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1. 发明授权

US5756600A Urethane-modified epoxy vinyl ester resin 失效
标题翻译：聚氨酯改性环氧乙烯基酯树脂
公开(公告)号：US5756600A
公开(公告)日：1998-05-26
申请号：US694688
申请日：1996-08-09
申请人： Hiroya Okumura , Toshiaki Uchida , Koichi Akiyama , Kenichi Morita , Takashi Shibata
发明人： Hiroya Okumura , Toshiaki Uchida , Koichi Akiyama , Kenichi Morita , Takashi Shibata
IPC分类号： C08F8/30 , C08F290/14 , C08G18/67 , C08K3/22 , C08K7/14 , C08L63/10
CPC分类号： C08G18/6705 , C08F290/14 , C08F8/30 , C08G18/672 , Y10T428/24994
摘要： A composition useful as a sheet or bulk molding compound comprises a urethane-modified vinyl ester resin (A), or acid-addition vinyl ester resn (A') obtained by reacting the hydroxyl groups in (A) with a polybasic acid anhydride (B), and a double bond(s)-containing monomer (C), wherein (A) is prepared by reacting a vinyl ester resin (F) derived from the reaction of an epoxy resin (D) and an unsaturated monobasic acid (E), with a polyisocyanate (H) and, optionally, a hydroxyl group(s)-containing (meth)acrylate (G) in an isocyanate:hydroxyl groups equivalent ratio of from 0.01-1.2:1.
摘要翻译：可用作片或模塑料的组合物包含通过使（A）中的羟基与多元酸酐（B）反应获得的氨基甲酸酯改性的乙烯基酯树脂（A）或酸加成乙烯基酯（A'））和含双键的单体（C），其中（A）通过使来自环氧树脂（D）的反应的乙烯基酯树脂（F）与不饱和一元酸（E）的反应制备，，异氰酸酯（H）和任选的含有（甲基）丙烯酸酯的羟基（G）的异氰酸酯：羟基当量比为0.01-1.2:1。

2. 发明授权

US5854313A Fine particles of high heat resistant polymer and epoxy esters 失效
标题翻译：高耐热聚合物和环氧酯的细颗粒
公开(公告)号：US5854313A
公开(公告)日：1998-12-29
申请号：US845206
申请日：1997-04-21
申请人： Yoshimasa Omori , Hiroya Okumura , Takashi Shibata
发明人： Yoshimasa Omori , Hiroya Okumura , Takashi Shibata
IPC分类号： C08F265/04 , C08F290/06 , C08G59/17 , C08L63/10 , C08K3/20
CPC分类号： C08L63/10 , C08F265/04 , C08F290/064 , C08G59/1466 , Y10S525/922
摘要： Fine particles of high heat resistant polymer obtained by emulsion polymerization or seeded polymerization of at least one epoxy ester (C) having two or more unsaturated bonds in one molecule and at least one reactive monomer (D) having at least one unsaturated double bond in one molecule, in the absence of a water-insoluble inorganic material as a dispersion stabilizer, the epoxy ester (C) being obtained by adding at least one unsaturated monobasic acid (B) to at least one epoxide (A-1) having at least one glycidyl group and one monocyclic hydrocarbon group in one molecule, and/or at least one epoxide (A-2) having at least one cycloaliphatic epoxy group in one molecule. The fine polymer particles have excellent heat resistance and solvent resistance, and an aqueous or alcoholic dispersion of such fine polymer particles is produced therefrom.
摘要翻译：通过在一个分子中具有两个或更多个不饱和键的至少一个环氧酯（C）和至少一个在一个分子中具有至少一个不饱和双键的反应性单体（D）的乳液聚合或接种聚合而获得的高耐热聚合物的细颗粒分子，在不存在作为分散稳定剂的水不溶性无机材料的情况下，环氧酯（C）是通过向至少一种具有至少一个的环氧化物（A-1）的至少一种环氧化物（A-1）加入至少一种不饱和一元酸一个分子中的缩水甘油基和一个单环烃基，和/或至少一个在一个分子中具有至少一个脂环族环氧基的环氧化物（A-2）。聚合物微粒具有优异的耐热性和耐溶剂性，由此生产这种聚合物微粒的水分散体或醇分散体。

