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1. 发明授权

US4537936A Diene rubber composition, method of preparing the same and tire employing said composition 失效
标题翻译：二烯橡胶组合物，其制备方法和采用所述组合物的轮胎
公开(公告)号：US4537936A
公开(公告)日：1985-08-27
申请号：US371020
申请日：1982-04-22
申请人： Hiroyoshi Takao , Keisaku Yamamoto , Akio Imai , Nobuyuki Yoshida , Hiroshi Furukawa , Yuichi Saito , Akio Okumura
发明人： Hiroyoshi Takao , Keisaku Yamamoto , Akio Imai , Nobuyuki Yoshida , Hiroshi Furukawa , Yuichi Saito , Akio Okumura
IPC分类号： B60C1/00 , C08F36/04 , C08L9/00 , C08L9/06
CPC分类号： C08F36/04 , B60C1/0016 , C08L9/00 , C08L9/06 , Y10S152/905
摘要： A diene rubber composition comprising 25 to 90 parts by weight of at least one high molecular weight diene rubber (A) having an intrinsic viscosity [.eta.] of at least 2.0 and a glass transition point of not lower than -50.degree. C. and 75 to 10 parts by weight of at least one low molecular weight diene rubber (B) having an intrinsic viscosity [.eta.] of 0.01 to 2.0, said composition having an average intrinsic viscosity of at least 1.8.Since this composition has an excellent wet grip and rolling resistance property and moreover has excellent processability, it is employed as tire tread rubber.
摘要翻译：一种二烯橡胶组合物，其包含25至90重量份的至少一种特性粘度η至少为2.0且玻璃化转变点不低于-50℃的高分子量二烯橡胶（A）和75 至10重量份的至少一种特性粘度η为0.01至2.0的低分子量二烯橡胶（B），所述组合物的平均特性粘度至少为1.8。由于该组合物具有优异的湿抓地性和滚动阻力性，而且具有优异的加工性，因此用作轮胎胎面胶。

2. 发明授权

US4436873A Conjugated diene block polymer and process for preparing the same 失效
标题翻译：共轭二烯嵌段聚合物及其制备方法
公开(公告)号：US4436873A
公开(公告)日：1984-03-13
申请号：US477583
申请日：1983-03-21
申请人： Hiroshi Furukawa , Yuichi Saito , Akio Imai , Keisaku Yamamoto , Hiroyoshi Takao , Nobuyuki Yoshida
发明人： Hiroshi Furukawa , Yuichi Saito , Akio Imai , Keisaku Yamamoto , Hiroyoshi Takao , Nobuyuki Yoshida
IPC分类号： C08F297/00 , C08F136/04 , C08F297/02
CPC分类号： C08F297/02 , C08F136/04
摘要： A conjugated diene block polymer composed of blocks having a different microstructure from each other such that one block contains 20 to 60% by mole of 1,2- and/or 3,4-bonding, the other block contains 50 to 90% by mole of 1,2- and/or 3,4-bonding, the difference in the 1,2- and/or 3,4-bonding content between the both blocks is from 20 to 50% mole and the average content of 1,2- and/or 3,4-bonding in the polymer is from 50 to 85% by mole. The block polymer has a high wet skid resistance and a low dynamic heat generating property, and is very useful as a material for automobile tires.
摘要翻译：共轭二烯嵌段聚合物由具有彼此不同微结构的嵌段组成，使得一个嵌段含有20至60摩尔％的1,2-和/或3,4-键，另一个嵌段含有50至90摩尔％的1,2-和/或3,4-键，两个嵌段之间的1,2-和/或3,4-键含量的差异为20-50％摩尔，平均含量为1,2 - 和/或3,4-键在聚合物中为50-85摩尔％。嵌段聚合物具有高的抗湿滑性和低动态发热性，并且作为汽车轮胎的材料是非常有用的。

