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1. 发明授权

US08536084B2 Photocatalyst material, method for decomposition of organic material, interior member, air purification device, and apparatus for preparation of oxidizing agent 有权
标题翻译：光催化剂材料，有机材料分解方法，内部构件，空气净化装置以及氧化剂的制备装置
公开(公告)号：US08536084B2
公开(公告)日：2013-09-17
申请号：US12736209
申请日：2009-03-19
申请人： Kazuhito Hashimoto , Hiroshi Irie , Syuhei Miura , Kazuhide Kamiya , Shinichiro Miki , Koichi Takahama , Mitsuo Yaguchi
发明人： Kazuhito Hashimoto , Hiroshi Irie , Syuhei Miura , Kazuhide Kamiya , Shinichiro Miki , Koichi Takahama , Mitsuo Yaguchi
IPC分类号： B01J23/888 , A61L2/08 , B32B19/00
CPC分类号： A61L9/18 , A61L9/205 , B01J23/72 , B01J23/888 , B01J35/004 , B01J37/0072 , B01J37/009 , B01J37/0211 , B01J37/0234 , B01J37/04
摘要： The present invention provides a tungsten trioxide microparticle carrying on its surface divalent copper salt. The divalent copper salt is utilized to perform a multi-electron reduction of oxygen. The tungsten trioxide exhibits a high oxidative decomposition activity when exposed to visible light.
摘要翻译：本发明提供了在其表面上具有二价铜盐的三氧化钨微粒。二价铜盐用于进行氧的多电子还原。当暴露于可见光时，三氧化钨显示出高的氧化分解活性。

2. 发明申请

US20110005916A1 PHOTOCATALYST MATERIAL, METHOD FOR DECOMPOSITION OF ORGANIC MATERIAL, INTERIOR MEMBER, AIR PURIFICATION DEVICE, AND APPARATUS FOR PREPARATION OF OXIDIZING AGENT 有权
标题翻译：光催化材料，有机材料分解方法，室内成员，空气净化装置及制备氧化剂的装置
公开(公告)号：US20110005916A1
公开(公告)日：2011-01-13
申请号：US12736209
申请日：2009-03-19
申请人： Kazuhito Hashimoto , Hiroshi Irie , Syuhei Miura , Kazuhide Kamiya , Shinichiro Miki , Koichi Takahama , Mitsuo Yaguchi
发明人： Kazuhito Hashimoto , Hiroshi Irie , Syuhei Miura , Kazuhide Kamiya , Shinichiro Miki , Koichi Takahama , Mitsuo Yaguchi
IPC分类号： C07B37/06 , B01J23/888
CPC分类号： A61L9/18 , A61L9/205 , B01J23/72 , B01J23/888 , B01J35/004 , B01J37/0072 , B01J37/009 , B01J37/0211 , B01J37/0234 , B01J37/04
摘要： The present invention provides a tungsten trioxide microparticle carrying on its surface divalent copper salt. The divalent copper salt is utilized to perform a multi-electron reduction of oxygen. The tungsten trioxide exhibits a high oxidative decomposition activity when exposed to visible light.
摘要翻译：本发明提供了在其表面上具有二价铜盐的三氧化钨微粒。二价铜盐用于进行氧的多电子还原。当暴露于可见光时，三氧化钨显示出高的氧化分解活性。

