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1. 发明授权

US09561468B2 Method and system for the purification of exhaust gas from an internal combustion engine 有权
标题翻译：用于净化内燃机废气的方法和系统
公开(公告)号：US09561468B2
公开(公告)日：2017-02-07
申请号：US14391926
申请日：2012-04-27
申请人： Manuel Moliner Marin , Cristina Franch Marti , Antonio Eduardo Palomares Gimeno , Avelino Corma Canós , Peter N. R. Vennestrøm , Marie Grill , Arkady Kustov , Joakim Reimer Thøgersen
发明人： Manuel Moliner Marin , Cristina Franch Marti , Antonio Eduardo Palomares Gimeno , Avelino Corma Canós , Peter N. R. Vennestrøm , Marie Grill , Arkady Kustov , Joakim Reimer Thøgersen
IPC分类号： B01D53/94 , F01N3/10 , F01N3/28 , F01N3/20 , F01N3/035 , B01J37/02 , B01J29/76 , B01J29/85 , B01J35/10
CPC分类号： B01D53/9418 , B01D53/9431 , B01D2251/206 , B01D2255/20761 , B01D2255/50 , B01D2255/915 , B01D2257/404 , B01D2258/012 , B01J23/72 , B01J29/76 , B01J29/85 , B01J35/1019 , B01J35/1038 , B01J37/0246 , B01J2229/20 , F01N3/023 , F01N3/035 , F01N3/2066 , F01N13/001 , F01N13/008 , F01N2330/06 , F01N2370/04 , F01N2610/02 , Y02T10/24
摘要： The invention provides a method and system for the purification of exhaust gas from an internal combustion engine, comprising a filter and a SCR catalyst. The filter is periodically regenerated increasing the temperature of the exhaust gas up to 850° C. and the water vapor content up to 100% by volume. The SCR catalyst comprises a hydrothermally microporous stable zeolite and/or zeotype having the AEI type framework and being promoted with copper.
摘要翻译：本发明提供一种用于净化来自内燃机的废气的方法和系统，该内燃机包括一个过滤器和一个SCR催化剂。周期性地再生过滤器，将排气温度提高到850℃，水汽含量高达100体积％。 SCR催化剂包含水热微孔稳定的沸石和/或具有AEI型骨架并且被铜促进的类型。

2. 发明申请

US20150118134A1 METHOD AND SYSTEM FOR THE PURIFICATION OF EXHAUST GAS FROM AN INTERNAL COMBUSTION ENGINE 有权
标题翻译：从内燃机中净化排气的方法和系统
公开(公告)号：US20150118134A1
公开(公告)日：2015-04-30
申请号：US14391926
申请日：2012-04-27
申请人： Manuel Moliner Marin , Cristina Franch Marti , Antonio Eduardo Palomares Gimeno , Avelino Corma Canós , Peter N.R. Vennestrøm , Marie Grill , Arkady Kustov , Joakim Reimer Thøgersen
发明人： Manuel Moliner Marin , Cristina Franch Marti , Antonio Eduardo Palomares Gimeno , Avelino Corma Canós , Peter N.R. Vennestrøm , Marie Grill , Arkady Kustov , Joakim Reimer Thøgersen
IPC分类号： B01D53/94
CPC分类号： B01D53/9418 , B01D53/9431 , B01D2251/206 , B01D2255/20761 , B01D2255/50 , B01D2255/915 , B01D2257/404 , B01D2258/012 , B01J23/72 , B01J29/76 , B01J29/85 , B01J35/1019 , B01J35/1038 , B01J37/0246 , B01J2229/20 , F01N3/023 , F01N3/035 , F01N3/2066 , F01N13/001 , F01N13/008 , F01N2330/06 , F01N2370/04 , F01N2610/02 , Y02T10/24
摘要： The invention provides a method and system for the purification of exhaust gas from an internal combustion engine, comprising a filter and a SCR catalyst. The filter is periodically regenerated increasing the temperature of the exhaust gas up to 850° C. and the water vapour content up to 100% by volume. The SCR catalyst comprises a hydrothermally microporous stable zeolite and/or zeotype having the AEI type framework and being promoted with copper.
摘要翻译：本发明提供一种用于净化来自内燃机的废气的方法和系统，该内燃机包括一个过滤器和一个SCR催化剂。周期性地再生过滤器，将排气温度提高到850℃，水汽含量高达100体积％。 SCR催化剂包含水热微孔稳定的沸石和/或具有AEI型骨架并且被铜促进的类型。

