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1. 发明授权

US4766155A Process for producing alcohols 失效
标题翻译：醇的制备方法
公开(公告)号：US4766155A
公开(公告)日：1988-08-23
申请号：US805395
申请日：1985-12-04
申请人： Jui-Yuan Sun , Erek J. Erekson
发明人： Jui-Yuan Sun , Erek J. Erekson
IPC分类号： C07C29/156 , C07C29/157 , C07C27/06
CPC分类号： C07C29/156 , C07C29/157
摘要： A process for producing alcohols by reacting carbon monoxide with hydrogen in the presence of a catalyst comprising (a) copper; (b) zinc; (c) at least one element selected from the group consisting of iron, cobalt, nickel, ruthenium, thorium and mixtures thereof; and (d) at least one element selected from the group consisting of alkali metals, alkaline earth metals and mixtures thereof.
摘要翻译：一种在催化剂存在下使一氧化碳与氢气反应生产醇的方法，包括：（a）铜; （b）锌; （c）选自铁，钴，镍，钌，钍及其混合物中的至少一种元素; 和（d）选自碱金属，碱土金属及其混合物中的至少一种元素。

2. 发明授权

US5204308A Anionicaly stabilized lithium catalysts and a method for stabilizing the lithium catalyst 失效
标题翻译：阴离子稳定的锂催化剂和稳定锂催化剂的方法
公开(公告)号：US5204308A
公开(公告)日：1993-04-20
申请号：US681958
申请日：1991-04-08
申请人： Anthony L. Lee , Erek J. Erekson , James T. Semrau , S. Peter Barone , Irving J. Solomon
发明人： Anthony L. Lee , Erek J. Erekson , James T. Semrau , S. Peter Barone , Irving J. Solomon
IPC分类号： B01J23/04 , B01J27/055 , B01J27/18 , C07C2/84
CPC分类号： B01J23/04 , B01J27/055 , B01J27/1806 , C07C2/84 , C07C2521/10 , C07C2527/167
摘要： An anionically stabilized lithium catalyst wherein the anion is sulfate, phosphate, aluminate, silicate and mixtures thereof. The anionically stabilized lithium catalyst may be supported on a metal oxide support of magnesium oxide, titanium oxide, zinc oxide, calcium oxide, barium oxide, strontium oxide, zirconium oxide, hafnium oxide, yttrium oxide, lanthanum oxide, samarium oxide, and mixtures thereof or when aluminate or silicate is used as the anion the aluminate or silicate may act as the support. The catalyst may be used to promote reactions at temperatures higher than prior lithium catalysts, particularly higher than about 600.degree. C., such as oxidative coupling of aliphatic and alicyclic hydrocarbons to produce higher molecular weight compounds and oxydehydrogenation of aliphatic and alicyclic hydrocarbons to produce unsaturated hydrocarbons or to change the functional group of the hydrocarbon.
摘要翻译：阴离子稳定的锂催化剂，其中阴离子是硫酸盐，磷酸盐，铝酸盐，硅酸盐及其混合物。阴离子稳定的锂催化剂可以负载在氧化镁，氧化钛，氧化锌，氧化钙，氧化钡，氧化锶，氧化锆，氧化铪，氧化钇，氧化镧，氧化钐及其混合物的金属氧化物载体上或者当使用铝酸盐或硅酸盐作为阴离子时，铝酸盐或硅酸盐可以用作载体。催化剂可用于在高于先前的锂催化剂的温度下促进反应，特别是高于约600℃，例如脂族和脂环族烃的氧化偶联以产生较高分子量的化合物，以及脂族和脂环族烃的氧化脱氢产生不饱和的烃或改变烃的官能团。

