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1. 发明申请

US20060293484A1 Low viscosity, ethylenically-unsaturated polyurethanes 审中-公开
标题翻译：低粘度，烯属不饱和聚氨酯
公开(公告)号：US20060293484A1
公开(公告)日：2006-12-28
申请号：US11165681
申请日：2005-06-24
申请人： Carol Kinney , Charles Gambino , Michael Dvorchak , Myron Shaffer
发明人： Carol Kinney , Charles Gambino , Michael Dvorchak , Myron Shaffer
IPC分类号： C08G18/00
CPC分类号： C08G18/73 , C08G18/6725 , C08G18/7837 , C08G18/792 , C08G18/797 , C09D175/16
摘要： The present invention relates to low viscosity, ethylenically-unsaturated polyurethanes which are substantially free from isocyanate groups, are liquid at 25° C., have a total content of ethylenically unsaturated groups (calculated as C═C, MW 24) of 1 to 12% by weight and contain the reaction product of A) 4-isocyanatomethyl-1,8-octamethylene diisocyanate (NTI) with B) a hydroxyl component comprising i) 5 to 100 hydroxyl equivalent % of one or more hydroxy functional lactone ester (meth)acrylates having a number average molecular weight of about 200 to 1000, ii) up to 95 hydroxyl equivalent % of a monohydroxy-functional, ethylenically unsaturated compound other than B-i), and iii) up to 20 hydroxyl equivalent % of a saturated hydroxyl compound or an unsaturated hydroxyl compound other than B-i) or B-ii), wherein i) the hydroxyl equivalent %'s of components B-i), B-ii) and B-iii) add up to 100%, based on the total weights of components B-i), B-ii) and B-iii) and ii) the NCO:OH equivalent ratio of component A) to component B) is 1.10:1 to 1:1.10. The present invention also relates to a one-component coating composition containing these ethylenically unsaturated polyurethanes.
摘要翻译：本发明涉及基本上不含异氰酸酯基团的低粘度烯键式不饱和聚氨酯，在25℃下为液体，烯属不饱和基团的总含量（以CC，MW 24计算）为1〜12％，含量为1〜12％含有A）4-异氰酸甲酯基-1,8-八亚甲基二异氰酸酯（NTI）与B）羟基组分的反应产物，其包含i）5至100个羟基当量％的一种或多种羟基官能的内酯酯（甲基）丙烯酸酯，其具有数均分子量为约200至1000，ii）除Bi之外的至多95羟基当量％的单羟基官能的烯键式不饱和化合物），和iii）饱和羟基化合物或不饱和羟基化合物的至多20羟基当量％除了Bi）或B-ii）之外的羟基化合物，其中i）组分Bi），B-ii）和B-iii的羟基当量％）基于组分Bi）的总重量加起来为100％，B-ii）和B-iii）和ii）NCO:OH等同物组分A）与组分B）的比例为1.10:1-1:1.10。本发明还涉及含有这些烯属不饱和聚氨酯的单组分涂料组合物。

