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1. 发明授权

US07604794B2 Zeolite catalyst for skeletal isomerisation of olefins 有权
标题翻译：用于烯烃骨架异构化的沸石催化剂
公开(公告)号：US07604794B2
公开(公告)日：2009-10-20
申请号：US10549169
申请日：2004-03-09
申请人： Marja Tiitta , Elina Harlin , Jaana Makkonen , Narendra Kumar , Dmitry Yu Murzin , Tapio Salmi
发明人： Marja Tiitta , Elina Harlin , Jaana Makkonen , Narendra Kumar , Dmitry Yu Murzin , Tapio Salmi
IPC分类号： C01B39/04 , C01B39/48 , C07C5/27
CPC分类号： C10G45/64 , B01J29/7046 , B01J29/87 , C01B39/48 , C07C5/2708 , C07C2529/70 , C07C11/02 , C07C11/09 , C07C11/10 , C07C11/107
摘要： The present invention relates to an active and selective zeolite catalyst having MTT structure that is useful in skeletal isomerisation of light olefins. The method for the manufacture of the zeolite catalyst having MTT structure comprises the steps of a) preparing of a gel mixture capable of forming crystalline material, and the mixture comprising sources of alkali or alkaline earth metal (M), of an oxide of a trivalent element (X), of an oxide of a tetravalent element (Y), water and a directing agent (R), and the mixture having a composition, in terms of molar ratios, within the given ranges; b) maintaining the mixture under sufficient conditions, including a temperature of from about 100° C. to about 250° C., under dynamic mode of stirring until crystals of the material are formed, recovering the material; and c) removing the directing agent (R) partly or totally with a calcination procedure.
摘要翻译：本发明涉及具有MTT结构的活性和选择性沸石催化剂，其可用于轻质烯烃的骨架异构化。制备具有MTT结构的沸石催化剂的方法包括以下步骤：a）制备能够形成结晶材料的凝胶混合物，以及包含碱金属或碱土金属（M）源的混合物，其为三价氧化物元素（X），四价元素（Y）的氧化物，水和导向剂（R）的组分，所述混合物的摩尔比在组合物的给定范围内; b）在动态搅拌模式下将混合物保持在足够的条件下，包括约100℃至约250℃的温度，直到形成材料晶体，回收材料; 和c）用煅烧程序部分或全部地去除引导剂（R）。

2. 发明申请

US20060275207A1 Zeolite catalyst for skeletal isomerisation of olefins 有权
标题翻译：用于烯烃骨架异构化的沸石催化剂
公开(公告)号：US20060275207A1
公开(公告)日：2006-12-07
申请号：US10549169
申请日：2004-03-09
申请人： Marja Tiitta , Elina Harlin , Jaana Makkonen , Narendra Kumar , Dintry Yu Murzin , Tapio Salmi
发明人： Marja Tiitta , Elina Harlin , Jaana Makkonen , Narendra Kumar , Dintry Yu Murzin , Tapio Salmi
IPC分类号： C01B39/00 , B01J29/06
CPC分类号： C10G45/64 , B01J29/7046 , B01J29/87 , C01B39/48 , C07C5/2708 , C07C2529/70 , C07C11/02 , C07C11/09 , C07C11/10 , C07C11/107
摘要： The present invention relates to an active and selective zeolite catalyst having MTT structure that is useful in skeletal isomerisation of light olefins. It also relates to a method for the manufacture of said catalyst. The method for the manufacture of the zeolite catalyst having MTT structure comprises the steps of a) Preparing of a gel mixture capable of forming crystalline material, and said mixture comprising sources of alkali or alkaline earth metal (M,) of an oxide of a trivalent element (X), of an oxide of a tetravalent element (Y), water and a directing agent (R), and said mixture having a composition, in terms of molar ratios, within the following ranges; (I) b) Maintaining of said mixture under sufficient conditions, including a temperature of from about 100° C. to about 250° C., under dynamic mode of stirring until crystals of said material are formed, recovering the material, and b) Removing of said directing agent (R) partly or totally with a calcination procedure, whereby a zeolite catalyst having MTT structure is obtained.
摘要翻译：本发明涉及具有MTT结构的活性和选择性沸石催化剂，其可用于轻质烯烃的骨架异构化。它还涉及制备所述催化剂的方法。制备具有MTT结构的沸石催化剂的方法包括以下步骤：a）制备能够形成结晶材料的凝胶混合物，所述混合物包含三价氧化物的碱金属或碱土金属（M i）源，元素（X），四价元素（Y）的氧化物，水和导向剂（R），所述混合物的摩尔比在下列范围内的组成：（I）b）在充分的条件下，包括约100℃至约250℃的温度，在动态搅拌模式下保持所述混合物，直至形成所述材料的晶体，回收该材料，和b）通过煅烧步骤部分或全部除去所述导向剂（R），由此得到具有MTT结构的沸石催化剂。

