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1. 发明授权

US07285607B2 Polymerisation of olefinic compounds 失效
标题翻译：烯烃化合物的聚合
公开(公告)号：US07285607B2
公开(公告)日：2007-10-23
申请号：US11130106
申请日：2005-05-17
申请人： Kevin Blann , Deon De Wet-Roos , Dawid Johannes Joubert , Esna Killian , John Thomas Dixon , Nonhlanhla Jillian Phelembe , Aletta Du Toit
发明人： Kevin Blann , Deon De Wet-Roos , Dawid Johannes Joubert , Esna Killian , John Thomas Dixon , Nonhlanhla Jillian Phelembe , Aletta Du Toit
IPC分类号： C08F4/74 , C08F4/76 , C08F4/78 , C08F10/00 , C08F4/622 , C08F4/69
CPC分类号： B01J31/2204 , B01J31/18 , B01J31/188 , B01J31/2409 , B01J2231/12 , B01J2231/20 , B01J2531/46 , B01J2531/56 , B01J2531/62 , C08F110/02 , C08F2410/04 , C08F2500/08 , C08F2500/02 , C08F2500/23 , C08F2500/17 , C08F2500/20 , C08F4/69146 , C08F4/6497
摘要： This invention relates to a process for producing a polymeric product by the polymerisation of at least one olefinic compound in the form of an olefin or a compound including an olefinic moiety by contacting the at least one olefinic compound with a polymerisation catalyst. The catalyst comprises the combination of a source of a Group IV to VI transition metal; and a ligating compound of the formula (R1)mX1(Y)X2(R2)n. The process is characterised therein that when R1 and R2 are independently a hydrocarbyl group or a heterohydrocarbyl group which contains at least one non-polar substituent, the olefinic compound is contacted with the polymerisation catalyst at a reaction temperature from and above 70° C.; and where R1 and R2 are independently a hydrocarbyl group or a heterohydrocarbyl group which contains no substituent, the olefinic compound is contacted with the polymerisation catalyst at a reaction temperature from and above 90° C.
摘要翻译：本发明涉及通过使烯烃或包含烯属部分的化合物的形式聚合至少一种烯烃化合物来生产聚合产物的方法，该方法包括使至少一种烯烃化合物与聚合催化剂接触。催化剂包括IV-VI族过渡金属源的组合; 和式<？in-line-formula description =“In-line Formulas”的连接化合物end =“lead”？（R 1）（Y）X 2（R 2）N 2 在线公式描述=“In 线式“end =”tail“？>该方法的特征在于当R 1和R 2独立地是烃基或至少含有至少一个非极性取代基，烯烃化合物在70℃以上的反应温度下与聚合催化剂接触。并且其中R 1和R 2独立地是不含取代基的烃基或杂烃基，所述烯烃化合物与所述聚合催化剂在反应温度下高于90°C

2. 发明授权

US06391987B1 Gas-phase polymerization process for producing propylene/1-pentene copolymers 失效
标题翻译：用于生产丙烯/ 1-戊烯共聚物的气相聚合方法
公开(公告)号：US06391987B1
公开(公告)日：2002-05-21
申请号：US09470219
申请日：1999-12-22
申请人： Ioan Tincul , Ignatius Hendrik Potgieter , Dawid Johannes Joubert , Antonie Hermanus Potgieter
发明人： Ioan Tincul , Ignatius Hendrik Potgieter , Dawid Johannes Joubert , Antonie Hermanus Potgieter
IPC分类号： C08F4614
CPC分类号： C08F10/00 , C08F210/06 , C08F4/6555 , C08F4/6492 , C08F4/655 , C08F4/6543 , C08F2/34 , C08F210/14 , C08F2500/12
摘要： Process for producing a propylene/1-pentene polymer in the presence of a Ziegler-Natta catalyst system with the monomer reactants being in the vapor phase while the reaction is in process and with no liquid component being present in the reaction zone while the reaction is in progress. Different ways of introducing the reactants are disclosed (partly in liquid phase then immediately evaporated or not, preheated or not, mixed with the comonomer or not).
摘要翻译：在齐格勒 - 纳塔催化剂体系存在下制备丙烯/ 1-戊烯聚合物的方法，其中单体反应物处于气相中，同时反应在反应过程中并且在反应区中不存在液体组分进行中。公开了不同的引入反应物的方法（部分为液相，然后立即蒸发或不蒸发，预热或不与共聚单体混合）。

