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1. 发明授权

US06395858B1 Aminopropyl-functional siloxane oligomers 有权
标题翻译：氨基丙基官能的硅氧烷低聚物
公开(公告)号：US06395858B1
公开(公告)日：2002-05-28
申请号：US09427479
申请日：1999-10-27
申请人： Helmut Mack , Dieter Barfurth , Roland Edelmann , Albert-Johannes Frings , Michael Horn , Peter Jenkner , Ralf Laven , Jaroslaw Monkiewicz , Burkhard Standke
发明人： Helmut Mack , Dieter Barfurth , Roland Edelmann , Albert-Johannes Frings , Michael Horn , Peter Jenkner , Ralf Laven , Jaroslaw Monkiewicz , Burkhard Standke
IPC分类号： C08G7726
CPC分类号： C08G77/045 , C07F7/21 , C08G77/26
摘要： The present invention relates to mixtures of catenate and cyclic siloxane oligomers of the formulae I and II where the substituents R consist of (i) aminopropyl-functional groups of the formula —(CH2)3—NH2 or —(CH2)3—NHR′ or —(CH2)3—NH(CH2)2—NH2 or —(CH2)3—NH(CH2)2—NH(CH2)2—NH2,in which R′ is a linear, branched or cyclic alkyl group of 1 to 18 carbon atoms or an aryl group of 6 to 12 carbon atoms, and (ii) methoxy, ethoxy, 2-methoxyethoxy and/or propoxy groups, and (iii) if desired, alkyl, alkenyl, isoalkyl or cycloalkyl groups of 1 to 18 carbon atoms and/or aryl groups of 6 to 12 carbon atoms, and where not more than one aminopropyl-functional group is attached to one silicon atom and the degree of oligomerization of compounds of the formula I is within the range 2
摘要翻译：本发明涉及式I和II的链状酯和环状硅氧烷低聚物的混合物，其中取代基R由（i）式 - （CH 2）3 -NH 2或 - （CH 2）3 -NHR'的氨基丙基官能团或 - （CH 2）3 -NH（CH 2）2 -NH 2或 - （CH 2）3 -NH（CH 2）2 -NH（CH 2）2 -NH 2，其中R'是直链，支链或环状烷基， 18个碳原子或6至12个碳原子的芳基，和（ii）甲氧基，乙氧基，2-甲氧基乙氧基和/或丙氧基，和（iii）如果需要，可以是1-18的烷基，烯基，异烷基或环烷基 6〜12个碳原子的碳原子和/或芳基，并且其中不超过一个氨基丙基官能团连接到一个硅原子上，并且式I化合物的低聚度在2 = 0.5的商。本发明还涉及制备所述混合物及其应用的特殊方法。

2. 发明授权

US06403228B1 Functional organylorganyloxysilanes on a carrier in cable compounds 失效
标题翻译：电缆化合物中载体上的功能性有机酰基氧基硅烷
公开(公告)号：US06403228B1
公开(公告)日：2002-06-11
申请号：US09604273
申请日：2000-06-26
申请人： Helmut Mack , Ralf Laven , Peter Jenkner , Roland Edelmann , Dieter Barfurth , Albert-Johannes Frings , Burkhard Standke , Jaroslaw Monkiewicz , Michael Horn
发明人： Helmut Mack , Ralf Laven , Peter Jenkner , Roland Edelmann , Dieter Barfurth , Albert-Johannes Frings , Burkhard Standke , Jaroslaw Monkiewicz , Michael Horn
IPC分类号： B32B904
CPC分类号： H01B3/44 , Y10T428/31663 , Y10T428/31801 , Y10T428/31855
摘要： The invention relates to the use of (1) a liquid functional organylorganyloxysilane bound to a carrier, or of a liquid (co)condensate derived from a functional organylorganyloxysilane and bound to a carrier for preparing cable compounds which comprise (2) a thermoplastic base polymer having polar functional groups and (3) a reinforcing or extending mineral filler.
摘要翻译：本发明涉及（1）与载体或衍生自功能性有机酰基氧基硅烷的液体（共）缩合物结合并结合到用于制备电缆化合物的载体的液体功能性有机羧基氧基硅烷的用途，其包含（2）热塑性基础聚合物具有极性官能团和（3）增强或延伸的矿物填料。