3. 发明授权

US4523618A Branched polymer, process for the preparation thereof, tire tread rubber composition and tire 失效
标题翻译：支化聚合物，其制备方法，轮胎胎面橡胶组合物和轮胎
公开(公告)号：US4523618A
公开(公告)日：1985-06-18
申请号：US480348
申请日：1983-03-30
申请人： Keisaku Yamamoto , Nobuyuki Yoshida , Yasushi Okamoto , Akio Imai , Tomoaki Seki , Hiroshi Furukawa , Yuichi Saito
发明人： Keisaku Yamamoto , Nobuyuki Yoshida , Yasushi Okamoto , Akio Imai , Tomoaki Seki , Hiroshi Furukawa , Yuichi Saito
IPC分类号： C08F4/00 , B60C1/00 , C08C19/44 , C08F4/42 , C08F236/00 , C08F236/10 , C08L9/00 , B60C11/00
CPC分类号： C08C19/44 , B60C1/0016 , C08L9/00 , Y10S152/905 , Y10T152/10495
摘要： A branched polymer which is a butadiene homopolymer or a copolymer of an aromatic vinyl compound and butadiene and has a glass transition temperature of not less than -50.degree. C. and of which at least 70% by weight of the polymer chains has a branched structure in which high molecules are coupled by a trifunctional or tetrafunctional coupling agent, has an excellent roll processability as required in mixing a rubber component with additives and provides a rubber component for tire tread showing a low rolling resistance and an excellent wet skid resistance characteristic.
摘要翻译：作为丁二烯均聚物或芳族乙烯基化合物与丁二烯的共聚物的分支聚合物，其玻璃化转变温度不低于-50℃，其中至少70重量％的聚合物链具有支链结构其中高分子通过三官能或四官能偶联剂偶联，根据需要在橡胶组分与添加剂混合时具有优异的辊加工性，并提供了具有低滚动阻力和优异的抗湿滑性能的轮胎胎面用橡胶组分。

4. 发明授权

US4471093A Elastomer composition comprising a blend of SBR rubbers 失效
标题翻译：包含SBR橡胶的混合物的弹性体组合物
公开(公告)号：US4471093A
公开(公告)日：1984-09-11
申请号：US470506
申请日：1983-02-28
申请人： Hiroshi Furukawa , Yuichi Saito , Keisaku Yamamoto , Akio Imai , Nobuyuki Yoshida , Yasushi Okamoto
发明人： Hiroshi Furukawa , Yuichi Saito , Keisaku Yamamoto , Akio Imai , Nobuyuki Yoshida , Yasushi Okamoto
IPC分类号： B60C1/00 , C08L9/06 , C08L7/00
CPC分类号： C08L7/00 , B60C1/0016 , C08L9/06
摘要： A rubber composition having improved rolling resistance and wet grip characteristics with improved processability, abrasion resistance and durability which contains as a rubber component a mixture of a high molecular weight styrene-butadiene rubber having a specific microstructure and a low molecular weight styrene-butadiene and/or butadiene rubber having a specific microstructure. The composition is particularly suitable for use in tread of tires.
摘要翻译：一种具有改善的滚动阻力和湿抓地性能的橡胶组合物，具有改进的加工性，耐磨性和耐久性，其包含作为橡胶组分的具有特定微结构的高分子量苯乙烯 - 丁二烯橡胶和低分子量苯乙烯 - 丁二烯和/ 或具有特定微结构的丁二烯橡胶。该组合物特别适用于轮胎胎面。

