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1. 发明授权

US4518472A Delustering coating composition excellent in abrasion resistance 失效
标题翻译：具有优异耐磨性的清漆涂料组合物
公开(公告)号：US4518472A
公开(公告)日：1985-05-21
申请号：US525895
申请日：1983-08-24
申请人： Kazuo Kishida , Isao Sasaki , Kenji Kushi , Masahiro Sugimori
发明人： Kazuo Kishida , Isao Sasaki , Kenji Kushi , Masahiro Sugimori
IPC分类号： C08F2/48 , C08F285/00 , C08J7/04 , C09D4/06 , C08F220/00 , C09D3/00
CPC分类号： C08J7/047 , C08F285/00 , C09D4/06 , C08J2333/06 , C08J2433/00
摘要： A coating composition curable by an activation energy ray, which comprises (a) 100 parts by weight of a monomer mixture (A) comprising at least 30% by weight of a compound having at least 3 acryloyloxy and/or methacryloyloxy groups in the molecule and up to 70% by weight of a compound having 1 to 2 .alpha.,.beta.-ethylenically unsaturated bonds in the molecule, (b) 0.01 to 6.0 parts by weight of at least one photosensitizer and (c) 0.5 to 30 parts by weight of an emulsion type crosslinked polymer or copolymer of a reactive monomer having one .alpha.,.beta.-ethylenically unsaturated bond in the molecule and a reactive monomer having at least two .alpha.,.beta.-ethylenically unsaturated bonds in the molecule.
摘要翻译：一种由活化能射线固化的涂料组合物，其包含（a）100重量份的包含至少30重量％的分子中具有至少3个丙烯酰氧基和/或甲基丙烯酰氧基的化合物的单体混合物（A），和至多70重量％的分子中具有1至2个α，β-烯属不饱和键的化合物，（b）0.01至6.0重量份的至少一种光敏剂和（c）0.5至30重量份的分子中具有一个α，β-烯属不饱和键的反应性单体的乳液型交联聚合物或共聚物，以及在分子中具有至少两个α，β-烯属不饱和键的反应性单体。

2. 发明授权

US4367245A Coating composition and process for preparing synthetic resin shaped articles by using same 失效
标题翻译：涂料组合物及其制备方法
公开(公告)号：US4367245A
公开(公告)日：1983-01-04
申请号：US246942
申请日：1981-03-24
申请人： Kazuo Kishida , Isao Sasaki , Kenji Kushi , Misao Tamura
发明人： Kazuo Kishida , Isao Sasaki , Kenji Kushi , Misao Tamura
IPC分类号： C08F20/00 , B05D3/06 , B05D7/02 , C08F2/48 , C08F20/10 , C08F20/26 , C08F22/10 , C08F220/28 , C08F290/00 , C08F299/02 , C08J7/04 , C09D4/00 , C09D133/04
CPC分类号： C08F22/105 , C09D4/00
摘要： A coating composition for the preparation of synthetic resin shaped articles excellent in abrasion resistance and weatherability is described. This composition comprises (a) a polyfunctional monomer mixture comprising (i) 25-75 wt. % of at least one polyfunctional monomer of the formula (I): ##STR1## wherein at least three of X.sub.11, X.sub.12, X.sub.13, X.sub.22, X.sub.23 -X.sub.n2, X.sub.n3 and X.sub.14 are CH.sub.2 .dbd.CH.C00-- and the remaining groups are --OH, and n is an integer of 1-5, (ii) 25-75 wt. % of at least one polyfunctional monomer of the formula (II): ##STR2## wherein at least three of the R groups are CH.sub.2 .dbd.CH COO-- and each of the remaining is H or --OH, n.sub.1, n.sub.2, n.sub.3, n.sub.4, m.sub.1, m.sub.2, m.sub.3 and m.sub.4 are integers of 0, 1 or 2, and X is an integer of 1 to 10 and (iii) 0 to 50 wt. % of a monomer containing one acryloyloxy group and having a boiling point of at least 150.degree. C. at normal pressure and a viscosity of not higher than 20 cps/20.degree. C., and (b) 0.01-6.0 wt. parts, based on 100 wt. parts of the polyfunctional monomer mixture, of at least one photosensitizer. The coating composition is coated on a synthetic resin shaped article and then, irradiated with utraviolet rays in air to form a crosslinked coating film having a thickness of 1-30 microns.
摘要翻译：描述了用于制备耐磨性和耐候性优异的合成树脂成型制品的涂料组合物。该组合物包含（a）多官能单体混合物，其包含（i）25-75wt。％的至少一种式（I）的多官能单体：其中X11，X12，X13，X22，X23-Xn2，Xn3和X14中的至少三个是CH2 = CH。 C00-，其余基团为-OH，n为1-5的整数，（ii）25-75wt。％的至少一种式（II）的多官能单体：其中至少三个R基团是CH 2 = CH COO-，并且其中每一个是H或-OH， n1，n2，n3，n4，m1，m2，m3和m4为0,1或2的整数，X为1〜10的整数，（iii）0〜50重量％％的含有1个丙烯酰氧基的单体，沸点在常压下为至少150℃，粘度不高于20cps / 20℃，（b）0.01-6.0wt。基于100wt。部分多官能单体混合物，至少一种光敏剂。将涂料组合物涂布在合成树脂成型制品上，然后在空气中用紫外线照射，形成厚度为1-30微米的交联涂膜。

