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1. 发明授权

US4918233A Production of ethylenediamine from monoethanolamine and ammonia 失效
标题翻译：从单乙醇胺和氨生产乙二胺
公开(公告)号：US4918233A
公开(公告)日：1990-04-17
申请号：US883000
申请日：1986-07-08
申请人： Michel Deeba , Michael E. Ford , Thomas A. Johnson
发明人： Michel Deeba , Michael E. Ford , Thomas A. Johnson
IPC分类号： C07C209/16 , C07C211/10
CPC分类号： C07C209/16
摘要： This invention relates to a process for producing ethylene diamine in high selectivity and high conversion by reacting monoethanolamine with ammonia in the presence of a catalyst. The catalyst which permits the production of ethylenediamine in high selectivity and high conversion is a hydrogen mordenite catalyst that has been treated in such a manner as to raise the silicon to aluminum ratio of the mordenite, such treatment, then being referred to as partial dealumination.
摘要翻译：本发明涉及通过在催化剂存在下使单乙醇胺与氨反应而以高选择性和高转化率生产乙二胺的方法。允许以高选择性和高转化率生产乙二胺的催化剂是已经以使升丝剂的硅与铝比例升高的方式处理的氢丝光沸石催化剂，这种处理，然后被称为部分脱铝。

2. 发明授权

US08568675B2 Palladium-supported catalyst composites 有权
标题翻译：钯负载催化剂复合材料
公开(公告)号：US08568675B2
公开(公告)日：2013-10-29
申请号：US12707416
申请日：2010-02-17
申请人： Michel Deeba , Tian Luo , Josephine Ramos
发明人： Michel Deeba , Tian Luo , Josephine Ramos
IPC分类号： B01J23/00 , B01J21/00 , B01J8/02 , B01D50/00 , B01D53/56 , B01D53/94 , C01B21/00 , C01B23/00 , C01B25/00 , C01B31/00 , C01B33/00 , C01B35/00 , C01G28/00 , C01G30/00
CPC分类号： B01J23/63 , B01D53/945 , B01D2251/2062 , B01D2255/1023 , B01D2255/1025 , B01D2255/206 , B01D2255/2092 , B01D2255/9022 , B01D2255/9025 , B01D2258/012 , B01D2258/014 , B01J23/002 , B01J23/10 , B01J37/0244 , B01J37/0248 , B01J2523/00 , F01N3/035 , F01N3/103 , Y02T10/22 , B01J2523/36 , B01J2523/3706 , B01J2523/3712 , B01J2523/3725 , B01J2523/48 , B01J2523/3718
摘要： Provided are catalyst composites that can be used in methods for treating exhaust gas from internal combustion engines, including diesel and gasoline engines, systems including such catalyst composites and methods of using the catalyst composites to treat internal combustion engine exhaust. The catalyst composites may provide diesel oxidation catalysts and three-way catalysts. A catalyst composite is provided which a catalytic material on a carrier, the catalytic material including a palladium component dispersed on a first support comprising at least 60% by weight of a zirconia component, and one or more rare earth oxides selected from the group consisting of lanthana, neodymia, praseodymia, yttria, the first support optionally containing no more than 15% by weight ceria, and being free of alumina. Layered catalyst composites having one or more washcoats on the carrier are also provided.
摘要翻译：提供了可用于处理来自内燃机（包括柴油和汽油发动机）的废气的方法中的催化剂复合材料，包括这种催化剂复合材料的系统以及使用催化剂复合材料来处理内燃机排气的方法。催化剂复合材料可提供柴油氧化催化剂和三元催化剂。提供一种催化剂复合材料，催化剂材料在载体上，催化材料包括分散在包含至少60重量％的氧化锆组分的第一载体上的钯组分和一种或多种选自以下的稀土氧化物：氧化镧，氧化钕，氧化镨，第一载体，任选地含有不超过15重量％的二氧化铈，并且不含氧化铝。还提供了在载体上具有一层或多层面漆的层状催化剂复合材料。