5. 发明授权

US4385151A Composition containing isoprene polymer 失效
标题翻译：含异戊二烯聚合物的组合物
公开(公告)号：US4385151A
公开(公告)日：1983-05-24
申请号：US324548
申请日：1981-11-24
申请人： Hiroshi Furukawa , Yuichi Saito , Akio Imai , Keisaku Yamamoto , Tomoaki Seki , Nobuyuki Yoshida
发明人： Hiroshi Furukawa , Yuichi Saito , Akio Imai , Keisaku Yamamoto , Tomoaki Seki , Nobuyuki Yoshida
IPC分类号： C08L9/00 , C08K3/06
CPC分类号： C08L9/00
摘要： A rubber composition containing an isoprene homopolymer or copolymer having a glass transition temperature of not less than -50.degree. C. and a Mooney viscosity of 20 to 120. The composition can provide a cured rubber having a high wet road gripping force and a small dynamic heat generating characteristic, and is very suitable for use in tires of automobiles.
摘要翻译：一种橡胶组合物，其含有玻璃化转变温度不低于-50℃，门尼粘度为20〜120的异戊二烯均聚物或共聚物。该组合物可以提供具有高湿道路夹紧力和小动态发热特性，非常适合用于汽车轮胎。

6. 发明授权

US4743652A Elastomeric copolymer of aromatic vinyl compounds and butadiene 失效
标题翻译：芳族乙烯基化合物和丁二烯的弹性共聚物
公开(公告)号：US4743652A
公开(公告)日：1988-05-10
申请号：US5400
申请日：1987-02-02
申请人： Nobuyuki Yoshida , Yasushi Okamoto , Akio Imai , Tomoaki Seki , Hiroshi Furukawa , Yuichi Saito
发明人： Nobuyuki Yoshida , Yasushi Okamoto , Akio Imai , Tomoaki Seki , Hiroshi Furukawa , Yuichi Saito
IPC分类号： C08F236/00 , C08C19/30 , C08C19/44 , C08F8/00 , C08F212/00 , C08F212/06 , C08F236/10 , C08F8/42
CPC分类号： C08C19/44
摘要： An elastomeric copolymer of an aromatic vinyl compound and butadiene prepared by a solution polymerization method, which has a glass transition temperature of not less than -50.degree. C. and contains polymer chains modified with a trifunctional or tetrafunctional coupling agent, and which contains not less than 3% by weight to less than 23% by weight, based on the whole polymer chains, of polymer chains having a molecular weight of at least 5 times a molecular weight corresponding to a peak appearing on the low molecular weight side of a high performance liquid chromatogram of the elastomeric copolymer. The elastomeric copolymer has an excellent processability and shows a low rolling resistance and a high wet grip characteristic when used as a rubber component in tires.
摘要翻译：通过溶液聚合法制备的芳族乙烯基化合物和丁二烯的弹性体共聚物，其具有不低于-50℃的玻璃化转变温度，并且包含用三官能或四官能偶联剂改性的聚合物链，并且不少于基于整个聚合物链，分子量至少为分子量的5倍的聚合物链的3重量％至小于23重量％，该分子量对应于高性能的低分子量侧上出现的峰弹性共聚物的液相色谱图。弹性体共聚物在轮胎中用作橡胶组分时具有优异的加工性能，并且具有低滚动阻力和高湿抓地性能。