3. 发明授权

US4388345A Coating composition and process for preparing synthetic resin shaped articles by using same 失效
标题翻译：涂料组合物及其制备方法
公开(公告)号：US4388345A
公开(公告)日：1983-06-14
申请号：US343221
申请日：1982-01-27
申请人： Kazuo Kishida , Isao Sasaki , Kenji Kushi , Misao Tamura
发明人： Kazuo Kishida , Isao Sasaki , Kenji Kushi , Misao Tamura
IPC分类号： C09D5/00 , C08J7/04 , C08J7/16 , C09D4/00 , B05D3/06
CPC分类号： C08J7/16 , C09D4/00 , C08J2331/00 , Y10T428/31507
摘要： A shaped article of synthetic resins, such as polydiethylene glycol bisallylcarbonate, is coated with the following coating composition and then irradiated with ultraviolet rays, whereby the coating composition deposited on the shaped article is cured to form a coating film having an excellent abrasion resistance, surface smoothness, adhesion to the substrate resin, flexibility, heat resistance, solvent resistance and durability. The coating composition comprised of (a) a mixture of, based on the weight of the mixture, (i) 25-99.95 wt. % of at least one polyfunctional monomer having at least three acryloyloxy or methacryloyloxy groups, (ii) 0-50 wt. % of at least one mono- or bi-functional monomer having one or two polymerizable unsaturated groups and (iii) 0.05-25 wt. % of at least one organic acid which has at least one halogen substituent (fluorine, chlorine or bromine) and which is liquid at normal temperature and pressure, and (b) 0.01-10 wt. parts, based on 100 wt. parts of said mixture, of a photosensitizer. The coating composition may contain 0.05-25 wt. % of at least one compound having an acrylamide or methacrylamide group and a hydroxyl group or groups.
摘要翻译：合成树脂如聚二甘醇双烯丙基碳酸酯的成形制品用以下涂料组合物涂覆，然后用紫外线照射，由此沉积在成型制品上的涂料组合物固化以形成具有优异耐磨性，表面平滑性，与基材树脂的粘合性，柔软性，耐热性，耐溶剂性和耐久性。涂料组合物包含（a）基于混合物重量的混合物，（i）25-99.95wt。至少一种具有至少三个丙烯酰氧基或甲基丙烯酰氧基的多官能单体的％，（ii）0-50wt。％的至少一种具有一个或两个可聚合不饱和基团的单官能或双官能单体和（iii）0.05-25wt。至少一种具有至少一个卤素取代基（氟，氯或溴）并在常温常压下为液体的有机酸的％，和（b）0.01-10重量％基于100wt。所述混合物的一部分，光敏剂。涂料组合物可以含有0.05-25wt。％的至少一种具有丙烯酰胺或甲基丙烯酰胺基团和羟基或基团的化合物。