3. 发明授权

US07125623B2 Separator for solid polymer type fuel cell and process for producing the same 有权
公开(公告)号：US07125623B2
公开(公告)日：2006-10-24
申请号：US09950081
申请日：2001-09-12
申请人： Hiroya Okumura , Takashi Shibata
发明人： Hiroya Okumura , Takashi Shibata
IPC分类号： H01M8/02 , H01B1/20
CPC分类号： C04B26/06 , C04B26/14 , C04B2111/00853 , C04B2111/94 , H01B1/122 , H01M8/0213 , H01M8/0226 , Y02P70/56 , C04B14/022
摘要： A separator for solid polymer-type fuel cell is produced by molding the resin composition which comprises an electroconductive agent and a radical-polymerizable thermosetting resin system by a resin molding method. The electroconductive agent comprises a carbon powder. The radical-polymerizable thermosetting resin system may comprise a radical-polymerizable resin (especially, a vinyl ester-series resin) and a radical-polymerizable diluent. It is preferred that the double bond equivalent of the radical-polymerizable resin may about 200 to 1,000 and that the hardened radical-polymerizable thermosetting resin system has a glass transition temperature of 120° C. or more. The weight ratio of the electroconductive agent to the radical-polymerizable thermosetting resin system may be about 55/45 to 95/5. Such a separator is suitable for fuel cell (in particular, solid polymer-type fuel cell), and can be produced with advantageous for commercial production.

4. 发明授权

US5886205A Process for producing silicon-containing isocyanate compound 失效
标题翻译：含硅异氰酸酯化合物的制造方法
公开(公告)号：US5886205A
公开(公告)日：1999-03-23
申请号：US843638
申请日：1997-04-10
申请人： Takashi Uchida , Hiroya Okumura , Takashi Shibata , Masaaki Sasaki
发明人： Takashi Uchida , Hiroya Okumura , Takashi Shibata , Masaaki Sasaki
IPC分类号： B01J31/12 , C07B61/00 , C07F7/08 , C07F7/10 , C07F7/18
CPC分类号： C07F7/0889 , C07F7/1892
摘要： A process for producing silicon-containing isocyanate compounds of the general formula II, comprising thermally induced decomposition of a silicon-containing carbamic ester of the general formula I at a pH of not higher than 8 in the presence of a catalyst of at least one metal or its compound.General Formula I: ##STR1## General Formula II: ##STR2## wherein R.sup.1 to R.sup.6 and R.sup.8 each represent a hydrocarbon group, R.sup.7 represents an alkylene group having 1 to 8 carbon atoms, n, m and l represent an integer of 0 to 3 and m+n+l=3, and a, b and c represent integers of 0 to 3, 0 to 2, and 0 to 8, respectively.
摘要翻译：一种制备通式II的含硅异氰酸酯化合物的方法，包括在至少一种金属的催化剂存在下，在不高于8的pH下热分解通式I的含硅氨基甲酸酯或其化合物。通式I：通式II：其中R 1至R 6和R 8各自表示烃基，R 7表示具有1至8个碳原子的亚烷基，n，m和l表示0至3的整数和m + n + 1 = 3，a，b和c分别表示0至3,0至2和0至8的整数。