3. 发明授权

US06239194B1 Surface-modified fillers, process for their preparation and their use 有权
标题翻译：表面改性填料，其制备方法及其用途
公开(公告)号：US06239194B1
公开(公告)日：2001-05-29
申请号：US09300450
申请日：1999-04-28
申请人： Burkhard Standke , Jaroslaw Monkiewicz , Albert-Johannes Frings , Ralf Laven , Roland Edelmann , Peter Jenkner , Helmut Mack , Dieter Barfurth , Michael Horn
发明人： Burkhard Standke , Jaroslaw Monkiewicz , Albert-Johannes Frings , Ralf Laven , Roland Edelmann , Peter Jenkner , Helmut Mack , Dieter Barfurth , Michael Horn
IPC分类号： C08K320
CPC分类号： C09C3/12 , C01P2006/22 , C08K9/06 , C09J11/06 , Y10T428/2995
摘要： The present invention relates to surface-modified fillers obtained by mixing a filler with water, adding an water-based organosiloxane composition with very thorough mixing, wherein the organosiloxanes are soluble in water and contain, in addition to OH groups, at least one amino-functional group and optionally a functional group from the series consisting of alkyl, haloalkyl, alkenyl, glycidyl ether alkyl, acryloxyalkyl and methacryloxyalkyl, and wherein a functional group is bonded to each silicon atom of the organosiloxane, and drying the mixture. The present invention also provides a process for the surface modification of fillers, their use and ethylene-vinyl acetate copolymer compositions which include the surface-modified fillers.
摘要翻译：本发明涉及通过将填料与水混合，加入具有非常充分混合的水基有机硅氧烷组合物而得到的表面改性填料，其中有机硅氧烷可溶于水并且除OH基之外还含有至少一个氨基 - 官能团和任选的由烷基，卤代烷基，烯基，缩水甘油醚烷基，丙烯酰氧基烷基和甲基丙烯酰氧基烷基组成的系列的官能团，并且其中官能团键合到有机硅氧烷的每个硅原子上，并干燥该混合物。本发明还提供了填料及其用途的表面改性方法和包括表面改性填料的乙烯 - 乙酸乙烯酯共聚物组合物。

4. 发明授权

US06255513B1 Stable compositions of water-soluble amino-and alkenyl-functional organosiloxanes, process for their preparation and their use 有权
标题翻译：水溶性氨基和烯基官能的有机硅氧烷的稳定组合物，其制备方法及其应用
公开(公告)号：US06255513B1
公开(公告)日：2001-07-03
申请号：US09300448
申请日：1999-04-28
申请人： Burkhard Standke , Jaroslaw Monkiewicz , Albert-Johannes Frings , Ralf Laven , Roland Edelmann , Peter Jenkner , Helmut Mack , Dieter Barfurth , Michael Horn
发明人： Burkhard Standke , Jaroslaw Monkiewicz , Albert-Johannes Frings , Ralf Laven , Roland Edelmann , Peter Jenkner , Helmut Mack , Dieter Barfurth , Michael Horn
IPC分类号： C07F710
CPC分类号： C08G77/20 , C08G77/26 , Y10T428/2995
摘要： The present invention relates to a stable composition of water-soluble organosiloxanes obtained by reacting a) a water-soluble amino-functional alkoxysilane with at least one water-insoluble alkenyl-functional alkoxysilane b) by adding water to form a mixture, and c) removing the alcohol formed during step b) from the mixture, where the amino-functional alkoxysilane and the water are used in the reaction at least in amounts such that substantially all of the alkoxy groups of the water-insoluble silane can react and such that when a resulting composition is diluted with water, essentially no alcohol is liberated by hydrolysis, and the composition, during an/or after the reaction, has a pH of from 2 to 6, the pH being preferably adjusted by adding an organic or inorganic, optionally aqueous, acid. In addition, the present invention discloses a process for the preparation of such a composition and also its use.
摘要翻译：本发明涉及水溶性有机硅氧烷的稳定组合物，该组合物通过使水溶性氨基官能化烷氧基硅烷与至少一种水不溶性烯基官能烷氧基硅烷b）反应而得到，所述组合物通过加入水以形成混合物，和c）除去醇在步骤b）中形成的步骤b）中，其中氨基官能的烷氧基硅烷和水在反应中使用至少使得水不溶性硅烷的基本上所有的烷氧基基本上可以反应，并且使得当得到的组合物用水稀释，基本上没有通过水解释出醇，并且在反应过程中或之后，组合物的pH为2-6，优选通过加入有机或无机的任选含水酸来调节pH 。此外，本发明公开了一种制备这种组合物的方法及其用途。

