent. High proton conductivity is provided by sulfonic acid groups connected to the benzene rings. Reduction of methanol crossover is realized by introduction of a rigid structure with aromatic rings, or a combination of a rigid structure with aromatic rings and a three-dimensional cross-linked structure.
摘要翻译：一种由电解质组合物制成的固体电解质膜的制造方法，该电解质组合物显示低甲醇交叉并且具有高质子传导性。该方法包括将包含有机溶剂的电解质组合物和具有特定结构的含全氟环丁烷的聚合物涂覆在基材上，然后除去溶剂。由苯连接的磺酸基提供高质子传导性。通过引入具有芳环的刚性结构或者具有芳环的刚性结构和三维交联结构的组合来实现甲醇交换的还原。

7. 发明授权

US5350523A Anion exchange method 失效
标题翻译：阴离子交换法
公开(公告)号：US5350523A
公开(公告)日：1994-09-27
申请号：US936337
申请日：1992-08-28
申请人： Masao Tomoi , Atsuo Kiyokawa , Hiromasa Ogawa , Teruo Onozuka , Tsuyoshi Ito
发明人： Masao Tomoi , Atsuo Kiyokawa , Hiromasa Ogawa , Teruo Onozuka , Tsuyoshi Ito
IPC分类号： B01J41/04 , B01J41/14 , C02F1/42 , B01J41/12
CPC分类号： B01J41/043 , B01J41/14
摘要： An anion exchange method conducted at a high temperature, which comprises using a crosslinked anion exchanger which comprises structural units having a quaternary ammonium group of the following formula (a) and structural units derived from an unsaturated hydrocarbon group-containing crosslinkable monomer, and of which at least 90% of anion exchange groups are present in the form of a group represented by ##STR1## as defined in the following formula (a): ##STR2## wherein R is a --(CH.sub.2).sub.n --group (n=an integer of from 3 to 18) which may include a cyclic hydrocarbon, each of R.sub.1, R.sub.2 and R.sub.3 which are independent from one another, is a C.sub.1 -C.sub.8 hydrocarbon group or a C.sub.1 -C.sub.8 alkanol group, the benzene ring of the formula (a) may be substituted by an alkyl group or a halogen atom, or may be condensed with other aromatic ring, and X is an anion.
摘要翻译：在高温下进行的阴离子交换法，其包括使用交联阴离子交换剂，其包含具有下式（a）的季铵基的结构单元和源自不饱和烃基的可交联单体的结构单元，其中至少90％的阴离子交换基团以如下式（a）所定义的由下式（a）表示的基团的形式存在：其中R是 - （CH 2）n - 基（n = 3〜18的整数），其可以包括彼此独立的R 1，R 2和R 3中的每一个为环烃，为C 1 -C 8烃基或C 1 -C 8链烷醇基，苯环为式（a）可以被烷基或卤原子取代，或者可以与其它芳香环稠合，X是阴离子。

8. 发明申请

US20090220839A1 Proton conductor 审中-公开
标题翻译：质子导体
公开(公告)号：US20090220839A1
公开(公告)日：2009-09-03
申请号：US11661304
申请日：2005-07-04
申请人： Toshiyuki Oyama , Masao Tomoi
发明人： Toshiyuki Oyama , Masao Tomoi
IPC分类号： H01M8/10
CPC分类号： C08F222/40 , C08F212/08 , C08F212/36 , H01B1/122 , H01M8/1023 , H01M8/1072 , H01M2300/0082 , H01M2300/0091 , Y02P70/56
摘要： The present invention provides a proton conductor, which can be used as a electrolyte of fuel cells and the like, and is a compatibilized material made of an ionic liquid and a polymer. The present invention is a proton conductor consisting of a compatibilized material made of a salt of Brönsted base and Brönsted acid, wherein said salt has at least one heteroatom accompanied with protons, and a polymer, wherein said polymer is produced by copolymerizing a vinyl compound, a divinyl compound and a maleimide compound and said maleimide compound is represented by the chemical formula 1 below: wherein R1 is a hydrogen atom, an alkyl group which may contain a substituent, an aryl group or an aralkyl group.
摘要翻译：本发明提供一种质子导体，其可以用作燃料电池等的电解质，并且是由离子液体和聚合物制成的增容材料。本发明是由布朗斯台德碱和布朗斯台德酸盐形成的增容材料构成的质子导体，其中所述盐具有至少一个伴有质子的杂原子和聚合物，其中所述聚合物通过共聚乙烯基化合物，二乙烯基化合物和马来酰亚胺化合物，所述马来酰亚胺化合物由下述化学式1表示：其中R1是氢原子，可以含有取代基的烷基，芳基或芳烷基。