3. 发明申请

US20110198210A1 PHOTOCATALYTIC MATERIAL, METHOD OF DECOMPOSING ORGANIC SUBSTANCE, INTERIOR MEMBER, AIR CLEANING DEVICE, AND DEVICE FOR PRODUCING OXIDIZING AGENT 失效
标题翻译：光化学材料，分解有机物质的方法，室内成员，空气净化装置和用于生产氧化剂的装置
公开(公告)号：US20110198210A1
公开(公告)日：2011-08-18
申请号：US13124669
申请日：2009-10-29
申请人： Kazuhito Hashimoto , Hiroshi Irie , Huogen Yu , Kazuhide Kamiya , Koichi Takahama , Shinichiro Miki , Mitsuo Yaguchi
发明人： Kazuhito Hashimoto , Hiroshi Irie , Huogen Yu , Kazuhide Kamiya , Koichi Takahama , Shinichiro Miki , Mitsuo Yaguchi
IPC分类号： B01J19/08 , B01J23/72 , B01J23/745 , B01J21/06
CPC分类号： B01J35/004 , A61L9/205 , B01J21/063 , B01J23/72 , B01J23/745 , B01J23/83
摘要： A divalent copper salt and/or trivalent iron salt is supported on a surface of a metal ion-doped titanium oxide obtained by doping titanium oxide with metal ions to give a metal ion-doped titanium oxide with a valence band potential of 3 V or more (vs. SHE, pH=0) and a bandgap of 3 V or less between the valence band and an energy level of electrons excited from the valence band (including conduction band minimum potential and isolated potential). The metal ion-doped titanium oxide can be made to exhibit strong oxidative decomposition activity when irradiated with visible light based on the fact the divalent copper salt or trivalent iron salt functions as a catalyst for multi-electron reduction of oxygen.
摘要翻译：二价铜盐和/或三价铁盐负载在通过用金属离子掺杂二氧化钛而获得的金属离子掺杂的氧化钛的表面上，得到价带电位为3V或更高的金属离子掺杂的氧化钛（与SHE，pH = 0）和价带之间的3V或更小的带隙与从价带激发的电子的能级（包括导带最小电位和隔离电位）之间的带隙。基于二价铜盐或三价铁盐作为多电子还原氧的催化剂的事实，可以使金属离子掺杂的氧化钛在用可见光照射时表现出强的氧化分解活性。

4. 发明授权

US08603302B2 Photocatalytic material, method of decomposing organic substance, interior member, air cleaning device, and device for producing oxidizing agent 失效
标题翻译：光催化材料，分解有机物的方法，内部构件，空气净化装置以及用于生产氧化剂的装置
公开(公告)号：US08603302B2
公开(公告)日：2013-12-10
申请号：US13124669
申请日：2009-10-29
申请人： Kazuhito Hashimoto , Hiroshi Irie , Huogen Yu , Kazuhide Kamiya , Koichi Takahama , Shinichiro Miki , Mitsuo Yaguchi
发明人： Kazuhito Hashimoto , Hiroshi Irie , Huogen Yu , Kazuhide Kamiya , Koichi Takahama , Shinichiro Miki , Mitsuo Yaguchi
IPC分类号： C07C1/00 , C07C2/00 , C07C4/00 , C07C5/00 , C07C6/00 , B01J23/70 , B01J23/72 , B01J23/00 , A62B7/08 , C09D1/00
CPC分类号： B01J35/004 , A61L9/205 , B01J21/063 , B01J23/72 , B01J23/745 , B01J23/83
摘要： A divalent copper salt and/or trivalent iron salt is supported on a surface of a metal ion-doped titanium oxide obtained by doping titanium oxide with metal ions to give a metal ion-doped titanium oxide with a valence band potential of 3 V or more (vs. SHE, pH=0) and a bandgap of 3 V or less between the valence band and an energy level of electrons excited from the valence band (including conduction band minimum potential and isolated potential). The metal ion-doped titanium oxide can be made to exhibit strong oxidative decomposition activity when irradiated with visible light based on the fact the divalent copper salt or trivalent iron salt functions as a catalyst for multi-electron reduction of oxygen.
摘要翻译：二价铜盐和/或三价铁盐负载在通过用金属离子掺杂二氧化钛而获得的金属离子掺杂的氧化钛的表面上，得到价带电位为3V或更高的金属离子掺杂的氧化钛（与SHE，pH = 0）和价带之间的3V或更小的带隙与从价带激发的电子的能级（包括导带最小电位和隔离电位）之间的带隙。基于二价铜盐或三价铁盐作为多电子还原氧的催化剂的事实，可以使金属离子掺杂的氧化钛在用可见光照射时表现出强的氧化分解活性。

