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1. 发明授权

US06784332B1 Processes employing hydrocarbon conversion catalyst 失效
标题翻译：使用烃转化催化剂的方法
公开(公告)号：US06784332B1
公开(公告)日：2004-08-31
申请号：US09691494
申请日：2000-10-18
申请人： James B. Kimble , Charles A. Drake , Jianhua Yao , An-hsiang Wu
发明人： James B. Kimble , Charles A. Drake , Jianhua Yao , An-hsiang Wu
IPC分类号： C07C510
CPC分类号： B01J29/40 , B01J2229/26 , B01J2229/36 , B01J2229/42 , C10G35/095
摘要： A hydrocarbon conversion process comprising contacting a hydrocarbon stream such as, for example, gasoline, with a catalyst composition to effect the conversion of the hydrocarbon to olefins and C6 to C8 aromatic hydrocarbons such as toluene and xylenes. The catalyst composition comprises a zeolite, a promoter and optionally a binder.
摘要翻译：烃转化方法包括使烃流例如汽油与催化剂组合物接触，以使碳氢化合物转化为烯烃和C 6至C 8芳族烃如甲苯和二甲苯。催化剂组合物包含沸石，助催化剂和任选的粘合剂。

2. 发明授权

US06593503B1 Process for making aromatic hydrocarbons using an acid treated zeolite 失效
标题翻译：使用酸处理的沸石制备芳烃的方法
公开(公告)号：US06593503B1
公开(公告)日：2003-07-15
申请号：US08695482
申请日：1996-08-12
申请人： An-hsiang Wu , Charles A. Drake , Ralph J. Melton
发明人： An-hsiang Wu , Charles A. Drake , Ralph J. Melton
IPC分类号： C07C600
CPC分类号： C07C6/10 , C07C2529/40 , C07C15/02
摘要： A catalyst composition and a process for converting a hydrocarbon stream such as, for example, gasoline to C6 to C8 aromatic hydrocarbons such as toluene and xylenes are disclosed. The catalyst composition includes an alumina, a silica, and a metal wherein the weight ratio of aluminum to silicon is in the range of from about 0.002:1 to about 0.6:1. The process includes contacting a hydrocarbon stream with the catalyst composition under a condition sufficient to effect the conversion of a hydrocarbon to a C6 to C8 aromatic hydrocarbon. Also disclosed is a process for producing the catalyst composition which includes: (1) contacting a zeolite with an effective amount of an acid under a condition sufficient to effect a reduction in aluminum content of the zeolite to produce an acid-leached zeolite; and (2) impregnating the acid-leached zeolite with an effective amount of a metal compound under a condition sufficient to effect the production of a metal-promoted zeolite.
摘要翻译：公开了一种催化剂组合物和将烃流例如汽油转化为C 6至C 8芳族烃如甲苯和二甲苯的方法。催化剂组合物包括氧化铝，二氧化硅和金属，其中铝与硅的重量比在约0.002:1至约0.6:1的范围内。该方法包括使烃流与催化剂组合物在足以使碳氢化合物转化为C 6至C 8芳族烃的条件下接触。还公开了一种生产催化剂组合物的方法，其包括：（1）在足以使沸石的铝含量降低以产生酸浸出的沸石的条件下使沸石与有效量的酸接触; 和（2）在足以产生金属促进的沸石的条件下，用有效量的金属化合物浸渍酸浸出的沸石。

