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1. 发明授权

US5849434A Non-aqueous electrolyte lithium secondary battery 失效
标题翻译：非水电解质锂二次电池
公开(公告)号：US5849434A
公开(公告)日：1998-12-15
申请号：US685562
申请日：1996-07-24
申请人： Hitoshi Miura , Atsushi Terahara , Katsuhiko Iwasaki , Kenichiro Kami , Taketsugu Yamamoto
发明人： Hitoshi Miura , Atsushi Terahara , Katsuhiko Iwasaki , Kenichiro Kami , Taketsugu Yamamoto
IPC分类号： H01M4/58 , H01M4/62 , H01M4/64
CPC分类号： H01M4/621 , H01M4/587
摘要： A non-aqueous electrolyte lithium secondary battery, comprising a cathode containing, as active material, a material that can be doped/undoped with lithium ions, an anode containing, as active material, a carbonaceous material that can be doped/undoped with lithium ions, a separator interposed between the cathode and anode and an electrolyte prepared by dissolving lithium salt in an organic solvent, wherein the anode contains a polymer having carbonate groups represented by the structural formula �I!: ##STR1## said polymer having a number average molecular weight of not less than 300 and not more than 200,000. The lithium secondary battery has cycle life and high-rate capacity which are improved without reducing low-temperature capacity.
摘要翻译：一种非水电解质锂二次电池，其包含含有作为活性材料的能够掺杂/未掺杂锂离子的材料的阴极，含有可掺杂/未掺杂锂离子的碳质材料作为活性材料的阳极插入在阴极和阳极之间的隔膜和通过将锂盐溶解在有机溶剂中而制备的电解质，其中阳极含有具有由结构式[I]表示的碳酸酯基团的聚合物：所述聚合物具有数均分子量不小于300，不大于20万。锂二次电池具有循环寿命和高速率容量，在不降低低温容量的情况下得到改进。

2. 发明授权

US5985477A Polymer electrolyte for fuel cell 失效
标题翻译：用于燃料电池的聚合物电解质
公开(公告)号：US5985477A
公开(公告)日：1999-11-16
申请号：US997564
申请日：1997-12-23
申请人： Katsuhiko Iwasaki , Taketsugu Yamamoto , Hiroshi Harada , Atsushi Terahara , Kunihisa Satoh
发明人： Katsuhiko Iwasaki , Taketsugu Yamamoto , Hiroshi Harada , Atsushi Terahara , Kunihisa Satoh
IPC分类号： C08G75/20 , C08G75/00 , H01M8/02 , H01M8/10
CPC分类号： H01M8/1083 , H01M8/0289 , H01M8/1027 , H01M8/1032 , H01M8/1067 , H01M8/1072 , H01M8/1081 , Y02P70/56
摘要： Provided is a polymer electrolyte which is cheap and easily synthesized, and has a high water resistance and high output performance.The polymer electrolyte comprising a sulfonated polymer having an ion-exchange group equivalent weight of 500 to 2500 g/mol, which is obtainable by sulfonating a structural unit represented by the structural formula (II) of a copolymer having 95 to 40 mol % of a structural unit represented by the following structural formula (I) and 5 to 60 mol % of a structural unit represented by the following structural formula (II), ##STR1##
摘要翻译：提供一种廉价且易于合成的高分子电解质，具有高耐水性和高输出性能。该聚合物电解质包含离子交换基团当量为500〜2500g / mol的磺化聚合物，其可通过将具有95〜40mol％的结构式（II）的结构式（II）表示的结构单元磺化，由下述结构式（I）表示的结构单元和5〜60摩尔％的由下述结构式（II）表示的结构单元，

