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1. 发明授权

US06489370B2 Method of manufacturing a synthesis gas to be employed for the synthesis of gasoline, kerosene and gas oil 有权
标题翻译：制造用于合成汽油，煤油和瓦斯油的合成气的方法
公开(公告)号：US06489370B2
公开(公告)日：2002-12-03
申请号：US09764379
申请日：2001-01-19
申请人： Masaki Iijima , Kazuto Kobayashi , Kazuhiro Morita
发明人： Masaki Iijima , Kazuto Kobayashi , Kazuhiro Morita
IPC分类号： C07C2700
CPC分类号： C10G2/30 , C01B3/382 , C01B3/384 , C01B2203/0811 , C01B2203/0816 , C01B2203/0866 , C01B2203/142 , C01B2203/143 , C01B2203/148 , C10G2300/1025 , C10G2300/807 , C10G2400/02 , C10G2400/06 , C10G2400/08 , Y02P20/129
摘要： A method for manufacturing a synthesis gas, which makes it possible to procure CO2 inside a synthesis gas-manufacturing plant utilizing the Fisher-Tropsch reaction system, thereby enabling the synthesis gas to be cheaply manufactured by way of the Fisher-Tropsch reaction system without being restricted by the location of CO2 gas source such as an ammonia plant, the synthesis gas comprising a molar ratio of H2/CO suited for synthesizing gasoline, kerosene and gas oil. This method comprises the steps of, feeding a steam-mixed natural gas to a reformer provided with a combustion radiation portion for burning a fuel, the reformer being heated by the combustion radiation portion, recovering carbon dioxide from a combustion exhaust gas generated at the combustion radiation portion, and adding the carbon dioxide to the steam-mixed natural gas at a location on an upstream side of the reformer.
摘要翻译：一种制造合成气的方法，其可以利用费 - 托反应体系在合成气制造厂内获得二氧化碳，从而能够通过费 - 托反应系统廉价地制造合成气，而不会受氨气装置等二氧化碳气体源的位置限制，合成气体包含适合合成汽油，煤油和瓦斯油的H2 / CO摩尔比。该方法包括以下步骤：将蒸汽混合天然气供给到设置有用于燃烧燃料的燃烧辐射部分的重整器，重整器由燃烧辐射部分加热，从燃烧产生的燃烧废气中回收二氧化碳辐射部分，并且在重整器的上游侧的位置处将二氧化碳加入到蒸汽混合天然气中。

2. 发明授权

US06486218B2 Method of manufacturing methanol 失效
标题翻译：制造甲醇的方法
公开(公告)号：US06486218B2
公开(公告)日：2002-11-26
申请号：US09931095
申请日：2001-08-17
申请人： Kazuto Kobayashi , Masaki Iijima , Kazuhiro Morita
发明人： Kazuto Kobayashi , Masaki Iijima , Kazuhiro Morita
IPC分类号： C07C2700
CPC分类号： C07C29/1518 , C07C31/04
摘要： A natural gas having steam and carbon dioxide added thereto is supplied into a reaction tube of a reformer provided with the reaction tube and a combustion radiation section for heating the reaction tube by combustion of a fuel so as to carry out a reaction between the hydrocarbon contained in the natural gas and the steam added to the natural gas, thereby forming a synthetic gas containing hydrogen, carbon monoxide and carbon dioxide. Then, the synthetic gas is subjected to a reaction in the presence of a methanol synthesizing catalyst. A crude methanol obtained is subjected to a gas-liquid separation. Further, a liquid crude methanol separated in the separation is distilled. In the particular methanol manufacturing process, a part of the purge gas obtained in the separation is recycled into the natural gas having steam and carbon dioxide added thereto in advance.
摘要翻译：将具有蒸汽和二氧化碳的天然气供给到设置有反应管的重整器的反应管中，以及用于通过燃料燃烧来加热反应管的燃烧放射部，以便在所含有的烃之间进行反应在天然气中加入天然气中的蒸汽，从而形成含有氢，一氧化碳和二氧化碳的合成气体。然后，合成气体在甲醇合成催化剂的存在下进行反应。将得到的粗甲醇进行气液分离。此外，在分离中分离的液体粗甲醇被蒸馏。在特定的甲醇制造方法中，将分离中获得的吹扫气体的一部分预先循环到具有蒸汽和二氧化碳的天然气中。

