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1. 发明授权

US06784332B1 Processes employing hydrocarbon conversion catalyst 失效
标题翻译：使用烃转化催化剂的方法
公开(公告)号：US06784332B1
公开(公告)日：2004-08-31
申请号：US09691494
申请日：2000-10-18
申请人： James B. Kimble , Charles A. Drake , Jianhua Yao , An-hsiang Wu
发明人： James B. Kimble , Charles A. Drake , Jianhua Yao , An-hsiang Wu
IPC分类号： C07C510
CPC分类号： B01J29/40 , B01J2229/26 , B01J2229/36 , B01J2229/42 , C10G35/095
摘要： A hydrocarbon conversion process comprising contacting a hydrocarbon stream such as, for example, gasoline, with a catalyst composition to effect the conversion of the hydrocarbon to olefins and C6 to C8 aromatic hydrocarbons such as toluene and xylenes. The catalyst composition comprises a zeolite, a promoter and optionally a binder.
摘要翻译：烃转化方法包括使烃流例如汽油与催化剂组合物接触，以使碳氢化合物转化为烯烃和C 6至C 8芳族烃如甲苯和二甲苯。催化剂组合物包含沸石，助催化剂和任选的粘合剂。

2. 发明授权

US06395949B1 Acid treated zeolite containing phosphorus used as a catalyst in processes for converting hydrocarbons, and use of binary hydrocarbon mixtures as diluents in processes for converting hydrocarbons 失效
标题翻译：含有磷的酸处理沸石在用于转化烃的方法中用作催化剂，并且在转化烃的方法中使用二元烃混合物作为稀释剂
公开(公告)号：US06395949B1
公开(公告)日：2002-05-28
申请号：US09627103
申请日：2000-07-27
申请人： Charles A. Drake , Jianhua Yao
发明人： Charles A. Drake , Jianhua Yao
IPC分类号： C07C402
CPC分类号： C10G35/095 , B01J27/182 , B01J29/40 , C10G2400/22 , C10G2400/30
摘要： A method of increasing total diluent conversion in a process for the conversion of cracked gasoline and a first diluent comprising iso-pentane to aromatics and light olefins by contacting the cracked gasoline, the first diluent and a second diluent comprising either propane or 1-hexene with a zeolite catalyst containing phosphorus. The zeolite catalyst comprises a calcined, acid-leached zeolite and phosphorus. Also described is a method of making such catalyst.
摘要翻译：一种在裂化汽油转化方法中提高总稀释剂转化率的方法，以及将包含异戊烷的第一稀释剂与芳族化合物和轻质烯烃转化的方法，该方法是将裂化汽油，第一稀释剂和包含丙烷或1-己烯的第二稀释剂与含磷的沸石催化剂。沸石催化剂包括煅烧的，酸浸的沸石和磷。还描述了制备这种催化剂的方法。

3. 发明授权

US6084142A Method of making an improved zeolite catalyst, a product from such method, and the use thereof in the conversion of hydrocarbons 失效
标题翻译：制备改进的沸石催化剂的方法，这种方法的产物及其在烃转化中的用途
公开(公告)号：US6084142A
公开(公告)日：2000-07-04
申请号：US76690
申请日：1998-05-12
申请人： Jianhua Yao , Charles A. Drake
发明人： Jianhua Yao , Charles A. Drake
IPC分类号： C10G11/05 , C10G35/095 , C07C15/00
CPC分类号： C10G35/095 , C10G2400/20
摘要： An improved zeolite catalyst containing a zeolite and a zinc component manufactured by a novel method having certain process steps necessary for providing the improved zeolite catalyst. The process steps include incorporation of a zinc component with such zeolite followed by a steam treatment. An acid treatment can be conducted after the steam treatment. Processes are also disclosed for using the improved zeolite catalyst in the conversion of hydrocarbons, preferably non-aromatic hydrocarbons, to lower olefins (such as ethylene, propylene, and butene) and aromatic hydrocarbons (such as benzene, toluene, and xylene).
摘要翻译：一种含有沸石和锌组分的改进的沸石催化剂，其通过具有提供改进的沸石催化剂所需的一些工艺步骤的新方法制备。工艺步骤包括将锌组分与这种沸石并入，然后进行蒸汽处理。蒸汽处理后可以进行酸处理。还公开了使用改进的沸石催化剂将烃，优选非芳族烃转化为低级烯烃（如乙烯，丙烯和丁烯）和芳族烃（如苯，甲苯和二甲苯）的方法。