2. 发明申请

US20060089480A1 Biuretized isocyanates and blocked biuretized isocyanates 审中-公开
标题翻译：自动化的异氰酸酯和封闭的缩二脲化异氰酸酯
公开(公告)号：US20060089480A1
公开(公告)日：2006-04-27
申请号：US10970763
申请日：2004-10-21
申请人： Richard Roesler , Yuliya Berezkin , Carol Kinney , Kyli Martin , Myron Shaffer
发明人： Richard Roesler , Yuliya Berezkin , Carol Kinney , Kyli Martin , Myron Shaffer
IPC分类号： C08G18/00
CPC分类号： C08G18/8032 , C08G18/7831 , C08G18/792
摘要： The present invention is directed to a biuret group-containing polyisocyanate composition having an isocyanate functionality of at least 4 prepared by a process comprising reacting a polyisocyanate adduct which a) is prepared from an aliphatic and/or cycloaliphatic diisocyanate; b) has an average isocyanate functionality of at least 2.5, and c) contains isocyanurate groups, with a secondary monoamine at an isocyanate to amine equivalent ratio of from about 4:1 to about 14:1 to incorporate biuret groups into said polyisocyanate. The invention is also directed to a blocked biuret group-containing polyisocyanate composition which is prepared by reacting the biuret-containing polyisocyanate with a blocking agent.
摘要翻译：本发明涉及具有至少4的异氰酸酯官能度的含缩二脲基团的多异氰酸酯组合物，其通过以下方法制备，所述方法包括使由脂族和/或脂环族二异氰酸酯制备的a）的多异氰酸酯加合物反应; b）具有至少2.5的平均异氰酸酯官能度，和c）含有异氰脲酸酯基团，其中异氰酸酯与胺当量比为约4:1至约14:1的仲单胺，以将缩二脲基团引入所述多异氰酸酯中。本发明还涉及含缩二脲基团的多异氰酸酯组合物，其通过使含缩合脲的多异氰酸酯与封闭剂反应制备。

3. 发明申请

US20060089481A1 Blocked biuretized isocyanates 审中-公开
标题翻译：封闭的缩二脲化异氰酸酯
公开(公告)号：US20060089481A1
公开(公告)日：2006-04-27
申请号：US10970771
申请日：2004-10-21
申请人： Richard Roesler , Yuliya Berezkin , Carol Kinney , Kyli Martin , Myron Shaffer , Poli Yu , Dorota Greszta-Franz , Reinhard Halpaap , Joachim Petzoldt
发明人： Richard Roesler , Yuliya Berezkin , Carol Kinney , Kyli Martin , Myron Shaffer , Poli Yu , Dorota Greszta-Franz , Reinhard Halpaap , Joachim Petzoldt
IPC分类号： C08G18/00
CPC分类号： C08G18/8093 , C08G18/2895 , C08G18/305 , C08G18/42 , C08G18/7831 , C08G18/792 , C08G18/8032 , C09D175/06
摘要： The present invention is directed to blocked biuret group-containing polyisocyanate compositions, wherein the blocking agent is selected from the group consisting of di-C1-C12-alkyl and/or alkoxyalkyl malonates and acetoacetic acid C1-C12-alkyl and/or alkoxyalkyl esters.
摘要翻译：本发明涉及封闭的含缩二脲基团的多异氰酸酯组合物，其中所述封闭剂选自二-C 1 -C 12 - 烷基和/ 或烷氧基烷基丙二酸酯和乙酰乙酸C 1 -C 12 - 烷基和/或烷氧基烷基酯。

4. 发明申请

US20070142610A1 Polyurethane elastomers comprising allophanate modified isocyanates 审中-公开
标题翻译：包含脲基甲酸酯改性异氰酸酯的聚氨酯弹性体
公开(公告)号：US20070142610A1
公开(公告)日：2007-06-21
申请号：US11300957
申请日：2005-12-15
申请人： Stephen Harasin , Richard Roesler , Rick Starcher , Carol Kinney , James Garrett
发明人： Stephen Harasin , Richard Roesler , Rick Starcher , Carol Kinney , James Garrett
IPC分类号： C08G18/77
CPC分类号： C08G18/7837 , C08G18/10 , C08G18/1858 , C08G18/2063 , C08G18/4866 , C08G18/6674
摘要： This invention relates to polyurethane elastomers and to a process for their production. These elastomers comprise the reaction product of a polyisocyanate component comprising an allophanate modified (cyclo)aliphatic polyisocyanate which has an NCO group content of about 15 to about 35% or a prepolymer thereof, with an isocyanate-reactive component comprising a low unsaturation polyether polyols, a low molecular weight organic compound containing two hydroxyl groups and which is free of amine groups, and, optionally, one or more organic compounds having a molecular weight of about 200 to about 500, a hydroxyl functionality of 3 to 4 and comprising an amine-initiated polyether polyol.
摘要翻译：本发明涉及聚氨酯弹性体及其生产方法。这些弹性体包括包含NCO基团含量为约15至约35％的脲基甲酸酯改性（环）脂族多异氰酸酯或其预聚物的多异氰酸酯组分与包含低不饱和聚醚多元醇的异氰酸酯反应性组分的多异氰酸酯组分的反应产物，含有两个羟基并且不含胺基的低分子量有机化合物，以及任选的一种或多种分子量为约200至约500，羟基官能度为3至4的有机化合物，引发的聚醚多元醇。