4. 发明授权

US4339474A Coating composition and process for preparing synthetic resin shaped articles by using same 失效
标题翻译：涂料组合物及其制备方法
公开(公告)号：US4339474A
公开(公告)日：1982-07-13
申请号：US239202
申请日：1981-03-03
申请人： Kazuo Kishida , Isao Sasaki , Kenji Kushi , Misao Tamura
发明人： Kazuo Kishida , Isao Sasaki , Kenji Kushi , Misao Tamura
IPC分类号： C08F2/48 , C09D4/06 , B05D3/06 , C08F8/00
CPC分类号： C09D4/06
摘要： A coating composition for the preparation of synthetic resin shaped articles excellent in abrasion resistance and weatherability is described. This composition comprises (a) a polyfunctional monomer composition comprising (i) 40-100 wt. % of a polyfunctional monomer containing at least three methacryloyloxy or acryloyloxy groups in the molecule and having a MW of not higher than about 900 and (ii) 0-60 wt. % of a mono- or bi-functional monomer having one or two methacryloyloxy or acryloyloxy groups in the molecule and having a MW of not higher than about 300 per methacryloyloxy or acryloyloxy group, (b) 5-35 parts by wt., based on 100 wt. parts of the monomer composition, of at least one ultraviolet absorber, (c) 0.5-8 wt. parts, based on 100 parts by wt. of the monomer composition, of at least one polymeric material selected from polymers of alkyl methacrylates and alkyl acrylates, and (d) 0.01-6 parts by wt., based on 100 parts by wt. of the monomer composition, of a photosensitizer. The coating composition is coated on a synthetic resin shaped article and then, irradiated with ultraviolet rays in an inert gas or air to form a crosslinked coating film having a thickness of 1 to 30 microns.
摘要翻译：描述了用于制备耐磨性和耐候性优异的合成树脂成型制品的涂料组合物。该组合物包含（a）多官能单体组合物，其包含（i）40-100wt。％的分子中含有至少三个甲基丙烯酰氧基或丙烯酰氧基并具有不高于约900的MW的多官能单体和（ii）0-60重量％％的分子中具有1个或2个甲基丙烯酰氧基或丙烯酰氧基的单功能或双官能单体，每个甲基丙烯酰氧基或丙烯酰氧基具有不高于约300的MW，（b）5-35重量份，基于 100重量单体组合物的部分，至少一种紫外线吸收剂，（c）0.5-8wt。部分，基于100重量份。至少一种选自甲基丙烯酸烷基酯和丙烯酸烷基酯的聚合物的聚合物材料，和（d）基于100重量份的重量比为0.01-6重量份。的单体组合物。将涂料组合物涂布在合成树脂成形制品上，然后在惰性气体或空气中用紫外线照射，形成厚度为1至30微米的交联涂膜。