5. 发明授权

US06500883B1 Organosilane-and/or organosiloxane-containing agent for filled polyamide 失效
标题翻译：用于填充聚酰胺的有机硅烷和/或含有机硅氧烷的试剂
公开(公告)号：US06500883B1
公开(公告)日：2002-12-31
申请号：US09660173
申请日：2000-09-12
申请人： Helmut Mack , Peter Jenkner , Roland Edelmann , Dieter Barfurth , Alber-Johannes Frings , Burkhard Standke , Jaroslaw Monkiewicz , Michael Horn , Thomas Schlosser
发明人： Helmut Mack , Peter Jenkner , Roland Edelmann , Dieter Barfurth , Alber-Johannes Frings , Burkhard Standke , Jaroslaw Monkiewicz , Michael Horn , Thomas Schlosser
IPC分类号： C08K906
CPC分类号： C08K9/06 , C08L77/00
摘要： Fillers surface-modified by treatment with an organosilane- and/or organosiloxane-containing agent for preparing filled polyamide compositions.
摘要翻译：用用于制备填充的聚酰胺组合物的有机硅烷和/或含有机硅氧烷的试剂进行表面改性的填料。

6. 发明授权

US07625975B2 Composition acting as coupling agent for filled and peroxidically crosslinking rubber compounds 失效
标题翻译：用作填充和过氧化交联橡胶化合物的偶联剂的组合物
公开(公告)号：US07625975B2
公开(公告)日：2009-12-01
申请号：US10524689
申请日：2003-06-20
申请人： Dieter Barfurth , Helmut Mack , Burkhard Standke
发明人： Dieter Barfurth , Helmut Mack , Burkhard Standke
IPC分类号： C08L9/00
CPC分类号： C08K5/5425 , C08L21/00 , Y10T428/2991 , Y10T428/2995 , Y10T428/31663
摘要： The present invention relates to a composition acting as coupling agent between fillers and peroxidically crosslinking elastomers in rubber compounds, which comprises, as component comprising silicon compounds, a mixture a) of vinylalkoxysiloxanes with alkylalkoxy-siloxanes, or b) of vinylalkoxysiloxanes with phenylalkoxy-siloxanes, or c) of vinylalkoxysiloxanes with phenyl/alkyl-alkoxysiloxanes or d) of acrylic or methacrylic alkoxysiloxanes with alkylalkoxysiloxanes, or e) of acrylic or methacrylic alkoxysiloxanes with phenylalkoxysiloxanes, or f) of acrylic or methacrylic alkoxysiloxanes with phenyl/alkylalkoxysiloxanes, or g) of at least one co-oligomeric organosiloxane which, as organofunctional groups, bears at least one group from the series vinyl, acrylic and methacrylic, and at least one group from the series alkyl and phenyl, and at least one alkoxy or hydroxy group. The present invention further relates to the use of a composition of the invention as a coupling agent in filled and peroxidically crosslinking rubber compounds, to rubber compounds obtained in this way, and to items made therefrom.
摘要翻译：本发明涉及在橡胶化合物中作为填料和过氧化交联弹性体之间的偶联剂的组合物，其包含作为包含硅化合物的组分的乙烯基烷氧基硅氧烷与烷基烷氧基硅氧烷的混合物，或b）乙烯基烷氧基硅氧烷与苯基烷氧基硅氧烷或c）具有苯基/烷基 - 烷氧基硅氧烷的乙烯基烷氧基硅氧烷或d）丙烯酸或甲基丙烯酸烷氧基硅氧烷与烷基烷氧基硅氧烷，或e）丙烯酸或甲基丙烯酸烷氧基硅氧烷与苯基烷氧基硅氧烷，或f）丙烯酸或甲基丙烯酸烷氧基硅氧烷与苯基/烷基烷氧基硅氧烷，或g）的至少一种共低聚有机硅氧烷，其作为有机官能团，从乙烯基，丙烯酸和甲基丙烯酸系列中至少包含一个基团，以及至少一个来自烷基和苯基的基团，以及至少一个烷氧基或羟基。本发明还涉及本发明的组合物作为填充和过氧化交联的橡胶化合物中的偶联剂，以这种方式获得的橡胶化合物以及由其制备的物质的用途。