3. 发明授权

US08329970B2 Deoxygenation of materials of biological origin 有权
标题翻译：生物来源材料脱氧
公开(公告)号：US08329970B2
公开(公告)日：2012-12-11
申请号：US12579224
申请日：2009-10-14
申请人： Elina Harlin , Helka Turunen , Johan-Fredrik Selin , Marja Tiitta , Mohamed Lashdaf
发明人： Elina Harlin , Helka Turunen , Johan-Fredrik Selin , Marja Tiitta , Mohamed Lashdaf
IPC分类号： C07C1/00 , C10L5/00
CPC分类号： C10G3/45 , B01J31/1616 , B01J31/20 , B01J2231/60 , B01J2531/64 , B01J2531/72 , B01J2531/82 , B01J2531/845 , C07C1/2078 , C07C1/213 , C07C2521/08 , C07C2521/18 , C07C2523/46 , C07C2531/20 , C10G3/47 , C10G3/48 , C10G2300/1014 , C10G2300/1018 , C10G2300/1022 , C10G2300/4037 , C10G2300/805 , C10G2400/02 , C10G2400/04 , C10G2400/08 , C10G2400/18 , Y02E50/30 , Y02T50/678 , C07C9/15
摘要： The present invention relates to a method for the deoxygenation of materials of biological origin and particularly to the removal of oxygen from biomass derived organic compounds with carbon monoxide, to yield linear and branched hydrocarbons suitable as biofuels or as blending stocks or components for biofuels, such as gas, gasoline, diesel fuel and aviation fuel, as well as solvents. The method comprises contacting a feedstock with carbon monoxide in the presence of a catalyst comprising a metal selected from a group consisting of ruthenium, manganese, rhodium, rhenium, osmium, iridium, molybdenum, copper, zinc, palladium, platinum and cobalt, in the presence of water, under alkaline conditions at a temperature from 150 to 350° C. and under a pressure from 0.1 to 150 bar, to produce hydrocarbons.
摘要翻译：本发明涉及一种生物来源的材料的脱氧方法，特别是涉及从具有一氧化碳的生物质衍生的有机化合物中除去氧气，以产生适合作为生物燃料的直链和支链烃或作为生物燃料的原料或组分，例如作为天然气，汽油，柴油和航空燃料，以及溶剂。该方法包括在催化剂存在下使原料与一氧化碳接触，所述催化剂包含选自钌，锰，铑，铼，锇，铱，钼，铜，锌，钯，铂和钴的金属，在碱性条件下，在150至350℃的温度和0.1至150巴的压力下，存在水，以产生烃。

4. 发明申请

US20050137435A1 Process for producing gasoline components 有权
标题翻译：生产汽油组分的方法
公开(公告)号：US20050137435A1
公开(公告)日：2005-06-23
申请号：US10740457
申请日：2003-12-22
申请人： Marja Tiitta , Elina Harlin , Antti Pyhalahti
发明人： Marja Tiitta , Elina Harlin , Antti Pyhalahti
IPC分类号： C07C2/06 , C07C2/12 , C07C5/25 , C07C11/16
CPC分类号： C07C5/2518 , C07C2/12 , C07C2529/40 , C07C11/02
摘要： Process for producing gasoline components. The process comprises feeding a fresh olefinic hydrocarbon feedstock to a reaction zone, in which its structure is first isomerized. The isomerized hydrocarbon is drawn out of the first reaction zone and conducted to a second reaction zone, where the isomerized hydrocarbon is dimerized. The dimerized reaction product is drawn out of the second reaction zone and separated from the flow in a separation zone. Because there are more isoolefins present in the dimerization unit feed, more isoolefin dimers useful as fuel components can be produced.
摘要翻译：生产汽油组分的方法。该方法包括将新鲜的烯烃原料进料至反应区，其中其结构首先被异构化。将异构化烃从第一反应区抽出并进入第二反应区，异构化的烃被二聚化。将二聚反应产物从第二反应区抽出并与分离区中的流分离。由于在二聚单元进料中存在更多的异烯烃，因此可以生产可用作燃料组分的更多异烯烃二聚体。