3. 发明申请

US20110268634A1 Process For The Preparation Of Coated Monoliths 有权
标题翻译：涂层整体制备工艺
公开(公告)号：US20110268634A1
公开(公告)日：2011-11-03
申请号：US13077225
申请日：2011-03-31
申请人： Markus Linsenbühler , Bernd Sachweh , Saadallah Nemeh , Michel Deeba , Michael Mertler , Matthias Wilhelm Meier
发明人： Markus Linsenbühler , Bernd Sachweh , Saadallah Nemeh , Michel Deeba , Michael Mertler , Matthias Wilhelm Meier
IPC分类号： B01J37/02 , B01J29/06 , B01J35/02 , B01J21/06 , B01D53/86 , B01J27/224 , B01J21/04
CPC分类号： B01J37/0215 , B01D53/94 , B01D53/944 , B01D53/9445 , B01D2255/1021 , B01D2255/2092 , B01J35/023 , B01J35/04 , B01J37/0036 , B01J37/0232 , B01J37/0248 , B05D1/02 , B05D7/22 , Y02A50/2324 , Y02T10/22
摘要： The invention relates to a monolithic support member comprising channels with walls separating the channels from each other and having a coating deposited thereon, the non-coated channels having a polygonal cross-section profile, wherein the mean thickness dC of the coating in a corner of said cross-section profile is smaller than or equal to the mean thickness dE of the coating on an edge of said cross-section profile plus 85 micrometer; and further relates to a method for the preparation of such coated monolithic support member, the method comprising (i) providing a suspension having a viscosity in the range of from 0.5 to 100 mPas and having a solid content in the range of from 1 to 40 wt.-%, (ii) dispersing the suspension into a gas stream to obtain a gas stream comprising droplets having a droplet size in the range of from d10 greater than or equal to 1 micrometer to d90 smaller than or equal to 100 micrometer; and (iii) directing said gas stream comprising said droplet towards the monolithic support member along the axial direction of the channels of the support; and still further relates to the use of such coated monolithic support member, in particular as catalytic article in the automotive exhaust gas treatment.
摘要翻译：本发明涉及一种整体式支撑构件，其包括具有将通道彼此分离并且具有沉积在其上的涂层的通道，所述非涂覆通道具有多边形横截面轮廓，其中涂层的平均厚度dC在所述横截面轮廓小于或等于所述横截面轮廓边缘上的涂层的平均厚度dE加上85微米; 并且还涉及一种制备这种涂覆的整体式支撑构件的方法，该方法包括（i）提供粘度范围为0.5-100mPa·s且固体含量在1至40范围内的悬浮液（ii）将悬浮液分散到气流中以获得包含液滴尺寸在d10大于或等于1微米至小于等于100微米的d90的液滴的气流; 和（iii）沿着所述支撑件的通道的轴向将包括所述液滴的所述气流引向所述整体式支撑构件; 并且还涉及这种涂覆的整体式支撑构件的使用，特别是作为汽车废气处理中的催化剂。

4. 发明申请

US20100212293A1 Palladium-Supported Catalyst Composites 有权
标题翻译：钯负载催化剂复合材料
公开(公告)号：US20100212293A1
公开(公告)日：2010-08-26
申请号：US12707416
申请日：2010-02-17
申请人： Michel Deeba , Tian Luo , Josephine Ramos
发明人： Michel Deeba , Tian Luo , Josephine Ramos
IPC分类号： F01N3/20 , B01J23/10 , F01N3/035
CPC分类号： B01J23/63 , B01D53/945 , B01D2251/2062 , B01D2255/1023 , B01D2255/1025 , B01D2255/206 , B01D2255/2092 , B01D2255/9022 , B01D2255/9025 , B01D2258/012 , B01D2258/014 , B01J23/002 , B01J23/10 , B01J37/0244 , B01J37/0248 , B01J2523/00 , F01N3/035 , F01N3/103 , Y02T10/22 , B01J2523/36 , B01J2523/3706 , B01J2523/3712 , B01J2523/3725 , B01J2523/48 , B01J2523/3718
摘要： Provided are catalyst composites that can be used in methods for treating exhaust gas from internal combustion engines, including diesel and gasoline engines, systems including such catalyst composites and methods of using the catalyst composites to treat internal combustion engine exhaust. The catalyst composites may provide diesel oxidation catalysts and three-way catalysts. A catalyst composite is provided which a catalytic material on a carrier, the catalytic material including a palladium component dispersed on a first support comprising at least 60% by weight of a zirconia component, and one or more rare earth oxides selected from the group consisting of lanthana, neodymia, praseodymia, yttria, the first support optionally containing no more than 15% by weight ceria, and being free of alumina. Layered catalyst composites having one or more washcoats on the carrier are also provided.
摘要翻译：提供了可用于处理来自内燃机（包括柴油和汽油发动机）的废气的方法中的催化剂复合材料，包括这种催化剂复合材料的系统以及使用催化剂复合材料来处理内燃机排气的方法。催化剂复合材料可提供柴油氧化催化剂和三元催化剂。提供一种催化剂复合材料，催化剂材料在载体上，催化材料包括分散在包含至少60重量％的氧化锆组分的第一载体上的钯组分和一种或多种选自以下的稀土氧化物：氧化镧，氧化钕，氧化镨，第一载体，任选地含有不超过15重量％的二氧化铈，并且不含氧化铝。还提供了在载体上具有一层或多层面漆的层状催化剂复合材料。

