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1. 发明授权

US07641787B2 Compositions and processes for reducing NOx emissions during fluid catalytic cracking 失效
标题翻译：在流化床催化裂化过程中减少NOx排放的组成和方法
公开(公告)号：US07641787B2
公开(公告)日：2010-01-05
申请号：US12291379
申请日：2008-11-07
申请人： George Yaluris , Michael Scott Ziebarth , Xinjin Zhao
发明人： George Yaluris , Michael Scott Ziebarth , Xinjin Zhao
IPC分类号： C10G11/05 , C10G47/16 , C10G47/18 , C10G47/20 , B01J29/90
CPC分类号： B01J29/80 , B01J29/06 , B01J29/084 , B01J29/18 , B01J29/60 , B01J29/70 , B01J29/7007 , B01J35/0006 , B01J37/0045 , B01J2229/42 , C10G11/02 , C10G11/05 , C10G11/182 , C10G2300/405 , C10G2300/80 , C10G2400/20
摘要： Compositions for reduction of NOx generated during a catalytic cracking process, preferably, a fluid catalytic cracking process, are disclosed. The compositions comprise a fluid catalytic cracking catalyst composition, preferably containing a Y-type zeolite, and a particulate NOx composition containing particles of a zeolite having a pore size ranging from about 3 to about 7.2 Angstroms and a SiO2 to Al2O3 molar ratio of less than about 500. Preferably, the NOx reduction composition contains NOx reduction zeolite particles bound with an inorganic binder. In the alternative, the NOx reduction zeolite particles are incorporated into the cracking catalyst as an integral component of the catalyst. Compositions in accordance with the invention are very effective for the reduction of NOx emissions released from the regenerator of a fluid catalytic cracking unit operating under FCC process conditions without a substantial change in conversion or yield of cracked products. Processes for the use of the compositions are also disclosed.
摘要翻译：公开了用于还原在催化裂化过程中产生的NOx，优选流化催化裂化过程的组合物。该组合物包含优选含有Y型沸石的流化催化裂化催化剂组合物和含有孔径范围为约3至约7.2埃的沸石和SiO 2与Al 2 O 3摩尔比小于优选地，NOx还原组合物含有与无机粘合剂结合的NOx还原沸石颗粒。另外，作为催化剂的组成成分，将NOx还原型沸石粒子并入裂化催化剂中。根据本发明的组合物对于在FCC工艺条件下操作的流化床催化裂化装置的再生器中释放的NO x排放的降低非常有效，而没有破裂产物的转化率或产率的显着变化。还公开了使用组合物的方法。

2. 发明授权

US09931595B2 Ferrierite composition for reducing NOx emissions during fluid catalytic cracking 有权
公开(公告)号：US09931595B2
公开(公告)日：2018-04-03
申请号：US12833336
申请日：2010-07-09
申请人： George Yaluris , Michael Scott Ziebarth , Xinjin Zhao
发明人： George Yaluris , Michael Scott Ziebarth , Xinjin Zhao
IPC分类号： B01D53/86 , B01J23/00 , B01J23/42 , B01J23/83 , B01J29/65 , B01J29/80 , B01J35/00 , C10G11/18 , B01J29/08 , B01J37/00
CPC分类号： B01D53/8628 , B01D2255/50 , B01D2258/00 , B01J23/42 , B01J23/83 , B01J29/084 , B01J29/65 , B01J29/80 , B01J35/0006 , B01J35/002 , B01J37/0045 , B01J2229/18 , B01J2229/42 , C10G11/18 , C10G11/182 , C10G2300/405
摘要： Compositions for reduction of NOx generated during a catalytic cracking process, preferably, a fluid catalytic cracking process, are disclosed. The compositions comprise a fluid catalytic cracking catalyst composition, preferably containing a Y-type zeolite, and a particulate NOx reduction composition containing ferrierite zeolite particles. Preferably, the NOx reduction composition contains ferrierite zeolite particles bound with an inorganic binder. In the alternative, the ferrierite zeolite particles are incorporated into the cracking catalyst as an integral component of the catalyst. NOx reduction compositions in accordance with the invention are very effective for the reduction of NOx emissions released from the regenerator of a fluid catalytic cracking unit operating under FCC process conditions without a substantial change in conversion or yield of cracked products. Processes for the use of the compositions are also disclosed.