5. 发明授权

US07329788B2 Process for producing gasoline components 有权
标题翻译：生产汽油组分的方法
公开(公告)号：US07329788B2
公开(公告)日：2008-02-12
申请号：US10740457
申请日：2003-12-22
申请人： Marja Tiitta , Elina Harlin , Antti Pyhälahti
发明人： Marja Tiitta , Elina Harlin , Antti Pyhälahti
IPC分类号： C07C2/06 , C07C5/25
CPC分类号： C07C5/2518 , C07C2/12 , C07C2529/40 , C07C11/02
摘要： Process for producing gasoline components. The process comprises feeding a fresh olefinic hydrocarbon feedstock to a reaction zone, in which its structure is first isomerized. The isomerized hydrocarbon is drawn out of the first reaction zone and conducted to a second reaction zone, where the isomerized hydrocarbon is dimerized. The dimerized reaction product is drawn out of the second reaction zone and separated from the flow in a separation zone. Because there are more isoolefins present in the dimerization unit feed, more isoolefin dimers useful as fuel components can be produced.
摘要翻译：生产汽油组分的方法。该方法包括将新鲜的烯烃原料进料至反应区，其中其结构首先被异构化。将异构化烃从第一反应区抽出并进入第二反应区，异构化的烃被二聚化。将二聚反应产物从第二反应区抽出并与分离区中的流分离。由于在二聚单元进料中存在更多的异烯烃，因此可以生产可用作燃料组分的更多异烯烃二聚体。

6. 发明申请

US20070006523A1 Process for the manufacture of diesel range hydro-carbons 有权
标题翻译：制造柴油机油碳氢化合物的方法
公开(公告)号：US20070006523A1
公开(公告)日：2007-01-11
申请号：US11477921
申请日：2006-06-30
申请人： Jukka Myllyoja , Pekka Aalto , Elina Harlin
发明人： Jukka Myllyoja , Pekka Aalto , Elina Harlin
IPC分类号： C10L1/18
CPC分类号： C10L1/08 , C10G3/46 , C10G3/47 , C10G3/50 , C10G45/64 , C10G2300/1014 , C10G2300/1018 , C10G2300/202 , C10G2300/205 , C10G2300/802 , C10G2400/04 , Y02E50/13 , Y02P30/20
摘要： The invention relates to chemical industry and is directed to the production of middle distillate from vegetable oils. In the first step of the production method, the fatty acids or triglycerides of said vegetable oils are hydrogenated to give n-paraffins, and in the second step, the n-paraffins are catalytically converted to paraffins with branched chains. Using this process having two steps, a high-quality middle distillate useful as a component of diesel fuels without any particular specifications may be produced.
摘要翻译：本发明涉及化学工业，涉及从植物油生产中间馏分。在制备方法的第一步中，将所述植物油的脂肪酸或甘油三酯氢化得到正链烷烃，在第二步中，正链烷烃被催化转化成具有支链的链烷烃。使用具有两个步骤的方法，可以生产用作柴油燃料组分的高品质中间馏分，而没有任何特定的规格。