3. 发明授权

US06475409B2 Method of manufacturing synthesis gas 失效
公开(公告)号：US06475409B2
公开(公告)日：2002-11-05
申请号：US09801718
申请日：2001-03-09
申请人： Masaki Iijima , Kazuto Kobayashi , Kazuhiro Morita
发明人： Masaki Iijima , Kazuto Kobayashi , Kazuhiro Morita
IPC分类号： C07C102
CPC分类号： C01B3/384 , C01B3/38 , C01B3/382 , C01B2203/0233 , C01B2203/0238 , C01B2203/025 , C01B2203/0475 , C01B2203/0495 , C01B2203/06 , C01B2203/061 , C01B2203/062 , C01B2203/0811 , C01B2203/0816 , C01B2203/0866 , C01B2203/0894 , C01B2203/1052 , C01B2203/1241 , C01B2203/1294 , C01B2203/142 , C01B2203/143 , C01B2203/146 , C01B2203/148 , Y02P20/129
摘要： A method of manufacturing a synthesis gas, which makes use of a synthesis plant comprising a reformer having a steam reforming reaction tube, a combustion radiation portion provided around the reaction tube, for heating the reaction tube, and a convection portion communicating the combustion radiation portion. A steam-containing natural gas is prepared by adding stream to a natural gas. The steam-containing natural gas is preheated by passing the natural gas through a convection portion of reformer, the natural gas preheated being subsequently fed to the reaction tube. After being preheated in the convection portion, carbon dioxide is fed to the reaction tube, thereby producing a synthesis gas containing hydrogen and carbon monoxide.

4. 发明授权

US06726852B2 Method of manufacturing synthesis gas 有权
标题翻译：制造合成气的方法
公开(公告)号：US06726852B2
公开(公告)日：2004-04-27
申请号：US09801720
申请日：2001-03-09
申请人： Masaki Iijima , Kazuto Kobayashi , Kazuhiro Morita
发明人： Masaki Iijima , Kazuto Kobayashi , Kazuhiro Morita
IPC分类号： C01J300
CPC分类号： C10L3/10 , C01B3/38 , C01B3/384 , C01B2203/0233 , C01B2203/0238 , C01B2203/0475 , C01B2203/06 , C01B2203/061 , C01B2203/062 , C01B2203/0811 , C01B2203/0816 , C01B2203/0866 , C01B2203/0894 , C01B2203/1052 , C01B2203/1241 , C01B2203/127 , C01B2203/1294 , C01B2203/148 , Y02C10/06
摘要： A method of manufacturing a synthesis gas containing hydrogen and carbon monoxide comprises steps of removing only hydrogen sulfide from a natural gas containing hydrogen sulfide and carbon dioxide by permitting the natural gas to pass through a hydrogen sulfide-removing device filled with a hydrogen sulfide absorbent, adding carbon dioxide and steam to the natural gas which the hydrogen sulfide has been removed to prepare a mixed gas, and feeding the mixed gas into a reaction tube of a reformer, thereby permitting mainly a steam reforming reaction to take place in the mixed gas. This method enables hydrogen sulfide in natural gas to be removed while permitting the carbon dioxide of natural gas to be effectively utilized, thereby reducing the quantity of carbon dioxide to be added to the natural gas to be transferred to the reformer.
摘要翻译：制造含有氢和一氧化碳的合成气的方法包括通过允许天然气通过填充有硫化氢吸收剂的硫化氢去除装置，仅从含有硫化氢和二氧化碳的天然气中除去硫化氢的步骤，向已除去硫化氢的天然气中加入二氧化碳和蒸汽以制备混合气体，并将混合气体进料到重整器的反应管中，从而主要在混合气体中进行蒸汽重整反应。该方法能够除去天然气中的硫化氢，同时能够有效地利用天然气的二氧化碳，从而减少要添加到转移到重整器中的天然气中的二氧化碳的量。

