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1. 发明授权

US5536788A Carboxyl-containing isobutene copolymers 失效
公开(公告)号：US5536788A
公开(公告)日：1996-07-16
申请号：US490031
申请日：1995-06-13
申请人： Andreas Deckers , Hans-Joachim Muller , Roger Klimesch , Eckehardt Wistuba , Heinz Plaumann , Erich Kolk , Gunther Isbarn , Karl-Heinz Fauth , Joachim Krobb
发明人： Andreas Deckers , Hans-Joachim Muller , Roger Klimesch , Eckehardt Wistuba , Heinz Plaumann , Erich Kolk , Gunther Isbarn , Karl-Heinz Fauth , Joachim Krobb
IPC分类号： C08F4/04 , C08F4/14 , C08F4/32 , C08F8/46 , C08F255/08 , C09J151/06 , C08F220/02 , C08F222/04
CPC分类号： C09J151/06 , C08F255/08 , C08F8/32 , C08F8/46 , C08G18/6204 , C08F210/14 , C08F2800/10 , C08F2810/20
摘要： Carboxyl-containing isobutene copolymers are obtainablea) by cationic polymerization of a mixture of from 1 to 99 mol % of isobutene and from 99 to 1 mol % of a 2-methylalk-1-ene at less than 20.degree. C. in the presence of a halogen-containing Lewis acid andb) subsequent grafting of the isobutene copolymer obtainable in this manner with an .alpha.,.beta.-ethylenically unsaturated carboxylic acid or carboxylic acid derivative at above 100.degree. C. and in the presence of a free radical initiator.Such carboxyl-containing isobutene copolymers are particularly suitable as adhesive raw materials or as sealing compounds.

2. 发明授权

US5473022A Carboxyl-containing isobutene copolymers 失效
标题翻译：含羧基异丁烯共聚物
公开(公告)号：US5473022A
公开(公告)日：1995-12-05
申请号：US300185
申请日：1994-09-02
申请人： Andreas Deckers , Hans-Joachim Muller , Roger Klimesch , Eckehardt Witsuba , Heinz Plaumann , Erich Kolk , Gunther Isbarn , Karl-Heinz Fauth , Joachim Krobb
发明人： Andreas Deckers , Hans-Joachim Muller , Roger Klimesch , Eckehardt Witsuba , Heinz Plaumann , Erich Kolk , Gunther Isbarn , Karl-Heinz Fauth , Joachim Krobb
IPC分类号： C08F4/04 , C08F4/14 , C08F4/32 , C08F8/46 , C08F255/08 , C09J151/06
CPC分类号： C09J151/06 , C08F255/08 , C08F8/32 , C08F8/46 , C08G18/6204 , C08F210/14 , C08F2800/10 , C08F2810/20
摘要： Carboxyl-containing isobutene copolymers are obtainablea) by cationic polymerization of a mixture of from 1 to 99 mol % of isobutene and from 99 to 1 mol % of a 2-methylalk-1-ene at less than 20.degree. C. in the presence of a halogen-containing Lewis acid andb) subsequent grafting of the isobutene copolymer obtainable in this manner with an .alpha.,.beta.-ethylenically unsaturated carboxylic acid or carboxylic acid derivative at above 100.degree. C. and in the presence of a free radical initiator.Such carboxyl-containing isobutene copolymers are particularly suitable as adhesive raw materials or as sealing compounds.
摘要翻译：含羧基的异丁烯共聚物可以通过在低于20℃的存在下通过阳离子聚合1至99mol％的异丁烯和99至1mol％的2-甲基-1-烯的混合物获得，的含卤素的路易斯酸，以及b）随后在100℃下和在自由基引发剂存在下用α，β-烯键式不饱和羧酸或羧酸衍生物以这种方式获得的异丁烯共聚物接枝。这种含羧基的异丁烯共聚物特别适用作粘合剂原料或密封剂。