3. 发明授权

US06248685B1 Catalyst 失效
标题翻译：催化剂
公开(公告)号：US06248685B1
公开(公告)日：2001-06-19
申请号：US09194673
申请日：1999-04-01
申请人： Dawid Johannes Joubert , Ignatius Hendrik Potgieter , Ioan Tincul
发明人： Dawid Johannes Joubert , Ignatius Hendrik Potgieter , Ioan Tincul
IPC分类号： B01J3100
CPC分类号： C08F210/16 , C08F10/00 , Y10S526/916 , C08F4/6555 , C08F210/14 , C08F210/08 , C08F2500/12
摘要： A method of making a catalyst suitable for the polymerization of olefins includes the steps of mixing an ether having a total number of carbon atoms equal to or greater than 8, with hydrated magnesium chloride, to produce partially activated magnesium chloride; mixing an alkyl aluminum with the partially activated magnesium chloride to form unwashed activated magnesium chloride; and washing the activated magnesium chloride with an inert saturated hydrocarbon liquid, to obtain an activated magnesium chloride-containing slurry. A plurality of alcohols are mixed with the activated magnesium chloride-containing slurry to form an activated magnesium chloride/alcohol complex. Titanium tetrachloride is mixed with the activated magnesium chloride/alcohol complex, to form a magnesium chloride supported titanium catalyst.
摘要翻译：制备适合于烯烃聚合的催化剂的方法包括将总数等于或大于8的碳原子的醚与水合氯化镁混合以产生部分活化的氯化镁的步骤; 将烷基铝与部分活化的氯化镁混合以形成未洗涤的活化氯化镁; 并用惰性饱和烃液体洗涤活化的氯化镁，得到活化的含氯化镁的浆料。将多种醇与活化的含氯化镁的浆料混合以形成活化的氯化镁/醇络合物。将四氯化钛与活化的氯化镁/醇络合物混合，形成载有氯化镁的钛催化剂。

4. 发明授权

US06391951B1 Propylene pentene-1 copolymers, method of preparation thereof and composition containing them 失效
标题翻译：丙烯戊烯-1共聚物，其制备方法和含有它们的组合物
公开(公告)号：US06391951B1
公开(公告)日：2002-05-21
申请号：US09615249
申请日：2000-07-13
申请人： Dawid Johannes Joubert , Antonie Hermanus Potgieter , Ignatius Hendrik Potgieter , Ioan Tincul
发明人： Dawid Johannes Joubert , Antonie Hermanus Potgieter , Ignatius Hendrik Potgieter , Ioan Tincul
IPC分类号： C08K549
CPC分类号： C08K5/1345 , C08F210/06 , C08K5/527 , C08F210/14 , C08L23/10 , C08F2500/12
摘要： The invention provides a copolymer of propylene and pentene, together with a process for producing such copolymer and a polymer composition. In the process, propylene and pentene are reacted in a reaction zone at a pressure of 60 kg/cm2 and temperature of 0-100° C. for 20-480 minutes in the presence of a Ziegler-Natta catalyst or catalyst system. The polymer composition has several components, namely the above copolymer, a phenolic stabilizer, an organic phosphite stabilizer, a thioether stabilizer and at least one metal salt of a higher aliphatic acid, with the proviso that at least one of the organic phosphite stabilizer, the thioether stabilizer and said salt must be present, so that up to two thereof can optionally be omitted.
摘要翻译：本发明提供丙烯和戊烯的共聚物，以及制备这种共聚物和聚合物组合物的方法。在该过程中，丙烯和戊烯在反应区中在齐格勒 - 纳塔催化剂或催化剂体系存在下，在60kg / cm2的压力和0-100℃的温度下反应20-480分钟。聚合物组合物具有若干组分，即上述共聚物，酚类稳定剂，有机亚磷酸酯稳定剂，硫醚稳定剂和至少一种高级脂肪酸的金属盐，条件是至少有一种有机亚磷酸酯稳定剂，必须存在硫醚稳定剂和所述盐，使得可以任选地省略其中两个。