5. 发明申请

US20070269353A1 Emission Treatment System with NSR and SCR Catalysts 有权
标题翻译：具有NSR和SCR催化剂的排放处理系统
公开(公告)号：US20070269353A1
公开(公告)日：2007-11-22
申请号：US11748759
申请日：2007-05-15
申请人： Yuejin Li , Michel Deeba , Joseph Dettling , Joseph Patchett , Stanley Roth
发明人： Yuejin Li , Michel Deeba , Joseph Dettling , Joseph Patchett , Stanley Roth
IPC分类号： B01D53/88 , F01N3/08
CPC分类号： F01N3/035 , B01D53/9418 , B01D53/9422 , B01D53/9459 , B01D2255/202 , B01D2255/204 , B01D2255/2063 , B01D2255/2068 , B01D2255/20738 , B01D2255/20761 , B01D2255/50 , B01D2255/9022 , B01D2255/908 , B01D2255/91 , B01D2255/9155 , B01D2258/012 , F01N3/0814 , F01N3/0842 , F01N3/2073 , F01N13/009 , F01N13/0093 , F01N2570/04 , F01N2570/16 , F01N2610/02 , F01N2610/03 , Y02T10/24
摘要： Provided is an emissions treatment system for an exhaust stream, having a NOx storage reduction (NSR) catalyst with a NOx sorbent at a concentration of at least 0.1 g/in3 and a platinum group metal component dispersed on a refractory metal oxide support; and, an SCR catalyst disposed downstream of the NSR catalyst. The emissions treatment system is advantageously used for the treatment of exhaust streams from diesel engines and lean burn gasoline engines.
摘要翻译：提供了一种排气流的排放处理系统，其具有NOx吸附剂浓度为至少0.1g / in 3以上的NOx吸收剂的NOx储存还原（NSR）催化剂和分散在耐火金属氧化物载体; 以及设置在NSR催化剂下游的SCR催化剂。排放物处理系统有利地用于处理来自柴油发动机和贫燃汽油发动机的废气流。

6. 发明授权

US06586254B1 Method and apparatus for accelerated catalyst poisoning and deactivation 失效
标题翻译：加速催化剂中毒和失活的方法和装置
公开(公告)号：US06586254B1
公开(公告)日：2003-07-01
申请号：US09594399
申请日：2000-06-15
申请人： Sanath V. Kumar , Michel Deeba , Patrick L. Burk
发明人： Sanath V. Kumar , Michel Deeba , Patrick L. Burk
IPC分类号： G01N3110
CPC分类号： F01N11/00 , F01N2550/02 , F01N2550/20 , G01N31/10 , Y02T10/47
摘要： An article, apparatus and method for simulating poisoning and deactivating catalysts with catalyst poison compounds at least one catalyst poison compound selected from the group consisting of a compound comprising phosphorous, a compound comprising zinc compound and a compound comprising phosphorous and zinc.
摘要翻译：一种用于模拟使用催化剂毒物化合物中毒和使催化剂失活的物品，装置和方法，所述催化剂毒物化合物选自由磷组成的组中的至少一种催化剂毒物化合物，包含锌化合物的化合物和包含磷和锌的化合物。