3. 发明授权

US5532321A Copolymers and blends which are self-curable under the action of atmospheric humidity 失效
标题翻译：在大气湿度作用下可自行固化的共聚物和共混物
公开(公告)号：US5532321A
公开(公告)日：1996-07-02
申请号：US238901
申请日：1994-05-06
申请人： Juergen Barwich , Heinz Plaumann , Eckehardt Wistuba
发明人： Juergen Barwich , Heinz Plaumann , Eckehardt Wistuba
IPC分类号： C08L31/02 , C08F218/04 , C08F220/12 , C08L31/04 , C08L33/04 , C08L33/06 , C08L43/00 , C08L43/04 , C09D133/04 , C09D133/06 , C09D137/00 , C09D143/04 , C09J131/00 , C09J131/02 , C09J133/04 , C09J133/06 , C09J137/00 , C09J143/04 , C09K3/10 , C08F222/06
CPC分类号： C09J143/04 , C08F218/04 , C08F220/12 , C09D143/04
摘要： Essentially isocyanate-free, ketimine- and aldimine-free, one-component sealing, adhesive or coating materials which are self-curable under the action of atmospheric humidity containing a copolymer A composed of50-99.8% by weight of a C.sub.1 -C.sub.16 -alkyl (meth)acrylate or vinyl ester of carboxylic acids of 1 to 20 carbon atoms a),0.1-20% by weight of an unsaturated carboxylic anhydride b),0.1-10% by weight of an Si-containing compound c) capable of undergoing hydrolysis and0-40% by weight of a further, copolymerizable unsaturated compound d)or containing a mixture of copolymers comprising5-95% by weight, based on the mixture, of a copolymer B), composed of50-99.9% by weight of a C.sub.1 -C.sub.16 -alkyl (meth)acrylate or vinyl ester of carboxylic acids of 1 to 20 carbon atoms a),0-20% by weight of an unsaturated carboxylic anhydride b)0.1-10% by weight of an Si-containing compound c) capable of undergoing hydrolysis and0-40% by weight of a further, copolymerizable unsaturated compound d)and5-95% by weight, based on the mixture, of a copolymer C) composed of50-99.9% by weight of a C.sub.1 -C.sub.16 -alkyl (meth)acrylate or vinyl ester of carboxylic acids of 1 to 20 carbon atoms a),0.1-20% by weight of an unsaturated carboxylic anhydride b),0-10% by weight of an Si-containing compound c) capable of undergoing hydrolysis and0-40% by weight of a further, copolymerizable unsaturated compound d),the K value of one of the copolymers B) or C) being from 12 to 40 and that of the other copolymer being from 30 to 70 and the K values of the two copolymers differing by at least 5K value units, where the K value is measured according to DIN 53,726.
摘要翻译：基本上无异氰酸酯，不含酮亚胺和不含亚胺基的单组分密封，粘合剂或涂层材料，其在大气湿度的作用下可自行固化，包含由50-99.8重量％的C1-C16- （甲基）丙烯酸烷基酯或1-20个碳原子的羧酸乙烯基酯a），0.1-20重量％的不饱和羧酸酐b），0.1-10重量％的含Si化合物c）进行水解和0-40重量％的另外的可共聚不饱和化合物d）或含有基于混合物的基于混合物的5-95重量％的共聚物B）的共混物的混合物，共聚物B）由50-99.9％碳原子数1〜20的（甲基）丙烯酸C 1 -C 16烷基酯或碳酸乙烯酯的重量a），0〜20重量％的不饱和羧酸酐b）0.1-10重量％的Si- 含有能够进行水解的化合物c）和0-40重量％的另外的可共聚不饱和化合物d）和5- 95重量％的基于混合物的由50-99.9重量％的（甲基）丙烯酸C 1 -C 16烷基酯或1至20个碳原子的羧酸乙烯基酯组成的共聚物C）a），0.1 -20重量％的不饱和羧酸酐b），0-10重量％的能够进行水解的含Si化合物c）和0-40重量％的另外的可共聚不饱和化合物d），K 共聚物B）或C）之一的值为12〜40，另一种共聚物的值为30〜70，两种共聚物的K值相差至少5K值，其中K值根据根据DIN 53,726。

4. 发明授权

US07442441B2 Composite structure, a resin composition for use in the composite structure, and a process for making the same 有权
标题翻译：复合结构体，用于复合结构体的树脂组合物及其制造方法
公开(公告)号：US07442441B2
公开(公告)日：2008-10-28
申请号：US10834652
申请日：2004-04-29
申请人： Calvin T. Peeler , Aaron M. Rath , Heinz Plaumann , James F. Turnbach
发明人： Calvin T. Peeler , Aaron M. Rath , Heinz Plaumann , James F. Turnbach
IPC分类号： B32B27/36 , B05D1/36
CPC分类号： B32B27/36 , B32B5/08 , B32B27/08 , B32B27/18 , B32B27/20 , B32B27/40 , B32B2250/24 , B32B2262/0261 , B32B2262/0269 , B32B2262/067 , B32B2262/101 , B32B2262/106 , B32B2262/14 , B32B2307/306 , B32B2605/00 , B32B2605/08 , B32B2605/12 , Y10T428/31551 , Y10T428/31565
摘要： The subject invention discloses a composite structure and a resin component for use in the composite structure. The composite structure includes a first layer, comprising a styrenated unsaturated polyester, and a second layer. The first layer is a show surface of the composite structure. The second layer includes the reaction product of the resin component and an isocyanate component. The resin component includes an isocyanate-reactive component, an amine-based catalyst, and a temperature-activated catalyst that is different from the amine-based catalyst. The amine-based catalyst is active at ambient temperature for initiating an exothermic reaction between the isocyanate component and the resin component thereby establishing a reaction temperature greater than the ambient temperature. The temperature-activated catalyst is active at the reaction temperature for completing a cure of the isocyanate component with the resin component.
摘要翻译：本发明公开了一种用于复合结构的复合结构和树脂组分。复合结构包括第一层，其包含苯乙烯化的不饱和聚酯和第二层。第一层是复合结构的显示表面。第二层包括树脂组分和异氰酸酯组分的反应产物。树脂组分包括与胺类催化剂不同的异氰酸酯反应性组分，胺类催化剂和温度活化催化剂。胺基催化剂在环境温度下是有活性的，用于引发异氰酸酯组分和树脂组分之间的放热反应，从而建立大于环境温度的反应温度。温度活化的催化剂在反应温度下是有活性的，以完成用树脂组分固化异氰酸酯组分。