5. 发明授权

US4460742A Delustered thermoplastic resin composition 失效
标题翻译：消光热塑性树脂组合物
公开(公告)号：US4460742A
公开(公告)日：1984-07-17
申请号：US324269
申请日：1981-11-23
申请人： Kazuo Kishida , Akira Hasegawa , Masahiro Sugimori
发明人： Kazuo Kishida , Akira Hasegawa , Masahiro Sugimori
IPC分类号： C08L101/00 , C08L1/00 , C08L7/00 , C08L21/00 , C08L23/00 , C08L23/06 , C08L25/14 , C08L27/00 , C08L27/06 , C08L33/00 , C08L33/02 , C08L33/06 , C08L33/08 , C08L33/10 , C08L51/00 , C08L51/02 , C08L55/02 , C08L67/00 , C08L77/00 , C08L33/04 , C08L51/06
CPC分类号： C08L33/08 , C08L23/06 , C08L27/06 , C08L33/10 , C08L55/02 , C08L25/14 , C08L33/06 , C08L51/003
摘要： A delustered thermoplastic resin composition which comprises 100 parts by weight of a thermoplastic resin (B); and 0.1 to 40 parts by weight of a resin (A) which essentially consists of:80 to 20 parts by weight of a polymer or a copolymer component (I) obtained by polymerizing;(a) 30 to 100% by weight of at least one monomer selected from the group consisting of an alkyl methacrylate in which the alkyl group has 1 to 4 carbon atoms and an aromatic vinyl compound;(b) 0 to 70% by weight of an alkyl acrylate in which the alkyl group has 1 to 13 carbon atoms;(c) 0 to 50% by weight of a monoethylenically unsaturated monomer other than those of (a) and (b); and(d) 0 to 5 parts by weight of a crosslinking monomer per 100 parts by weight of the total amount of the above components (a), (b), and (c); and 20 to 80 parts by weight of a copolymer component (II) obtained by polymerizing;(e) 30 to 90% by weight of an aromatic vinyl compound;(f) 10 to 60% by weight of at least one alkyl acrylate monomer in which the alkyl group has 1 to 13 carbon atoms;(g) 0 to 20% by weight of a monoethylenically unsaturated monomer other than those of (e) and (f); and(h) 0.05 to 10 parts by weight of a crosslinking monomer per 100 parts by weight of the total amount of the above components (e), (f) and (g).
摘要翻译：一种消光热塑性树脂组合物，其包含100重量份的热塑性树脂（B）; 和0.1〜40重量份的树脂（A），其基本上由以下组成：通过聚合得到的聚合物或共聚物成分（I）为80〜20重量份; （a）30〜100重量％的至少一种选自甲基丙烯酸烷基酯中具有1〜4个碳原子的烷基和芳香族乙烯基化合物的单体; （b）0〜70重量％的烷基具有1〜13个碳原子的丙烯酸烷基酯; （c）0至50重量％的除（a）和（b）之外的单烯属不饱和单体; 和（d）每100重量份上述组分（a），（b）和（c）的总量为0-5重量份的交联单体; 和20〜80重量份通过聚合得到的共聚物组分（II）; （e）30〜90重量％的芳族乙烯基化合物; （f）10至60重量％的至少一种烷基丙烯酸酯单体，其中烷基具有1至13个碳原子; （g）除（e）和（f）以外的单烯属不饱和单体0〜20重量％（e），（f）和（g）的总量相对于100重量份的交联单体为0.05〜10重量份。

6. 发明授权

US4508875A Multi-layer structure polymer composition 失效
标题翻译：多层结构聚合物组成
公开(公告)号：US4508875A
公开(公告)日：1985-04-02
申请号：US526546
申请日：1983-08-26
申请人： Kazuo Kishida , Akira Hasegawa , Masahiro Sugimori
发明人： Kazuo Kishida , Akira Hasegawa , Masahiro Sugimori
IPC分类号： C08F265/04 , C08F285/00 , C08F265/06
CPC分类号： C08F265/04 , C08F285/00 , C08L33/10 , C08L67/00 , C08L69/00 , C08L77/00 , C08F220/14 , C08L51/06 , Y10S525/902
摘要： A multi-layer structure polymer composition having a gel content of at least 50% which is constituted of an innermost layer polymer (A) consisting mainly of alkyl acrylate and having a degree of swelling of 10 or lower, and having a glass transition temperature lower than 10.degree. C., a crosslinked elastomer polymer (B) consisting mainly of alkyl acrylate and having a degree of swelling slightly higher than that of said polymer (A) and having a glass transition temperature not higher than 0.degree. C., said innermost layer polymer (A) and said crosslinked elastomer polymer (B) constituting a double layer elastomer structure polymer, as well as an outermost layer polymer (C) consisting mainly of alkyl methacrylate and having a glass transition temperature not lower than 60.degree. C., and at least one intermediate layer (D) existing between said polymer (B) layer and said polymer (C) layer, the amount of alkyl acrylate in said intermediate layer (D) linearly decreasing from said polymer (B) layer to said polymer (C) layer. Said polymer composition does not readily show the phenomenon of whitening even if dipped in hot water or boiling water and is excellent in weather resistance, solvent resistance, stress-whitening resistance, water-whitening resistance and transparency.
摘要翻译：一种凝胶含量为至少50％的多层结构聚合物组合物，其由主要由丙烯酸烷基酯组成并具有10或更低的膨胀度并且玻璃化转变温度较低的最内层聚合物（A）所述最内层的玻璃化转变温度不高于10℃的交联弹性体聚合物（B），其主要由丙烯酸烷基酯组成，其膨胀度略高于所述聚合物（A）层叠聚合物（A）和构成双层弹性体结构聚合物的所述交联弹性体聚合物（B）以及主要由甲基丙烯酸烷基酯组成并且玻璃化转变温度不低于60℃的最外层聚合物（C）和存在于所述聚合物（B）层和所述聚合物（C）层之间的至少一个中间层（D），所述中间层（D）中的丙烯酸烷基酯的量从所述聚合物（B）层线性减小到所述聚合物（C）层。所述聚合物组合物即使浸渍在热水或沸水中也不容易显示白化现象，并且耐候性，耐溶剂性，耐应力白化性，耐水白色性和透明性优异。