5. 发明授权

US06592986B1 Material for molding thermosetting resin sheet, production process, and molded product 失效
标题翻译：用于模制热固性树脂板的材料，生产工艺和模制产品
公开(公告)号：US06592986B1
公开(公告)日：2003-07-15
申请号：US09701135
申请日：2000-11-24
申请人： Masahiro Hakotani , Koichi Akiyama , Hiromu Miyashita , Takashi Shibata
发明人： Masahiro Hakotani , Koichi Akiyama , Hiromu Miyashita , Takashi Shibata
IPC分类号： B32B2738
CPC分类号： H05K9/0088 , B29C70/025 , B29C70/502 , B29C70/882 , C08K7/04 , H01B1/22 , H01B1/24 , H05K9/009 , Y10T428/249933 , Y10T428/24994 , Y10T428/249952 , Y10T428/26 , Y10T428/31511
摘要： The present invention presents an SMC with which the electrically conductive layer does not break down or become non-uniform during molding and with which molded articles with excellent electromagnetic wave shielding capability and electric conductivity can be produced. This SMC is a thermosetting resin sheet molding compound having at least one continuous layer of electrically conductive fibers with a fiber length of 50 &mgr; to 5 mm, and it is further preferred that electrically conductive powder is uniformly dispersed throughout the entire molding compound. These SMCs can be produced by impregnating a reinforcing material with a thermosetting resin composition which is combined with the above-mentioned electrically conductive fibers, or the electrically conductive fibers and electrically conductive powder, and forming at least one continuous layer of these electrically conductive fibers adjacent to this reinforcement layer.
摘要翻译：本发明提出了一种SMC，其导电层在成型期间不会分解或变得不均匀，并且可以制造具有优异的电磁波屏蔽能力和导电性的模制品。该SMC是具有纤维长度为50〜5mm的至少一层连续导电性纤维的热固性树脂片状成型用化合物，进一步优选导电性粉末均匀地分散在整个成型料中。这些SMC可以通过用与上述导电纤维或导电纤维和导电粉末组合的热固性树脂组合物浸渍增强材料并且形成相邻的这些导电纤维的至少一个连续层来生产到这个加强层。

6. 发明授权

US06245419B1 Resin composition having excellent vibration-damping properties and molded article made thereof 失效
标题翻译：具有优异的阻尼性能的树脂组合物和由其制成的模塑制品
公开(公告)号：US06245419B1
公开(公告)日：2001-06-12
申请号：US09390767
申请日：1999-09-07
申请人： Masahiro Hakotani , Koichi Akiyama , Takashi Shibata , Kaneo Hamajima , Osamu Kito , Hiroyuki Takahashi , Kazuhiro Uchida
发明人： Masahiro Hakotani , Koichi Akiyama , Takashi Shibata , Kaneo Hamajima , Osamu Kito , Hiroyuki Takahashi , Kazuhiro Uchida
IPC分类号： B32B700
CPC分类号： C08G63/52 , C08L67/06 , Y10T428/249921
摘要： An unsaturated polyester resin composition having excellent vibration-damping properties, comprising an unsaturated polyester resin (A) having a glass transition temperature (Tg) of 0° C. or more and less than 60° C. In the composition, the unsaturated polyester resin (A) may be blended with an unsaturated polyester resin (B) having a glass transition temperature (Tg) of 150° C. or more and less than 200° C. or an unsaturated polyester resin (C) having a glass transition temperature (Tg) of 200° C. or more. Further, the composition may contain an elastomer (D) having a glass transition temperature (Tg) of −50° C. or more and less than 100° C. Since the unsaturated polyester resin composition has excellent vibration-damping properties and moldability in a wide temperature range, it is very useful to provide molded articles such as vibration-damping structural components, especially automobile engine-related components, having excellent heat resistance and chemical resistance as well as having excellent vibration-damping properties and moldability.
摘要翻译：具有优异的阻尼性能的不饱和聚酯树脂组合物，其包含玻璃化转变温度（Tg）为0℃以上且小于60℃的不饱和聚酯树脂（A）。在该组合物中，不饱和聚酯树脂（A）可以与玻璃化转变温度（Tg）为150℃以上且小于200℃的不饱和聚酯树脂（B）或具有玻璃化转变温度的不饱和聚酯树脂（C） Tg）为200℃以上。此外，组合物可以含有玻璃化转变温度（Tg）为-50℃以上且小于100℃的弹性体（D）。由于不饱和聚酯树脂组合物具有优异的阻尼性和成型性宽的温度范围，提供具有优异的耐热性和耐化学性以及具有优异的减振性和成型性的减振结构部件，特别是汽车发动机相关部件的模制品非常有用。

