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1. 发明授权

US4423185A Thermoplastic resinous composition 失效
标题翻译：热塑性树脂组合物
公开(公告)号：US4423185A
公开(公告)日：1983-12-27
申请号：US126273
申请日：1980-03-03
申请人： Koichi Matsumoto , Yoshihiko Katayama , Hisaya Sakurai
发明人： Koichi Matsumoto , Yoshihiko Katayama , Hisaya Sakurai
IPC分类号： B32B27/06 , C08L23/02 , C08L51/06 , C08L75/04
CPC分类号： C08L51/06 , B32B27/06 , C08L23/025 , C08L75/04 , Y10T428/31551 , Y10T428/31855
摘要： Disclosed is a soft and flexible thermoplastic resinous composition having high impact and tear resistances, a good processability and a good thermal adhesion to a wide variety of plastic and other materials. The resinous composition consists essentially of 5 to 70 wt. % of a thermoplastic polyurethane elastomer and 30 to 95 wt. % of a modified polyolefin or an olefin copolymer, having functional groups of at least one type selected from carboxyl, carboxylate salt, carboxylic anhydride, amide, hydroxyl and epoxy groups. A typical application of the thermoplastic resious composition is a laminate having at least two laminae bonded to each other, at least one of the laminae being comprised of the above-mentioned resinous composition and the other being comprised of at least one material selected from vinyl chloride polymer resins, vinylidene chloride polymer resins, thermoplastic polyester resins, ethylene/vinyl alcohol copolymer resins, polyamide resins, polyacrylonitrile and nitrile copolymer resins, polystyrene and styrene copolymer resins, polymethyl methacrylate and acrylic copolymer resins, polyurethane resins, olefin polymer resins, polyacetal resins, polyvinyl acetal resins, polycarbonate resins, polyphenylene oxide resins, polysulfone resins, epoxy resins, phenol-formaldehyde resins, unsaturated polyester resins, melamine-formaldehyde resins, urea-formaldehyde resins, natural and synthetic rubbers, cellulosic materials, cement, glass and other ceramic materials and metals.
摘要翻译：公开了一种柔软和柔性的热塑性树脂组合物，具有高抗冲击性和抗撕裂性，良好的可加工性和对多种塑料和其它材料的良好的热粘合性。树脂组合物基本上由5-70wt。％的热塑性聚氨酯弹性体和30〜95重量％％的具有至少一种选自羧基，羧酸盐，羧酸酐，酰胺，羟基和环氧基团的官能团的改性聚烯烃或烯烃共聚物。热塑性塑料组合物的典型应用是具有彼此结合的至少两个层的层压体，至少一层由上述树脂组合物组成，另一层由至少一种选自氯乙烯聚合物树脂，偏二氯乙烯聚合物树脂，热塑性聚酯树脂，乙烯/乙烯醇共聚物树脂，聚酰胺树脂，聚丙烯腈和腈共聚物树脂，聚苯乙烯和苯乙烯共聚物树脂，聚甲基丙烯酸甲酯和丙烯酸共聚物树脂，聚氨酯树脂，烯烃聚合物树脂，聚缩醛树脂聚乙烯醇缩醛树脂，聚碳酸酯树脂，聚苯醚树脂，聚砜树脂，环氧树脂，酚醛树脂，不饱和聚酯树脂，三聚氰胺 - 甲醛树脂，脲甲醛树脂，天然和合成橡胶，纤维素材料，水泥，玻璃等陶瓷材料和金属。