7. 发明授权

US4464513A Delustered thermoplastic resin composition 失效
标题翻译：消光热塑性树脂组合物
公开(公告)号：US4464513A
公开(公告)日：1984-08-07
申请号：US400619
申请日：1982-07-22
申请人： Kazuo Kishida , Akira Hasegawa , Masahiro Sugimori
发明人： Kazuo Kishida , Akira Hasegawa , Masahiro Sugimori
IPC分类号： C08L25/00 , C08L1/00 , C08L7/00 , C08L21/00 , C08L23/00 , C08L23/06 , C08L25/04 , C08L25/14 , C08L27/00 , C08L27/06 , C08L33/00 , C08L33/02 , C08L33/06 , C08L51/00 , C08L51/02 , C08L51/04 , C08L55/02 , C08L67/00 , C08L75/04 , C08L77/00 , C08L101/00
CPC分类号： C08L55/02 , C08L101/00 , C08L23/06 , C08L25/04 , C08L27/06 , C08L33/06 , C08L51/04 , C08L75/04 , C08L2205/02 , C08L2205/22
摘要： A delustered thermoplastic resin composition obtained by incorporating in 100 parts by weight of a thermoplastic resin up to 40 parts by weight of a cross-linked polymer having an average particle diameter of 35-500.mu. which polymer is obtained by suspension-polymerizing a non-crosslinking monomer composition comprising 50-70 wt. % of a vinyl aromatic monomer, 10-40 wt. % of at least one monomer selected from the group consisting of alkyl acrylates having 1-13 carbon atoms in the alkyl group, 10-40 wt. % of a monomer selected from alkyl methacrylates having 1-4 carbon atoms in the alkyl group and 0-40 wt. % of another monoethylenically unsaturated monomer with 0.5-5 parts by weight, per 100 parts by weight of the non-cross-linking monomer composition, of a cross-linking monomer having at least two double bonds in the molecule.
摘要翻译：一种消光热塑性树脂组合物，其通过在100重量份的热塑性树脂中加入最多40重量份的平均粒径为35-500μm的交联聚合物，该聚合物通过将非聚合物悬浮聚合而获得，交联单体组合物，其包含50-70wt。％的乙烯基芳族单体，10-40wt。％的至少一种选自烷基中具有1-13个碳原子的丙烯酸烷基酯的单体，10-40wt。选自烷基中具有1-4个碳原子的甲基丙烯酸烷基酯的单体的％和0-40重量％％的另一种单烯属不饱和单体，相对于每100重量份的非交联单体组合物，分子中具有至少两个双键的交联单体为0.5-5重量份。