3. 发明授权

US6087031A Polymer electrolyte and process for producing the same 失效
标题翻译：聚合物电解质及其制备方法
公开(公告)号：US6087031A
公开(公告)日：2000-07-11
申请号：US997547
申请日：1997-12-23
申请人： Katsuhiko Iwasaki , Taketsugu Yamamoto , Atsushi Terahara , Michihisa Isobe
发明人： Katsuhiko Iwasaki , Taketsugu Yamamoto , Atsushi Terahara , Michihisa Isobe
IPC分类号： C08G75/23 , C08J5/20 , H01M8/02 , H01M8/10
CPC分类号： H01M8/1072 , C08J5/20 , H01M8/1027 , H01M8/1032 , H01M8/1067 , Y02P70/56
摘要： A polymer electrolyte comprising a sulfonated polyethersulfone having an ion-exchange group equivalent weight of 870 to 5000 g/mol, which is obtainable by sulfonating a polyethersulfone having the structural unit represented by the following structural formula, ##STR1## The polymer electrolyte is cheap, easily mold-processable by virtue of soluble property in organic solvent and thermoplastic property, easily film-processable, highly water-resistant, and suitable for a fuel cell.
摘要翻译：包含具有870〜5000g / mol的离子交换基当量的磺化聚醚砜的聚合物电解质，其可通过磺化具有由下列结构式表示的结构单元的聚醚砜获得。该聚合物电解质便宜，由于在有机溶剂中的可溶性和热塑性能可加工，易于加工膜，高度防水，并且适用于燃料电池。

4. 发明授权

US06379846B1 Non-aqueous electrolyte and lithium secondary battery using the same 有权
标题翻译：非水电解质和锂二次电池使用相同
公开(公告)号：US06379846B1
公开(公告)日：2002-04-30
申请号：US09525225
申请日：2000-03-14
申请人： Atsushi Terahara , Taketsugu Yamamoto , Kenji Nakane
发明人： Atsushi Terahara , Taketsugu Yamamoto , Kenji Nakane
IPC分类号： H01M1022
CPC分类号： H01M10/052 , H01M4/505 , H01M6/168 , H01M10/0525 , H01M10/0567
摘要： The present invention provides a non-aqueous electrolyte solution comprising a non-aqueous solvent and a lithium electrolyte, wherein the non-aqueous solvent is obtained by adding a phosphoric acid compound prepared by substituting at least one hydrogen atom in phosphoric acid or polyphosphoric acid with a group represented by the general formula [1]: wherein, X represents Si, Ge or Sn atom, and each of R1 to R3 independently represents an alkyl group having 1 to 10 carbon atoms, an alkenyl group having 1 to 10 carbon atoms or an aryl group having 6 to 10 carbon atoms.
摘要翻译：本发明提供一种包含非水溶剂和锂电解质的非水电解质溶液，其中非水溶剂是通过将磷酸或多磷酸中的至少一个氢原子取代而制备的磷酸化合物与由通式[1]表示的基团：其中，X表示Si，Ge或Sn原子，R 1至R 3各自独立地表示具有1至10个碳原子的烷基，具有1至10个碳原子的烯基或具有6-10个碳原子的芳基。