5. 发明申请

US20060223969A1 Low surface energy polyisocyanates and their use in one- or two-component coating compositions 审中-公开
标题翻译：低表面能多异氰酸酯及其在单组分或双组分涂料组合物中的用途
公开(公告)号：US20060223969A1
公开(公告)日：2006-10-05
申请号：US11096590
申请日：2005-03-31
申请人： Richard Roesler , Carol Kinney , Aaron Lockhart , James Garrett
发明人： Richard Roesler , Carol Kinney , Aaron Lockhart , James Garrett
IPC分类号： C08G18/00
CPC分类号： C08G18/61 , C08G18/289 , C08G18/73 , C08G18/755 , C08G18/7831 , C08G18/7837 , C08G18/792 , C08G18/797 , C08G18/798 , C09D175/04
摘要： The present invention is directed to a polyisocyanate mixture i) having an NCO content of 5 to 35% by weight and a monomeric diisocyanate content of less than 3% by weight, and prepared from a polyisocyanate adduct, ii) containing allophanate groups in an amount such that there are more equivalents of allophanate groups than urethane groups and such that the polyisocyanate mixture remains stable and homogeneous in storage for 1 month at 25° C. and iii) containing siloxane groups (calculated as SiO, MW 44) in an amount of 0.002 to 50% by weight, wherein the preceding percentages are based on the solids content of the polyisocyanate mixture and wherein the siloxane groups are incorporated by reacting an isocyanate group with a compound containing one or more hydroxyl groups directly attached to a carbon atom and one or more siloxane groups. The present invention is also directed to a process for the production of this polyisocyanate mixture and to its use, optionally in blocked form, as an isocyanate component in one- or two-component coating compositions.
摘要翻译：本发明涉及NCO含量为5〜35重量％，单体二异氰酸酯含量小于3重量％，由多异氰酸酯加合物制备的多异氰酸酯混合物i），ii）含有量的脲基甲酸酯基使得比氨基甲酸酯基团具有更多当量的脲基甲酸酯基团，并且使得多异氰酸酯混合物在25℃下保存稳定和均匀储存1个月，和iii）含有硅氧烷基团（以SiO，MW 44计） 0.002至50重量％，其中前述百分比基于多异氰酸酯混合物的固体含量，并且其中硅氧烷基团通过使异氰酸酯基团与含有一个或多个直接连接到碳原子上的羟基的化合物反应而引入，一个或更多的硅氧烷基团。本发明还涉及在单组分或双组分涂料组合物中制备该多异氰酸酯混合物及其用途，任选为封闭形式的异氰酸酯组分的方法。