3. 发明授权

US09561498B2 Process for the direct synthesis of Cu-SAPO-34 有权
标题翻译：直接合成Cu-SAPO-34的方法
公开(公告)号：US09561498B2
公开(公告)日：2017-02-07
申请号：US14395872
申请日：2012-04-27
申请人： Raquel Martinez Franco , Manuel Moliner Marin , Avelino Corma Canós , Arkady Kustov , Joakim Reimer Thøgersen
发明人： Raquel Martinez Franco , Manuel Moliner Marin , Avelino Corma Canós , Arkady Kustov , Joakim Reimer Thøgersen
IPC分类号： C01B39/54 , B01J29/85 , C01B37/08 , B01D53/86 , B01J37/08
CPC分类号： B01J29/85 , B01D53/8628 , B01D2255/50 , B01D2257/404 , B01J37/08 , B01J2229/183 , C01B37/08 , C01B39/54
摘要： A process for the direct synthesis of Cu-SAPO-34 comprising at least the steps: preparation of a mixture of water, at least one silicon source, at least one Al source, at least one P source, at least one Cu source, at least one 0SDA1 (any polyamine), and at least one OSDA2 source (where OSDA2 is any organic molecule capable of directing the synthesis of SAPO 34); and where the final synthesis mixture has the molar composition: a Si:0.5 Al:c Cu:d OSDA1:e OSDA2:f H2O wherein a is in the range from 0.01 to 0.3; b is in the range from 0.2 to 0.49; c is in the range from 0.001 to 0.6; d is in the range from 0.001 to 0.6; e is in the range from 0.001 to 2; f is in the range 1 to 200; hydrothermal treatment of the mixture at 80−200° C. until formation of the crystalline material, and recovery of the crystalline material.
摘要翻译：一种用于直接合成Cu-SAPO-34的方法，至少包括以下步骤：制备水，至少一种硅源，至少一种Al源，至少一种P源，至少一种Cu源，至少一个0SDA1（任何多胺）和至少一个OSDA2源（其中OSDA2是能够指导SAPO 34的合成的任何有机分子）; 并且其中最终合成混合物具有以下摩尔组成：Si：0.5 Al：c Cu：d OSDA1：e OSDA2：fH2O，其中a在0.01至0.3的范围内; b在0.2〜0.49的范围内; c在0.001至0.6的范围内; d在0.001至0.6的范围内; e在0.001至2的范围内; f在1到200的范围内; 在80-200℃下对混合物进行水热处理，直到形成结晶材料，并回收结晶材料。

4. 发明申请

US20150110711A1 PROCESS FOR THE DIRECT SYNTHESIS OF CU-SAPO-34 有权
标题翻译： CU-SAPO-34的直接合成方法
公开(公告)号：US20150110711A1
公开(公告)日：2015-04-23
申请号：US14395872
申请日：2012-04-27
申请人： Raquel Martínez Franco , Manuel Moliner Marin , Avelino Corma Canós , Arkady Kustov , Joakim Reimer Thøgersen
发明人： Raquel Martínez Franco , Manuel Moliner Marin , Avelino Corma Canós , Arkady Kustov , Joakim Reimer Thøgersen
IPC分类号： B01J29/85 , B01D53/86 , B01J37/08 , C01B39/54
CPC分类号： B01J29/85 , B01D53/8628 , B01D2255/50 , B01D2257/404 , B01J37/08 , B01J2229/183 , C01B37/08 , C01B39/54
摘要： Process for the direct synthesis of Cu-SAPO-34 comprising at least the following steps: preparation of a mixture containing water, at least one silicon source, at least one Al source, at least one P source, at least one Cu source, at least one OSDA1 (where OSDA1 is any polyamine), and at least one OSDA2 (where OSDA2 is any organic molecule capable of directing the synthesis of the SAPO-34); and where the final synthesis mixture has the next molar composition: a Si:0.5 Al:b P:c Cu:d OSDA1:e OSDA2:f H20 wherein a is in the range from 0.01 to 0.3; wherein b is in the range from 0.2 to 0.49; wherein c is in the range from 0.001 to 0.6; wherein d is in the range from 0.001 to 0.6; wherein e is in the range from 0.001 to 2; wherein f is in the range from 1 to 200; hydrothermal treatment of the mixture at 80-200° C. until formation of the crystalline material, and recovery of the crystal-line material.
摘要翻译：用于直接合成Cu-SAPO-34的方法包括至少以下步骤：制备含有水，至少一种硅源，至少一种Al源，至少一种P源，至少一种Cu源的混合物，至少一个OSDA1（其中OSDA1是任何多胺）和至少一个OSDA2（其中OSDA2是能够指导SAPO-34的合成的任何有机分子）; 并且其中最终合成混合物具有下一摩尔组成：a Si：0.5 Al:b P：c Cu：d OSDA1：e OSDA2：fH20其中a在0.01至0.3的范围内; 其中b在0.2〜0.49的范围内; 其中c在0.001至0.6的范围内; 其中d在0.001至0.6的范围内; 其中e在0.001至2的范围内; 其中f在1至200的范围内; 在80-200℃下对混合物进行水热处理，直到形成结晶材料，并回收晶体线材料。