7. 发明授权

US4876377A Alkylation of aromatic amines with olefins on partially dealuminated zeolites 失效
标题翻译：芳烃与烯烃在部分脱铝沸石上烷基化
公开(公告)号：US4876377A
公开(公告)日：1989-10-24
申请号：US171602
申请日：1988-03-22
申请人： Rakesh Agrawal , Steven R. Auvil , Michel Deeba
发明人： Rakesh Agrawal , Steven R. Auvil , Michel Deeba
IPC分类号： C07C209/68
CPC分类号： C07C209/68 , B01J2229/16
摘要： This invention pertains to an improved process for the alkylation of aromatic amines. The improvement resides in the use with particular aromatic amines and olefins a catalyst which is a highly acidic partially dealuminated zeolite having an increased silica to alumina molar ratio over the original zeolite and an acidity factor of at least 0.3. The partially dealuminated zeolites are preferably exchanged with hydrogen or rare earth metal and are particularly effective for producing an alkylated aromatic amine where the alkyl group is ortho to the amine. The highly acidic partially dealuminated H-mordenite and partially dealuminated HY faujasite are very effective for the alkylation of aniline with propylene.
摘要翻译：本发明涉及芳族胺的烷基化改进方法。改进在于与特定的芳族胺和烯烃一起使用催化剂，催化剂是与原沸石相比具有增加的二氧化硅与氧化铝摩尔比并且酸度因子至少为0.3的高度酸性部分脱铝的沸石。部分脱铝的沸石优选与氢或稀土金属交换，并且对于制备其中烷基是胺的邻位的烷基化芳族胺特别有效。高度酸性的部分脱铝的H-丝光沸石和部分脱铝的HY八面沸石对于用丙烯烷基化苯胺非常有效。

8. 发明授权

US4398041A Process for manufacturing alkylamines 失效
标题翻译：制备烷基胺的方法
公开(公告)号：US4398041A
公开(公告)日：1983-08-09
申请号：US344246
申请日：1982-01-29
申请人： Robert N. Cochran , Michel Deeba
发明人： Robert N. Cochran , Michel Deeba
IPC分类号： C07C85/06
CPC分类号： C07C209/16
摘要： A process for converting a C.sub.1 -C.sub.4 alcohol to a non-equilibrium controlled distribution of mono-, di- and trialkylamines is disclosed. A mixture of the alcohol and ammonia is reacted in a first conversion reactor containing a shape selective catalyst to yield a first product stream comprising the mono- and disubstituted alkylamines and substantially no trisubstituted alkylamine. A predetermined fraction of the first product stream is removed and the remainder of the stream is reacted in a second conversion reactor containing a catalyst which yields a second product stream comprising an equilibrium controlled distribution of the mono-, di- and trisubstituted alkylamine. The fraction of the first product stream and the second product stream are combined to yield an alkylamines stream comprising a non-equilibrium controlled alkylamines distribution.
摘要翻译：公开了将C1-C4醇转化为单 - ，二 - 和三烷基胺的非平衡受控分布的方法。醇和氨的混合物在含有形状选择性催化剂的第一转化反应器中反应，得到包含单取代烷基胺和二取代烷基胺并基本上不含三取代烷基胺的第一产物流。除去预定部分的第一产物流，并将剩余的物流在包含催化剂的第二转化反应器中反应，该催化剂产生包含单取代，二取代和三取代的烷基胺的平衡受控分布的第二产物流。将第一产物流和第二产物流的级分组合以产生包含非平衡控制的烷基胺分布的烷基胺流。