5. 发明申请

US20120237396A1 VISIBLE LIGHT-RESPONSIVE PHOTOCATALYST COATING MATERIAL, COATED ARTICLE, ALLERGEN INACTIVATION METHOD 有权
标题翻译：可见光反应性光催化涂层材料，涂层制品，过敏灭活方法
公开(公告)号：US20120237396A1
公开(公告)日：2012-09-20
申请号：US13512379
申请日：2010-08-26
申请人： Shinichiro Miki , Koichi Takahama , Kensaku Kinugawa , Kazuhito Hashimoto , Kayano Sunada
发明人： Shinichiro Miki , Koichi Takahama , Kensaku Kinugawa , Kazuhito Hashimoto , Kayano Sunada
IPC分类号： B01J31/26 , B01J31/38 , B01J31/34 , A61L2/23
CPC分类号： B01J35/004 , A61L2/0076 , A61L9/205 , B01J21/063 , B01J23/72 , B01J23/888 , B01J37/038 , C08K3/22 , C08K5/5415 , C08K5/5419 , C08K9/02 , C09D5/1618 , C09D7/62 , C09D183/04
摘要： Object of the present invention is to provide visible light-responsive photocatalyst coating material which can form a coating film exhibiting superior allergen inactivation property through irradiation of visible light. The visible light-responsive photocatalyst coating material comprises: photocatalyst material having visible light-activity composed of metal oxide particle with divalent copper salt supported on the surface thereof, said metal oxide particle having optical semiconductor-characteristics and potential of valence band of said metal oxide particle being 3[V] or more (vs. SHE, pH=0); binder component including component having siloxane bond or component forming siloxane bond through reaction; and chloride ionic compound. When visible light is irradiated to the coating film, the metal oxide particle exhibits photocatalyst activity in the presence of the copper-divalent ion and chloride ion, thereby significantly high allergen inactivation property is exhibited. Additionally, it can prevent the separation of the photocatalyst coating material from the coating film.
摘要翻译：本发明的目的是提供可见光响应光催化剂涂料，其可以通过照射可见光而形成显示出优异的变应原灭活性能的涂膜。可见光响应光催化剂涂料包括：具有由其表面上负载有二价铜盐的金属氧化物颗粒组成的可见光活性的光催化剂材料，所述金属氧化物颗粒具有光学半导体特性和所述金属氧化物的价带电位颗粒为3 [V]以上（相对于SHE，pH = 0）; 粘合剂组分包括具有硅氧烷键或通过反应形成硅氧烷键的组分的组分; 和氯离子化合物。当可见光被照射到涂膜时，金属氧化物颗粒在铜 - 二价离子和氯离子的存在下显示出光催化活性，从而显示出高的变应原灭活性能。另外，可以防止光催化剂涂料与涂膜分离。

6. 发明授权

US09138734B2 Visible light-responsive photocatalyst coating material, coated article, allergen inactivation method 有权
标题翻译：可见光响应光催化剂涂层材料，涂层制品，过敏原灭活方法
公开(公告)号：US09138734B2
公开(公告)日：2015-09-22
申请号：US13512379
申请日：2010-08-26
申请人： Shinichiro Miki , Koichi Takahama , Kensaku Kinugawa , Kazuhito Hashimoto , Kayano Sunada
发明人： Shinichiro Miki , Koichi Takahama , Kensaku Kinugawa , Kazuhito Hashimoto , Kayano Sunada
IPC分类号： C09D183/04 , C09D7/12 , C09D5/16 , B01J35/02 , B01J37/02 , B01J35/00 , B01J21/06 , B01J23/72 , B01J23/888 , B01J37/03 , A61L9/20 , A61L2/00 , C08K3/22 , C08K5/5415 , C08K5/5419 , C08K9/02
CPC分类号： B01J35/004 , A61L2/0076 , A61L9/205 , B01J21/063 , B01J23/72 , B01J23/888 , B01J37/038 , C08K3/22 , C08K5/5415 , C08K5/5419 , C08K9/02 , C09D5/1618 , C09D7/62 , C09D183/04
摘要： Object of the present invention is to provide visible light-responsive photocatalyst coating material which can form a coating film exhibiting superior allergen inactivation property through irradiation of visible light. The visible light-responsive photocatalyst coating material comprises: photocatalyst material having visible light-activity composed of metal oxide particle with divalent copper salt supported on the surface thereof, said metal oxide particle having optical semiconductor-characteristics and potential of valence band of said metal oxide particle being 3[V] or more (vs. SHE, pH=0); binder component including component having siloxane bond or component forming siloxane bond through reaction; and chloride ionic compound. When visible light is irradiated to the coating film, the metal oxide particle exhibits photocatalyst activity in the presence of the copper-divalent ion and chloride ion, thereby significantly high allergen inactivation property is exhibited. Additionally, it can prevent the separation of the photocatalyst coating material from the coating film.
摘要翻译：本发明的目的是提供可见光响应光催化剂涂料，其可以通过照射可见光而形成显示出优异的变应原灭活性能的涂膜。可见光响应光催化剂涂料包括：具有由其表面上负载有二价铜盐的金属氧化物颗粒组成的可见光活性的光催化剂材料，所述金属氧化物颗粒具有光学半导体特性和所述金属氧化物的价带电位颗粒为3 [V]以上（相对于SHE，pH = 0）; 粘合剂组分包括具有硅氧烷键或通过反应形成硅氧烷键的组分的组分; 和氯离子化合物。当可见光被照射到涂膜时，金属氧化物颗粒在铜 - 二价离子和氯离子的存在下显示出光催化活性，从而显示出高的变应原灭活性能。另外，可以防止光催化剂涂料与涂膜分离。