5. 发明授权

US5795677A Non-aqueous electrolyte and lithium secondary battery 失效
标题翻译：非水电解质和锂二次电池
公开(公告)号：US5795677A
公开(公告)日：1998-08-18
申请号：US685666
申请日：1996-07-24
申请人： Taketsugu Yamamoto , Hitoshi Miura
发明人： Taketsugu Yamamoto , Hitoshi Miura
IPC分类号： H01M6/16 , H01M10/0569 , H01M6/14
CPC分类号： H01M6/164 , H01M10/0569 , H01M2300/0034
摘要： The present invention provides a non-aqueous electrolyte that includes a non-aqueous solvent and a lithium salt. The non-aqueous electrolyte contains a halogen-substituted ether compound represented by the general formula (I): R.sub.1 --O--R.sub.2 (I) wherein R.sub.1 is an alkyl or halogen-substituted alkyl group having 2 or less carbon atoms and R.sub.2 is a halogen-substituted alkyl group having 2 to 10 carbon atoms. Additionally, the non-aqueous electrolyte contains at least one compound that is capable of dissolving the lithium salt in an amount of not less than 0.5 mol/liter. When this compound is added to the halogen-substituted ether compound, a mixed solvent is formed that is used as the non-aqueous solvent. The present invention also provides a lithium secondary battery that comprises a cathode that can be doped/undoped with lithium ions, an anode of a lithium metal or alloy or an anode that can be doped/undoped with lithium ions, and the non-aqueous electrolyte described above. A lithium secondary battery that uses the non-aqueous electrolyte of the present invention is superior in cycle life, in repeating charging/discharging and low-temperature capacity, is particularly superior in high-rate capacity, and causes little deterioration of high-rate capacity due to cycles.
摘要翻译：本发明提供一种包含非水溶剂和锂盐的非水电解质。非水电解质含有由通式（I）表示的卤素取代的醚化合物：R1-O-R2（I）其中R1是具有2个或更少碳原子的烷基或卤素取代的烷基，R2是具有2〜10个碳原子的卤素取代的烷基。此外，非水电解质含有至少一种能够以0.5摩尔/升的量溶解锂盐的化合物。当将该化合物加入到卤素取代的醚化合物中时，形成用作非水溶剂的混合溶剂。本发明还提供一种锂二次电池，其包括可以掺杂/未掺杂锂离子的阴极，锂金属或合金的阳极或可以掺杂/未掺杂锂离子的阳极，并且非水电解质如上所述。使用本发明的非水电解质的锂二次电池的循环寿命优异，重复充放电和低温容量优异，高容量特性优异，高容量容量几乎不劣化由于循环。

6. 发明授权

US09502714B2 Mixed metal oxide, electrode, and sodium secondary battery 有权
标题翻译：混合金属氧化物，电极和钠二次电池
公开(公告)号：US09502714B2
公开(公告)日：2016-11-22
申请号：US13256159
申请日：2010-03-10
申请人： Satoru Kuze , Masami Makidera , Taketsugu Yamamoto
发明人： Satoru Kuze , Masami Makidera , Taketsugu Yamamoto
IPC分类号： H01M4/131 , H01M4/50 , C01G45/12 , C01G49/00 , C01G51/00 , C01G53/00 , H01M2/16 , H01M4/48 , H01M4/485 , H01M10/054 , H01M10/0565 , H01M10/0568 , H01M10/0569 , H01M10/36 , H01M4/505 , H01M4/525 , H01M4/02
CPC分类号： H01M4/50 , C01G45/1228 , C01G49/0018 , C01G49/0027 , C01G49/0036 , C01G51/006 , C01G51/42 , C01G53/42 , C01G53/50 , C01P2002/52 , C01P2002/54 , C01P2002/72 , C01P2004/32 , C01P2004/54 , C01P2006/16 , C01P2006/40 , C01P2006/80 , H01M2/16 , H01M2/1686 , H01M4/483 , H01M4/485 , H01M4/505 , H01M4/525 , H01M10/054 , H01M10/0565 , H01M10/0568 , H01M10/0569 , H01M10/36 , H01M2004/028 , H01M2200/10 , H01M2300/002 , H01M2300/0025 , H01M2300/0088 , Y02E60/122
摘要： Disclosed is a mixed metal oxide comprising Na, M1, and M2, where M1 represents at least one element selected from the group consisting of Mg, Ca, Sr, and Ba; and M2 represents at least one element selected from the group consisting of Mn, Fe, Co, and Ni, wherein the molar ratio of Na:M1:M2 is a:b:1, where a is a value within the range of not less than 0.5 and less than 1; b is a value within the range of more than 0 and not more than 0.5; and “a+b” is a value within the range of more than 0.5 and not more than 1. An electrode having an active material containing the mixed metal oxide is also disclosed. Further disclosed is an electrode containing the electrode active material as well as a sodium secondary battery comprising the electrode as a positive electrode.
摘要翻译：公开了包含Na，M1和M2的混合金属氧化物，其中M1表示选自Mg，Ca，Sr和Ba中的至少一种元素; M2表示选自Mn，Fe，Co和Ni中的至少一种元素，其中Na：M1：M2的摩尔比为a：b：1，其中a为不小于大于0.5且小于1; b是大于0且不大于0.5的范围内的值; 并且“a + b”是大于0.5且不大于1的范围内的值。还公开了具有含有该混合金属氧化物的活性物质的电极。还公开了含有电极活性物质的电极以及包含该电极作为正电极的钠二次电池。