7. 发明申请

US20070032609A1 Composition acting as coupling agent for filled and peroxidically crosslinking rubber compounds 失效
标题翻译：用作填充和过氧化交联橡胶化合物的偶联剂的组合物
公开(公告)号：US20070032609A1
公开(公告)日：2007-02-08
申请号：US10524689
申请日：2003-06-20
申请人： Dieter Barfurth , Helmut Mack , Burkhard Standke
发明人： Dieter Barfurth , Helmut Mack , Burkhard Standke
IPC分类号： C08L83/04 , B32B27/00 , B32B27/18 , B32B9/04
CPC分类号： C08K5/5425 , C08L21/00 , Y10T428/2991 , Y10T428/2995 , Y10T428/31663
摘要： The present invention relates to a composition acting as coupling agent between fillers and peroxidically crosslinking elastomers in rubber compounds, which comprises, as component comprising silicon compounds, a mixture a) of vinylalkoxysiloxanes with alkylalkoxy-siloxanes, or b) of vinylalkoxysiloxanes with phenylalkoxy-siloxanes, or c) of vinylalkoxysiloxanes with phenyl/alkyl-alkoxysiloxanes or d) of acrylic or methacrylic alkoxysiloxanes with alkylalkoxysiloxanes, or e) of acrylic or methacrylic alkoxysiloxanes with phenylalkoxysiloxanes, or f) of acrylic or methacrylic alkoxysiloxanes with phenyl/alkylalkoxysiloxanes, or g) of at least one co-oligomeric organosiloxane which, as organofunctional groups, bears at least one group from the series vinyl, acrylic and methacrylic, and at least one group from the series alkyl and phenyl, and at least one alkoxy or hydroxy group. The present invention further relates to the use of a composition of the invention as a coupling agent in filled and peroxidically crosslinking rubber compounds, to rubber compounds obtained in this way, and to items made therefrom.
摘要翻译：本发明涉及在橡胶化合物中作为填料和过氧化交联弹性体之间的偶联剂的组合物，其包含作为包含硅化合物的组分的乙烯基烷氧基硅氧烷与烷基烷氧基硅氧烷的混合物，或b）乙烯基烷氧基硅氧烷与苯基烷氧基硅氧烷或c）具有苯基/烷基 - 烷氧基硅氧烷的乙烯基烷氧基硅氧烷或d）丙烯酸或甲基丙烯酸烷氧基硅氧烷与烷基烷氧基硅氧烷，或e）丙烯酸或甲基丙烯酸烷氧基硅氧烷与苯基烷氧基硅氧烷，或f）丙烯酸或甲基丙烯酸烷氧基硅氧烷与苯基/烷基烷氧基硅氧烷，或g）的至少一种共低聚有机硅氧烷，其作为有机官能团，从乙烯基，丙烯酸和甲基丙烯酸系列中至少包含一个基团，以及至少一个来自烷基和苯基的基团，以及至少一个烷氧基或羟基。本发明还涉及本发明的组合物作为填充和过氧化交联的橡胶化合物中的偶联剂，以这种方式获得的橡胶化合物以及由其制备的物质的用途。