3. 发明申请

US20100276337A1 FERRIERITE COMPOSITION FOR REDUCING NOX EMISSIONS DURING FLUID CATALYTIC CRACKING 有权
标题翻译：用于在流体催化裂化过程中减少NO x排放的FERRIERITE组合物
公开(公告)号：US20100276337A1
公开(公告)日：2010-11-04
申请号：US12833336
申请日：2010-07-09
申请人： George Yaluris , Michael Scott Ziebarth , Xinjin Zhao
发明人： George Yaluris , Michael Scott Ziebarth , Xinjin Zhao
IPC分类号： C10G11/00
CPC分类号： B01D53/8628 , B01D2255/50 , B01D2258/00 , B01J23/42 , B01J23/83 , B01J29/084 , B01J29/65 , B01J29/80 , B01J35/0006 , B01J35/002 , B01J37/0045 , B01J2229/18 , B01J2229/42 , C10G11/18 , C10G11/182 , C10G2300/405
摘要： Compositions for reduction of NOx generated during a catalytic cracking process, preferably, a fluid catalytic cracking process, are disclosed. The compositions comprise a fluid catalytic cracking catalyst composition, preferably containing a Y-type zeolite, and a particulate NOx reduction composition containing ferrierite zeolite particles. Preferably, the NOx reduction composition contains ferrierite zeolite particles bound with an inorganic binder. In the alternative, the ferrierite zeolite particles are incorporated into the cracking catalyst as an integral component of the catalyst. NOx reduction compositions in accordance with the invention are very effective for the reduction of NOx emissions released from the regenerator of a fluid catalytic cracking unit operating under FCC process conditions without a substantial change in conversion or yield of cracked products. Processes for the use of the compositions are also disclosed.
摘要翻译：公开了用于还原在催化裂化过程中产生的NOx，优选流化催化裂化过程的组合物。该组合物包含优选含有Y型沸石的流化催化裂化催化剂组合物和含有镁碱沸石颗粒的颗粒NOx还原组合物。优选地，NOx还原组合物含有与无机粘合剂结合的镁碱沸石颗粒。替代方案中，镁碱沸石颗粒作为催化剂的组成成分加入到裂化催化剂中。根据本发明的NOx还原组合物对于在FCC工艺条件下操作的流化催化裂化装置的再生器中释放的NOx排放的降低非常有效，而没有破裂产物的转化率或产率的显着变化。还公开了使用组合物的方法。

4. 发明申请

US20090068079A1 Compositions and processes for reducing NOx emissions during fluid catalytic cracking 失效
标题翻译：在流化床催化裂化过程中减少NOx排放的组成和方法
公开(公告)号：US20090068079A1
公开(公告)日：2009-03-12
申请号：US12291379
申请日：2008-11-07
申请人： George Yaluris , Michael Scott Ziebarth , Xinjin Zhao
发明人： George Yaluris , Michael Scott Ziebarth , Xinjin Zhao
IPC分类号： B01D53/86
CPC分类号： B01J29/80 , B01J29/06 , B01J29/084 , B01J29/18 , B01J29/60 , B01J29/70 , B01J29/7007 , B01J35/0006 , B01J37/0045 , B01J2229/42 , C10G11/02 , C10G11/05 , C10G11/182 , C10G2300/405 , C10G2300/80 , C10G2400/20
摘要： Compositions for reduction of NOx generated during a catalytic cracking process, preferably, a fluid catalytic cracking process, are disclosed. The compositions comprise a fluid catalytic cracking catalyst composition, preferably containing a Y-type zeolite, and a particulate NOx composition containing particles of a zeolite having a pore size ranging from about 3 to about 7.2 Angstroms and a SiO2 to Al2O3 molar ratio of less than about 500. Preferably, the NOx reduction composition contains NOx reduction zeolite particles bound with an inorganic binder. In the alternative, the NOx reduction zeolite particles are incorporated into the cracking catalyst as an integral component of the catalyst. Compositions in accordance with the invention are very effective for the reduction of NOx emissions released from the regenerator of a fluid catalytic cracking unit operating under FCC process conditions without a substantial change in conversion or yield of cracked products. Processes for the use of the compositions are also disclosed.
摘要翻译：公开了用于还原在催化裂化过程中产生的NOx，优选流化催化裂化过程的组合物。该组合物包含优选含有Y型沸石的流化催化裂化催化剂组合物和含有孔径范围为约3至约7.2埃的沸石和SiO 2与Al 2 O 3摩尔比小于优选地，NOx还原组合物含有与无机粘合剂结合的NOx还原沸石颗粒。另外，作为催化剂的组成成分，将NOx还原型沸石粒子并入裂化催化剂中。根据本发明的组合物对于在FCC工艺条件下操作的流化床催化裂化装置的再生器中释放的NO x排放的降低非常有效，而没有破裂产物的转化率或产率的显着变化。还公开了使用组合物的方法。