5. 发明授权

US07857981B2 Bimetallic catalyst for the treatment of water containing nitrates 失效
标题翻译：用于处理含硝酸盐的水的双金属催化剂
公开(公告)号：US07857981B2
公开(公告)日：2010-12-28
申请号：US12195401
申请日：2008-08-20
申请人： Avelino Corma Canós , Antonio Eduardo Palomares Gimeno , Jose Gregorio Prato Moreno
发明人： Avelino Corma Canós , Antonio Eduardo Palomares Gimeno , Jose Gregorio Prato Moreno
IPC分类号： C02F1/70 , A62D3/37 , B01J23/00 , B01J21/00 , B01J20/00
CPC分类号： C02F1/70 , B01J23/005 , B01J23/007 , B01J23/89 , B01J23/8926 , B01J35/1019 , B01J37/0205 , B01J37/03 , C02F2101/163 , C02F2101/166 , C02F2101/38
摘要： A catalyst which, by means of a reduction reaction at ambient temperature, permits the elimination of nitrates and nitrites in waters. The catalyst comprises a combination of a noble metal and a non-noble metal supported on or incorporated into the structure of a support which, in elemental and anhydrous form, has the formula XYMgAl, in which X is at least one noble metal, Y is at least one non-noble metal, Mg is magnesium and Al is aluminum, the Mg and Al preferably forming the structure of a hydrotalcite or a mixed oxide deriving from a hydrotalcite.
摘要翻译：通过在环境温度下的还原反应允许在水中除去硝酸盐和亚硝酸盐的催化剂。该催化剂包含贵金属和非贵金属的组合，其负载在或并入其中以元素和无水形式具有式XYMgAl的载体结构，其中X为至少一种贵金属，Y为至少一种非贵金属，Mg是镁，Al是铝，Mg和Al优选形成由水滑石衍生的水滑石或混合氧化物的结构。

6. 发明申请

US20120330065A1 PRODUCTION OF MYRTANAL FROM BETA-PINENE EPOXIDE 有权
标题翻译：由环戊二烯环氧化物生产木质素
公开(公告)号：US20120330065A1
公开(公告)日：2012-12-27
申请号：US13517403
申请日：2010-12-17
申请人： Avelino Corma Canós , Michael Renz , Olalla De La Torre Alfaro
发明人： Avelino Corma Canós , Michael Renz , Olalla De La Torre Alfaro
IPC分类号： C07C45/58
CPC分类号： B01J29/7615 , B01J29/7057 , B01J29/7815 , B01J35/002 , C01B39/02 , C07C45/58 , C07C47/347
摘要： The present invention refers to a process for the production of myrtanal from β-pinene epoxide that comprises at least of putting this epoxide in contact with a microporous and crystalline catalyst with pores of a diameter of at least 0.52 nm with an empirical formula for the calcinated and dehydrated form of Hw(MwTixSnyZrzSi1-w-x-y-z)O2 where M is at least a metal with valence+3 selected from Al, B, Ga, Fe, Cr and combinations of these; w is a molar fraction of M with a value of between 0 and 2(x+y+z); x is a molar fraction of titanium and has a value of between 0 and 0.06; y is a molar fraction of tin and has a value of between 0 and 0.06; z is a molar fraction of zirconium and has a value of between 0 and 0.06; and where at least one of the three values “x”, “y” or “z” is different from zero. In the present invention, the microporous and crystalline catalyst preferably has pores of at least 0.52 nm and has a crystalline structure with an X-ray diffractogram of a zeolite beta.
摘要翻译：本发明涉及一种从环氧丙烷生产木药的方法，该方法至少包括使该环氧化物与直径为至少0.52nm的孔的微孔和结晶催化剂接触，其经验公式为煅烧和脱水形式的Hw（MwTixSnyZrzSi1-wxyz）O2，其中M至少为选自Al，B，Ga，Fe，Cr的价数+3的金属及其组合; w是0至2（x + y + z）之间的M的摩尔分数; x是钛的摩尔分数，其值在0和0.06之间; y是锡的摩尔分数，其值在0和0.06之间; z是锆的摩尔分数，其值在0和0.06之间; 并且其中三个值x，y或z中的至少一个不同于零。在本发明中，微孔和结晶催化剂优选具有至少0.52nm的孔，并具有具有β沸石的X射线衍射图的晶体结构。

