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1. 发明授权

US08119852B2 Process for manufacturing neohexene 失效
标题翻译：制备新己烯的方法
公开(公告)号：US08119852B2
公开(公告)日：2012-02-21
申请号：US12448216
申请日：2007-12-11
申请人： Jean Marie Basset , Francois Stoffelbach , Mostafa Taoufik , Jean Thivolle-Cazat
发明人： Jean Marie Basset , Francois Stoffelbach , Mostafa Taoufik , Jean Thivolle-Cazat
IPC分类号： C07C6/04
CPC分类号： C10L1/06 , B01J21/04 , B01J31/121 , B01J37/0209 , B01J2531/66 , C07C6/04 , C07C2521/04 , C07C2531/12 , C07C11/107
摘要： The present invention relates to a process for manufacturing neohexene, comprising contacting isobutene with a supported catalyst comprising a tungsten compound chosen from tungsten hydrides, organometallic tungsten compounds and organometallic tungsten hydrides, and a support comprising an oxide of aluminum, so as to form a reaction mixture comprising neohexene, and preferably separating neohexene from the reaction mixture, so as to isolate it. The contacting leads to the direct production of neohexene, in particular in a single (reaction) stage and with a high molar selectivity for neohexene. The contacting can be performed at a temperature of 50 to 600 ° C., under a total absolute pressure of 0.01 to 100 MPa.
摘要翻译：本发明涉及一种制备新己烯的方法，包括使异丁烯与包含选自氢化钨，有机金属钨化合物和有机金属氢化钨的钨化合物的负载催化剂和包含铝氧化物的载体接触，以形成反应包含新己烯的混合物，优选从反应混合物中分离新己烯，以便将其分离。接触导致新己烯的直接生产，特别是在单一（反应）阶段和对新己烯的高摩尔选择性。接触可以在50〜600℃的温度下，在0.01〜100MPa的绝对压力下进行。

2. 发明申请

US20090306441A1 Method for treatment of oil and/or gas field waste and by product materials 审中-公开
标题翻译：用于处理油和/或气田废物和产品材料的方法
公开(公告)号：US20090306441A1
公开(公告)日：2009-12-10
申请号：US12308747
申请日：2007-06-12
申请人： Jean Marie Basset , Francois Stoffelbach , Mostafa Taoufik , Jean Thivolle-Cazat
发明人： Jean Marie Basset , Francois Stoffelbach , Mostafa Taoufik , Jean Thivolle-Cazat
IPC分类号： C10L1/16 , C07C6/00
CPC分类号： B01J31/121 , B01J21/04 , B01J31/2265 , B01J37/0203 , B01J37/0207 , B01J37/0209 , B01J2531/66 , C07C6/10 , C07C2521/04 , C07C2531/12 , C10L1/06 , C07C9/16
摘要： The present invention relates to a process for preparing 2,3-dimethylbutane which comprises contacting in a reaction zone isobutane with a supported catalyst comprising a tungsten hydride and a support comprising an aluminium oxide, so as to form a reaction mixture comprising 2,3-dimethylbutane. The contacting essentially leads to performing a metathesis reaction of the isobutane, with a very high specificity in the formation of 2,3-dimethylbutane. The catalyst is preferably a tungsten hydride grafted onto a support based on aluminium oxide. The support can be chosen from aluminium oxides, mixed aluminium oxides and modified aluminium oxides. The reaction mixture can be isolated and preferably subjected to one or more fractionating operations in order to recover 2,3-dimethylbutane and optionally one or more other components of the reaction mixture, such as C5+ alkanes. The process can comprise isolating from the reaction mixture the C5+ alkanes including 2,3-dimethylbutane as a single component, which can be blended with gasoline to enhance the gasoline octane number, or be used as a gasoline blendstock. At least one separated fraction containing 2,3-dimethylbutane can be isolated from the single component, which can be blended with gasoline to enhance the gasoline octane number, or be used as a gasoline blendstock.
摘要翻译：本发明涉及一种制备2,3-二甲基丁烷的方法，该方法包括使反应区异丁烷与包含氢化钨的载体催化剂和包含氧化铝的载体接触，以形成包含2,3-二甲基丁烷的反应混合物，二甲基丁烷。该接触基本上导致进行异丁烷的复分解反应，在2,3-二甲基丁烷的形成中具有非常高的特异性。催化剂优选为基于氧化铝接枝到载体上的氢化钨。载体可以选自氧化铝，混合氧化铝和改性氧化铝。可以分离反应混合物，并优选进行一次或多次分馏操作，以回收2,3-二甲基丁烷和任选的一种或多种其它反应混合物的组分，例如C5 +烷烃。该方法可以包括从反应混合物中分离出包含2,3-二甲基丁烷作为单一组分的C5 +烷烃，其可以与汽油混合以增强汽油辛烷值，或者用作汽油混合料。可以从单一成分中分离出含有2,3-二甲基丁烷的至少一个分离馏分，其可以与汽油混合以提高汽油辛烷值，或者用作汽油混合料。