4. 发明授权

US06638892B1 Syngas conversion and catalyst system employed therefor 有权
标题翻译：合成气转化和催化剂体系
公开(公告)号：US06638892B1
公开(公告)日：2003-10-28
申请号：US10125661
申请日：2002-04-18
申请人： An-hsiang Wu , Jianhua Yao , Charles A. Drake
发明人： An-hsiang Wu , Jianhua Yao , Charles A. Drake
IPC分类号： B01J2300
CPC分类号： C07C41/01 , B01J23/80 , B01J29/084 , B01J29/85 , B01J35/0006 , C07C1/20 , C07C2529/85 , C07C11/02 , C07C43/043
摘要： A process for the conversion of syngas by contact of syngas under conversion conditions with catalyst having as components zinc oxide, copper oxide, aluminum oxide, Y zeolite and clay in which (A) in a one step process for conversion of syngas to dimethyl ether, the catalyst has as components an extruded mixture of zinc oxide, copper oxide, gamma aluminum oxide, Y zeolite and clay; (B) in a two step process for conversion of syngas to light olefins, a catalyst system is employed that has in the first step a catalyst mixture of zinc oxide, copper oxide, aluminum oxide, Y zeolite and clay and the catalyst employed in the second step is SAPO-34; SAPO-34 modified with lanthanum(III) nitrate hexahydrate; SAPO-34 modified with magnesium nitrate hexahydrate; SAPO-34 modified with tributyl borate or SAPO-34 modified with triethyl phosphate or (C) in a two step process for conversion of syngas to light olefins, the pressure on the effluent from the contact of syngas with a mixture of zinc oxide, copper oxide, aluminum oxide, Y zeolite and clay is reduced before contact with a second catalyst of SAPO-34. The catalyst systems employed in the processes herein.
摘要翻译：通过合成气在转化条件下与作为组分氧化锌，氧化铜，氧化铝，Y沸石和粘土的组分的催化剂接触合成气的方法，其中（A）在将合成气转化为二甲醚的一步法中，催化剂具有氧化锌，氧化铜，γ氧化铝，Y沸石和粘土的挤出混合物的组分; （B）在将合成气转化为轻质烯烃的两步法中，采用了催化剂体系，该催化剂体系在第一步中是氧化锌，氧化铜，氧化铝，Y沸石和粘土的催化剂混合物，第二步是SAPO-34; 用硝酸镧（III）六水合物修饰的SAPO-34; SAPO-34用硝酸镁六水合物改性; 用硼酸三丁酯或用三乙基磷酸酯改性的SAPO-34改性的SAPO-34或（C）在将合成气转化为轻质烯烃的两步法中，合成气与氧化锌，铜的混合物接触的流出物的压力氧化物，氧化铝，Y沸石和粘土在与SAPO-34的第二催化剂接触之前还原。本文工艺中使用的催化剂体系。

5. 发明授权

US6156689A Catalyst composition comprising zinc compound or boron compound and hydrocarbon conversion process 失效
标题翻译：包含锌化合物或硼化合物和烃转化方法的催化剂组合物
公开(公告)号：US6156689A
公开(公告)日：2000-12-05
申请号：US956082
申请日：1997-10-23
申请人： James B. Kimble , Charles A. Drake , Jianhua Yao , An-hsiang Wu
发明人： James B. Kimble , Charles A. Drake , Jianhua Yao , An-hsiang Wu
IPC分类号： B01J29/40 , C10G35/095 , B01J29/06
CPC分类号： B01J29/40 , C10G35/095 , B01J2229/26 , B01J2229/36 , B01J2229/42
摘要： A catalyst composition, a process for producing the composition, and a hydrocarbon conversion process for converting a hydrocarbon stream such as, for example, gasoline, to olefins and C.sub.6 to C.sub.8 aromatic hydrocarbons such as toluene and xylenes are disclosed. The catalyst composition comprises a zeolite, a promoter and optionally a binder. The process for producing the composition comprises the steps: (1) combining a zeolite with a promoter under a condition sufficient to produce a modified zeolite; and (2) steaming the modified zeolite. The hydrocarbon conversion process comprises contacting a hydrocarbon stream with the catalyst composition under a condition sufficient to effect the conversion of a hydrocarbon to an olefin and a C.sub.6 to C.sub.8 aromatic hydrocarbon.
摘要翻译：公开了一种催化剂组合物，该组合物的制备方法以及用于将烃流例如汽油转化为烯烃和C 6至C 8芳族烃如甲苯和二甲苯的烃转化方法。催化剂组合物包含沸石，助催化剂和任选的粘合剂。制备组合物的方法包括以下步骤：（1）在足以产生改性沸石的条件下将沸石与促进剂组合; 和（2）蒸发改性沸石。烃转化方法包括在足以使烃转化为烯烃和C 6至C 8芳族烃的条件下使烃流与催化剂组合物接触。