5. 发明授权

US06191246B1 Ethylene-pentene-hexene copolymer, process for its preparation and use for the production of films 失效
标题翻译：乙烯 - 戊烯 - 己烯共聚物，其制备方法和用于制备薄膜的方法
公开(公告)号：US06191246B1
公开(公告)日：2001-02-20
申请号：US08945495
申请日：1998-01-12
申请人： Dawid Johannes Joubert , Ignatius Hendrik Potgieter , Ioan Tincul , Peter Loggenberg
发明人： Dawid Johannes Joubert , Ignatius Hendrik Potgieter , Ioan Tincul , Peter Loggenberg
IPC分类号： C08F21014
CPC分类号： C08K5/098 , C08F210/16 , C08K5/13 , Y10S526/905 , Y10S526/916 , C08F4/6555 , C08L23/02 , C08F210/14 , C08F2500/12
摘要： The invention provides a polymer which is a polymerization product obtained by polymerizing at least ethylene, 1-pentene and 1-hexene; and a process for producing a polymer by reacting at least ethylene, 1-pentene and 1-hexene in a reaction zone at a pressure between atmospheric and 60 kg/cm3 and at a temperature between 30° C. and 120° C., in the presence of a catalyst system. The invention also provides a polymer composition which comprises a terpolymer of ethylene, 1-pentene and 1-hexene, a phenolic stabilizer component, a metal salt of a higher aliphatic acid, and, optionally, at least one organic phosphite stabilizer.
摘要翻译：本发明提供一种聚合物，其是通过至少聚合乙烯，1-戊烯和1-己烯而获得的聚合产物; 以及通过在反应区中至少使乙烯，1-戊烯和1-己烯在大气压和60kg / cm 3之间的压力下和在30℃和120℃之间的温度下，在催化剂体系的存在。本发明还提供一种聚合物组合物，其包含乙烯，1-戊烯和1-己烯的三元共聚物，酚类稳定剂组分，高级脂族酸的金属盐和任选的至少一种有机亚磷酸酯稳定剂。

6. 发明授权

US06417300B1 Terpolymerization 失效
标题翻译：三聚合
公开(公告)号：US06417300B1
公开(公告)日：2002-07-09
申请号：US09194672
申请日：1999-05-12
申请人： Dawid Johannes Joubert , Ignatius Hendrik Potgieter , Ioan Tincul
发明人： Dawid Johannes Joubert , Ignatius Hendrik Potgieter , Ioan Tincul
IPC分类号： C08F1014
CPC分类号： C08F210/16 , C08F10/00 , Y10S526/916 , C08F4/6555 , C08F210/14 , C08F210/08 , C08F2500/12
摘要： Disclosed are terpolymers and processes of terpolymerization, wherein the terpolymer comprises units derived from ethylene, 1-pentene and another alpha-olefin containing at least six carbon atoms.
摘要翻译：公开了三元共聚物和三元共聚方法，其中三元共聚物包含衍生自乙烯，1-戊烯和另外含有至少6个碳原子的α-烯烃的单元。

7. 发明授权

US6111047A Propylene/pentene-1 copolymers and method of preparation thereof 失效
标题翻译：丙烯/戊烯-1共聚物及其制备方法
公开(公告)号：US6111047A
公开(公告)日：2000-08-29
申请号：US875782
申请日：1997-10-28
申请人： Dawid Johannes Joubert , Antonie Hermanus Potgieter , Ignatius Hendrik Potgieter , Ioan Tincul
发明人： Dawid Johannes Joubert , Antonie Hermanus Potgieter , Ignatius Hendrik Potgieter , Ioan Tincul
IPC分类号： C08F210/06 , C08K5/134 , C08K5/527 , C08F10/14 , C08F110/14
CPC分类号： C08K5/1345 , C08F210/06 , C08K5/527
摘要： The invention provides a copolymer of propylene and pentene, together with a process for producing such copolymer. The copolymer has a random arrangement of propylene and 1-pentene, is theromplastic, has crystalline and amorphous sequences, and has a melt flow index in the range of about 0.01 to about 200 g/10 minutes. In the process, propylene and pentene are reacted in a reaction zone at a pressure of 60 kg/cm.sup.2 and temperature of 0-100.degree. C. for 20-480 minutes in the presence of a Ziegler-Natta catalyst or catalyst system.
摘要翻译： PCT No.PCT / GB96 / 00201 Sec。 371日期1997年10月28日第 102（e）日期1997年10月28日PCT 1996年1月30日PCT PCT。公开号WO96 / 24623 日期：1996年8月15日本发明提供丙烯和戊烯的共聚物，以及制备这种共聚物的方法。该共聚物具有丙烯和1-戊烯的随机排列，是具有结晶和无定形序列的成纤维，具有约0.01至约200g / 10分钟范围内的熔体流动指数。在该过程中，丙烯和戊烯在反应区中在齐格勒 - 纳塔催化剂或催化剂体系存在下，在60kg / cm 2的压力和0-100℃的温度下反应20-480分钟。

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