5. 发明授权

US06782714B2 Plant and method for producing liquefied natural gas 有权
标题翻译：生产液化天然气的工厂和方法
公开(公告)号：US06782714B2
公开(公告)日：2004-08-31
申请号：US10640016
申请日：2003-08-14
申请人： Masaki Iijima , Kazuto Kobayashi , Hiroyuki Osora , Yoshio Seiki
发明人： Masaki Iijima , Kazuto Kobayashi , Hiroyuki Osora , Yoshio Seiki
IPC分类号： F25J308
CPC分类号： B01D53/1475 , C01B32/50 , F25J1/0022 , F25J1/0282 , F25J3/0209 , F25J3/0266 , F25J2205/50 , F25J2210/70 , F25J2220/66 , F25J2230/20 , F25J2230/30 , F25J2230/80 , F25J2240/70 , F25J2260/80 , Y02C10/04 , Y02C10/06 , Y02C10/12 , Y02P20/152
摘要： A plant for producing liquefied natural gas comprises a carbon dioxide recovery apparatus for natural gas absorbing and removing carbon dioxide from natural gas, a liquefying apparatus having a steam turbine, for liquefying the natural gas from which carbon dioxide has been removed by the carbon dioxide recovery apparatus, a boiler equipment for supplying steam to the steam turbine of the liquefying apparatus, and a carbon dioxide recovery apparatus for combustion exhaust gas including an absorption tower for absorbing carbon dioxide from combustion exhaust gas exhausted from the boiler equipment by absorbing liquid, and a regeneration tower for separating and recovering carbon dioxide from the absorbing liquid.
摘要翻译：用于生产液化天然气的设备包括用于从天然气中吸收和去除二氧化碳的天然气的二氧化碳回收装置，具有汽轮机的液化装置，用于液化通过二氧化碳回收除去二氧化碳的天然气设备，用于向液化装置的蒸汽涡轮机供应蒸汽的锅炉设备和用于燃烧废气的二氧化碳回收设备，其包括用于通过吸收液体从从锅炉设备排出的燃烧废气中吸收二氧化碳的吸收塔，以及用于从吸收液中分离和回收二氧化碳的再生塔。

6. 发明授权

US06504068B1 Method for converting a plastic waste into oil in a stainless steel reactor 失效
标题翻译：在不锈钢反应器中将塑料废物转化为油的方法
公开(公告)号：US06504068B1
公开(公告)日：2003-01-07
申请号：US08870623
申请日：1997-06-06
申请人： Wataru Matsubara , Hiroshi Makihara , Kazuto Kobayashi , Masaki Iijima
发明人： Wataru Matsubara , Hiroshi Makihara , Kazuto Kobayashi , Masaki Iijima
IPC分类号： C07C100
CPC分类号： C10G1/10 , Y10S208/952
摘要： A method of converting a plastic waste into oil by decomposing the plastic waste by a reaction using water in a supercritical or near supercritical region as a reaction medium. In this method, the reaction is conducted by using a tubular continuous reactor. The present invention further provides an apparatus therefor. Moreover, the present invention provides a method of converting a plastic waste into oil by conducting the reaction after hydrogen chloride is removed by performing the pyrolysis of the plastic waste in the case that the plastic waste contain chlorine. The present invention further provides an apparatus for performing this method.
摘要翻译：通过使用超临界或近超临界区域中的水作为反应介质的反应分解塑料废物来将塑料废物转化为油的方法。在该方法中，通过使用管状连续反应器进行反应。本发明还提供了一种装置。此外，本发明提供了在塑料废物含有氯的情况下，通过进行塑料废物的热分解而在除去氯化氢之后通过进行反应来将塑料废物转化为油的方法。本发明还提供了一种用于执行该方法的装置。

7. 发明申请

US20070037998A1 Method and device for manufacturing dimethyl carbonate 有权
标题翻译：制造碳酸二甲酯的方法和装置
公开(公告)号：US20070037998A1
公开(公告)日：2007-02-15
申请号：US10553009
申请日：2004-04-16
申请人： Kazuto Kobayashi , Hiroyuki Osora , Yoshio Seiki , Masaki Iijima
发明人： Kazuto Kobayashi , Hiroyuki Osora , Yoshio Seiki , Masaki Iijima
IPC分类号： C07C69/96 , C07C27/26
CPC分类号： C07C29/1518 , C07C29/152 , C07C68/04 , Y02P20/142 , C07C31/04 , C07C69/96
摘要： The present invention provides a method and apparatus for producing dimethyl carbonate, wherein carbon dioxide is recovered from combustion exhaust gas of a steam reformer 10 and a boiler; and some of the recovered carbon dioxide is used for methanol synthesis as a raw material for the steam reformer 10, and the remaining carbon dioxide is allowed to react with some of the yielded methanol to synthesize dimethyl carbonate. According to the present invention, CO2, which has conventionally been discharged, is returned to the steam reformer and is used effectively to produce DMC, and also devices for producing methanol and DMC can be simplified.
摘要翻译：本发明提供一种生产二甲基碳酸酯的方法和装置，其中从蒸汽重整器10和锅炉的燃烧废气中回收二氧化碳; 一部分回收的二氧化碳用作甲醇合成用作蒸汽重整器10的原料，剩余的二氧化碳与一些生成的甲醇反应合成碳酸二甲酯。根据本发明，通常排出的CO 2返回到蒸汽重整器，并且有效地用于制造DMC，并且还可以简化用于生产甲醇和DMC的装置。