3. 发明申请

US20100028735A1 PROCESS FOR CONVERTING METHANE INTO A HIGHER ALKANE MIXTURE 审中-公开
标题翻译：将甲烷转化为较高的烷烃混合物的方法
公开(公告)号：US20100028735A1
公开(公告)日：2010-02-04
申请号：US12448275
申请日：2007-12-18
申请人： Jean Marie Basset , Sudhakar Chakka , Daravong Soulivong , Mostafa Taoufik , Jean Thivolle-Cazat
发明人： Jean Marie Basset , Sudhakar Chakka , Daravong Soulivong , Mostafa Taoufik , Jean Thivolle-Cazat
IPC分类号： H01M8/04 , C07C2/76 , C01B3/02
CPC分类号： C07C6/10 , C07C2521/08 , C07C2531/12 , C07C9/10 , C07C9/14 , C07C9/08
摘要： The present invention relates to a process for converting methane into a higher alkane mixture, preferably a liquid alkane mixture, comprising (C3+) alkanes having 3 carbon atoms and more, preferably (C4+) alkanes having 4 carbon atoms, especially (C5+) alkanes having 5 carbon atoms and more. The process comprises:—a stage (1) comprising contacting methane with a metal catalyst (C1) capable of producing, in contact with alkane, reactions involving the splitting and recombining of C—C and/or C—H and/or C-metal bonds, so as to form by a non-oxidative methane coupling reaction a mixture (M1) comprising ethane and hydrogen,—preferably a stage (2) comprising fractionating the mixture (M1) so as to separate and to isolate the ethane, and—a stage (3) comprising, preferably simultaneously, (i) contacting the mixture (M1) or preferably the ethane isolated in stage (2) with a metal catalyst (C2) capable of producing, in contact with alkane, reactions involving the splitting and recombining of C—C and/or C—H and/or C-metal bonds, said catalyst being identical to or different from catalyst (C1), so as to form by simultaneous ethane self- and cross-metathesis reactions a mixture (M2) comprising methane and the higher alkane mixture, and (ii) fractionating the mixture (M2) so as to separate and to isolate said higher alkane mixture, preferably in liquid form, and particularly the methane which is preferably recycled into stage (1). The hydrogen produced in stage (1) is preferably separated and isolated in stage (2) and then used for various applications and stages, e.g. for producing thermal and/or electrical energies preferably employed to run the process.
摘要翻译：本发明涉及一种将甲烷转化成高级烷烃混合物，优选液态烷烃混合物的方法，该混合物包含具有3个碳原子的（C3 +）烷烃和更多（优选具有4个碳原子的（C4 +）烷烃），特别是（C5 +）烷烃，其具有 5个碳原子和更多。该方法包括：a阶段（1）包括使甲烷与能够与烷烃接触的金属催化剂（C1）接触涉及CC和/或CH和/或C - 金属键的分解和重组的反应，因此通过非氧化甲烷偶联反应形成包含乙烷和氢气的混合物（M1），优选地包括分级分离混合物（M1）以分离和分离乙烷的阶段（2）和阶段（ 3）优选同时包含（i）将阶段（2）中分离的混合物（M1）或优选乙烷与能够与烷烃接触的金属催化剂（C2）接触涉及CC的分解和重组的反应和/或CH和/或C - 金属键，所述催化剂与催化剂（C1）相同或不同，以便通过同时进行乙烷自身和交叉复分解反应形成包含甲烷和高级烷烃的混合物（M2）混合物，和（ii）分离混合物（M2）以分离并且优选分离所述高级烷烃混合物，优选液体形式，特别是优选循环到阶段（1）中的甲烷。在阶段（1）中产生的氢优选在阶段（2）中分离和分离，然后用于各种应用和阶段，例如，用于产生优选用于运行该过程的热能和/或电能。

4. 发明申请

US20110160503A1 PROCESS FOR PREPARING A SUPPORTED CATALYST BASED ON Ni AND A METAL FROM GROUP IB, FOR THE SELECTIVE HYDROGENATION OF POLYUNSATURATED HYDROCARBONS 审中-公开
标题翻译：用于制备基于Ni和来自IB组的金属的支持催化剂的方法，用于选择性加氢聚合烃
公开(公告)号：US20110160503A1
公开(公告)日：2011-06-30
申请号：US12856932
申请日：2010-08-16
申请人： Lars FISCHER , Anne Claire Dubreuil , Cecile Thomazeau , Layane Deghedi , Jean Pierre Candy , Jean Marie Basset , Fabienne Le Peltier
发明人： Lars FISCHER , Anne Claire Dubreuil , Cecile Thomazeau , Layane Deghedi , Jean Pierre Candy , Jean Marie Basset , Fabienne Le Peltier
IPC分类号： C07C5/00 , B01J23/89 , B01J37/025 , B01J37/16 , B01J21/08 , B01J37/06
CPC分类号： C10G45/36 , B01J21/08 , B01J23/755 , B01J23/892 , B01J37/0203 , B01J37/0205 , B01J37/0213 , B01J37/18 , C07C5/05 , C07C2523/755 , C07C15/073
摘要： A process is described for preparing a catalyst comprising at least one porous support and at least one metallic phase containing nickel and at least one metal M from group IB in a proportion such that the molar ratio M/Ni is in the range 0.005 to 0.5, said process comprising at least the following steps in succession: a1) depositing nickel on at least said support in order to obtain a supported nickel-based monometallic catalyst; b1) depositing, in the presence of at least one reducing gas and in the absence of any aqueous solvent, at least one organometallic compound of at least said metal M onto said monometallic catalyst.
摘要翻译：描述了一种制备催化剂的方法，该催化剂包含至少一种多孔载体和至少一种含有镍和至少一种金属M的金属相，其比例使得M / Ni的摩尔比在0.005至0.5的范围内，所述方法至少包括以下步骤：a1）在至少所述载体上沉积镍以获得负载的镍基单金属催化剂; b1）在至少一种还原气体存在下，在不存在任何水性溶剂的情况下，将至少一种至少所述金属M的有机金属化合物沉积在所述单金属催化剂上。

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