8. 发明授权

US4452941A Thermoplastic acrylic resin composition 失效
标题翻译：热塑性丙烯酸树脂组合物
公开(公告)号：US4452941A
公开(公告)日：1984-06-05
申请号：US500571
申请日：1983-06-02
申请人： Kazuo Kishida , Akira Hasegawa , Masahiro Sugimori
发明人： Kazuo Kishida , Akira Hasegawa , Masahiro Sugimori
IPC分类号： C08F265/06 , C08F285/00 , C08L51/00 , C08L51/06
CPC分类号： C08F285/00 , C08F265/06 , C08L51/003
摘要： A novel acrylic thermoplastic resin composition, transparent and excellent in flexibility, consisting of at least two different multi-layer structure polymers. Polymer [I] contains an inner layer of crosslinked acrylic elastomer and an outer layer of acrylic resin, wherein the amount of elastomeric inner layer is minor in comparison with the amount of the resin outer layer; polymer [II] has the same fundamental polymer structure as multi-layer structure polymer [I] except that the amount of crosslinked elastomer inner layer is a major amount as compared to the amount of resin outer layer. It is preferred that an intermediate layer having an intermediate property exist between the inner and outer layers of the multi-layer structure polymers.
摘要翻译：一种由至少两种不同的多层结构聚合物组成的透明且柔软性优异的丙烯酸类热塑性树脂组合物。聚合物[I]含有交联的丙烯酸弹性体的内层和丙烯酸树脂的外层，其中弹性体内层的量与树脂外层的量相比较小; 聚合物[II]与多层结构聚合物[I]具有相同的基本聚合物结构，除了与树脂外层的量相比，交联的弹性体内层的量是主要量。优选在多层结构聚合物的内层和外层之间存在具有中等特性的中间层。

9. 发明授权

US4720516A Composite material with improved properties 失效
标题翻译：具有改善性能的复合材料
公开(公告)号：US4720516A
公开(公告)日：1988-01-19
申请号：US450378
申请日：1982-12-16
申请人： Kazuo Kishida , Isao Sasaki , Hiroshi Mori , Yasuaki Ii
发明人： Kazuo Kishida , Isao Sasaki , Hiroshi Mori , Yasuaki Ii
IPC分类号： C08L23/26 , C08G18/62 , C08K3/00 , C08K5/17 , C08K5/29 , C08K7/00 , C08K7/02 , C08L7/00 , C08L21/00 , C08L23/00 , C08L51/00 , C08L51/02 , C08L51/06 , C08L77/00 , C08L77/10 , C08L101/00 , C08K7/06 , C08K7/22
CPC分类号： C08G18/6204 , C08L51/06
摘要： A polyolefin resin composition comprising a polyolefin modified with an unsaturated carboxylic acid, at least one member selected from the group consisting of polyepoxides, polyisocyanates, and polyamines, and a reinforcement.
摘要翻译：一种聚烯烃树脂组合物，其包含用不饱和羧酸改性的聚烯烃，选自聚环氧化物，多异氰酸酯和多胺中的至少一种，以及增强剂。

10. 发明授权

US4504608A Flame retardant polyester resin compositions 失效
标题翻译：阻燃聚酯树脂组合物
公开(公告)号：US4504608A
公开(公告)日：1985-03-12
申请号：US461228
申请日：1983-01-26
申请人： Kazuo Kishida , Isao Sasaki , Hiroshi Mori
发明人： Kazuo Kishida , Isao Sasaki , Hiroshi Mori
IPC分类号： C08L67/00 , C08G59/00 , C08K3/00 , C08K3/22 , C08K5/3492 , C08K5/3495 , C08L63/00 , C08L67/02 , C08L63/02
CPC分类号： C08K5/34924
摘要： Flame retardant reinforced with polyester resin compositions are disclosed glass fiber and a system of flame retardants represented by the following general formulas (I) and (II), together with antimony trioxide. The flame retardant system is a blend of 1-20 parts by weight of component (I), and 2-30 parts by weight of component (II), provided the weight ratio (I)/(II) of the flame retardant component (I) to (II) is in the range of 0.2
摘要翻译：公开了用聚酯树脂组合物增强的阻燃剂，由下列通式（I）和（II）表示的玻璃纤维和阻燃剂体系以及三氧化锑。阻燃剂体系是1-20重量份组分（I）和2-30重量份组分（II）的混合物，只要阻燃组分的重量比（I）/（II） I）至（II）在0.2 <（I）/（II）<4的范围内，阻燃剂（I）+（II）的总量在3-40重量份的范围内。存在2至30重量份的三氧化锑，并且还存在5至60重量％的玻璃纤维，这两个百分比基于总树脂组合物的重量来表示。树脂组合物除了是阻燃剂外还具有出色的机械，热性能和成型性。其中X是氢，氯或溴，m的平均值为0至11，n的平均值为0至7，卤素含量为10重量％以上。 R1和R2的值在附件说明书中给出。

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