6. 发明授权

US5981418A Zeolite based catalyst containing zinc, boron and phosphorus and method of making such zeolite based catalyst 失效
公开(公告)号：US5981418A
公开(公告)日：1999-11-09
申请号：US57048
申请日：1998-04-08
申请人： Charles A. Drake , An-hsiang Wu , Jianhua Yao
发明人： Charles A. Drake , An-hsiang Wu , Jianhua Yao
IPC分类号： B01J29/06 , B01J29/40
CPC分类号： B01J29/061 , B01J2229/16
摘要： A novel composition including either a zeolite or an acid leached zeolite containing boron, zinc and phosphorus, used in the conversion of hydrocarbons. The novel composition is prepared by a novel method including incorporating into a zeolite or an acid treated zeolite material, preferably by use of a liquid solution, a zinc component, a boron component, and a phosphorus component.

7. 发明授权

US06235955B1 Hydrocarbon conversion processess 失效
标题翻译：烃转化过程
公开(公告)号：US06235955B1
公开(公告)日：2001-05-22
申请号：US09632892
申请日：2000-08-07
申请人： Jianhua Yao , Charles A. Drake
发明人： Jianhua Yao , Charles A. Drake
IPC分类号： C07C252
CPC分类号： C10G35/095 , B01J29/061 , C10G2400/20
摘要： A composition, a process for producing the composition, and a hydrocarbon conversion process for converting a hydrocarbon stream such as, for example, gasoline, to olefins and C6 to C8 aromatic hydrocarbons such as toluene and xylenes are disclosed. The composition comprises a silylated catalyst which comprises a zeolite, a clay or silica, and a promoter. The process for producing the composition comprises the steps: (1) combining a zeolite with a clay or silica and a promoter under a condition sufficient to bind the clay to the zeolite to produce a clay-bound zeolite; (2) heating the clay-bound zeolite to produce a modified zeolite; and (3) silylating the modified zeolite with a silylating agent. The hydrocarbon conversion process comprises contacting a hydrocarbon stream with the catalyst composition under a condition sufficient to effect the conversion of a hydrocarbon to an olefin and a C6 to C8 aromatic hydrocarbon.
摘要翻译：公开了一种组合物，该组合物的制备方法以及用于将烃流例如汽油转化为烯烃和C 6至C 8芳族烃如甲苯和二甲苯的烃转化方法。该组合物包含甲硅烷基化催化剂，其包含沸石，粘土或二氧化硅和助催化剂。制备组合物的方法包括以下步骤：（1）在足以将粘土结合到沸石以产生粘土结合的沸石的条件下，将沸石与粘土或二氧化硅和助催化剂组合; （2）加热粘土结合的沸石以产生改性沸石; 和（3）用甲硅烷基化剂使改性沸石甲硅烷基化。烃转化方法包括在足以使烃转化为烯烃和C 6至C 8芳族烃的条件下使烃流与催化剂组合物接触。