5. 发明授权

US07304011B2 Compositions and processes for reducing NOx emissions during fluid catalytic cracking 有权
标题翻译：在流化床催化裂化过程中减少NOx排放的组成和方法
公开(公告)号：US07304011B2
公开(公告)日：2007-12-04
申请号：US10824913
申请日：2004-04-15
申请人： George Yaluris , Michael Scott Ziebarth , Xinjin Zhao
发明人： George Yaluris , Michael Scott Ziebarth , Xinjin Zhao
IPC分类号： B01J29/80 , B01J29/06
CPC分类号： C10G11/05 , C10G2300/405 , C10G2300/80 , C10G2400/20
摘要： Compositions for reduction of NOx generated during a catalytic cracking process, preferably, a fluid catalytic cracking process, are disclosed. The compositions comprise a fluid catalytic cracking catalyst composition, preferably containing a Y-type zeolite, and a particulate NOx composition containing particles of a zeolite having a pore size ranging from about 3 to about 7.2 Angstoms and a SiO2 to Al2O3 molar ratio of less than about 500. Preferably, the NOx reduction composition contains NOx reduction zeolite particles bound with an inorganic binder. In the alternative, the NOx reduction zeolite particles are incorporated into the cracking catalyst as an integral component of the catalyst. Compositions in accordance with the invention are very effective for the reduction of NOx emissions released from the regenerator of a fluid catalytic cracking unit operating under FCC process conditions without a substantial change in conversion or yield of cracked products, e.g., gasoline and light olefins. Processes for the use of the compositions are also disclosed.
摘要翻译：公开了在催化裂化过程中产生的用于还原NO x x N的组合物，优选流化催化裂化过程。该组合物包含优选含有Y型沸石的流化催化裂化催化剂组合物和含有孔径为约3至约7.2埃的沸石颗粒的颗粒状NO x SiO 2 / SiO 2与Al 2 O 3摩尔比小于约500.优选地，NO x X 3还原组合物含有与无机粘合剂结合的NO x X 3还原沸石颗粒。在替代方案中，将NO x还原沸石颗粒作为催化剂的组成成分加入到裂化催化剂中。根据本发明的组合物对于在FCC工艺条件下操作的流化床催化裂化装置的再生器中释放的NO x NO x的排放非常有效，而没有破裂产物的转化率或产率的实质变化，例如汽油和轻质烯烃。还公开了使用组合物的方法。

