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1. 发明申请

US20070032691A1 Dehydrogenation process 有权
标题翻译：脱氢工艺
公开(公告)号：US20070032691A1
公开(公告)日：2007-02-08
申请号：US11196033
申请日：2005-08-03
申请人： Vladimir Fridman , Michael Urbancic , Andrzej Rokicki
发明人： Vladimir Fridman , Michael Urbancic , Andrzej Rokicki
IPC分类号： C07C5/327 , C07C5/373
CPC分类号： B01J35/10 , B01J23/26 , B01J23/8993 , B01J35/0006 , B01J35/1014 , B01J35/1019 , B01J37/10 , C07C5/333 , C07C5/3337 , C07C2521/04 , C07C2521/06 , C07C2521/10 , C07C2523/04 , C07C2523/26 , C07C2523/42 , C07C2523/755 , C07C11/02
摘要： A process for adiabatic, non-oxidative dehydrogenation of hydrocarbons including passing a hydrocarbon feed stream through a catalyst bed, wherein the catalyst bed includes a first layer of a catalyst and second layer of a catalyst, wherein the catalyst of the first layer has high activity but a higher capacity for producing coke than the catalyst of the second layer and the second catalyst also has high activity but a lower capacity for producing coke than the catalyst of the first layer.
摘要翻译：一种用于烃的绝热，非氧化脱氢的方法，包括使烃进料流通过催化剂床，其中催化剂床包括第一层催化剂和第二层催化剂，其中第一层的催化剂具有高活性但比第二层的催化剂生产焦炭的能力更高，第二催化剂的生产焦炭的活性高于第一层的催化剂，而且生产焦炭的能力较高。

2. 发明授权

US08063261B2 Multi-layered dehydrogenation catalyst system and process of use 失效
标题翻译：多层脱氢催化剂体系及其使用过程
公开(公告)号：US08063261B2
公开(公告)日：2011-11-22
申请号：US11129834
申请日：2005-05-16
申请人： Andrzej Rokicki , Vladimir Fridman , Michael Urbancic
发明人： Andrzej Rokicki , Vladimir Fridman , Michael Urbancic
IPC分类号： B01J23/26
CPC分类号： B01J21/066 , B01J21/04 , B01J23/26 , B01J35/0006 , C07C5/3332 , C07C2521/04 , C07C2521/06 , C07C2523/26 , Y02P20/52 , C07C11/06 , C07C11/08
摘要： A system for dehydrogenating a C3 or C4 hydrocarbon feed stream containing a first and second layer of catalysts placed in the hydrocarbon feed stream, wherein the feed stream first passes through the first layer and then the second layer of catalysts and wherein the catalysts of the first layer contain from about 50 to about 90 percent by weight of an eta-alumina carrier, from about 10 to about 50 percent by weight of chromia and from about 0.1 to about 5 percent by weight of a zirconium compound and wherein the catalysts of the second layer of catalysts contain from about 50 to about 90 percent by weight of an eta-alumina carrier and from about 10 to about 50 percent by weight of chromia, without an added zirconium compound.
摘要翻译：一种用于使包含置于烃进料流中的第一和第二层催化剂的C3或C4烃进料物流脱氢的系统，其中进料流首先通过第一层然后第二层催化剂，其中第一层催化剂层含有约50至约90重量％的氧化铝载体，约10至约50重量％的氧化铬和约0.1至约5重量％的锆化合物，并且其中第二催化剂层包含约50至约90重量％的氧化铝 - 氧化铝载体和约10至约50重量％的氧化铬，而不加入锆化合物。