3. 发明授权

US06420295B1 Hydrocarbon conversion catalyst composition and process therefor and therewith 失效
标题翻译：烃转化催化剂组合物及其工艺及其
公开(公告)号：US06420295B1
公开(公告)日：2002-07-16
申请号：US09634492
申请日：2000-08-08
申请人： An-hsiang Wu , Charles A. Drake
发明人： An-hsiang Wu , Charles A. Drake
IPC分类号： B01J2940
CPC分类号： B01J37/0203 , B01J29/061 , B01J29/40 , B01J37/086 , B01J2229/26 , B01J2229/36 , B01J2229/42 , C10G35/095
摘要： A catalyst composition, a process for producing the catalyst composition, and a hydroconversion process for converting a fluid stream comprising at least one saturated hydrocarbon to C6 to C8 aromatic hydrocarbons such as benzene, toluene, and xylenes are disclosed. The catalyst composition comprises a zeolite and a promoter. The process for producing the composition comprises the steps of: (1) combining a zeolite with a complexing ligand and a promoter compound under a condition sufficient to produce a modified zeolite; and (2) heating the modified zeolite to produce a promoted zeolite. The hydroconversion process comprises contacting a fluid stream with the catalyst composition under a condition sufficient to effect the conversion of a saturated hydrocarbon to a C6 to C8 aromatic hydrocarbon.
摘要翻译：公开了一种催化剂组合物，用于制备催化剂组合物的方法和用于将包含至少一种饱和烃的流体流转化为C 6至C 8芳族烃如苯，甲苯和二甲苯的加氢转化方法。催化剂组合物包含沸石和助催化剂。制备组合物的方法包括以下步骤：（1）在足以产生改性沸石的条件下将沸石与络合配体和助催化剂化合物结合; 和（2）加热改性沸石以产生促进的沸石。加氢转化方法包括在足以使饱和烃转化为C6至C8芳族烃的条件下使流体物流与催化剂组合物接触。

4. 发明授权

US06395949B1 Acid treated zeolite containing phosphorus used as a catalyst in processes for converting hydrocarbons, and use of binary hydrocarbon mixtures as diluents in processes for converting hydrocarbons 失效
标题翻译：含有磷的酸处理沸石在用于转化烃的方法中用作催化剂，并且在转化烃的方法中使用二元烃混合物作为稀释剂
公开(公告)号：US06395949B1
公开(公告)日：2002-05-28
申请号：US09627103
申请日：2000-07-27
申请人： Charles A. Drake , Jianhua Yao
发明人： Charles A. Drake , Jianhua Yao
IPC分类号： C07C402
CPC分类号： C10G35/095 , B01J27/182 , B01J29/40 , C10G2400/22 , C10G2400/30
摘要： A method of increasing total diluent conversion in a process for the conversion of cracked gasoline and a first diluent comprising iso-pentane to aromatics and light olefins by contacting the cracked gasoline, the first diluent and a second diluent comprising either propane or 1-hexene with a zeolite catalyst containing phosphorus. The zeolite catalyst comprises a calcined, acid-leached zeolite and phosphorus. Also described is a method of making such catalyst.
摘要翻译：一种在裂化汽油转化方法中提高总稀释剂转化率的方法，以及将包含异戊烷的第一稀释剂与芳族化合物和轻质烯烃转化的方法，该方法是将裂化汽油，第一稀释剂和包含丙烷或1-己烯的第二稀释剂与含磷的沸石催化剂。沸石催化剂包括煅烧的，酸浸的沸石和磷。还描述了制备这种催化剂的方法。

5. 发明授权

US06235954B1 Hydrocarbon hydrogenation catalyst and process 失效
公开(公告)号：US06235954B1
公开(公告)日：2001-05-22
申请号：US09408824
申请日：1999-09-29
申请人： An-hsiang Wu , Charles A. Drake
发明人： An-hsiang Wu , Charles A. Drake
IPC分类号： C07C505
CPC分类号： C10G45/34 , B01J29/076 , C07C5/03 , C07C2529/076
摘要： A catalyst composition and process for preparing such catalyst composition which can be useful in contacting a hydrocarbon-containing fluid which contains a highly unsaturated hydrocarbon such as 1,3-butadiene, in the presence of hydrogen, with such catalyst composition in a hydrogenation zone under a hydrogenation condition effective to hydrogenate such highly unsaturated hydrocarbon to a less unsaturated hydrocarbon such as n-butene is disclosed. Such process for preparing a catalyst composition includes (1) combining a zeolite, a Group VIB metal, and an inorganic support to form a modified zeolite; (2) calcining such modified zeolite under a calcining condition to produce a calcined, modified zeolite; and (3) contacting such calcined, modified zeolite with a carburizing agent under a carburizing condition to provide such catalyst composition.