6. 发明申请

US20050232839A1 Compositions and processes for reducing NOx emissions during fluid catalytic cracking 审中-公开
标题翻译：在流化床催化裂化过程中减少NOx排放的组成和方法
公开(公告)号：US20050232839A1
公开(公告)日：2005-10-20
申请号：US10909709
申请日：2004-08-02
申请人： George Yaluris , Michael Ziebarth , Xinjin Zhao
发明人： George Yaluris , Michael Ziebarth , Xinjin Zhao
IPC分类号： B01J29/06 , B01J29/08 , B01J29/18 , B01J29/60 , B01J29/70 , B01J29/80 , B01J35/00 , B01J37/00 , C10G11/02 , C10G11/05 , C10G11/18 , C10G11/00
CPC分类号： B01J29/80 , B01J29/06 , B01J29/084 , B01J29/18 , B01J29/60 , B01J29/70 , B01J29/7007 , B01J35/0006 , B01J37/0045 , B01J2229/42 , C10G11/02 , C10G11/05 , C10G11/182 , C10G2300/405 , C10G2300/80 , C10G2400/20
摘要： Compositions for reduction of NOx generated during a catalytic cracking process, preferably, a fluid catalytic cracking process, are disclosed. The compositions comprise a fluid catalytic cracking catalyst composition, preferably containing a Y-type zeolite, and a particulate NOx reduction composition containing particles of a zeolite having a pore size ranging from about 3 to about 7.2 Angstoms and a SiO2 to Al2O3 molar ratio of less than about 500. Preferably, the NOx reduction composition contains NOx reduction zeolite particles bound with an inorganic binder. In the alternative, the NOx reduction zeolite particles are incorporated into the cracking catalyst as an integral component of the catalyst. Compositions in accordance with the invention are very effective for the reduction of NOx emissions released from the regenerator of a fluid catalytic cracking unit operating under FCC process conditions without a substantial change in conversion or yield of cracked products. Processes for the use of the compositions are also disclosed.
摘要翻译：公开了在催化裂化过程中产生的用于还原NO x x N的组合物，优选流化催化裂化过程。组合物包含优选含有Y型沸石的流化催化裂化催化剂组合物和含有孔径范围为约3至约7.2埃的沸石颗粒的颗粒状NO x X还原组合物，以及 SiO 2 / Al 2 O 3摩尔比小于约500.优选地，还原反应组合物含有与无机粘合剂结合的NO x x N还原沸石颗粒。在替代方案中，将NO x还原沸石颗粒作为催化剂的组成成分加入到裂化催化剂中。根据本发明的组合物对于在FCC工艺条件下操作的流化床催化裂化装置的再生器中释放的NO x NO x的排放非常有效，而没有破裂产物的转化率或产率的显着变化。还公开了使用组合物的方法。

7. 发明申请

US20050100493A1 Ferrierite compositions for reducing NOx emissions during fluid catalytic cracking 审中-公开
标题翻译：用于在流化床催化裂化过程中减少NOx排放的镁碱沸石组合物
公开(公告)号：US20050100493A1
公开(公告)日：2005-05-12
申请号：US10702240
申请日：2003-11-06
申请人： George Yaluris , Michael Ziebarth , Xinjin Zhao
发明人： George Yaluris , Michael Ziebarth , Xinjin Zhao
IPC分类号： B01D53/86 , B01J23/42 , B01J23/83 , B01J29/08 , B01J29/65 , B01J29/80 , B01J35/00 , B01J37/00 , C10G11/18 , B01J29/04 , B01J21/00 , B01J29/00 , B01J29/87 , C01B21/00
CPC分类号： C10G11/18 , B01D53/8628 , B01D2255/50 , B01D2258/00 , B01J23/42 , B01J23/83 , B01J29/084 , B01J29/65 , B01J29/80 , B01J35/0006 , B01J35/002 , B01J37/0045 , B01J2229/18 , B01J2229/42
摘要： Compositions for reduction of NOx generated during a catalytic cracking process, preferably, a fluid catalytic cracking process, are disclosed. The compositions comprise a fluid catalytic cracking catalyst composition, preferably containing a Y-type zeolite, and a particulate NOx composition containing ferrierite zeolite particles. Preferably, the NOx reduction composition contains ferrierite zeolite particles bound with an inorganic binder. In the alternative, the ferrierite zeolite particles are incorporated into the cracking catalyst as an integral component of the catalyst. NOx reduction compositions in accordance with the invention are very effective for the reduction of NOx emissions released from the regenerator of a fluid catalytic cracking unit operating under FCC process conditions without a substantial change in conversion or yield of cracked products, e.g., gasoline and light olefins. Processes for the use of the compositions are also disclosed.
摘要翻译：公开了在催化裂化过程中产生的用于还原NO x x N的组合物，优选流化催化裂化过程。组合物包含优选含有Y型沸石的流化催化裂化催化剂组合物和含有镁碱沸石颗粒的颗粒状NO x组合物。优选地，NO x X还原组合物含有与无机粘合剂结合的镁碱沸石颗粒。替代方案中，镁碱沸石颗粒作为催化剂的组成成分加入到裂化催化剂中。根据本发明的NO x x还原组合物对于在FCC工艺条件下操作的流化催化裂化装置的再生器中释放的NO x x N 2排放非常有效，裂解产物（例如汽油和轻质烯烃）的转化率或产率的显着变化。还公开了使用组合物的方法。