7. 发明授权

US09337519B2 Air battery having an electrode and polymer film 有权
标题翻译：具有电极和聚合物膜的空气电池
公开(公告)号：US09337519B2
公开(公告)日：2016-05-10
申请号：US13391183
申请日：2010-08-12
申请人： Takashi Sato , Taketsugu Yamamoto
发明人： Takashi Sato , Taketsugu Yamamoto
IPC分类号： H01M8/22 , H01M12/06
CPC分类号： H01M12/06
摘要： An air battery containing an electrode and a polymer film, wherein the polymer film is disposed on the air intake side of the electrode, and the polymer film is a film of a polymer comprising a repeating unit represented by the following formula (1), wherein R1, R2, and m are defined in the specification.
摘要翻译：一种包含电极和聚合物膜的空气电池，其中聚合物膜设置在电极的进气侧，聚合物膜是包含由下式（1）表示的重复单元的聚合物的膜，其中 R1，R2和m在本说明书中定义。

8. 发明申请

US20110135990A1 SODIUM SECONDARY BATTERY 有权
标题翻译：钠二次电池
公开(公告)号：US20110135990A1
公开(公告)日：2011-06-09
申请号：US13056912
申请日：2009-07-29
申请人： Taketsugu Yamamoto , Hideaki Nakajima , Hiroshi Inukai , Shigekazu Ohmori , Chikara Murakami , Daisuke Nakaji , Hidekazu Yoshida , Maiko Saka
发明人： Taketsugu Yamamoto , Hideaki Nakajima , Hiroshi Inukai , Shigekazu Ohmori , Chikara Murakami , Daisuke Nakaji , Hidekazu Yoshida , Maiko Saka
IPC分类号： H01M4/583 , G01J3/44 , G01N23/201 , G01N25/20 , H01M4/04 , H01M2/18
CPC分类号： H01M4/136 , H01M4/58 , H01M4/587 , H01M10/0569 , Y10T29/49108
摘要： Disclosed is a sodium secondary battery. The sodium secondary battery comprises a first electrode and a second electrode comprising a carbonaceous material. The carbonaceous material satisfies one or more requirements selected from the group consisting of requirements 1, 2, 3 and 4. Requirement 1: R value (=ID/IG) obtained by Raman spectroscopic measurement is 1.07 to 3. Requirement 2: A value and σA value obtained by small angle X-ray scattering measurement are −0.5 to 0 and 0 to 0.010, respectively. Requirement 3: for an electrode comprising an electrode mixture obtained by mixing 85 parts by weight of the carbonaceous material with 15 parts by weight of poly(vinylidene fluoride), the carbonaceous material in the electrode after being doped and dedoped with sodium ions is substantially free from pores having a size of not less than 10 nm. Requirement 4: Q1 value obtained by a calorimetric differential thermal analysis is not more than 800 joules/g.
摘要翻译：公开了钠二次电池。钠二次电池包括第一电极和包含碳质材料的第二电极。碳质材料满足从要求1,2,3和4所选择的一个或多个要求。要求1：通过拉曼光谱测量获得的R值（= ID / IG）为1.07至3.要求2：A值和＆sgr。通过小角度X射线散射测量获得的值分别为-0.5至0和0至0.010。要求3：对于包含通过将85重量份的碳质材料与15重量份的聚（偏二氟乙烯）混合而获得的电极混合物的电极，掺杂并掺杂了钠离子的电极中的碳质材料基本上不含来自具有不小于10nm的尺寸的孔。要求4：通过量热差热分析获得的Q1值不超过800焦耳/ g。