7. 发明授权

US5811192A Titanium dioxide film having photocatalytic activity and substrate having the same 失效
标题翻译：具有光催化活性的二氧化钛膜和具有该催化活性的基材
公开(公告)号：US5811192A
公开(公告)日：1998-09-22
申请号：US713845
申请日：1996-09-12
申请人： Koichi Takahama , Hirotsugu Kishimoto , Takaharu Nakagawa , Shigehito Deki , Noboru Hashimoto
发明人： Koichi Takahama , Hirotsugu Kishimoto , Takaharu Nakagawa , Shigehito Deki , Noboru Hashimoto
IPC分类号： B01J35/00 , C01G23/053 , C03C17/25 , C03C25/42 , B32B15/04
CPC分类号： B01J35/004 , B01J35/002 , C01G23/053 , C03C17/256 , C03C25/42 , C03C2217/212 , C03C2217/71 , C03C2218/11
摘要： There is provided a substrate of which the surface is coated with a titanium dioxide film having a photocatalytic activity, which substrate is obtained by: depositing titanium dioxide in a film form on a surface of a substrate by contacting the substrate with a reaction solution containing ammonium titanium fluoride, water and an additive which shifts the following equilibrium reaction: (NH.sub.4).sub.2 TiF.sub.6 +2H.sub.2 O TiO.sub.2 +4HF+2NH.sub.4 F toward a right side, and calcining the deposited titanium dioxide film.
摘要翻译：提供了一种基材，其表面涂覆有具有光催化活性的二氧化钛膜，该基材通过以下方式获得：通过使底物与含有铵的反应溶液接触将沉积的二氧化钛以薄膜形式沉积在基材的表面上氟化钛，水和添加剂，将下列平衡反应：（NH4）2TiF6 + 2H2O <=> TiO2 + 4HF + 2NH4F向右侧移动，煅烧沉积的二氧化钛膜。

8. 发明授权

US07582351B2 Composite thin film holding substrate, transparent conductive film holding substrate, and panel light emitting body 有权
标题翻译：复合薄膜保持基板，透明导电膜保持基板和面板发光体
公开(公告)号：US07582351B2
公开(公告)日：2009-09-01
申请号：US10492534
申请日：2002-10-24
申请人： Hiroshi Yokogawa , Masaru Yokoyama , Kenji Kawano , Norihiro Itou , Koichi Takahama , Takeyuki Yamaki , Akira Tsujimoto , Yasuhisa Kishigami , Nobuhiro Ide
发明人： Hiroshi Yokogawa , Masaru Yokoyama , Kenji Kawano , Norihiro Itou , Koichi Takahama , Takeyuki Yamaki , Akira Tsujimoto , Yasuhisa Kishigami , Nobuhiro Ide
IPC分类号： B32B7/02 , B32B5/16 , H05B33/12
CPC分类号： G02B1/10 , C08K3/36 , C08K7/22 , C08L2205/20 , C09D7/70 , G02B1/11 , G02B5/0236 , G02B5/0242 , G02B5/0247 , G02B5/0278 , H01J5/16 , H01J2211/44 , H01L51/0096 , H01L51/5268 , Y02E10/549 , Y10T428/24942 , Y10T428/25 , Y10T428/259 , Y10T428/265 , Y10T428/31663
摘要： There is provided a composite thin film-holding substrate in which a composite thin film (4) comprising a filler (2) having a refractive index lower than that of a substrate (1) and a binder (3) having a refractive index higher than that of the filler (2) is formed on a surface of the substrate (1). Light is efficiently scattered when passing through the composite thin film (3) which comprises the filler (2) and the binder (3) having different refractive indexes from each other. In addition, the refractive index of a composite thin film (4) comprising a filler (2) having a low refractive index is low. As a result, the discharge efficiency of light which passes through the composite thin film (4) from the substrate (1) to the external is improved.
摘要翻译：提供一种复合薄膜保持基板，其中复合薄膜（4）包括折射率低于基板（1）的折射率的填料（2）和折射率高于填料（2）的表面形成在基材（1）的表面上。当通过包含彼此具有不同折射率的填料（2）和粘合剂（3）的复合薄膜（3）时，光被有效地分散。此外，包含低折射率的填料（2）的复合薄膜（4）的折射率低。结果，提高了通过复合薄膜（4）从基板（1）到外部的光的放电效率。