9. 发明授权

US08211392B2 Diesel oxidation catalyst composite with layer structure for carbon monoxide and hydrocarbon conversion 有权
标题翻译：柴油氧化催化剂复合材料，具有一氧化碳和烃转化的层结构
公开(公告)号：US08211392B2
公开(公告)日：2012-07-03
申请号：US12686817
申请日：2010-01-13
申请人： Gerd Grubert , Torsten Neubauer , Alfred H. Punke , Torsten W. Müller-Stach , Attilio Siani , Stanley A. Roth , Jeffrey B. Hoke , Shiang Sung , Yuejin Li , Xinyi Wei , Michel Deeba
发明人： Gerd Grubert , Torsten Neubauer , Alfred H. Punke , Torsten W. Müller-Stach , Attilio Siani , Stanley A. Roth , Jeffrey B. Hoke , Shiang Sung , Yuejin Li , Xinyi Wei , Michel Deeba
IPC分类号： B01D53/94 , B01J23/44 , B01J35/00 , F01N3/10
CPC分类号： B01J37/0244 , B01D53/944 , B01D2255/1021 , B01D2255/1023 , B01D2255/206 , B01D2255/20715 , B01D2255/502 , B01D2255/9022 , B01D2255/9025 , B01D2255/908 , B01D2255/912 , B01D2257/502 , B01D2257/702 , B01D2258/012 , B01J23/002 , B01J23/63 , B01J29/068 , B01J29/7415 , B01J35/023 , B01J37/0036 , B01J37/0246 , B01J37/0248 , B01J2523/00 , F01N2510/0682 , Y02A50/2341 , B01J2523/3706 , B01J2523/3712 , B01J2523/3718 , B01J2523/48
摘要： Provided is a catalyst composition, in particular a diesel oxidation catalyst, for the treatment of exhaust gas emissions, such as the oxidation of unburned hydrocarbons (HC), and carbon monoxide (CO). More particularly, the present invention is directed to a catalyst structure comprising at least two, specifically three distinct layers, at least one of which contains an oxygen storage component (OSC) that is present in a layer separate from the majority of the platinum group metal (PGM) components, such as palladium and platinum.
摘要翻译：提供了用于处理废气排放的催化剂组合物，特别是柴油氧化催化剂，例如未燃烧的烃（HC）和一氧化碳（CO）的氧化。更具体地说，本发明涉及一种催化剂结构，该催化剂结构包括至少两个，具体为三个不同的层，其中至少一个含有存储在与大多数铂族金属分开的层中的储氧组分（OSC）（PGM）组分，例如钯和铂。

10. 发明授权

US07879755B2 Catalyst compositions 有权
标题翻译：催化剂组合物
公开(公告)号：US07879755B2
公开(公告)日：2011-02-01
申请号：US11836476
申请日：2007-08-09
申请人： Knut Wassermann , Stephan Siemund , Michel Deeba , Harold Rabinowitz
发明人： Knut Wassermann , Stephan Siemund , Michel Deeba , Harold Rabinowitz
IPC分类号： B01J23/00 , B01J23/10 , B01J23/56 , B01J23/42 , B01J23/44 , B01D53/56 , B01D53/94 , B01J8/02 , C01B21/00 , C01B23/00 , C01B25/00 , C01B31/00 , C01B33/00 , C01B35/00 , C01G28/00 , C01G30/00
CPC分类号： B01J23/63 , B01D53/945 , B01D2255/1023 , B01D2255/206 , B01D2255/407 , B01D2255/908 , B01D2257/502 , B01J37/0036 , B01J37/0244 , B01J37/0248 , Y02T10/22
摘要： Provided are catalyst composites comprising: a catalytic material on a carrier, the catalytic material comprising a precious metal selected from a palladium component and an oxygen storage component, the oxygen storage component being present in an amount of at least 10% by weight, wherein substantially all of the oxygen storage component is in intimate contact with the palladium component and the catalytic material is effective to substantially simultaneously oxidize carbon monoxide and hydrocarbons and reduce nitrogen oxides. A catalyst composite comprising: a catalytic material on a carrier, the catalytic material comprising a palladium component and a ceria-zirconia composite support, the ceria being present in an amount in the range of 10 to 70% by weight, wherein substantially all of the ceria is in intimate contact with at least a portion of the palladium component. Methods of making and using these catalysts are also provided.
摘要翻译：提供了催化剂复合材料，其包括：载体上的催化材料，催化材料包含选自钯组分和储氧组分的贵金属，所述储氧组分的存在量为至少10重量％，其中基本上所有储氧组分与钯组分紧密接触，催化材料有效地基本上同时氧化一氧化碳和烃并还原氮氧化物。一种催化剂复合材料，包括：在载体上的催化材料，所述催化材料包含钯组分和二氧化铈 - 氧化锆复合载体，所述二氧化铈的存在量为10至70重量％，其中基本上全部二氧化铈与钯组分的至少一部分紧密接触。还提供了制备和使用这些催化剂的方法。

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