2. 发明授权

US4410595A Laminate of thermoplastic resinous composition 失效
标题翻译：热塑性树脂组合物层压板
公开(公告)号：US4410595A
公开(公告)日：1983-10-18
申请号：US413597
申请日：1982-08-31
申请人： Koichi Matsumoto , Yoshihiko Katayama , Hisaya Sakurai
发明人： Koichi Matsumoto , Yoshihiko Katayama , Hisaya Sakurai
IPC分类号： B32B27/00 , C08L51/06 , C08L75/04 , B32B27/36 , B32B27/38 , B32B27/40
CPC分类号： C08L75/04 , C08L51/06 , B32B2272/00 , Y10T428/31507 , Y10T428/31511 , Y10T428/31554 , Y10T428/31562 , Y10T428/31565 , Y10T428/31569 , Y10T428/31573 , Y10T428/31576 , Y10T428/3158 , Y10T428/31583 , Y10T428/31587 , Y10T428/31591 , Y10T428/31594 , Y10T428/31601 , Y10T428/31605 , Y10T428/31609
摘要： Disclosed is a soft and flexible thermoplastic resinous composition having high impact and tear resistances, a good processability and a good thermal adhesion to a wide variety of plastic and other materials. The resinous composition consists essentially of 5 to 70 wt. % of a thermoplastic polyurethane elastomer and 30 to 95 wt. % of a modified polyolefin or an olefin copolymer, having functional groups of at least one type selected from carboxyl, carboxylate salt, carboxylic anhydride, amide, hydroxyl and epoxy groups. A typical application of the thermoplastic resinous composition is a laminate having at least two lamine bonded to each other, at least one of the laminae being comprised of the above-mentioned resinous composition and the other being comprised of at least one material selected from vinyl chloride polymer resins, vinylidene chloride polymer resins, thermoplastic polyester resins, ethylene/vinyl alcohol copolymer resins, polyamide resins, polyacrylonitrile and nitrile copolymer resins, polystyrene and styrene copolymer resins, polymethyl methacrylate and acrylic copolymer resins, polyurethane resins, olefin polymer resins, polyacetal resins, polyvinyl acetal resins, polycarbonate resins, polyphenylene oxide resins, polysulfone resins, epoxy resins, phenol-formaldehyde resins, unsaturated polyester resins, melamine-formaldehyde resins, urea-formaldehyde resins, natural and synthetic rubbers, cellulosic materials, cement, glass and other ceramic materials and metals.
摘要翻译：公开了一种柔软和柔性的热塑性树脂组合物，具有高抗冲击性和抗撕裂性，良好的可加工性和对多种塑料和其它材料的良好的热粘合性。树脂组合物基本上由5-70wt。％的热塑性聚氨酯弹性体和30〜95重量％％的具有至少一种选自羧基，羧酸盐，羧酸酐，酰胺，羟基和环氧基团的官能团的改性聚烯烃或烯烃共聚物。热塑性树脂组合物的典型应用是具有彼此键合的至少两个胺的层压体，至少一个薄层由上述树脂组合物组成，另一个由至少一种选自氯乙烯聚合物树脂，偏二氯乙烯聚合物树脂，热塑性聚酯树脂，乙烯/乙烯醇共聚物树脂，聚酰胺树脂，聚丙烯腈和腈共聚物树脂，聚苯乙烯和苯乙烯共聚物树脂，聚甲基丙烯酸甲酯和丙烯酸共聚物树脂，聚氨酯树脂，烯烃聚合物树脂，聚缩醛树脂聚乙烯醇缩醛树脂，聚碳酸酯树脂，聚苯醚树脂，聚砜树脂，环氧树脂，酚醛树脂，不饱和聚酯树脂，三聚氰胺 - 甲醛树脂，脲甲醛树脂，天然和合成橡胶，纤维素材料，水泥，玻璃等陶瓷材料和金属。