6. 发明授权

US6124515A Catalytic conversion of a saturated hydrocarbon to an aromatic hydrocarbon 失效
标题翻译：将饱和烃催化转化成芳烃
公开(公告)号：US6124515A
公开(公告)日：2000-09-26
申请号：US404669
申请日：1999-09-23
申请人： An-hsiang Wu , Charles A. Drake
发明人： An-hsiang Wu , Charles A. Drake
IPC分类号： B01J29/06 , B01J29/40 , B01J37/02 , B01J37/08 , C10G35/095 , C07C2/52 , C07C6/00 , C10G35/06
CPC分类号： B01J37/0203 , B01J29/061 , B01J29/40 , B01J37/086 , C10G35/095 , B01J2229/26 , B01J2229/36 , B01J2229/42
摘要： A catalyst composition, a process for producing the catalyst composition, and a hydroconversion process for converting a fluid stream comprising at least one saturated hydrocarbon to C.sub.6 to C.sub.8 aromatic hydrocarbons such as benzene, toluene, and xylenes are disclosed. The catalyst composition comprises a zeolite and a promoter. The process for producing the composition comprises the steps of: (1) combining a zeolite with a complexing ligand and a promoter compound under a condition sufficient to produce a modified zeolite; and (2) heating the modified zeolite to produce a promoted zeolite. The hydroconversion process comprises contacting a fluid stream with the catalyst composition under a condition sufficient to effect the conversion of a saturated hydrocarbon to a C.sub.6 to C.sub.8 aromatic hydrocarbon.
摘要翻译：公开了一种催化剂组合物，用于制备催化剂组合物的方法和用于将包含至少一种饱和烃的流体流转化为C 6至C 8芳族烃如苯，甲苯和二甲苯的加氢转化方法。催化剂组合物包含沸石和助催化剂。制备组合物的方法包括以下步骤：（1）在足以产生改性沸石的条件下将沸石与络合配体和助催化剂化合物结合; 和（2）加热改性沸石以产生促进的沸石。加氢转化方法包括在足以使饱和烃转化为C6至C8芳族烃的条件下使流体物流与催化剂组合物接触。

7. 发明授权

US6084142A Method of making an improved zeolite catalyst, a product from such method, and the use thereof in the conversion of hydrocarbons 失效
标题翻译：制备改进的沸石催化剂的方法，这种方法的产物及其在烃转化中的用途
公开(公告)号：US6084142A
公开(公告)日：2000-07-04
申请号：US76690
申请日：1998-05-12
申请人： Jianhua Yao , Charles A. Drake
发明人： Jianhua Yao , Charles A. Drake
IPC分类号： C10G11/05 , C10G35/095 , C07C15/00
CPC分类号： C10G35/095 , C10G2400/20
摘要： An improved zeolite catalyst containing a zeolite and a zinc component manufactured by a novel method having certain process steps necessary for providing the improved zeolite catalyst. The process steps include incorporation of a zinc component with such zeolite followed by a steam treatment. An acid treatment can be conducted after the steam treatment. Processes are also disclosed for using the improved zeolite catalyst in the conversion of hydrocarbons, preferably non-aromatic hydrocarbons, to lower olefins (such as ethylene, propylene, and butene) and aromatic hydrocarbons (such as benzene, toluene, and xylene).
摘要翻译：一种含有沸石和锌组分的改进的沸石催化剂，其通过具有提供改进的沸石催化剂所需的一些工艺步骤的新方法制备。工艺步骤包括将锌组分与这种沸石并入，然后进行蒸汽处理。蒸汽处理后可以进行酸处理。还公开了使用改进的沸石催化剂将烃，优选非芳族烃转化为低级烯烃（如乙烯，丙烯和丁烯）和芳族烃（如苯，甲苯和二甲苯）的方法。