7. 发明申请

US20110071320A1 Allylic Oxidation Method for the Preparation of Fragrances Using Metal-Organic Compounds and Gold Catalysts 有权
标题翻译：使用金属有机化合物和金催化剂制备香料的烯丙基氧化方法
公开(公告)号：US20110071320A1
公开(公告)日：2011-03-24
申请号：US12888688
申请日：2010-09-23
申请人： Onofre Casanova Navarro , Avelino Corma Canós , Sara Iborra Jornet
发明人： Onofre Casanova Navarro , Avelino Corma Canós , Sara Iborra Jornet
IPC分类号： C07C45/28
CPC分类号： C07C45/34 , B01J23/66 , B01J35/0013 , B01J35/1019 , B01J37/031 , B01J37/035 , C07C29/50 , C07C45/39 , C07C2602/24 , C07C35/32 , C07C49/633
摘要： The present invention refers to a method for allylic catalytic oxidation to obtain α,β-unsaturated ketones and alcohols from bicyclic compounds reacted with oxygen and catalysts comprising metal-organic compounds and gold nanoparticles. The present invention also relates to a method for the preparation of fragrances using the above methods or products of the above method.
摘要翻译：本发明涉及一种烯丙基氧化以从与氧反应的二环化合物和包含金属 - 有机化合物和金纳米颗粒的催化剂中获得α，β-不饱和酮和醇的方法。本发明还涉及使用上述方法或上述方法的产品制备香料的方法。

8. 发明授权

US07611623B2 Separation method using an ITQ-29 zeolite material 失效
标题翻译：使用ITQ-29沸石材料的分离方法
公开(公告)号：US07611623B2
公开(公告)日：2009-11-03
申请号：US11662762
申请日：2005-09-15
申请人： Avelino Corma Canós , Fernando Rey Garcia , Susana Valencia Valencia
发明人： Avelino Corma Canós , Fernando Rey Garcia , Susana Valencia Valencia
IPC分类号： C07C7/13 , B01D53/85 , B01D53/86
CPC分类号： C07C7/12 , B01D53/02 , B01D2253/108 , B01D2257/702 , B01D2257/80 , C01B39/145
摘要： The invention relates to a method of separating the components of a mixture. The inventive method is characterised in that it comprises the following steps: (a) the bringing into contact of the components of a mixture selected from (i) at least two hydrocarbons, (ii) a mixture containing at least nitrogen and oxygen, and (iii) at least one hydrocarbon and water, with an ITQ-29 zeolite material having a T(IV)/T(III) ratio of greater than 7, whereby T(IV) denotes one or more tetravalent elements and T(III) denotes one or more trivalent elements; (b) preferential adsorption of one or more of the components by the ITQ-29 zeolite material and (c) recovery of one or more of the components, preferably for the separation of hydrocarbon mixtures, such as linear or branched olefins from paraffins.
摘要翻译：本发明涉及一种分离混合物组分的方法。本发明的方法的特征在于其包括以下步骤：（a）使选自（i）至少两种烃的混合物的组分与（ii）至少含有氮和氧的混合物和（ iii）至少一种烃和水，其具有T（IV）/ T（III）比大于7的ITQ-29沸石材料，由此T（IV）表示一种或多种四价元素，并且T（III）表示一种或多种三价元素; （b）通过ITQ-29沸石材料优先吸附一种或多种组分，和（c）回收一种或多种组分，优选用于从石蜡中分离烃混合物，例如直链或支链烯烃。