3. 发明授权

US4342708A Hydrocarbon-soluble diorganomagnesium compounds, hydrocarbon solutions containing the same and processes for preparation thereof 失效
标题翻译：烃溶性二有机镁化合物，含有它们的烃溶液及其制备方法
公开(公告)号：US4342708A
公开(公告)日：1982-08-03
申请号：US169233
申请日：1980-07-16
申请人： Hisaya Sakurai , Yoshihiko Katayama , Tadashi Ikegami , Shigeo Tsuyama
发明人： Hisaya Sakurai , Yoshihiko Katayama , Tadashi Ikegami , Shigeo Tsuyama
IPC分类号： C07F3/02 , C08F4/44
CPC分类号： C07F3/02
摘要： Novel hydrocarbon-soluble isopropyl group-containing diorganomagnesium compounds and hydrocarbon solutions thereof are disclosed. The compound of the present invention has a high weight percent of Mg per one mol thereof, and the hydrocarbon solution of the present invention has a very low viscosity as compared with the conventional solutions. The hydrocarbon solution of the present invention can be prepared according any of various processes. If the reaction is carried out in an ether medium, the ether is substituted with a hydrocarbon solvent by removing the ether from the reaction mixture by distillation in the presence of the hydrocarbon solvent.
摘要翻译：公开了新的含烃溶性异丙基二有机镁化合物及其烃溶液。本发明的化合物与其一摩尔具有高的重量百分数的Mg，与常规溶液相比，本发明的烃溶液具有非常低的粘度。本发明的烃溶液可以根据各种方法中的任一种制备。如果反应在醚介质中进行，则通过在烃溶剂的存在下通过蒸馏从反应混合物中除去醚而将醚用烃溶剂取代。

4. 发明授权

US4264472A Catalyst for preparing polyethylene 失效
标题翻译：催化剂用于制备聚乙烯
公开(公告)号：US4264472A
公开(公告)日：1981-04-28
申请号：US70589
申请日：1979-08-29
申请人： Tadashi Ikegami , Hisaya Sakurai , Yoshihiko Katayama , Shigeo Tsuyama , Yukitoshi Iwashita
发明人： Tadashi Ikegami , Hisaya Sakurai , Yoshihiko Katayama , Shigeo Tsuyama , Yukitoshi Iwashita
IPC分类号： C07F7/00 , C08F4/64 , C08F10/00 , C08F36/02
CPC分类号： C08F10/00 , C07F7/006
摘要： A catalyst for preparing an .alpha.-olefin polymer having a broad molecular weight distribution and excellent physical properties, which comprises a solid catalyst component (A) and an organometal compound (B), the solid catalyst component (A) being obtained by reduction with an organomagnesium solution of the thermal decomposition solid product of special titanium compounds.
摘要翻译：一种制备具有宽分子量分布和优异物理性质的α-烯烃聚合物的催化剂，其包含固体催化剂组分（A）和有机金属化合物（B），固体催化剂组分（A）通过用有机镁溶液中的特殊钛化合物的热分解固体产物。

5. 发明授权

US4376720A Olefin polymerization catalyst and olefin polymerization method using such catalyst 失效
标题翻译：烯烃聚合催化剂和使用这种催化剂的烯烃聚合方法
公开(公告)号：US4376720A
公开(公告)日：1983-03-15
申请号：US211991
申请日：1980-12-01
申请人： Hisaya Sakurai , Yoshihiko Katayama , Tadashi Ikegami , Shigeo Tsuyama
发明人： Hisaya Sakurai , Yoshihiko Katayama , Tadashi Ikegami , Shigeo Tsuyama
IPC分类号： C08F4/24 , C08F4/58 , C08F10/00 , C08F4/66 , C08F10/02
CPC分类号： C08F10/00
摘要： An olefin polymerization catalyst which shows an extremely high activity even at low temperatures and is suited for the production of blow molding polymers, said catalyst comprising a solid component constituted by a chromium compound supported by an inorganic oxide carrier, and an organomagnesium complex compound soluble in the inert hydrocarbons and represented by the general formula: M.sub..alpha. Mg.sub..beta. R.sub.p.sup.1 R.sub.q.sup.2 R.sub.r.sup.3 X.sub.s Y.sub.t (wherein .alpha.>0, .beta.>0, p.gtoreq.0, q.gtoreq.0, r.gtoreq.0, s>0, t.gtoreq.0, 0
摘要翻译：一种烯烃聚合催化剂，即使在低温下也显示出极高的活性，适用于生产吹塑聚合物，所述催化剂包括由无机氧化物载体担载的铬化合物构成的固体组分和可溶于惰性烃，由以下通式表示：MαMgβRp1Rq2Rr3XsYt（其中α> 0，β> 0，p> / = 0，q> / = 0，r> / = 0，s> 0，t> = 0,0（s + t）/（α+β）= 1.5和p + q + r + s + t =mα+2β; M是选自铝，锌，硼，铍和锂; m是M的化合价; R 1，R 2和R 3可以相同或不同，分别代表具有1-20个碳原子的烃基; X是OSiR5R6R7; Y是选自由OR4，OSiR5R6R7，NR8R9和SR10组成，其中R5，R6，R7，R8和R9分别表示烃基或氢原子，R4和R10表示引入烃基）。