6. 发明申请

US20070112164A1 Low surface energy, ethylenically unsaturated polyisocyanate addition compounds and their use in coating compositions 审中-公开
标题翻译：低表面能，烯键式不饱和多异氰酸酯加成化合物及其在涂料组合物中的应用
公开(公告)号：US20070112164A1
公开(公告)日：2007-05-17
申请号：US11281080
申请日：2005-11-17
申请人： Richard Roesler , James Garrett , Aaron Lockhart , Carol Kinney
发明人： Richard Roesler , James Garrett , Aaron Lockhart , Carol Kinney
IPC分类号： C08G18/00
CPC分类号： C08G18/289 , C08G18/61 , C08G18/672 , C08G18/7837 , C09D175/16
摘要： The present invention is directed to polyisocyanate addition compounds which i) are substantially free from isocyanate groups and are prepared from one or more monomeric polyisocyanates and/or polyisocyanate adducts, ii) contain allophanate groups, iii) contain siloxane groups (calculated as SiO, MW 44) in an amount of 0.002 to 50% by weight, and iv) contain ethylenically unsaturated groups (calculated as C═C, MW 24) in an amount of 2 to 40% by weight, wherein the preceding percentages are based on the solids content of the polyisocyanate addition compounds and wherein the siloxane groups are incorporated by reacting an isocyanate group with a compound containing one or more hydroxyl groups directly attached to a carbon atom and one or more siloxane groups to form urethane groups and/or allophanate groups, provided that more than 50 mole % of the groups that chemically incorporate siloxane groups into the polyisocyanate addition compounds are allophanate groups. The present invention also relates to the use of the polyisocyanate addition compounds in coating compositions curable by free radical polymerization.
摘要翻译：本发明涉及多异氰酸酯加成化合物，其i）基本上不含异氰酸酯基团，并且由一种或多种单体多异氰酸酯和/或多异氰酸酯加合物制备，ii）含有脲基甲酸酯基团，iii）含有硅氧烷基团（按SiO计，MW 44），其量为0.002至50重量％，和iv）含有2-40重量％的烯键式不饱和基团（以CC，MW 24计算），其中前述百分比基于所述多异氰酸酯加成化合物，其中所述硅氧烷基团通过使异氰酸酯基团与直接与碳原子连接的一个或多个羟基的化合物和一个或多个硅氧烷基团反应形成氨基甲酸酯基和/或脲基甲酸酯基而引入，条件是更多将硅氧烷基团化学引入到多异氰酸酯加成化合物中的基团的50摩尔％为脲基甲酸酯基。本发明还涉及多异氰酸酯加成化合物在通过自由基聚合可固化的涂料组合物中的用途。

7. 发明申请

US20070032625A1 Low surface energy polyisocyanates and their use in one-or two-component coating compositions 审中-公开
标题翻译：低表面能多异氰酸酯及其在单组分或双组分涂料组合物中的用途
公开(公告)号：US20070032625A1
公开(公告)日：2007-02-08
申请号：US11198733
申请日：2005-08-05
申请人： Richard Roesler , James Garrett , Aaron Lockhart , Carol Kinney
发明人： Richard Roesler , James Garrett , Aaron Lockhart , Carol Kinney
IPC分类号： C08G18/00
CPC分类号： C08G18/3812 , C08G18/10 , C08G18/2885 , C08G18/7831 , C08G18/792 , C09D175/04 , C08G18/307 , C08G18/42
摘要： The present invention is directed to a polyisocyanate mixture i) having a monomeric diisocyanate content of less than 3% by weight, ii) having a urethane group content of more than 50 equivalent %, based on the total equivalents of urethane and allophanate groups, and iii) containing fluorine (calculated as F, AW 19) in an amount of 0.001 to 50% by weight, wherein the preceding percentages are based on the solids content of the polyisocyanate mixture and wherein fluorine is incorporated by reacting a) an isocyanate group from a polyisocyanate adduct containing at least 60% by weight, based on the total weight of the polyisocyanate adduct, of a polyisocyanate adduct which is prepared from 1,6-hexamethylene diisocyanate, contains isocyanurate, iminooxadiazine dione and/or uretdione groups and has a viscosity at 25° C. and 100% solids of less than 2000 mPa·s, with b) a compound containing two or more carbon atoms, one or more hydroxyl groups and one or more fluorine atoms to form urethane groups. The present invention is also directed to the use of this polyisocyanate mixture, optionally in blocked form, as an isocyanate component in one- or two-component coating compositions.
摘要翻译：本发明涉及单体二异氰酸酯含量小于3重量％的二异氰酸酯混合物，ii）氨基甲酸酯基含量大于等于50当量的氨基甲酸酯和脲基甲酸酯基，和 iii）以0.001至50重量％的量含有氟（以F，AW 19计算），其中前述百分比基于多异氰酸酯混合物的固体含量，并且其中通过使a）异氰酸酯基团从基于多异氰酸酯加合物的总重量至少60重量％的由1,6-六亚甲基二异氰酸酯制备的多异氰酸酯加合物的多异氰酸酯加合物含有异氰脲酸酯，亚氨基恶二嗪二酮和/或脲二酮基团，并且具有粘度在25℃和100％固体含量小于2000mPa.s，b）含有两个或更多个碳原子的化合物，一个或多个羟基和一个或多个氟原子以形成氨基甲酸酯 e组。本发明还涉及这种多异氰酸酯混合物（任选地以封闭形式）作为单组分或双组分涂料组合物中的异氰酸酯组分的用途。