3. 发明授权

US4945078A Mixed basic metal sulfide catalyst 失效
标题翻译：混合碱性金属硫化物催化剂
公开(公告)号：US4945078A
公开(公告)日：1990-07-31
申请号：US359207
申请日：1989-05-31
申请人： Erek J. Erekson , Anthony L. Lee , S. Peter Barone , Irvine J. Solomon
发明人： Erek J. Erekson , Anthony L. Lee , S. Peter Barone , Irvine J. Solomon
IPC分类号： B01J23/00 , B01J23/02 , B01J23/06 , C07C2/84 , C07C5/333
CPC分类号： C07C2/84 , B01J23/00 , B01J23/02 , B01J23/06 , C07C5/3332 , C07C2521/02 , C07C2521/10 , C07C2523/02 , C07C2523/04 , C07C2523/06 , C07C2523/10 , C07C2523/12 , C07C2527/04
摘要： A mixed basic metal sulfide catalyst having the formula:xA.yB.zC.qSwherein A is an alkali metal selected from lithium, sodium, potassium, rubidium, cesium and mixtures thereof; B is a cation which has an ionization state 1 greater than the ionization state of C; B is selected from scandium, yttrium, lanthanum, actinium, aluminum, boron and mixtures thereof when C is selected from beryllium, magnesium, calcium, strontium, barium, radium, zinc, cadmium, mercury and mixtures thereof and B is selected from titanium, zirconium, hafnium, silicon and mixtures thereof when C is selected from scandium, yttrium, lanthanum, actinium, aluminum, boron and mixtures thereof; x and y are in mole fractions of z such that when z=1 then x=0.001 to 0.25, and y=0.001 to 0.25; and q is a number necessary to maintain charge balance with S being sulfur.The catalyst is useful for oxidative coupling of methane and aliphatic and alicyclic hydrocarbon compounds with an aromatic compound to produce higher molecular weight hydrocarbons; and for dehydrogenating hydrocarbon compounds to produce unsaturated aliphatic and alicyclic chains.
摘要翻译：一种具有下式的混合碱金属硫化物催化剂：其中A是选自锂，钠，钾，铷，铯的碱金属及其混合物; B是具有大于C的电离状态的电离状态1的阳离子; 当C选自铍，镁，钙，锶，钡，镭，锌，镉，汞及其混合物时，B选自钪，钇，镧，锕，铝，硼及其混合物，B选自钛，锆，铪，硅及其混合物，当C选自钪，钇，镧，锕，铝，硼及其混合物时; x和y是z的摩尔分数，使得当z = 1时x = 0.001至0.25，y = 0.001至0.25; 并且q是维持与S为硫的电荷平衡所必需的数字。该催化剂可用于甲烷和脂族和脂环族烃化合物与芳族化合物的氧化偶联以产生较高分子量的烃; 并且用于使烃化合物脱氢以产生不饱和脂族和脂环族链。

4. 发明授权

US4935572A Mixed basic metal oxide catalyst for oxidative coupling of methane 失效
标题翻译：用于甲烷氧化偶联的混合碱性金属氧化物催化剂
公开(公告)号：US4935572A
公开(公告)日：1990-06-19
申请号：US274415
申请日：1988-11-21
申请人： Erek J. Erekson , Anthony L. Lee
发明人： Erek J. Erekson , Anthony L. Lee
IPC分类号： B01J23/00 , B01J23/02 , B01J23/06 , C07C2/84 , C07C5/333
CPC分类号： C07C2/84 , B01J23/00 , B01J23/02 , B01J23/06 , C07C5/3332 , C07C2521/02 , C07C2521/10 , C07C2523/02 , C07C2523/04 , C07C2523/06 , C07C2523/10 , C07C2523/12 , Y10S585/921 , Y10S585/926 , Y10S585/943
摘要： A catalyst and process for oxidative coupling of methane, the catalyst being a mixed basic metal oxide catalyst. One preferred catalyst is boron/alkali metal promoted metal oxide.
摘要翻译：甲烷氧化偶联的催化剂和方法，催化剂是混合的碱性金属氧化物催化剂。一种优选的催化剂是硼/碱金属促进的金属氧化物。

5. 发明授权

US4826796A Mixed basic metal oxide catalyst for oxidative coupling of methane 失效
标题翻译：用于甲烷氧化偶联的混合碱性金属氧化物催化剂
公开(公告)号：US4826796A
公开(公告)日：1989-05-02
申请号：US172808
申请日：1988-03-28
申请人： Erek J. Erekson , Anthony L. Lee
发明人： Erek J. Erekson , Anthony L. Lee
IPC分类号： B01J23/02 , B01J23/06 , C07C2/84 , B01J21/02 , B01J23/04 , B01J23/10
CPC分类号： C07C2/84 , B01J23/02 , B01J23/06 , C07C2521/02 , C07C2521/10 , C07C2523/02 , C07C2523/04 , C07C2523/06 , C07C2523/10 , C07C2523/12
摘要： A catalyst and a process for oxidative coupling of methane, the catalyst being a mixed basic metal oxide catalyst. One preferred catalyst is boron/alkali metal promoted metal oxide.
摘要翻译：催化剂和甲烷的氧化偶联方法，催化剂是混合的碱性金属氧化物催化剂。一种优选的催化剂是硼/碱金属促进的金属氧化物。