8. 发明授权

US06924399B2 Method of manufacturing dimethyl ether 失效
标题翻译：制造二甲醚的方法
公开(公告)号：US06924399B2
公开(公告)日：2005-08-02
申请号：US10316086
申请日：2002-12-11
申请人： Masaki Iijima , Kazuto Kobayashi
发明人： Masaki Iijima , Kazuto Kobayashi
IPC分类号： C07C41/09 , C07C43/04 , C10L1/18
CPC分类号： C07C41/09 , C07C43/043
摘要： Dimethyl ether is obtained with at low cost by transporting methanol under room temperature and atmospheric pressure from the methanol producing district to the dimethyl ether consuming district or its neighboring district by converting the raw material containing the transported methanol into dimethyl ether in the consuming district or its neighboring district.
摘要翻译：通过将甲醇在室温和大气压下从甲醇生产区运送到二甲醚消费区或其邻近地区，通过将含有运输的甲醇的原料转化成二甲醚在消费区或其中的二甲醚获得二甲醚邻近区。

9. 发明授权

US06352674B2 Apparatus for converting a plastic waste into oil 失效
标题翻译：用于将塑料废物转化为油的装置
公开(公告)号：US06352674B2
公开(公告)日：2002-03-05
申请号：US09359383
申请日：1999-07-23
申请人： Wataru Matsubara , Hiroshi Makihara , Kazuto Kobayashi , Masaki Iijima
发明人： Wataru Matsubara , Hiroshi Makihara , Kazuto Kobayashi , Masaki Iijima
IPC分类号： F28D2100
CPC分类号： C10G1/10
摘要： A method of converting a plastic waste into oil by decomposing the plastic waste by a reaction using water in a supercritical or near supercritical region as a reaction medium. In this method, the reaction is conducted by using a tubular continuous reactor. The present invention further provides an apparatus therefor. Moreover, the present invention provides a method of converting a plastic waste into oil by conducting the reaction after hydrogen chloride is removed by performing the pyrolysis of the plastic waste in the case that the plastic waste contain chlorine. The present invention further provides an apparatus for performing this method.
摘要翻译：通过使用超临界或近超临界区域中的水作为反应介质的反应分解塑料废物来将塑料废物转化为油的方法。在该方法中，通过使用管状连续反应器进行反应。本发明还提供了一种装置。此外，本发明提供了在塑料废物含有氯的情况下，通过进行塑料废物的热分解而在除去氯化氢之后通过进行反应来将塑料废物转化为油的方法。本发明还提供了一种用于执行该方法的装置。

10. 发明授权

US6107532A Process and system for converting plastics waste into oil 失效
标题翻译：将塑料废物转化为油的工艺和制度
公开(公告)号：US6107532A
公开(公告)日：2000-08-22
申请号：US57725
申请日：1998-04-09
申请人： Yoshihisa Saito , Takehiko Moriya , Masaki Iijima , Wataru Matsubara , Kazuto Kobayashi , Naohiko Ukawa
发明人： Yoshihisa Saito , Takehiko Moriya , Masaki Iijima , Wataru Matsubara , Kazuto Kobayashi , Naohiko Ukawa
IPC分类号： B09B3/00 , C08J11/00 , C10G1/10 , C07C1/00 , C10L1/00
CPC分类号： C10G1/10
摘要： Disclosed is an economical process for treating a large amount of plastics waste in which thermoplastics, crosslinked plastics, thermosetting plastics or a mixture thereof can be continuously and rapidly degraded and converted into oil without sorting various types of plastics waste. According to this process, powdered plastics obtained by grinding thermoplastics, crosslinked plastics, thermosetting plastics or a mixture thereof is mixed with water to form a slurry, and a dispersing agent such as a water-absorbing resin, a water-soluble polymer or a surface-active agent is added thereto. The resulting mixed slurry is fed to a tubular continuous reactor where the powdered plastics is degraded under reaction conditions causing the water to be in or near its supercritical region. Finally, oil is recovered from the reaction product.
摘要翻译：公开了一种用于处理大量塑料废料的经济方法，其中热塑性塑料，交联塑料，热固性塑料或其混合物可以连续且快速地降解并转化成油而不分类各种塑料废料。根据该方法，将通过研磨热塑性塑料，交联塑料，热固性塑料或其混合物获得的粉末状塑料与水混合以形成浆料，并将分散剂如吸水树脂，水溶性聚合物或表面添加活性剂。将所得混合浆料进料到管状连续反应器中，其中粉末状塑料在引起水处于或接近其超临界区域的反应条件下降解。最后，从反应产物中回收油。

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