3. 发明授权

US07491860B2 Dehydrogenation process 有权
标题翻译：脱氢工艺
公开(公告)号：US07491860B2
公开(公告)日：2009-02-17
申请号：US11196033
申请日：2005-08-03
申请人： Vladimir Fridman , Michael Urbancic , Andrzej Rokicki
发明人： Vladimir Fridman , Michael Urbancic , Andrzej Rokicki
IPC分类号： C07C5/333 , B01J23/00 , C10G35/04
CPC分类号： B01J35/10 , B01J23/26 , B01J23/8993 , B01J35/0006 , B01J35/1014 , B01J35/1019 , B01J37/10 , C07C5/333 , C07C5/3337 , C07C2521/04 , C07C2521/06 , C07C2521/10 , C07C2523/04 , C07C2523/26 , C07C2523/42 , C07C2523/755 , C07C11/02
摘要： A process for adiabatic, non-oxidative dehydrogenation of hydrocarbons including passing a hydrocarbon feed stream through a catalyst bed, wherein the catalyst bed includes a first layer of a catalyst and second layer of a catalyst, wherein the catalyst of the first layer has high activity but a higher capacity for producing coke than the catalyst of the second layer and the second catalyst also has high activity but a lower capacity for producing coke than the catalyst of the first layer.
摘要翻译：一种用于烃的绝热，非氧化脱氢的方法，包括使烃进料流通过催化剂床，其中催化剂床包括第一层催化剂和第二层催化剂，其中第一层的催化剂具有高活性但比第二层的催化剂生产焦炭的能力更高，第二催化剂的生产焦炭的活性高于第一层的催化剂，而且生产焦炭的能力较高。

4. 发明申请

US20060149112A1 Multi-layered dehydrogenation catalyst system and process of use 失效
标题翻译：多层脱氢催化剂体系及其使用过程
公开(公告)号：US20060149112A1
公开(公告)日：2006-07-06
申请号：US11129834
申请日：2005-05-16
申请人： Andrzej Rokicki , Vladimir Fridman , Michael Urbancic
发明人： Andrzej Rokicki , Vladimir Fridman , Michael Urbancic
IPC分类号： C07C5/327
CPC分类号： B01J21/066 , B01J21/04 , B01J23/26 , B01J35/0006 , C07C5/3332 , C07C2521/04 , C07C2521/06 , C07C2523/26 , Y02P20/52 , C07C11/06 , C07C11/08
摘要： A system for dehydrogenating a C3 or C4 hydrocarbon feed stream containing a first and second layer of catalysts placed in the hydrocarbon feed stream, wherein the feed stream first passes through the first layer and then the second layer of catalysts and wherein the catalysts of the first layer contain from about 50 to about 90 percent by weight of an eta-alumina carrier, from about 10 to about 50 percent by weight of chromia and from about 0.1 to about 5 percent by weight of a zirconium compound and wherein the catalysts of the second layer of catalysts contain from about 50 to about 90 percent by weight of an eta-alumina carrier and from about 10 to about 50 percent by weight of chromia, without an added zirconium compound.
摘要翻译：一种用于使包含置于烃进料流中的第一和第二层催化剂的C3或C4烃进料物流脱氢的系统，其中进料流首先通过第一层然后第二层催化剂，其中第一层催化剂层含有约50至约90重量％的氧化铝载体，约10至约50重量％的氧化铬和约0.1至约5重量％的锆化合物，并且其中第二催化剂层包含约50至约90重量％的氧化铝 - 氧化铝载体和约10至约50重量％的氧化铬，而不加入锆化合物。