8. 发明授权

US07976697B2 NOX reduction compositions for use in partial burn FCC processes 有权
标题翻译：用于部分燃烧FCC工艺的NOX还原组合物
公开(公告)号：US07976697B2
公开(公告)日：2011-07-12
申请号：US11918085
申请日：2006-03-24
申请人： M. Sundaram Krishnamoorthy , Michael Scott Ziebarth , George Yaluris , Roger Jean Lussier , John Allen Rudesill
发明人： M. Sundaram Krishnamoorthy , Michael Scott Ziebarth , George Yaluris , Roger Jean Lussier , John Allen Rudesill
IPC分类号： C10G11/05 , B01J29/068 , B01J29/08
CPC分类号： B01J29/068 , B01J29/084 , B01J29/67 , B01J29/80 , B01J35/023 , B01J2229/20 , B01J2229/42 , C10G11/05 , C10G11/182 , C10G2300/405 , C10G2300/80
摘要： A NOx reduction composition and process of using the composition to reduce the content of NOx emissions and gas phase reduced nitrogen species released from the regeneration zone during fluid catalytic cracking of a hydrocarbon feedstock into lower molecular weight components is disclosed. The process comprises contacting a hydrocarbon feedstock during a fluid catalytic cracking (FCC) process wherein a regeneration zone of an fluid catalytic cracking unit (FCCU) is operated in a partial or incomplete combustion mode under FCC conditions, with a circulating inventory of an FCC cracking catalyst and a particulate NOx reduction composition. The NOx reduction composition has a mean particle size of greater than 45 μm and comprises (1) a zeolite component having (i) a pore size of form 2-7 A Angstroms and (ii) a SiO2 to Al2O3 molar ratio of less than 500, and (2) at least one noble metal selected from the group consisting of platinum, palladium, rhodium, iridium, osmium, ruthenium, rhenium and mixtures thereof.
摘要翻译：公开了一种NOx还原组合物和使用该组合物以减少在烃原料进入较低分子量组分的流化催化裂化期间从再生区释放的NOx排放物和气相还原氮物质的含量的方法。该方法包括在流化催化裂化（FCC）方法期间使烃原料接触，其中流化催化裂化装置（FCCU）的再生区在FCC条件下以部分或不完全燃烧模式操作，FCC循环库存催化剂和微粒NOx还原组合物。 NOx还原组合物具有大于45μm的平均粒度，并且包括（1）具有（i）2-7A埃的孔径和（ii）SiO 2与Al 2 O 3摩尔比小于500的沸石组分，和（2）选自铂，钯，铑，铱，锇，钌，铼中的至少一种贵金属及其混合物。