8. 发明申请

US20080146730A1 Polymer Dispersion Comprising Silicon Compounds 失效
标题翻译：包含硅化合物的聚合物分散体
公开(公告)号：US20080146730A1
公开(公告)日：2008-06-19
申请号：US10566371
申请日：2004-06-02
申请人： Dieter Barfurth , Helmut Mack
发明人： Dieter Barfurth , Helmut Mack
IPC分类号： C08L83/00
CPC分类号： C09J183/10 , C08F30/08 , C08F283/12 , C08L51/085 , C08L2666/02 , C09D151/085 , C09D183/10 , C09J151/085
摘要： The present invention relates to a polymer dispersion wherein the components of a physical mixture comprising (i) at least one unsaturated silane of the general formula (I): [H2C═CX(Y)n]Si(CH3)p(R)3-p in which X is a hydrogen atom or a methyl group, Y is a divalent group selected from —CH2— and —C(O)O—(CH2)3—, n is 0 or 1, R is an alkoxy group selected from methoxy, ethoxy, n-propoxy, isopropoxy, n-butoxy, isobutoxy, and 2-methoxyethoxy, and p is 0 or 1, and (ii) at least one organosilane of the general formula (II): R1Si(CH3)q(R2)3-q in which R1 is a linear, branched or cyclic alkyl group having 1 to 18 carbon atoms or is an aryl group or is a polyether group, R2 is an alkoxy group selected from methoxy, ethoxy, n-propoxy, isopropoxy, n-butoxy, isobutoxy and 2-methoxyethoxy, and q is 0 or 1, and/or at least one silicic ester of the general formula (III): Si(R3)4, in which groups R3 are identical or different and R3 is an alkoxy group selected from methoxy, ethoxy, n-propoxy, isopropoxy, n-butoxy and isobutoxy, are incorporated into the framework of the polymer, a process for preparing such a polymer dispersion, and its use.
摘要翻译：本发明涉及一种聚合物分散体，其中物理混合物的组分包含（i）至少一种通式（I）的不饱和硅烷：[H 2 C-CX（Y）_{是选自甲氧基，乙氧基，正丙氧基，异丙氧基，正丁氧基，异丁氧基和2-甲氧基乙氧基的烷氧基，q是0或1，和/或至少一个硅酸盐呃通式（III）：其中基团R 3相同或不同，R（O）3 > 3是选自甲氧基，乙氧基，正丙氧基，异丙氧基，正丁氧基和异丁氧基的烷氧基，并入聚合物的骨架中，制备这种聚合物分散体的方法及其用途。}