7. 发明授权

US4737535A Rubber composition for tire tread 失效
标题翻译：轮胎胎面橡胶组合物
公开(公告)号：US4737535A
公开(公告)日：1988-04-12
申请号：US817949
申请日：1985-12-17
申请人： Hiroshi Furukawa , Yuichi Saito , Akio Imai , Nobuyuki Yoshida
发明人： Hiroshi Furukawa , Yuichi Saito , Akio Imai , Nobuyuki Yoshida
IPC分类号： C08L7/00 , B60C1/00 , C08K3/04 , C08K5/04 , C08K5/10 , C08K5/11 , C08K13/02 , C08L9/06 , C08L21/00
CPC分类号： C08K5/10 , B60C1/0016 , C08L21/00
摘要： A tire tread rubber composition which is improved in grip characteristic, steering stability characteristics and low-temperature characteristics, containing 15 to 50 parts by weight of a particular styrene-butadiene rubber obtained by solution polymerization containing polymer chains modified with trifunctional and/or tetrafunctional coupling agents, 50 to 85 parts by weight of at least one rubber selected from the group consisting of emulsion-polymerized styrene-butadiene rubber, natural rubber, synthetic polyisoprene rubber and butadiene rubber, at least one compound as plasticizer selected from the group consisting of a sebacic acid ester, an adipic acid ester and a fatty acid ester, and carbon black having an average particle size of not more than 30 m.mu..
摘要翻译： PCT No.PCT / JP85 / 00217 Sec。 371日期1985年12月17日第 102（e）日期1985年12月17日PCT申请1985年4月18日PCT公布。公开号WO85 / 04888 日期：1985年11月7日。一种改进了抓地性能，操纵稳定特性和低温特性的胎面橡胶组合物，其含有15〜50重量份通过溶液聚合得到的特定苯乙烯 - 丁二烯橡胶，使用三官能和/或四官能偶联剂，50至85重量份的选自乳液聚合的丁苯橡胶，天然橡胶，合成聚异戊二烯橡胶和丁二烯橡胶中的至少一种橡胶，至少一种化合物作为增塑剂选自癸二酸酯，己二酸酯和脂肪酸酯，平均粒径不大于30μm的碳黑。

8. 发明授权

US4482678A Diene rubber composition and tire using it in tread 失效
标题翻译：二烯橡胶组合物和轮胎使用它在胎面
公开(公告)号：US4482678A
公开(公告)日：1984-11-13
申请号：US525698
申请日：1983-08-23
申请人： Hiroshi Furukawa , Yuichi Saito , Akio Imai , Nobuyuki Yoshida , Yasushi Okamoto
发明人： Hiroshi Furukawa , Yuichi Saito , Akio Imai , Nobuyuki Yoshida , Yasushi Okamoto
IPC分类号： C08L7/00 , B60C1/00 , B60C11/00 , C08C19/44 , C08L9/00 , C08L21/00 , C08L9/06
CPC分类号： B60C1/0016 , C08C19/44 , C08L9/00
摘要： A diene rubber composition comprising as a main rubber component an elastomeric polymer having a glass transition temperature of not less than -50.degree. C. selected from the group consisting of a butadiene homopolymer and a copolymer of butadiene and an aromatic vinyl compound, said elastomeric polymer being one prepared by a solution polymerization method and not less than 40% by weight to less than 65% by weight of the polymer chains thereof being branched polymer chains formed by coupling the polymer molecules with each other with a trifunctional or tetrafunctional coupling agent. The composition has excellent rolling resistance characteristic, wet grip characteristic, processability, tear strength and tackiness, and is suitable particularly for use in the tread portion of tires.
摘要翻译：一种二烯橡胶组合物，其包含玻璃化转变温度不低于-50℃的弹性体聚合物作为主要橡胶组分，所述玻璃化转变温度选自丁二烯均聚物和丁二烯与芳族乙烯基化合物的共聚物，所述弹性体聚合物是通过溶液聚合法制备的，其不低于40重量％至小于65重量％的聚合物链是通过用三官能或四官能偶联剂将聚合物分子彼此连接而形成的支链聚合物链。组合物具有优异的滚动阻力特性，湿抓地性，加工性，撕裂强度和粘性，并且特别适用于轮胎的胎面部分。