5. 发明申请

US20100217052A1 Catalyst For The Selective Hydrogenation Of Acetylenic Hydrocarbons And Method For Producing Said Catalyst 审中-公开
标题翻译：用于选择性氢化乙炔烃的催化剂及其制备方法
公开(公告)号：US20100217052A1
公开(公告)日：2010-08-26
申请号：US12601985
申请日：2008-05-30
申请人： Sybille Ungar , Richard Fischer , Andreas Trautwein , Steve Blankenship , Jennifer Boyer , Michael Urbancic , Andrzej Rokicki
发明人： Sybille Ungar , Richard Fischer , Andreas Trautwein , Steve Blankenship , Jennifer Boyer , Michael Urbancic , Andrzej Rokicki
IPC分类号： C07C5/08 , B01J31/12
CPC分类号： B01J23/44 , B01J23/40 , B01J23/48 , B01J23/50 , B01J23/74 , B01J35/002 , B01J35/006 , B01J35/008 , B01J35/1014 , B01J37/0203 , B01J37/0221 , B01J37/16 , C07C7/167 , C07C2521/04 , C07C2523/44 , C07C2523/56 , C10G45/40 , Y02P20/52 , C07C11/06 , C07C11/04
摘要： A method for producing a catalyst, in particular for the selective reduction of acetylenic compounds in hydrocarbon streams. An impregnation solution is provided, which contains a mixture of water and at least one water-miscible organic solvent as solvent in which at least one active metal compound and also preferably at least one promoter metal compound is dissolved. A support is provided, the support is impregnated with the impregnation solution, and the impregnated support is calcined. Palladium is preferably used as active metal and silver is preferably used as promoter metal. Also, a catalyst as is obtained by the method and also its preferred use for the selective hydrogenation of acetylenic compounds.
摘要翻译：一种制备催化剂的方法，特别是用于在烃流中选择性还原炔属化合物。提供浸渍溶液，其含有水和至少一种与水可混溶的有机溶剂作为溶剂的混合物，其中至少一种活性金属化合物和还优选至少一种助催化剂金属化合物溶解。提供支撑体，用浸渍溶液浸渍载体，并将浸渍的载体煅烧。优选使用钯作为活性金属，优选使用银作为助催化剂金属。另外，通过该方法得到的催化剂，也是炔属化合物的选择性氢化的优选用途。

6. 发明申请

US20070054801A1 Catalytically inactive heat generator and improved dehydrogenation process 有权
标题翻译：催化惰性热发生器和改进的脱氢工艺
公开(公告)号：US20070054801A1
公开(公告)日：2007-03-08
申请号：US11218949
申请日：2005-09-02
申请人： Vladimir Fridman , Jay Merriam , Michael Urbancic
发明人： Vladimir Fridman , Jay Merriam , Michael Urbancic
IPC分类号： B01J23/26
CPC分类号： B01J23/32 , B01J23/26 , B01J23/72 , B01J35/0006 , C07C5/322 , C07C2521/02 , C07C2521/04 , C07C2521/08 , C07C2521/10 , C07C2521/12 , C07C2523/02 , C07C2523/04 , C07C2523/06 , C07C2523/26 , C07C2523/34 , C07C2523/72 , C07C2523/889 , C07C2529/04 , Y02P20/52 , Y02P20/584 , C07C11/06
摘要： An improved dehydrogenation catalyst bed system for olefin production utilizing classical processing techniques is disclosed. The catalyst bed system comprises a dehydrogenation catalyst comprising an active component selected from an oxide of a metal of Group 4 or Group 5 or Group 6 and combinations thereof and a support selected from aluminum oxide, aluminas, alumina monohydrate, alumina trihydrate, alumina-silica, transition aluminas, alpha-alumina, silica, silicate, aluminates, calcined hydrotalcites, zeolites and combinations thereof mixed with a first inert material selected from any material that is catalytically inactive when subjected to reaction conditions that can effect dehydrogenation of olefins and that has a high density and high heat capacity and that is not capable of producing heat during any stage of the dehydrogenation process, and the dehydrogenation catalyst plus the first inert material then being physically mixed with a secondary component comprising a heat-generating inert material and a carrier capable of supporting the heat-generating inert material, wherein the secondary component is catalytically inert with respect to dehydrogenation reactions or to cracking or to coking and generates heat after being exposed to reducing and/or to oxidizing reaction conditions.
摘要翻译：公开了一种利用经典处理技术改进用于烯烃生产的脱氢催化剂床系统。催化剂床系统包括脱氢催化剂，其包含选自第4组或第5组或第6组金属的氧化物及其组合的活性组分和选自氧化铝，氧化铝，一水合氧化铝，三水合氧化铝，氧化铝 - 二氧化硅，过渡氧化铝，α-氧化铝，二氧化硅，硅酸盐，铝酸盐，煅烧水滑石，沸石及其混合物与第一惰性材料混合，所述第一惰性材料选自任何可能影响烯烃脱氢反应条件的催化无活性物质，高密度和高热容量，并且在脱氢过程的任何阶段都不能产生热量，然后脱氢催化剂加第一惰性材料与包含发热惰性材料和载体的次级组分物理混合支撑发热惰性材料，其中次要组分相对于脱氢反应是催化惰性的，或者在暴露于还原和/或氧化反应条件之后开裂或焦化并产生热量。