8. 发明授权

US09034472B2 Non-aqueous polyurethane coating compositions 有权
标题翻译：非水性聚氨酯涂料组合物
公开(公告)号：US09034472B2
公开(公告)日：2015-05-19
申请号：US13980104
申请日：2012-01-19
申请人： Ramesh Subramanian , Abdullah Ekin , Carol Kinney , Christine Mebane , Wolfgang Fischer , Helmut Kuczewski
发明人： Ramesh Subramanian , Abdullah Ekin , Carol Kinney , Christine Mebane , Wolfgang Fischer , Helmut Kuczewski
IPC分类号： B32B27/00 , B32B27/40 , C03C17/32 , C03C17/00 , C09D4/06 , C08G18/67
CPC分类号： C03C17/322 , C03C17/005 , C08G18/672 , C09D4/06 , Y10T428/1321 , Y10T428/31601
摘要： The present invention relates to a non-aqueous coating composition comprising: 1) 75 to 99 wt. %, preferably 85 to 95 wt. % of a hard urethane(meth)acrylate polymer or oligomer; and 2) 1 to 25 wt. %, preferably 5 to 15 wt. % of a soft unsaturated urethane(meth)acrylate polymer or oligomer containing allophanate groups.
摘要翻译：本发明涉及一种非水性涂料组合物，其包含：1）75〜99重量％％，优选85〜95重量％％的硬聚氨酯（甲基）丙烯酸酯聚合物或低聚物; 和2）1至25wt。％，优选5〜15wt。％的含有脲基甲酸酯基的软质不饱和聚氨酯（甲基）丙烯酸酯聚合物或低聚物。

9. 发明申请

US20070112163A1 Low surface energy, ethylenically unsaturated polyisocyanate addition compounds and their use in coating compositions 失效
标题翻译：低表面能，烯键式不饱和多异氰酸酯加成化合物及其在涂料组合物中的应用
公开(公告)号：US20070112163A1
公开(公告)日：2007-05-17
申请号：US11281079
申请日：2005-11-17
申请人： Carol Kinney , Richard Roesler , James Garrett , Aaron Lockhart
发明人： Carol Kinney , Richard Roesler , James Garrett , Aaron Lockhart
IPC分类号： C08G18/00
CPC分类号： C08G18/2885 , C08G18/672 , C08G18/791 , C08G18/798 , C09D175/16
摘要： The present invention is directed to polyisocyanate addition compounds which i) are substantially free from isocyanate groups and are prepared from one or more a) polyisocyanate adducts containing uretdione, biuret, allophanate, carbodiimide and/or oxadiazinetrione groups and/or b) NCO prepolymers, ii) contain urethane groups, iii) contain fluorine (calculated as F, AW 19) in an amount of 0.01 to 50% by weight, and iv) contain ethylenically unsaturated groups (calculated as C═C, MW 24) in an amount of 2 to 40% by weight, wherein the preceding percentages are based on the solids content of the polyisocyanate addition compounds and wherein fluorine is incorporated by reacting an isocyanate group with a compound containing two or more carbon atoms, one or more hydroxyl groups and one or more fluorine atoms to form urethane groups and optionally allophanate groups, provided that more than 50 mole % of the groups that chemically incorporate fluorine into the polyisocyanate addition compounds are urethane groups. The present invention also relates to the use of the polyisocyanate addition compounds in coating compositions curable by free radical polymerization.
摘要翻译：本发明涉及i）基本上不含异氰酸酯基并且由一种或多种a）含有脲二酮，缩二脲，脲基甲酸酯，碳二亚胺和/或恶二嗪二酮基团的多异氰酸酯加合物和/或b）NCO预聚物制备的多异氰酸酯加成化合物， ii）含有氨基甲酸酯基团，iii）含有0.01-50重量％的氟（按F，AW 19计算），和iv）含有烯键式不饱和基团（按CC，MW 24计算），其量为2至 40重量％，其中前述百分比基于多异氰酸酯加成化合物的固体含量，并且其中氟通过使异氰酸酯基团与含有两个或更多个碳原子的化合物，一个或多个羟基和一个或多个氟原子形成氨基甲酸酯基团和任选的脲基甲酸酯基团，条件是将多于50摩尔％的化学引入氟的多元醇加成化合物是氨基甲酸酯基团。本发明还涉及多异氰酸酯加成化合物在通过自由基聚合可固化的涂料组合物中的用途。