7. 发明申请

US20110015459A1 Process for the preparation of light fuels 有权
标题翻译：轻质燃料的制备工艺
公开(公告)号：US20110015459A1
公开(公告)日：2011-01-20
申请号：US12837627
申请日：2010-07-16
申请人： Pekka Aalto , Ville Alopaeus , Elina Harlin , Raimo Linnaila , Leena Rantanen-Kolehmainen
发明人： Pekka Aalto , Ville Alopaeus , Elina Harlin , Raimo Linnaila , Leena Rantanen-Kolehmainen
IPC分类号： C07C1/207
CPC分类号： C10G47/16 , C10G3/45 , C10G3/46 , C10G3/47 , C10G3/49 , C10G3/50 , C10G45/02 , C10G45/12 , C10G45/58 , C10G45/64 , C10G47/00 , C10G65/043 , C10G65/12 , C10G2300/1011 , C10G2300/4018 , C10G2400/02 , C10G2400/28 , Y02P30/20
摘要： In the process of the invention, an aliphatic C2-C14 hydrocarbon product is prepared from natural fats or derivatives thereof. The process comprises the steps of: (i) providing a natural fat or derivative thereof, (ii) deoxygenating a natural fat or derivative thereof originating from step (i) to yield an aliphatic C9-C28 hydrocarbon, (iii) hydrocracking an aliphatic C9-C28 hydrocarbon originating from step (ii) to yield a product comprising an aliphatic C2-C14 hydrocarbon, (iv) isomerising an aliphatic C2-C14 hydrocarbon originating from step (iii) into an isomerised aliphatic C2-C14 hydrocarbon, and optionally (v) recovering an isomerised C2-C14 hydrocarbon originating from step (iv) as said C2-C14 hydrocarbon product. Pure and high quality light fuel is easily obtained in sufficient amounts.
摘要翻译：在本发明的方法中，由天然脂肪或其衍生物制备脂族C 2 -C 14烃产物。该方法包括以下步骤：（i）提供天然脂肪或其衍生物，（ii）脱氧源自步骤（i）的天然脂肪或其衍生物以产生脂族C 9 -C 28烃，（iii）加氢裂化脂族C 9 来源于步骤（ii）的-C28烃产生包含脂族C 2 -C 14烃的产物，（iv）将由步骤（iii）衍生的脂族C 2 -C 14烃异构化成异构化的脂族C 2 -C 14烃，和任选地（v ）从所述C2-C14烃产物回收源自步骤（iv）的异构化的C 2 -C 14烃。能够容易地获得纯净和高质量的轻质燃料。

8. 发明申请

US20070287871A1 Silicoaluminophosphate isomerization catalyst 审中-公开
标题翻译：硅铝磷酸异构化催化剂
公开(公告)号：US20070287871A1
公开(公告)日：2007-12-13
申请号：US11725103
申请日：2007-03-16
申请人： Eelko Brevoord , Stephan Janbroers , Mark Harte , Pekka Aalto , Elina Harlin , Heidi Osterholm
发明人： Eelko Brevoord , Stephan Janbroers , Mark Harte , Pekka Aalto , Elina Harlin , Heidi Osterholm
IPC分类号： C07C5/31 , B01J27/182 , B01J27/185
CPC分类号： B01J29/85 , B01J29/068 , B01J35/023 , B01J2229/20 , B01J2229/42 , C07C5/2775 , C07C2529/85 , C10G45/64 , C10G2300/1014 , C10G2300/1018 , C10G2300/4018 , Y02P30/20 , C07C9/22 , C07C9/16
摘要： A catalyst system for treating a hydrocarbonaceous feed comprising a matrix selected from the group consisting of alumna, silica alumina, titanium alumina and mixtures thereof; a support medium substantially uniformly distributed through said matrix comprising a SAPO-11 molecular sieve; and 0.1 to 1.0 wt % (based on the total weight of the catalyst system) of a catalytically active metal phase supported on said medium and comprising a metal selected from the group consisting of platinum, palladium, ruthenium, rhodium or mixtures thereof. The catalyst system is characterized in that said SAPO-11 molecular sieve has: a) a silica to alumina molar ratio of 0.08 to 0.24; b) a phosphorous to alumina ratio of 0.75 to 0.83; c) a surface area of at least 150 m2/g; d) a crystallite size in the range 250 to 600 angstroms; and, e) a sodium content of less than 2000 ppm weight.
摘要翻译：一种用于处理含烃原料的催化剂体系，其包含选自校准物，二氧化硅氧化铝，钛氧化铝及其混合物的基质; 基本上均匀分布在包含SAPO-11分子筛的基质中的载体介质; 和0.1至1.0重量％（基于催化剂体系的总重量）负载在所述介质上的催化活性金属相，并且包含选自铂，钯，钌，铑或其混合物的金属。催化剂体系的特征在于所述SAPO-11分子筛具有：a）二氧化硅与氧化铝的摩尔比为0.08至0.24; b）磷与氧化铝的比例为0.75至0.83; c）表面积至少为150m 2 / g; d）微晶尺寸在250至600埃的范围内; 和e）小于2000ppm重量的钠含量。