8. 发明授权

US06218590B1 Zeolite material, a method of making such improved zeolite material and the use thereof in the conversion of non-aromatic hydrocarbons to aromatics and light olefins 失效
标题翻译：沸石材料，制备这种改进的沸石材料的方法及其在非芳族烃转化成芳族化合物和轻质烯烃的用途
公开(公告)号：US06218590B1
公开(公告)日：2001-04-17
申请号：US09510767
申请日：2000-02-23
申请人： Jianhua Yao , James B. Kimble , Charles A. Drake
发明人： Jianhua Yao , James B. Kimble , Charles A. Drake
IPC分类号： C07C252
CPC分类号： B01J37/0009 , B01J23/005 , B01J29/06 , B01J29/40 , B01J29/405 , B01J35/0006 , C10G35/095
摘要： A novel high stability catalyst composition comprising a mixture of zeolite and zinc spinel that has been treated with a reducing gas under high temperature conditions, a method of making such high stability catalyst, and the use thereof for converting paraffin hydrocarbons to olefins and aromatics.
摘要翻译：一种新型的高稳定性催化剂组合物，其包含在高温条件下用还原气体处理的沸石和尖晶石的混合物，制备这种高稳定性催化剂的方法及其用于将链烷烃转化为烯烃和芳族化合物的用途。

9. 发明授权

US6124227A Hydrocarbon conversion catalyst composition and processes therefor and therewith 失效
标题翻译：烃转化催化剂组合物及其工艺及其
公开(公告)号：US6124227A
公开(公告)日：2000-09-26
申请号：US143321
申请日：1998-08-28
申请人： Jianhua Yao , Charles A. Drake
发明人： Jianhua Yao , Charles A. Drake
IPC分类号： B01J29/06 , B01J31/02 , C10G11/05 , C10G35/095
CPC分类号： C10G35/095 , B01J29/061 , C10G2400/20
摘要： A composition, a process for producing the composition, and a hydrocarbon conversion process for converting a hydrocarbon stream such as, for example, gasoline, to olefins and C.sub.6 to C.sub.8 aromatic hydrocarbons such as toluene and xylenes are disclosed. The composition comprises a silylated catalyst which comprises a zeolite, a clay or silica, and a promoter. The process for producing the composition comprises the steps: (1) combining a zeolite with a clay or silica and a promoter under a condition sufficient to bind the clay to the zeolite to produce a clay-bound zeolite; (2) heating the clay-bound zeolite to produce a modified zeolite; and (3) silylating the modified zeolite with a silylating agent. The hydrocarbon conversion process comprises contacting a hydrocarbon stream with the catalyst composition under a condition sufficient to effect the conversion of a hydrocarbon to an olefin and a C.sub.6 to C.sub.8 aromatic hydrocarbon.
摘要翻译：公开了一种组合物，该组合物的制备方法以及用于将烃流例如汽油转化为烯烃和C 6至C 8芳族烃如甲苯和二甲苯的烃转化方法。该组合物包含甲硅烷基化催化剂，其包含沸石，粘土或二氧化硅和助催化剂。制备组合物的方法包括以下步骤：（1）在足以将粘土结合到沸石以产生粘土结合的沸石的条件下，将沸石与粘土或二氧化硅和助催化剂组合; （2）加热粘土结合的沸石以产生改性沸石; 和（3）用甲硅烷基化剂使改性沸石甲硅烷基化。烃转化方法包括在足以使烃转化为烯烃和C 6至C 8芳族烃的条件下使烃流与催化剂组合物接触。

10. 发明授权

US6090990A Method of making an improved catalyst containing zeolite treated with boron trichloride, the product from such method, and the use thereof in the conversion of hydrocarbons 失效
标题翻译：制备含有三氯化硼处理的沸石的改进的催化剂的方法，该方法的产物及其在烃转化中的用途
公开(公告)号：US6090990A
公开(公告)日：2000-07-18
申请号：US35198
申请日：1998-03-05
申请人： Jianhua Yao , Charles A. Drake
发明人： Jianhua Yao , Charles A. Drake
IPC分类号： B01J29/40 , B01J37/00 , B01J37/02 , C10G35/095 , C07C2/52 , C07C4/02 , C10G35/06
CPC分类号： B01J37/0238 , B01J29/40 , B01J37/0009 , C10G35/095 , B01J2229/26 , B01J2229/42 , Y10S585/906
摘要： An improved zeolite based catalyst comprising a mixture of a zeolite and a binder treated with boron trichloride and prepared by a novel method including exposing a mixture of a zeolite material and a binder to gaseous boron trichloride under suitable process conditions.
摘要翻译：一种改进的沸石基催化剂，其包括沸石和用三氯化硼处理的粘合剂的混合物，并通过新的方法制备，包括在合适的工艺条件下将沸石材料和粘合剂的混合物暴露于气态三氯化硼。

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