7. 发明申请

US20080097134A1 Endothermic Hydrocarbon Conversion Process 有权
标题翻译：吸热烃转化过程
公开(公告)号：US20080097134A1
公开(公告)日：2008-04-24
申请号：US11873367
申请日：2007-10-16
申请人： Vladimir Fridman , Michael Urbancic
发明人： Vladimir Fridman , Michael Urbancic
IPC分类号： C07C7/20
CPC分类号： B01J23/26 , B01J23/32 , B01J23/72 , B01J35/0006 , C07C5/3332 , C07C2521/02 , C07C2521/04 , C07C2521/08 , C07C2521/10 , C07C2521/12 , C07C2523/02 , C07C2523/04 , C07C2523/06 , C07C2523/26 , C07C2523/34 , C07C2523/72 , C07C2523/889 , C07C2529/04 , Y02P20/52 , C07C11/06 , C07C11/09
摘要： The present invention is an improved cyclic, endothermic hydrocarbon conversion process and a catalyst bed system for accomplishing the same. Specifically, the improved process comprises reacting a hydrocarbon with a multi-component catalyst bed in such a manner that the temperature within the catalyst bed remains within controlled temperature ranges throughout all stages of the process. The multi-component catalyst bed comprises a reaction-specific catalyst physically mixed with a heat-generating material.
摘要翻译：本发明是一种改进的循环，吸热烃转化方法和用于实现它的催化剂床系统。具体地，改进的方法包括使烃与多组分催化剂床反应，使得催化剂床内的温度在整个过程的所有阶段都保持在受控温度范围内。多组分催化剂床包括与发热材料物理混合的反应特异性催化剂。

8. 发明申请

US20130102819A1 CATALYST COMPOSITION FOR SELECTIVE HYDROGENATION WITH IMPROVED CHARACTERISTICS 审中-公开
标题翻译：具有改进特性的选择性氢化催化剂组合物
公开(公告)号：US20130102819A1
公开(公告)日：2013-04-25
申请号：US13276403
申请日：2011-10-19
申请人： Normen Szesni , Alfred Hagemeyer , Frank Grossmann , Richard Fischer , Michael Urbancic , Claus Lugmair , Mingyong Sun , Hongyi C. Hou , David Michael Lowe
发明人： Normen Szesni , Alfred Hagemeyer , Frank Grossmann , Richard Fischer , Michael Urbancic , Claus Lugmair , Mingyong Sun , Hongyi C. Hou , David Michael Lowe
IPC分类号： C07C5/09 , B01J23/50 , B01J23/52 , B01J31/02 , B01J23/62 , B01J23/89 , B01J23/644 , B01J23/58 , B01J23/44 , B01J23/60
CPC分类号： B01J23/44 , B01J21/04 , B01J23/50 , B01J23/52 , B01J23/58 , B01J23/60 , B01J23/62 , B01J23/626 , B01J23/628 , B01J23/6447 , B01J23/8926 , B01J31/0277 , B01J31/0279 , B01J31/0284 , B01J35/008 , B01J35/1009 , B01J35/1038 , B01J37/0201 , B01J37/024 , B01J37/16 , B01J2231/645 , B01J2531/824 , C07C7/167 , C10G45/40 , C10G2400/20 , Y02P20/52 , C07C11/04 , C07C11/06
摘要： This invention relates to heterogeneous catalysts useful for selective hydrogenation of unsaturated hydrocarbons, comprising palladium and optionally a promoter, supported on a substrate, having an uncoated BET surface area of ≦9 m2/g, the surface being coated with an ionic liquid. Also described are methods of making the catalysts and methods of selective hydrogenation of acetylene and/or dienes in front-end mixed olefin feed streams.
摘要翻译：本发明涉及可用于不饱和烃的选择性氢化的非均相催化剂，其包含负载在基材上的钯和任选的助催化剂，其具有未涂覆的BET表面积为9m 2 / g，该表面用离子液体涂覆。还描述了制备催化剂的方法和在前端混合烯烃进料流中乙炔和/或二烯烃的选择性氢化的方法。

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