9. 发明授权

US4647614A Diene elastomer compositions 失效
标题翻译：二烯弹性体组合物
公开(公告)号：US4647614A
公开(公告)日：1987-03-03
申请号：US804843
申请日：1985-12-05
申请人： Hiroyoshi Takao , Nobuyuki Yoshida , Akio Imai
发明人： Hiroyoshi Takao , Nobuyuki Yoshida , Akio Imai
IPC分类号： C08L7/00 , B60C1/00 , C08L9/00 , C08L9/06 , C08L21/00 , C08K3/04 , C08F136/00 , C08L47/00
CPC分类号： C08L9/00 , B60C1/0016
摘要： Disclosed is a diene elastomer composition especially suitable as tread rubber of tires which has low rolling resistance and high wet grip in combination. This elastomer composition contains a rubber material comprising an elastomeric polymer component of a butadiene polymer and/or a styrene-butadiene copolymer and a rubbery component. The elastomeric polymer is produced by using an organolithium compound as a polymerization initiator, and has a long chain end concentration (LCEC) of 1.5 or less as defined by the following formula: ##EQU1## wherein .alpha.: total number of terminal groups in long chain molecules per polymer,MW: a value obtained from intrinsic viscosity of the polymer as measured in toluene at 30.degree. C. by the following formulas:MW=70,660 x[.eta.].sup.1.282 for styrene-butadiene copolymer,MW=79,167 x[.eta.].sup.1.443 for butadiene polymer,.beta.i: weight fraction of component i when MW=(MW).sub.i.
摘要翻译：公开了一种二烯弹性体组合物，其特别适用于轮胎的胎面橡胶，其组合具有低滚动阻力和高湿抓地力。该弹性体组合物包含橡胶材料，其包含丁二烯聚合物和/或苯乙烯 - 丁二烯共聚物的弹性体聚合物组分和橡胶组分。弹性体聚合物通过使用有机锂化合物作为聚合引发剂制备，并且具有如下式所定义的1.5或更小的长链末端浓度（LCEC）：其中α：长链中的末端基团的总数每个聚合物的分子，＆upbar＆M：由在30℃下在甲苯中测量的聚合物的特性粘度得到的值，通过下列公式：＆lt;＆nbsp;＆nbsp;对于苯乙烯 - 丁二烯共聚物，M = 70,660×η1.282＆amp;＆amp; M = 79,167× 丁烯聚合物的η1.443，βi：当＆upbar＆M =（＆amp; upbar＆M）时组分i的重量分数i。

10. 发明授权

US5039756A Vulcanizable epoxy group-containing elastomer composition 失效
标题翻译：含可硫化环氧基的弹性体组合物
公开(公告)号：US5039756A
公开(公告)日：1991-08-13
申请号：US376490
申请日：1989-07-07
申请人： Keisaku Yamamoto , Nobuyuki Yoshida , Masahiro Fukuyama , Masahiro Ichinose
发明人： Keisaku Yamamoto , Nobuyuki Yoshida , Masahiro Fukuyama , Masahiro Ichinose
IPC分类号： C08L63/00 , C08F8/44 , C08G59/00 , C08G59/40 , C08G59/44 , C08G59/50 , C08G59/54 , C08G59/56 , C08K3/22 , C08K13/02
CPC分类号： C08F8/44 , C08K13/02
摘要： A vulcanizable epoxy group-containing elastomer composition is disclosed, which comprises:(A) an epoxy group-containing elastomer having compounded therewith(B) an organic compound having at least two linkages, per molecule, of the formula ##STR1## wherein X and Y are each oxygen atom or sulfur atom, or one of X and Y is oxygen atom and the other is sulfur atom;(C) a quaternary ammonium salt and/or a quaternary phosphonium salt;(D) a compound having one linkage, per molecule, of the formula ##STR2## wherein Z is oxygen atom or sulfur atom; and (E) calcium oxide or a combination of calcium oxide and calcium hydroxide.
摘要翻译：公开了一种可硫化的含环氧基的弹性体组合物，其包含：（A）与其混合的含环氧基的弹性体（B）每分子具有至少两个键的有机化合物，其中X和 Y分别是氧原子或硫原子，或X和Y中的一个是氧原子，另一个是硫原子; （C）季铵盐和/或季鏻盐; （D）每分子具有一个键的化合物，其中Z是氧原子或硫原子; 和（E）氧化钙或氧化钙和氢氧化钙的组合。

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