6. 发明授权

US4330651A Polymerization of .alpha.-olefins 失效
标题翻译： α-烯烃的聚合
公开(公告)号：US4330651A
公开(公告)日：1982-05-18
申请号：US177545
申请日：1980-08-13
申请人： Hisaya Sakurai , Yoshihiko Katayama , Tadashi Ikegami , Masayasu Furusato
发明人： Hisaya Sakurai , Yoshihiko Katayama , Tadashi Ikegami , Masayasu Furusato
IPC分类号： C08F10/00 , C08F4/02
CPC分类号： C08F10/00 , Y10S526/904
摘要： A catalyst for the solution polymerization of .alpha.-olefins is prepared by admixing component (A) with an organometal component (B), component (A) being prepared by reacting a specific hydrocarbon-soluble organomagnesium compound with an aluminum compound and contacting the obtained product with a titanium and/or vanadium compound.
摘要翻译：通过将组分（A）与有机金属组分（B）混合，通过使特定的可溶于烃的有机镁化合物与铝化合物反应制备的组分（A）来制备用于α-烯烃溶液聚合的催化剂，并将获得的产物与钛和/或钒化合物。

7. 发明授权

US4230831A Polyethylene blend composition 失效
标题翻译：聚乙烯共混组合物
公开(公告)号：US4230831A
公开(公告)日：1980-10-28
申请号：US078737
申请日：1979-09-25
申请人： Hisaya Sakurai , Yoshihiko Katayama , Tadashi Ikegami , Kisoo Moriguchi , Shigeru Mizutani
发明人： Hisaya Sakurai , Yoshihiko Katayama , Tadashi Ikegami , Kisoo Moriguchi , Shigeru Mizutani
IPC分类号： C08L23/00 , C08L7/00 , C08L21/00 , C08L23/06 , C08L33/00 , C08L33/02 , C08L101/00
CPC分类号： C08L23/06 , C08L2205/02 , C08L2205/025 , C08L2205/03
摘要： An intimately melted and homogenized polyethylene composition having excellent physical properties and moldability and comprising a high-medium density polyethylene having a high molecular weight (A), a high-medium density polyethylene having a low molecular weight (B) and a low density polyethylene (C) characterized in that:(i) the average molecular weight of (A) is 100,000-1,000,000, the average molecular weight of (B) is 1,000-100,000, the molecular weight ratio of (A) to (B) is 5-200, and (C) has an intrinsic viscosity [.eta.] of 0.70 dl/g or more in decalin at 135.degree. C. and an expansion factor of 3.3 or more, and(ii) the mixing ratio (A)/(B) is 30/70 to 80/20 and the mixing ratio of (C) in the composition is within the range from 1% by weight to less than 15% by weight.
摘要翻译：具有优异的物理性能和成型性的密实熔融均质的聚乙烯组合物，其包含高分子量（A）的高介质密度聚乙烯，具有低分子量（B）和低密度聚乙烯的高中密度聚乙烯其特征在于：（i）（A）的平均分子量为100,000-1,000,000，（B）的平均分子量为1,000-100,000，（A）与（B）的分子量比为5- 200和（C）在135℃的萘烷中的特性粘度η为0.70dl / g以上，膨胀系数为3.3以上，（ii）混合比（A）/（B）为30/70〜80/20，组合物中（C）的混合比在1重量％以下且小于15重量％的范围内。