6. 发明授权

US5097086A Liquid catalyst for oxidative coupling reactions 失效
标题翻译：用于氧化偶联反应的液体催化剂
公开(公告)号：US5097086A
公开(公告)日：1992-03-17
申请号：US708460
申请日：1991-05-31
申请人： Anthony L. Lee , Robert F. Zabransky , Erek J. Erekson , S. Peter Barone , Irvine J. Solomon
发明人： Anthony L. Lee , Robert F. Zabransky , Erek J. Erekson , S. Peter Barone , Irvine J. Solomon
IPC分类号： C07C5/48
CPC分类号： C07C5/48
摘要： A liquid catalyst composition for the oxidative coupling of methane and other hydrocarbon compounds to produce higher hydrocarbons and for the oxidative dehydrogenation of aliphatic and alicyclic hydrocarbon compounds, aliphatic and alicyclic substituted aromatic hydrocarbons, and mixtures thereof is disclosed.
摘要翻译：公开了用于氧化偶合甲烷和其它烃化合物以产生高级烃和用于脂族和脂环族烃化合物，脂族和脂环族烃化合物及其混合物的氧化脱氢的液体催化剂组合物。

7. 发明授权

US5043505A Oxidative coupling of aliphatic and alicyclic compounds and mixed basic metal oxide catalyst therefore 失效
标题翻译：因此，脂肪族和脂环族化合物与混合的碱性金属氧化物催化剂的氧化偶联
公开(公告)号：US5043505A
公开(公告)日：1991-08-27
申请号：US517068
申请日：1990-05-07
申请人： Erek J. Erekson , Anthony L. Lee , S. Peter Barone , Irvine J. Solomon
发明人： Erek J. Erekson , Anthony L. Lee , S. Peter Barone , Irvine J. Solomon
IPC分类号： B01J23/00 , B01J23/02 , B01J23/04 , B01J23/06 , B01J23/20 , B01J27/04 , C07C2/84 , C07C2/00 , B01J21/02
CPC分类号： B01J23/02 , B01J23/00 , B01J23/04 , B01J23/06 , B01J23/20 , B01J27/04 , C07C2/84 , C07C2521/02 , C07C2521/10 , C07C2523/02 , C07C2523/04 , C07C2523/06 , C07C2523/10 , C07C2523/12 , C07C2527/04 , Y10S585/921 , Y10S585/926 , Y10S585/943
摘要： A catalytic process for gas phase oxidative coupling of aliphatic and alicyclic hydrocarbon compounds to produce higher molecular weight hydrocarbon compounds, the catalyst being a mixed basic metal oxide or sulfide catalyst. One preferred mixed basic metal oxide catalyst is boron/alkali metal promoted metal oxide.
摘要翻译：用于气相氧化偶联脂族和脂环族烃化合物以产生较高分子量烃化合物的催化方法，该催化剂为混合的碱性金属氧化物或硫化物催化剂。一种优选的混合碱性金属氧化物催化剂是硼/碱金属促进的金属氧化物。

8. 发明授权

US4956327A Mixed basic metal oxide/sulfide catalyst 失效
标题翻译：混合碱性金属氧化物/硫化物催化剂
公开(公告)号：US4956327A
公开(公告)日：1990-09-11
申请号：US359500
申请日：1989-05-31
申请人： Erek J. Erekson , Anthony L. Lee , S. Peter Barone , Irvine J. Solomon
发明人： Erek J. Erekson , Anthony L. Lee , S. Peter Barone , Irvine J. Solomon
IPC分类号： B01J23/00 , B01J23/02 , B01J23/04 , B01J23/20 , B01J27/04
CPC分类号： B01J23/20 , B01J23/00 , B01J23/02 , B01J23/04 , B01J27/04 , C07C2527/04
摘要： A mixed basic metal oxide/sulfide catalyst having the formulaxA.yB.zC.qDwherein A is an alkali metal selected from lithium, sodium, potassium, rubidium, cesium and mixtures thereof; B is a cation which has an ionization state 2 and 3 greater than the ionization state of C; B is selected from titanium, zirconium, hafnium, tantalum, niobium, vanadium and mixtures thereof; C is selected from magnesium, calcium, strontium, barium and mixtures thereof; D is selected from oxygen, sulfur and mixtures thereof; x and y are in mole fractions of z such that when z=1 then x=0.001 to 0.25, and y=0.001 to 0.25; and q is a number necessary to maintain charge balance with D. The sulfide form provides tolerance for sulfur containing feedstocks. The catalyst is useful for oxidative coupling of methane and aliphatic and alicyclic hydrocarbon compounds with an aromatic compound to produce higher molecular weight hydrocarbons and for dehydrogenating hydrocarbon compounds to produce unsaturated aliphatic and alicyclic chains.
摘要翻译：具有式xA.yB.zC.qD的混合碱式金属氧化物/硫化物催化剂，其中A是选自锂，钠，钾，铷，铯的碱金属及其混合物; B是具有大于C的电离状态的电离状态2和3的阳离子; B选自钛，锆，铪，钽，铌，钒及其混合物; C选自镁，钙，锶，钡及其混合物; D选自氧，硫及其混合物; x和y是z的摩尔分数，使得当z = 1时x = 0.001至0.25，y = 0.001至0.25; 并且q是与D保持电荷平衡所必需的数字。硫化物形式提供含硫原料的耐受性。催化剂可用于甲烷和脂族和脂环族烃化合物与芳族化合物的氧化偶联以产生较高分子量的烃和用于使烃化合物脱氢以产生不饱和脂族和脂环族链。