9. 发明申请

US20090050527A1 NOchi Reduction Compositions for Use in Partial Burn FCC Processes 有权
标题翻译：用于部分燃烧FCC过程的NOC还原组合物
公开(公告)号：US20090050527A1
公开(公告)日：2009-02-26
申请号：US11918085
申请日：2006-03-24
申请人： M. Sundaram Krishnamoorthy , Michael Scott Ziebarth , George Yaluris , Roger Jean Lussier , John Allen Rudesill
发明人： M. Sundaram Krishnamoorthy , Michael Scott Ziebarth , George Yaluris , Roger Jean Lussier , John Allen Rudesill
IPC分类号： C10G11/00 , B01J29/068 , B01J21/12
CPC分类号： B01J29/068 , B01J29/084 , B01J29/67 , B01J29/80 , B01J35/023 , B01J2229/20 , B01J2229/42 , C10G11/05 , C10G11/182 , C10G2300/405 , C10G2300/80
摘要： A NOx reduction composition and process of using the composition to reduce the content of NOx emissions and gas phase reduced nitrogen species released from the regeneration zone during fluid catalytic cracking of a hydrocarbon feedstock into lower molecular weight components is disclosed. The process comprises contacting a hydrocarbon feedstock during a fluid catalytic cracking (FCC) process wherein a regeneration zone of an fluid catalytic cracking unit (FCCU) is operated in a partial or incomplete combustion mode under FCC conditions, with a circulating inventory of an FCC cracking catalyst and a particulate NOx reduction composition. The NOx reduction composition has a mean particle size of greater than 45 μm and comprises (1) a zeolite component having (i) a pore size of form 2-7 A Angstroms and (ii) a SiO2 to Al2O3 molar ratio of less than 500, and (2) at least one noble metal selected from the group consisting of platinum, palladium, rhodium, iridium, osmium, ruthenium, rhenium and mixtures thereof.
摘要翻译：公开了一种NOx还原组合物和使用该组合物以减少在烃原料进入较低分子量组分的流化催化裂化期间从再生区释放的NOx排放物和气相还原氮物质的含量的方法。该方法包括在流化催化裂化（FCC）方法期间使烃原料接触，其中流化催化裂化装置（FCCU）的再生区在FCC条件下以部分或不完全燃烧模式操作，FCC循环库存催化剂和微粒NOx还原组合物。 NOx还原组合物具有大于45μm的平均粒度，并且包括（1）具有（i）2-7A埃的孔径和（ii）SiO 2与Al 2 O 3摩尔比小于500的沸石组分，和（2）选自铂，钯，铑，铱，锇，钌，铼中的至少一种贵金属及其混合物。

10. 发明申请

US20050230285A1 Compositions and processes for reducing NOx emissions during fluid catalytic cracking 有权
标题翻译：在流化床催化裂化过程中减少NOx排放的组成和方法
公开(公告)号：US20050230285A1
公开(公告)日：2005-10-20
申请号：US10824913
申请日：2004-04-15
申请人： George Yaluris , Michael Ziebarth , Xinjin Zhao
发明人： George Yaluris , Michael Ziebarth , Xinjin Zhao
IPC分类号： C10G11/05
CPC分类号： C10G11/05 , C10G2300/405 , C10G2300/80 , C10G2400/20
摘要： Compositions for reduction of NOx generated during a catalytic cracking process, preferably, a fluid catalytic cracking process, are disclosed. The compositions comprise a fluid catalytic cracking catalyst composition, preferably containing a Y-type zeolite, and a particulate NOx composition containing particles of a zeolite having a pore size ranging from about 3 to about 7.2 Angstoms and a SiO2 to Al2O3 molar ratio of less than about 500. Preferably, the NOx reduction composition contains NOx reduction zeolite particles bound with an inorganic binder. In the alternative, the NOx reduction zeolite particles are incorporated into the cracking catalyst as an integral component of the catalyst. Compositions in accordance with the invention are very effective for the reduction of NOx emissions released from the regenerator of a fluid catalytic cracking unit operating under FCC process conditions without a substantial change in conversion or yield of cracked products, e.g., gasoline and light olefins. Processes for the use of the compositions are also disclosed.
摘要翻译：公开了在催化裂化过程中产生的用于还原NO x x N的组合物，优选流化催化裂化过程。该组合物包含优选含有Y型沸石的流化催化裂化催化剂组合物和含有孔径为约3至约7.2埃的沸石颗粒的颗粒状NO x SiO 2 / SiO 2与Al 2 O 3摩尔比小于约500.优选地，NO x X 3还原组合物含有与无机粘合剂结合的NO x X 3还原沸石颗粒。在替代方案中，将NO x还原沸石颗粒作为催化剂的组成成分加入到裂化催化剂中。根据本发明的组合物对于在FCC工艺条件下操作的流化床催化裂化装置的再生器中释放的NO x NO x的排放非常有效，而没有破裂产物的转化率或产率的实质变化，例如汽油和轻质烯烃。还公开了使用组合物的方法。

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