9. 发明申请

US20100287821A9 Process for the manufacture of diesel range hydro-carbons 有权
标题翻译：制造柴油机油碳氢化合物的方法
公开(公告)号：US20100287821A9
公开(公告)日：2010-11-18
申请号：US11477921
申请日：2006-06-30
申请人： Jukka Myllyoja , Pekka Aalto , Elina Harlin
发明人： Jukka Myllyoja , Pekka Aalto , Elina Harlin
IPC分类号： C10L1/18
CPC分类号： C10L1/08 , C10G3/46 , C10G3/47 , C10G3/50 , C10G45/64 , C10G2300/1014 , C10G2300/1018 , C10G2300/202 , C10G2300/205 , C10G2300/802 , C10G2400/04 , Y02E50/13 , Y02P30/20
摘要： The invention relates to a process for the manufacture of diesel range hydrocarbons wherein a feed comprising fresh feed is hydrotreated in a hydrotreating step and isomerised in an isomerisation step and the fresh feed contains at least 20% by weight triglyceride C12-C16 fatty acids or C12-C16 fatty acid esters or C12-C16 fatty acids or combinations of thereof and feed contains 50-20000 w-ppm sulphur calculated as elemental sulphur.
摘要翻译：本发明涉及一种用于制造柴油范围烃的方法，其中将包含新鲜进料的进料在加氢处理步骤中加氢处理并在异构化步骤中异构化，并且新鲜进料含有至少20重量％的甘油三酯C12-C16脂肪酸或C12 -C16脂肪酸酯或C12-C16脂肪酸或其与饲料的组合含有以元素硫计算的50-20000W-ppm硫。

10. 发明授权

US09005429B2 Process for the manufacture of hydrocarbon components 有权
标题翻译：用于制造烃类成分的方法
公开(公告)号：US09005429B2
公开(公告)日：2015-04-14
申请号：US12495263
申请日：2009-06-30
申请人： Varpu Markkanen , Petri Lindqvist , Elina Harlin , Pekka Aalto , Jukka Myllyoja , Ville Alopaeus
发明人： Varpu Markkanen , Petri Lindqvist , Elina Harlin , Pekka Aalto , Jukka Myllyoja , Ville Alopaeus
IPC分类号： C10G3/00 , C10G65/04 , C10G45/64
CPC分类号： C10G65/043 , C10G3/46 , C10G3/50 , C10G45/64 , C10G2300/1014 , C10G2300/1018 , C10G2300/1055 , C10G2300/4081 , C10G2400/02 , C10G2400/04 , C10G2400/08 , Y02P30/20
摘要： The present invention relates to hydrocarbons and particularly to the manufacture of hydrocarbon components suitable as aviation fuels or jet fuels and as blending stocks for aviation fuels. The process comprises the stages, wherein in the first stage an oil feed of biological origin and hydrogen gas are subjected to conditions sufficient to effect hydrodeoxygenation in the presence of a hydrodeoxygenation catalyst to yield n-paraffins; in the second stage the n-paraffins and hydrogen gas are subjected to conditions sufficient to effect isomerization in the presence of an isomerization catalyst to yield isoparaffins and separating fractions; and recycling the fraction boiling at a temperature above 200° C. under atmospheric pressure obtained from the second stage to reisomerization, where isomerization is effected in the presence of an isomerization catalyst.
摘要翻译：本发明涉及碳氢化合物，特别涉及适用于航空燃料或喷气燃料的烃类组分的制造以及用于航空燃料的混合原料。该方法包括以下阶段，其中在第一阶段中，在加氢脱氧催化剂存在下，生物来源和氢气的进料经受足以进行加氢脱氧的条件以产生正链烷烃; 在第二阶段中，正链烷烃和氢气在异构化催化剂存在下进行足以实现异构化的条件，得到异链烷烃和分离馏分; 并将在第二阶段获得的大气压下在高于200℃的温度下沸腾的馏分再循环进行再异构化，其中异构化在异构化催化剂存在下进行。

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