9. 发明授权

US06303229B2 Hydrophilic inorganic coating film and composition made from alkoxysilane and silica 失效
标题翻译：亲水性无机涂膜和由烷氧基硅烷和二氧化硅制成的组合物
公开(公告)号：US06303229B2
公开(公告)日：2001-10-16
申请号：US09445350
申请日：1999-12-08
申请人： Koichi Takahama , Minoru Inoue , Junko Ikenaga , Shoichi Nakamoto
发明人： Koichi Takahama , Minoru Inoue , Junko Ikenaga , Shoichi Nakamoto
IPC分类号： B32B904
CPC分类号： C09D183/02 , Y10T428/31663
摘要： The present invention provides a process for forming a hydrophilic inorganic coated film on a surface of a base material, the process comprising the steps of: (1) preparing an inorganic coating composition which contains, as a major component, a silicone resin obtained by hydrolyzing and condensation-polymerizing only the tetra-functional alkoxysilane represented by the formula: Si(OR)4 [wherein R represents an alkyl group having carbon atoms up to and including 7 or an aryl group], and has a total solid content of not more than 5% by weight; (2) applying the inorganic coating composition to a surface of the base material to form a coated layer; and (3) drying and curing the coated layer to form a cured coated film having a thickness of 0.01 to 0.5 &mgr;m. The hydrophilic inorganic coated film formed by the process of the present invention is highly hydrophilic just after the film is formed, even in the case that it is not irradiated with ultraviolet rays.
摘要翻译：本发明提供了在基材表面形成亲水性无机涂膜的方法，该方法包括以下步骤：（1）制备一种无机涂料组合物，其中以无机涂料组合物为主要成分，并且仅使由式（Si）（OR）4表示的四官能烷氧基硅烷进行缩聚：[其中，R表示碳原子数为7以上的烷基或芳基]，总固体成分不多超过5％重量; （2）将无机涂料组合物涂布在基材的表面上以形成涂层; 和（3）干燥和固化涂层以形成厚度为0.01至0.5μm的固化涂膜。通过本发明的方法形成的亲水性无机涂膜即使在没有用紫外线照射的情况下，在形成膜之后即具有高亲水性。

10. 发明授权

US5364823A Method for manufacturing inorganic porous layered member 失效
标题翻译：无机多孔层叠体的制造方法
公开(公告)号：US5364823A
公开(公告)日：1994-11-15
申请号：US93496
申请日：1987-07-17
申请人： Koichi Takahama , Shozo Hirao , Masaru Yokoyama , Takashi Kishimoto , Hiroshi Yokokawa
发明人： Koichi Takahama , Shozo Hirao , Masaru Yokoyama , Takashi Kishimoto , Hiroshi Yokokawa
IPC分类号： C04B35/14 , C04B14/20 , C04B38/00 , B01J21/16 , B01J20/12
CPC分类号： C04B14/206
摘要： This invention relates to a method for manufacturing an inorganic porous layered member which can maintain a sufficient distance between layers to show a high degree of heat insulating properties. In the manufacturing method for the inorganic porous layered member according to the present invention, an inorganic layered compound 12 having swelling charecteristics is swelled, and an inorganic pillar and an organic pillar are intercalated to form inorganic compound 16 between layers 14 of the inorganic layered compound 12. Fine gaps are thus formed in a wide range by the intercalation of the inorganic compound 16 between the layers 14 to maintain a sufficient distance between the layers 14, and the inorganic porous layered member 10 having high heat insulating properties is thus produced.
摘要翻译： PCT No.PCT / JP87 / 00317 Sec。 371日期1987年7月17日 102（e）1987年7月17日PCT PCT 1987年5月19日PCT公布。出版物WO88 / 02356 日本公开日1988年7月4日。本发明涉及一种无机多孔层状部件的制造方法，其能够在层间保持足够的距离以显示出高绝热性。在本发明的无机多孔层叠体的制造方法中，具有溶胀性的无机层状化合物12膨胀，并且插入无机柱和有机柱，以在无机层状化合物的层14之间形成无机化合物16 因此，通过层14之间的无机化合物16的插入，在宽范围内形成微细的间隙，以保持层14之间的足够的距离，从而制得具有高绝热性的无机多孔层叠体10。

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