9. 发明授权

US07638255B2 Method for forming image through reaction development 失效
标题翻译：通过反应开发形成图像的方法
公开(公告)号：US07638255B2
公开(公告)日：2009-12-29
申请号：US10491771
申请日：2002-10-04
申请人： Masao Tomoi , Takafumi Fukushima , Hiroshi Itatani
发明人： Masao Tomoi , Takafumi Fukushima , Hiroshi Itatani
IPC分类号： G03F7/00 , G03F7/004
CPC分类号： G03F7/039 , G03F7/0233 , G03F7/0392 , G03F7/322 , Y10S430/114
摘要： The invention relates to a reaction development patterning process wherein a photo resist layer masked by a desired pattern is irradiated using ultraviolet light and this layer is subsequently washed using a solvent solution containing alkali characterized by said photo resist layer comprising a condensation type polymer containing in the main chain carbonyl groups (C═O) bonded to hetero atoms and a photo acid generating agent and said alkali being an amine. This reaction development patterning process is characterized by being able to use as a photo resist target resins containing bonds having low reactivity toward nucleophilic reagents, for example, condensation type polymers containing any one of bonds such as carbonate, ester, urethane and amide.
摘要翻译：本发明涉及一种反应发展图案化工艺，其中用紫外光照射所需图案掩蔽的光致抗蚀剂层，随后使用含有碱的溶剂溶液洗涤该层，其特征在于所述光致抗蚀剂层包含含有与杂原子键合的主链羰基（CO）和光酸产生剂，所述碱是胺。该反应发展图案化方法的特征在于能够使用含有对亲核试剂具有低反应性的键的光致抗蚀剂靶树脂，例如含有碳酸酯，酯，氨基甲酸酯和酰胺之类的任何一种键的缩合型聚合物。

10. 发明授权

US5518627A Method for treating water or an aqueous solution 失效
标题翻译：处理水或水溶液的方法
公开(公告)号：US5518627A
公开(公告)日：1996-05-21
申请号：US396795
申请日：1995-03-01
申请人： Masao Tomoi , Teruo Onozuka , Manabu Shindo , Hideaki Kiniwa , Hirohisa Kubota , Shintaro Sawada
发明人： Masao Tomoi , Teruo Onozuka , Manabu Shindo , Hideaki Kiniwa , Hirohisa Kubota , Shintaro Sawada
IPC分类号： B01J41/04 , C02F1/42
CPC分类号： B01J41/043 , Y10S210/90 , Y10S210/917
摘要： A method for demineralizing water or an aqueous solution, which comprises contacting the water or the aqueous solution to be treated to a strongly basic anion exchanger made of a crosslinked polymer having a constituting unit of the following formula (I): ##STR1## wherein A is a C.sub.1-2 linear alkylene group, B is a C.sub.4-8 linear alkylene group, each of R1, R2 and R3 which may be the same or different, is a C.sub.1-4 alkyl group or a C.sub.2-4 alkanol group, X is a counter ion coordinated on the ammonium group, and the benzene ring D may have an alkyl group or a halogen atom as a substituent.
摘要翻译：一种使水或水溶液软化矿物的方法，其包括将待处理的水或溶液与由具有下式（I）的构成单元的交联聚合物制成的强碱性阴离子交换剂接触：）其中A为C1-2直链亚烷基，B为C4-8直链亚烷基，R 1，R 2和R 3可相同或不同，为C 1-4烷基或C 2-4链烷醇基团，X是在铵基上配位的抗衡离子，苯环D可以具有烷基或卤素原子作为取代基。

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