9. 发明授权

US06858746B2 Process for the hydrosilylation of unsaturated aliphatic compounds 有权
标题翻译：不饱和脂肪族化合物的氢化硅烷化方法
公开(公告)号：US06858746B2
公开(公告)日：2005-02-22
申请号：US10267819
申请日：2002-10-10
申请人： Sabine Giessler , Helmut Mack , Dieter Barfurth
发明人： Sabine Giessler , Helmut Mack , Dieter Barfurth
IPC分类号： C07F7/08 , C07F7/14 , C07F7/18
CPC分类号： C07F7/14 , C07F7/0829 , C07F7/1876
摘要： A compound having at least one H—Si group is reacted with an unsaturated aliphatic compound in the presence of a platinum catalyst and at least one organic additive component. The combination of platinum catalyst and additive component is one of: (i) a solution of a Pt(0) complex catalyst in a solvent, with at least one organic amide, or (ii) a solution of a Pt(0) complex catalyst in a solvent, with at least one organic amine, or (iii) a solution of a Pt(0) complex catalyst, in a solvent, with at least one organic nitrite.
摘要翻译：具有至少一个H-Si基团的化合物与不饱和脂族化合物在铂催化剂和至少一种有机添加剂组分的存在下反应。铂催化剂和添加剂组分的组合是以下之一：（i）Pt（0）配合物催化剂在溶剂中与至少一种有机酰胺的溶液，或（ii）Pt（0）配位催化剂在溶剂中与至少一种有机胺，或（iii）Pt（0）配合物催化剂在溶剂中的溶液与至少一种有机亚硝酸盐反应。

10. 发明授权

US07847018B2 Polymer dispersion comprising silicon compounds 失效
标题翻译：包含硅化合物的聚合物分散体
公开(公告)号：US07847018B2
公开(公告)日：2010-12-07
申请号：US10566371
申请日：2004-06-02
申请人： Dieter Barfurth , Helmut Mack
发明人： Dieter Barfurth , Helmut Mack
IPC分类号： C08L83/06
CPC分类号： C09J183/10 , C08F30/08 , C08F283/12 , C08L51/085 , C08L2666/02 , C09D151/085 , C09D183/10 , C09J151/085
摘要： The present invention relates to a polymer dispersion wherein the components of a physical mixture comprising (i) at least one unsaturated silane of the general formula (I): [H2C═CX(Y)n]Si(CH3)p(R)3-p in which X is a hydrogen atom or a methyl group, Y is a divalent group selected from —CH2— and —C(O)O—(CH2)3—, n is 0 or 1, R is an alkoxy group selected from methoxy, ethoxy, n-propoxy, isopropoxy, n-butoxy, isobutoxy, and 2-methoxyethoxy, and p is 0 or 1, and (ii) at least one organosilane of the general formula (II): R1Si(CH3)q(R2)3-q in which R1 is a linear, branched or cyclic alkyl group having 1 to 18 carbon atoms or is an aryl group or is a polyether group, R2 is an alkoxy group selected from methoxy, ethoxy, n-propoxy, isopropoxy, n-butoxy, isobutoxy and 2-methoxyethoxy, and q is 0 or 1, and/or at least one silicic ester of the general formula (III): Si(R3)4, in which groups R3 are identical or different and R3 is an alkoxy group selected from methoxy, ethoxy, n-propoxy, isopropoxy, n-butoxy and isobutoxy, are incorporated into the framework of the polymer, a process for preparing such a polymer dispersion, and its use.
摘要翻译：本发明涉及一种聚合物分散体，其中物理混合物的组分包含（i）至少一种通式（I）的不饱和硅烷：[H 2C≡CX（Y）n] Si（CH 3）p（R）3 -p，其中X是氢原子或甲基，Y是选自-CH 2 - 和-C（O）O-（CH 2）3 - 的二价基团，n是0或1，R是选择的烷氧基甲氧基，乙氧基，正丙氧基，异丙氧基，正丁氧基，异丁氧基和2-甲氧基乙氧基，p为0或1，和（ii）至少一种通式（II）的有机硅烷：R1Si（CH3）q （R2）3-q，其中R1是具有1至18个碳原子的直链，支链或环状烷基，或者是芳基或是聚醚基，R2是选自甲氧基，乙氧基，正丙氧基，异丙氧基，正丁氧基，异丁氧基和2-甲氧基乙氧基，q为0或1，和/或至少一种通式（III）的硅酸酯：Si（R3）4，其中基团R3相同或不同， R3是选自甲氧基，乙氧基，正丙氧基的烷氧基 y，异丙氧基，正丁氧基和异丁氧基引入聚合物的骨架中，制备这种聚合物分散体的方法及其用途。

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