7. 发明授权

US5077326A Unsaturated polyester compositions molding materials therefrom and molded products therefrom 失效
标题翻译：不饱和聚酯组合物由其模塑材料和模制产品
公开(公告)号：US5077326A
公开(公告)日：1991-12-31
申请号：US363215
申请日：1989-06-08
申请人： Takashi Shibata , Koichi Akiyama , Sanzi Aoki , Yasuhiro Mishima , Hisayuki Iwai , Ken Hatta
发明人： Takashi Shibata , Koichi Akiyama , Sanzi Aoki , Yasuhiro Mishima , Hisayuki Iwai , Ken Hatta
IPC分类号： C08L67/06
CPC分类号： C08L67/06
摘要： A quickly curable unsaturated polyester composition with high surface quality contains an unsaturated polyester, a vinyl monomer, either an alkane polyol polyacrylate or an alkane polyol polymethylacrylate, a thermoplastic resin, and one or more curing catalysts selected from t-butylperoxy benzoate, t-butylperoxy octoate and 2,5-dimethyl-2,5-di(benzoilperoxy) hexane. Molding compounds are obtained by impregnating glass fibers with such composition and molded products obtained by curing such molding material have improved surface smoothness.
摘要翻译：具有高表面质量的快速固化不饱和聚酯组合物包含不饱和聚酯，乙烯基单体，烷基多元醇聚丙烯酸酯或烷基多元醇聚甲基丙烯酸酯，热塑性树脂和一种或多种选自叔丁基过氧苯甲酸酯，叔丁基过氧化物辛酸酯和2,5-二甲基-2,5-二（苯甲酰过氧）己烷。通过用这种组合物浸渍玻璃纤维获得成型化合物，并且通过固化这种成型材料获得的模制产品具有改善的表面平滑度。

8. 发明授权

US5395865A Unsaturated polyester compositions, molding materials and molded products 失效
标题翻译：不饱和聚酯组合物，成型材料和模制产品
公开(公告)号：US5395865A
公开(公告)日：1995-03-07
申请号：US973056
申请日：1992-11-06
申请人： Koichi Akiyama , Takashi Shibata , Hiroma Miyashita , Sanji Aoki , Ken Hatta , Takashi Ino , Yasuhiro Mishima
发明人： Koichi Akiyama , Takashi Shibata , Hiroma Miyashita , Sanji Aoki , Ken Hatta , Takashi Ino , Yasuhiro Mishima
IPC分类号： C08K5/13 , C08L67/06
CPC分类号： C08K5/13
摘要： Quickly curable unsaturated polyester composition with improved surface characteristics and stability in storage contains 20-40 weight parts of unsaturated polyester, 20-60 weight parts of vinyl monomer, 0.01-1.0 weight parts of BHT (ditertiary butyl hydroxy toluene), and 10-40 weight parts of thermoplastic resin such that the total is 100 weight parts. In addition, 0.001-0.1 weight parts of compound with effect of inhibiting polymerization at temperatures over 100.degree. C. are contained against the total of 100 weight parts. Molding materials are obtained by impregnating glass fibers with such compositions and products are obtained by curing such molding materials.
摘要翻译：具有改善的表面特性和储存稳定性的快速固化的不饱和聚酯组合物包含20-40重量份的不饱和聚酯，20-60重量份的乙烯基单体，0.01-1.0重量份的BHT（二叔丁基羟基甲苯）和10-40 重量份的热塑性树脂，总共为100重量份。此外，相对于总共100重量份，含有0.001-0.1重量份的在100℃以上抑制聚合作用的化合物。通过用这种组合物浸渍玻璃纤维获得成型材料，并且通过固化这种成型材料获得产品。