10. 发明申请

US20070112162A1 Low surface energy, ethylenically unsaturated polyisocyanate addition compounds and their use in coating compositions 审中-公开
标题翻译：低表面能，烯键式不饱和多异氰酸酯加成化合物及其在涂料组合物中的应用
公开(公告)号：US20070112162A1
公开(公告)日：2007-05-17
申请号：US11281006
申请日：2005-11-17
申请人： Carol Kinney , Richard Roesler , James Garrett , Aaron Lockhart
发明人： Carol Kinney , Richard Roesler , James Garrett , Aaron Lockhart
IPC分类号： C08G18/00
CPC分类号： C08G18/5015 , C08G18/2885 , C08G18/3812 , C08G18/672 , C08G18/7837 , C08G18/8054 , C08G18/8087 , C09D175/16
摘要： The present invention is directed to polyisocyanate addition compounds which i) are substantially free from isocyanate groups and are prepared from one or more monomeric polyisocyanates and/or polyisocyanate adducts, ii) contain allophanate groups, iii) contain fluorine (calculated as F, AW 19) in an amount of 0.01 to 50% by weight, and iv) contain ethylenically unsaturated groups (calculated as C═C, MW 24) in an amount of 2 to 40% by weight, wherein the preceding percentages are based on the solids content of the polyisocyanate addition compounds and wherein fluorine is incorporated by reacting an isocyanate group with a compound containing two or more carbon atoms, one or more hydroxyl groups and one or more fluorine atoms to form urethane groups and/or allophanate groups, provided that more than 50 mole % of the groups that chemically incorporate fluorine into the polyisocyanate addition compounds are allophanate groups. The present invention also relates to the use of the polyisocyanate addition compounds in coating compositions curable by free radical polymerization.
摘要翻译：本发明涉及多异氰酸酯加成化合物，其i）基本上不含异氰酸酯基团，并且由一种或多种单体多异氰酸酯和/或多异氰酸酯加合物制备，ii）含有脲基甲酸酯基团，iii）含氟（按F，AW 19计算），并且iv）含有2-40重量％的烯键式不饱和基团（按CC，MW 24计算），其中前述百分比基于固体含量多异氰酸酯加成化合物，其中通过使异氰酸酯基团与含有两个或更多个碳原子，一个或多个羟基和一个或多个氟原子的化合物反应形成氨基甲酸酯基和/或脲基甲酸酯基而引入氟，条件是超过50摩尔将氟化学引入多异氰酸酯加成化合物的基团的百分比是脲基甲酸酯基。本发明还涉及多异氰酸酯加成化合物在通过自由基聚合可固化的涂料组合物中的用途。

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