8. 发明授权

US4219453A Inorganic filler-incorporated ethylene polymer film 失效
标题翻译：无机填料加入乙烯聚合物膜
公开(公告)号：US4219453A
公开(公告)日：1980-08-26
申请号：US942713
申请日：1978-09-15
申请人： Hisaya Sakurai , Kisoo Moriguchi , Yoshihiko Katayama
发明人： Hisaya Sakurai , Kisoo Moriguchi , Yoshihiko Katayama
IPC分类号： C08L23/00 , B29C49/00 , B29C55/00 , B29C55/28 , C08K3/00 , C08K5/09 , C08K5/098 , C08K5/13 , C08K13/02 , C08L101/00 , C08K3/24 , C08K3/26 , C08K3/30
CPC分类号： C08K5/098 , C08K13/02 , C08K3/0033 , C08K3/22 , C08K3/24 , C08K5/09 , C08K5/13
摘要： An ethylene polymer film exhibiting improved impact strength and tear strength is provided. This film is made of an inorganic filler-incorporated ethylene polymer composition which is comprised of:(a) 35-90 wt.%, based on the ethylene polymer composition, of an ethylene polymer having a melt index of 0.005-0.2 and a specific gravity of 0.94- 0.98 as measured at a temperature of 23.degree. C.,(b) 10-65 wt.%, based on the ethylene polymer composition, of a finely divided inorganic filler particle having an average particle size of 0.01-10 microns,(c) 0.1-10 wt.parts, based on 100 wt.parts of the ingredient (b), of a higher fatty acid,(d) 0.5-15 wt.parts, based on 100 wt.parts of the ingredient (b), of a metal salt of a higher fatty acid, and(e) 0.05-5 wt.parts, based on 100 wt.parts of the ingredient (b), of a stabilizer composition predominantly comprised of a phenolic stabilizer.The ethylene polymer film is produced by extruding the ethylene polymer composition at 150.degree.-250.degree. C. through a ring die having lips with a gap of 0.7-3.0 mm, at a blow ratio of 2/1-8/1 and a frost line height of 200-2,000 mm.
摘要翻译：提供了表现出改善的冲击强度和撕裂强度的乙烯聚合物膜。该膜由无机填料掺入的乙烯聚合物组合物制成，该组合物包含：（a）基于乙烯聚合物组合物的35-90重量％的熔体指数为0.005-0.2的乙烯聚合物和具体的在23℃的温度下测得的重量为0.94-0.98，（b）基于乙烯聚合物组合物的10-65重量％的平均粒径为0.01-10微米的细碎无机填料颗粒，（c）基于100重量份成分（b）的0.1-10重量份高级脂肪酸，（d）0.5-15重量份，基于100重量份的成分（ b），高级脂肪酸的金属盐，和（e）基于100重量份成分（b）的0.05-5重量份的主要由酚类稳定剂组成的稳定剂组合物。乙烯聚合物膜通过在150-250℃下通过具有间隙为0.7-3.0mm的唇缘的环模具以2 / 1-8 / 1的吹塑比和霜线高200-2000毫米。