9. 发明授权

US5354585A Molding materials and molded products thereform 失效
标题翻译：成型材料和成型品
公开(公告)号：US5354585A
公开(公告)日：1994-10-11
申请号：US834822
申请日：1992-02-13
申请人： Takashi Shibata , Koichi Akiyama , Shinichiro Asao
发明人： Takashi Shibata , Koichi Akiyama , Shinichiro Asao
IPC分类号： B29C70/02 , B32B27/12 , B32B5/18 , B32B5/16
CPC分类号： B32B27/12 , B29C70/025 , B29C70/026 , Y10T428/1359 , Y10T428/1362 , Y10T428/1372 , Y10T428/1376 , Y10T428/249971 , Y10T428/249972 , Y10T428/249979 , Y10T428/24998 , Y10T428/249988 , Y10T428/252 , Y10T428/2982 , Y10T428/2996 , Y10T442/675 , Y10T442/676
摘要： A molding material is disclosed, comprising a film (A) coated on one surface with a thermosetting resin composition containing a hollow filler, a film (B) on which no resin composition is applied, and a reinforcing fiber layer positioned between the coated surface of film (A) and film (B), wherein the reinforcing fiber layer is impregnated with the liquid component of the resin composition coated on film (A). A piled material is also disclosed, comprising the two portions of the said molding material, wherein the respective molding materials are positioned on top of the other portion in a face-to-face relationship having their respective film (A) sides facing inwardly to each other, where the respective films (A) have been stripped off prior to positioning. A molded product prepared by curing the said piled material from which the films (B) have been stipped off prior to curing, under heating and compressing conditions are very useful for preparing a structural member which is lightweight and has high mechanical strength, due to its lower specific gravity and higher mechanical strength.
摘要翻译：公开了一种成型材料，其包括在一个表面上涂覆有含有中空填料的热固性树脂组合物的膜（A），其上没有施加树脂组合物的膜（B）和位于涂覆表面之间的增强纤维层膜（A）和膜（B），其中，所述增强纤维层浸渍有涂覆在膜（A）上的树脂组合物的液体成分。还公开了一种堆叠材料，其包括所述模制材料的两个部分，其中相应的模制材料以面对面关系定位在另一部分的顶部上，其中它们各自的膜（A）侧面向内朝向每个另一方面，在定位之前已经剥离各个膜（A）。在加热和压缩条件下固化所述薄膜（B）已被固化的所述堆叠材料制成的模制产品对于制备重量轻且机械强度高的结构件是非常有用的，较低的比重和较高的机械强度。

10. 发明授权

US5246983A Unsaturated polyester resin compositions, molding compounds and molded products therefrom 失效
标题翻译：不饱和聚酯树脂组合物，模塑料及其成型品
公开(公告)号：US5246983A
公开(公告)日：1993-09-21
申请号：US717818
申请日：1991-06-19
申请人： Takashi Shibata , Hiromu Miyashita , Sanzi Aoki , Koichi Akiyama
发明人： Takashi Shibata , Hiromu Miyashita , Sanzi Aoki , Koichi Akiyama
IPC分类号： C08J9/32
CPC分类号： C08J9/32 , C08J2367/00
摘要： A resin composition comprising (a) an unsaturated polyester, (b) a vinyl monomer, (c) a thermoplastic resin, (d) a curing agent and (e) a hollow filler with a number average particle diameter of not more than 20 .mu., wherein (e) occurs in a proportion of 10 to 150 parts by weight to 100 parts by weight of (a), (b) and (c) combined, and the molding compounds obtainable by impregnating glass fiber with the said resin composition are very useful in that, because of their lower specific gravity, they provide lightweight products with excellent surface quality which are great use as automotive exterior body panels and other parts.
摘要翻译：一种树脂组合物，其包含（a）不饱和聚酯，（b）乙烯基单体，（c）热塑性树脂，（d）固化剂和（e）数均粒径不大于20微米的中空填料其中（e）以（a），（b）和（c）的100重量份的比例为10〜150重量份的组合，通过与所述树脂组合物浸渍玻璃纤维而获得的成型化合物为非常有用，因为它们的比重较低，它们提供具有优异表面质量的轻质产品，其作为汽车外壳面板和其它部件是非常有用的。

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