8. 发明授权

US6080697A Process for making a composition that is useful for converting lower value aromatics to higher value aromatics 失效
标题翻译：制备可用于将较低价值芳族化合物转化为较高价值芳族化合物的组合物的方法
公开(公告)号：US6080697A
公开(公告)日：2000-06-27
申请号：US167910
申请日：1998-10-07
申请人： An-hsiang Wu , Charles A. Drake
发明人： An-hsiang Wu , Charles A. Drake
IPC分类号： B01J29/00 , B01J29/06 , B01J29/40 , B01J29/82 , B01J37/00 , B01J29/04 , B01J27/14 , B01J31/00
CPC分类号： B01J29/06 , B01J29/005 , B01J37/0009 , B01J2229/12 , B01J2229/32 , B01J2229/34 , B01J2229/42 , B01J29/40 , B01J29/82
摘要： A process to produce a composition is provided. Said process comprises: contacting a zeolite component, a silicon component, a Group 14 metal component, and a phosphorus component together to form a first mixture; treating said first mixture to form a second mixture; contacting said second mixture with a binder component to form a third mixture; agglomerating said third mixture to form a fourth mixture; and treating said fourth mixture to form said composition.
摘要翻译：提供了制备组合物的方法。所述方法包括：将沸石组分，硅组分，第14族金属组分和磷组分一起接触以形成第一混合物; 处理所述第一混合物以形成第二混合物; 使所述第二混合物与粘合剂组分接触以形成第三混合物; 将所述第三混合物附聚以形成第四混合物; 并处理所述第四混合物以形成所述组合物。

9. 发明授权

US6063974A Silylated water vapor treated zinc or gallium promoted zeolite and use thereof for the conversion of non-aromatic hydrocarbons to olefins and aromatic hydrocarbons 失效
标题翻译：硅烷化水蒸汽处理的锌或镓促进沸石及其用于将非芳族烃转化为烯烃和芳族烃的沸石
公开(公告)号：US6063974A
公开(公告)日：2000-05-16
申请号：US60579
申请日：1998-04-15
申请人： Charles A. Drake , An-hsiang Wu
发明人： Charles A. Drake , An-hsiang Wu
IPC分类号： B01J29/06 , B01J31/02 , C10G35/095 , C07C2/52 , C07C4/02 , C07C4/12 , C10G35/06
CPC分类号： C10G35/095 , B01J29/061
摘要： A hydrocarbon conversion process in which the rate of coke formation is reduced without a significant sacrifice in light olefin and BTX yield by the use of a silylated, stabilized metal promoted zeolite catalyst. Another embodiment includes a novel silylated spinel/zeolite catalyst. Another embodiment includes a process for producing a zinc or gallium promoted zeolite in which the promoter is stabilized by a high temperature water vapor treatment in the presence of a metal oxide such as alumina and thereafter the stabilized catalyst precursor is calcined and silylated.
摘要翻译：一种烃转化方法，其中通过使用甲硅烷基化稳定的金属促进的沸石催化剂，在轻烯烃中显着降低焦炭形成速率并降低BTX产率。另一个实施方案包括新的甲硅烷基化尖晶石/沸石催化剂。另一个实施方案包括一种生产锌或镓的促进沸石的方法，其中助催化剂在金属氧化物如氧化铝存在下通过高温水蒸汽处理而稳定，之后将稳定的催化剂前体煅烧并进行甲硅烷基化。

10. 发明授权

US6034020A Zeolite-based catalyst material, the preparation thereof and the use thereof 失效
标题翻译：沸石催化剂材料，其制备方法及其用途
公开(公告)号：US6034020A
公开(公告)日：2000-03-07
申请号：US222469
申请日：1998-12-29
申请人： Charles A. Drake , An-hsiang Wu
发明人： Charles A. Drake , An-hsiang Wu
IPC分类号： B01J29/48 , C10G35/06 , C10G35/095 , B01J29/04 , B01J21/00 , B01J29/06 , C07C15/00
CPC分类号： C10G35/095 , B01J29/48 , B01J2229/36
摘要： A process for producing catalyst compositions for converting a cracked gasoline feedstock to a product that is principally lower olefins. The catalyst compositions produced thereby. A process for converting a cracked gasoline feedstock to a product that is principally lower olefins.
摘要翻译：用于生产用于将裂化汽油原料转化为主要是低级烯烃的产物的催化剂组合物的方法。由此生产的催化剂组合物。将裂化汽油原料转化为主要是低级烯烃的产物的方法。

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