9. 发明申请

US20110008668A1 POWDER FOR POSITIVE ELECTRODE ACTIVE MATERIAL, POSITIVE ACTIVE ELECTRODE ACTIVE MATERIAL, AND SODIUM SECONDARY BATTERY 有权
标题翻译：活性电极活性材料，阳极活性电极活性材料和钠二次电池用粉末
公开(公告)号：US20110008668A1
公开(公告)日：2011-01-13
申请号：US12866148
申请日：2009-02-03
申请人： Masami Makidera , Taketsugu Yamamoto
发明人： Masami Makidera , Taketsugu Yamamoto
IPC分类号： H01M4/50 , H01B1/02 , H01M4/52 , H01M2/14
CPC分类号： H01M2/1653 , H01M4/505 , H01M4/525 , H01M10/056 , Y10T428/2982
摘要： The present invention provides a positive electrode active material that can suppress the necessity of performing sieving and is suitable for use in secondary batteries, particularly sodium secondary batteries. Also provided is a powder for a positive electrode active material as a raw material for the positive electrode active material. The powder for a positive electrode active material of the present invention comprises Mn-containing particles. In the cumulative particle size distribution on the volume basis of particles constituting the powder, D50, which is the particle diameter at a 50% cumulation measured from the smallest particle, is in the range of from 0.1 μm to 10 μm, and 90 vol % or more of the particles constituting the powder are in the range of from 0.3 times to 3 times D50. The powder for a positive electrode active material comprises Mn-containing particles, and 90 vol % or more of the particles constituting the powder are in the range of from 0.6 μm to 6 μm. The positive electrode active material is a powdery positive electrode active material obtained by calcining a mixture of the powder for positive electrode active material and a sodium compound. The positive electrode for sodium rechargeable batteries comprises the positive electrode active material.
摘要翻译：本发明提供能够抑制进行筛分的必要性的正极活性物质，适用于二次电池，特别是钠二次电池。还提供了作为正极活性物质的原料的正极活性物质的粉末。本发明的正极活性物质用粉末含有Mn粒子。在构成粉末的粒子的体积基础上的累积粒度分布中，从最小粒子测定的50％累积时的粒径D50为0.1μm〜10μm，90体积％或更多的构成粉末的颗粒在D50的0.3倍至3倍的范围内。用于正极活性物质的粉末包含含Mn颗粒，并且构成粉末的颗粒的90体积％以上在0.6μm至6μm的范围内。正极活性物质是通过煅烧正极活性物质粉末和钠化合物的混合物而获得的粉末状正极活性物质。钠可充电电池用正极包含正极活性物质。

10. 发明授权

US09899665B2 Sodium secondary battery comprising carbonaceous material 有权
公开(公告)号：US09899665B2
公开(公告)日：2018-02-20
申请号：US13056912
申请日：2009-07-29
申请人： Taketsugu Yamamoto , Hideaki Nakajima , Hiroshi Inukai , Shigekazu Ohmori , Chikara Murakami , Daisuke Nakaji , Hidekazu Yoshida , Maiko Saka
发明人： Taketsugu Yamamoto , Hideaki Nakajima , Hiroshi Inukai , Shigekazu Ohmori , Chikara Murakami , Daisuke Nakaji , Hidekazu Yoshida , Maiko Saka
IPC分类号： H01M4/136 , H01M4/58 , H01M4/04 , H01M4/587 , H01M10/0569
CPC分类号： H01M4/136 , H01M4/58 , H01M4/587 , H01M10/0569 , Y10T29/49108
摘要： Disclosed is a sodium secondary battery. The sodium secondary battery comprises a first electrode and a second electrode comprising a carbonaceous material. The carbonaceous material satisfies one or more requirements selected from the group consisting of requirements 1, 2, 3 and 4. Requirement 1: R value (=ID/IG) obtained by Raman spectroscopic measurement is 1.07 to 3. Requirement 2: A value and σA value obtained by small angle X-ray scattering measurement are −0.5 to 0 and 0 to 0.010, respectively. Requirement 3: for an electrode comprising an electrode mixture obtained by mixing 85 parts by weight of the carbonaceous material with 15 parts by weight of poly(vinylidene fluoride), the carbonaceous material in the electrode after being doped and dedoped with sodium ions is substantially free from pores having a size of not less than 10 nm. Requirement 4: Q1 value obtained by a calorimetric differential thermal analysis is not more than 800 joules/g.

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