9. 发明授权

US4950830A Dehydration of aliphatic and alicyclic hydrocarbons and aliphatic and alicyclic substituted aromatic hydrocarbons 失效
标题翻译：脂肪族和脂环族烃类和脂族和脂环族取代芳烃的脱水
公开(公告)号：US4950830A
公开(公告)日：1990-08-21
申请号：US274499
申请日：1988-11-21
申请人： Erek J. Erekson , Anthony L. Lee
发明人： Erek J. Erekson , Anthony L. Lee
IPC分类号： B01J23/00 , B01J23/02 , B01J23/06 , C07C2/84 , C07C5/333
CPC分类号： C07C2/84 , B01J23/00 , B01J23/02 , B01J23/06 , C07C5/3332 , C07C2521/02 , C07C2521/10 , C07C2523/02 , C07C2523/04 , C07C2523/06 , C07C2523/10 , C07C2523/12
摘要： A process for dehydrogenation of aliphatic and alicyclic hydrocarbon compounds and aliphatic and alicyclic substituted aromatic hydrocarbon compounds to form unsaturated aliphatic and alicyclic hydrocarbon chains. The catalyst is mixed basic metal oxide catalyst, one preferred catalyst is boron/alkali metal promoted metal oxide. Reaction of ethylbenzene according to this invention results in conversion to styrene.
摘要翻译：一种脂肪族和脂环族烃化合物和脂肪族和脂环族取代芳烃化合物脱氢形成不饱和脂肪族和脂环族烃链的方法。催化剂是混合碱性金属氧化物催化剂，一种优选的催化剂是硼/碱金属促进的金属氧化物。根据本发明的乙苯的反应导致转化为苯乙烯。

10. 发明授权

US4950827A Oxidative coupling of aliphatic and alicyclic hydrocarbons with aliphatic and alicyclic substituted aromatic hydrocarbons 失效
标题翻译：脂肪族和脂环族烃与脂族和脂环族取代芳烃的氧化偶联
公开(公告)号：US4950827A
公开(公告)日：1990-08-21
申请号：US274454
申请日：1988-11-21
申请人： Erek J. Erekson , Anthony L. Lee
发明人： Erek J. Erekson , Anthony L. Lee
IPC分类号： B01J23/00 , B01J23/02 , B01J23/06 , C07C2/84 , C07C5/333
CPC分类号： C07C2/84 , B01J23/00 , B01J23/02 , B01J23/06 , C07C5/3332 , C07C2521/02 , C07C2521/10 , C07C2523/02 , C07C2523/04 , C07C2523/06 , C07C2523/10 , C07C2523/12 , Y10S585/921 , Y10S585/926 , Y10S585/943
摘要： A catalyst and a process for oxidative coupling of aliphatic and alicyclic hydrocarbon compounds with aliphatic and alicyclic substituted aromatic hydrocarbon compounds to form a longer substituent hydrocarbon on the aromatic ring. The catalyst is mixed basic metal oxide catalyst, one preferred catalyst is boron/alkali metal promoted metal oxide. Reaction of methane with toluene and oxygen according to this invention results in conversion to styrene.
摘要翻译：脂肪族和脂环族烃化合物与脂肪族和脂环族取代芳烃化合物氧化偶合的催化剂和方法，在芳香环上形成更长的取代烃。催化剂是混合碱性金属氧化物催化剂，一种优选的催化剂是硼/碱金属促进的金属氧化物。根据本发明，甲烷与甲苯和氧的反应导致转化为苯乙烯。

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