9. 发明授权

US07439411B2 Zeolite catalyst for the alkylation of aromatic compounds with olefins, alcohols or polyalkylated aromatic compounds 失效
标题翻译：用于用烯烃，醇或多烷基化芳族化合物烷基化芳族化合物的沸石催化剂
公开(公告)号：US07439411B2
公开(公告)日：2008-10-21
申请号：US11033047
申请日：2005-01-11
申请人： Avelino Corma Canós , Fernando Rey García , María José Díaz Cabañas
发明人： Avelino Corma Canós , Fernando Rey García , María José Díaz Cabañas
IPC分类号： C07C2/66
CPC分类号： C07C2/66 , C07C6/126 , C07C2521/04 , C07C2521/06 , C07C2521/08 , C07C2521/16 , C07C2523/02 , C07C2529/70 , C07C15/085 , C07C15/28 , C07C15/30 , C07C15/24
摘要： The invention relates to a method of preparing an alkylated aromatic compound. The inventive method is characterized in that it comprises an alkylation reaction of an aromatic compound with an alkylating agent which is selected from an olefin, an alcohol and a polyalkylated aromatic compound, in the presence of a catalyst which is a porous crystalline material with the following chemical composition in the calcined form: X2O3:n YO2:m ZO2, wherein (n+m) is at least 5, X is at least a trivalent element, Z is Ge, Y is at least a tetravalent element different from Ge and the n/m ratio is at least 1. Said method is particularly suitable for obtaining cumene.
摘要翻译：本发明涉及一种制备烷基化芳族化合物的方法。本发明的方法的特征在于它包括芳族化合物与选自烯烃，醇和多烷基化芳族化合物的烷基化剂在催化剂的存在下的烷基化反应，催化剂是多孔结晶材料，其具有以下煅烧形式的化学组成：X 2 O 3：n Y 2 O 2：m ZO 2，其中（ n + m）至少为5，X为至少三价元素，Z为Ge，Y为至少与Ge不同的四价元素，n / m比为1以上。所述方法特别适用于获得枯烯。

10. 发明授权

US07029651B2 Microporous crystalline material (ITQ-19) with laminar characteristics, preparation method and use thereof as a catalyst in the catalytic conversion of organic compounds 失效
标题翻译：具有层状特性的微孔结晶材料（ITQ-19），其制备方法和用途作为催化转化有机化合物中的催化剂
公开(公告)号：US07029651B2
公开(公告)日：2006-04-18
申请号：US10630368
申请日：2003-07-30
申请人： Avelino Corma Canós , Urbano Díaz Morales , Vicente Fornes Segui
发明人： Avelino Corma Canós , Urbano Díaz Morales , Vicente Fornes Segui
IPC分类号： C01B39/48
CPC分类号： C01B33/38 , B01J29/035 , B01J29/70 , C01B37/02 , C01B39/48 , C10G45/64
摘要： The invention relates to a novel microporous crystalline material ITQ-19 used in the catalytic conversion of organic compounds, such as, for example, the dewaxing and isodewaxing of paraffins and the disproportionation of toluene. Said material has a characteristic X-ray diffractogram, a high absorption capacity and the empirical formula x(M1/nXO2):yYO2:(1−y)SiO2 wherein x has a value less than 0.2; y has a value less than 0.1; M is at least an inorganic cation with a +n charge; X is at least a chemical element having oxidation state +3, preferably selected among Al, Ga, B, Cr, Fe; Y is at least a chemical element with oxidation stated +4, preferably selected among Ge, Ti, Sn, V. The inventive material can be obtained by means of a preparation process involving the use of one or more organic additives in a reaction mix which is crystallized by heating.
摘要翻译：本发明涉及用于有机化合物的催化转化的新型微孔结晶材料ITQ-19，例如石蜡的脱蜡和异戊二烯化和甲苯的歧化。所述材料具有特征X射线衍射图，高吸收能力和经验公式x（M 1 / n 2 X 2 2）：y Y 2 O 2 >：（1-y）SiO 2其中x的值小于0.2; y的值小于0.1; M至少为+ n电荷的无机阳离子; X至少是氧化态为+3的化学元素，优选选自Al，Ga，B，Cr，Fe; Y至少是一种化学元素，其氧化值为+4，优选选自Ge，Ti，Sn，V。本发明的材料可以通过涉及在反应混合物中使用一种或多种有机添加剂的制备方法获得，通过加热结晶。

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