9. 发明授权

US4381252A Catalyst for producing polyolefins 失效
标题翻译：催化剂生产聚烯烃
公开(公告)号：US4381252A
公开(公告)日：1983-04-26
申请号：US269240
申请日：1981-06-01
申请人： Hisaya Sakurai , Yoshihiko Katayama , Tadashi Ikegami , Masayasu Furusato
发明人： Hisaya Sakurai , Yoshihiko Katayama , Tadashi Ikegami , Masayasu Furusato
IPC分类号： C08F4/64 , C08F10/00
CPC分类号： C08F10/00
摘要： A catalyst suitable for polymerizing an .alpha.-olefin, comprising a solid catalyst component [A] and an organometal compound [B], the solid catalyst component [A] being prepared by reacting an organomagnesium compound (1) soluble in a hydrocarbon medium and represented by the general formula,MgR.sub.p.sup.1 R.sub.q.sup.2 X.sub.r.Z.sub.swhereinR.sup.1 is a hydrocarbon group having 2 to 3 carbon atoms;R.sup.2 is a hydrocarbon group having 4 to 20 carbon atoms and the difference in number of carbon atoms between R.sup.1 and R.sup.2 is at least 2;X is an electronegative group having an oxygen atom, a nitrogen atom or a sulfur atom;Z is an organometal compound of aluminum, boron, beryllium, zinc, silicon or lithium;p and q each is a number above 0 to 1;r is a number from 0 to 1;p+q+r=2; ands is a number from 0.02 to 0.09,with a titanium and/or vanadium compound (2) having at least one halogen atom; and a process for polymerizing an .alpha.-olefin employing the same catalyst.
摘要翻译：一种适用于聚合α-烯烃的催化剂，包括固体催化剂组分[A]和有机金属化合物[B]，固体催化剂组分[A]是通过使可溶于烃介质的有机镁化合物（1）通式为MgRp1Rq2Xr.Zs，其中R1为碳原子数2〜3的烃基; R2是碳原子数为4〜20的烃基，R1和R2之间的碳原子数不同，为2以上。 X是具有氧原子，氮原子或硫原子的电负性基团; Z是铝，硼，铍，锌，硅或锂的有机金属化合物; p和q各自为0至1以上的数字; r是从0到1的数字; p + q + r = 2; 和s为0.02至0.09的数，其中钛和/或钒化合物（2）具有至少一个卤素原子; 以及使用相同催化剂聚合α-烯烃的方法。

10. 发明授权

US4335229A Process for polymerizing an .alpha.-olefin 失效
标题翻译：聚合α-烯烃的方法
公开(公告)号：US4335229A
公开(公告)日：1982-06-15
申请号：US177546
申请日：1980-08-13
申请人： Hisaya Sakurai , Yoshihiko Katayama , Tadashi Ikegami , Masayasu Furusato
发明人： Hisaya Sakurai , Yoshihiko Katayama , Tadashi Ikegami , Masayasu Furusato
IPC分类号： C08F4/62 , C08F4/76 , C08F10/00 , C08F4/64
CPC分类号： C08F10/00 , Y10S526/904
摘要： A process for polymerizing an .alpha.-olefin comprising contacting the olefin in liquid phase at a temperature of about 120.degree. to about 320.degree. C. with a catalyst comprising a component (A) and an organometal component (B), the component (A) being produced by reacting a hydrocarbon-soluble organomagnesium component (i) of the formula,M.sub..alpha. MgR.sub.p.sup.1 R.sub.q.sup.2 X.sub.r.sup.1 X.sub.s.sup.2 D.sub.twherein.alpha., p, q, r and s each independently is 0 or a number greater than 0,t is a number greater than 0,p+q+r+s=m.alpha.+2,O.ltoreq.(r+s)/(.alpha.+1)
摘要翻译：一种聚合α-烯烃的方法，包括使液相中的烯烃在约120℃至约320℃的温度下与包含组分（A）和有机金属组分（B）的催化剂接触，组分（A）其中α，p，q，r和s各自独立地为0或大于0的数，t是大于0的数，p是大于0的数，p + q + r + s =mα+2，O（=（r + s）/（α+ 1））2，m是M的化合价，M是周期的第1〜表中，R 1和R 2各自独立地为具有1至20个碳原子的烃基，X 1和X 2各自独立地为氢原子，卤素原子或含有O，N或S的有机负电子基团，D为电子给体，与（ⅱ）硼，硅，锗，锡，磷，锑，铋或锌的卤化物，并使（ⅰ）+（ⅱ）与（ⅲ）钛的化合物和 /或钛+钒浓度为至多约2摩尔/升惰性反应溶剂的钒化合物，（A）中Mg /（Ti + V）的原子比为约3至约500。

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