5. 发明申请

US20050038132A1 Composition for forming a foamed article and an article of furniture having the foamed article disposed therein 审中-公开
标题翻译：用于形成发泡制品的组合物和其中设置有发泡制品的家具制品
公开(公告)号：US20050038132A1
公开(公告)日：2005-02-17
申请号：US10892413
申请日：2004-07-15
申请人： Raghuram Gummaraju , Gene Scheffler , Heinz Plaumann , Theodore Smiecinski , Todd Green
发明人： Raghuram Gummaraju , Gene Scheffler , Heinz Plaumann , Theodore Smiecinski , Todd Green
IPC分类号： C08G18/00 , C08G18/66 , C08J9/00 , C08J9/12 , C08J9/30
CPC分类号： C08G18/6688 , C08G18/3275 , C08G18/4841 , C08G18/632 , C08G18/7621 , C08G2101/0008 , C08G2101/005 , C08G2101/0083 , C08J9/30 , C08J2375/04
摘要： The subject invention provides a foamed article having random cell structures formed by a process comprising the steps of providing a resin component and an isocyanate component and providing a first nucleation gas and a second nucleation gas, both under low pressure. The first and the second nucleation gases are added into at least one of the resin component and the isocyanate component. The resin component and the isocyanate component are reacted to form the foamed article having a first cell structure resulting from the addition of the first nucleation gas and a second cell structure that is different than the first cell structure resulting from the addition of the second nucleation gas. The foamed article is particularly suited for replacing metal springs in an article of furniture while still maintaining the feel and comfort of the metal springs.
摘要翻译：本发明提供了一种发泡制品，其具有通过包括以下步骤形成的无规细胞结构的方法：提供树脂组分和异氰酸酯组分，并在低压下提供第一成核气体和第二成核气体。将第一和第二成核气体加入到至少一种树脂组分和异氰酸酯组分中。使树脂组分和异氰酸酯组分反应形成具有由添加第一成核气体而产生的第一单元结构的发泡制品和与添加第二成核气体所产生的第一单元结构不同的第二单元结构。发泡制品特别适用于在家具制品中更换金属弹簧，同时仍保持金属弹簧的感觉和舒适性。

6. 发明申请

US20060100404A1 Method of reducing a content of a residual styrene monomer in a polyol 失效
公开(公告)号：US20060100404A1
公开(公告)日：2006-05-11
申请号：US10985104
申请日：2004-11-10
申请人： Karl Gust , Heinz Plaumann , Joseph Borst
发明人： Karl Gust , Heinz Plaumann , Joseph Borst
IPC分类号： C08F4/32
CPC分类号： C08G63/90 , C08F6/006 , C08F283/06 , C08F212/08
摘要： A method of reducing a content of a residual styrene monomer in a polyol utilizes a polyol, a peroxide, an adjustment of temperature, and an application of a vacuum to separate the residual styrene monomer from the polyol. The residual styrene monomer is classified as a volatile organic compound. The peroxide includes monoperoxycarbonates and peroxyketals. Peroxide radicals, present in the peroxide, react with and polymerize the residual styrene monomer to form a polymer having decreased volatility. Applying the vacuum physically separates the residual styrene monomer from the polyol by increasing a vapor pressure of the residual styrene monomer. Separating the residual styrene monomer from the polyol forms an improved polyol which includes less than 20 parts per million of the residual styrene monomer in the polyol.

7. 发明授权

US5990203A Method for improving the compatibility of random vinyl substituted aromatic/C.sub.4 -C.sub.6 conjugated diolefin polymer/asphalt mixtures 失效
标题翻译：提高无规乙烯基取代芳香族/ C4-C6共轭二烯烃聚合物/沥青混合物相容性的方法
公开(公告)号：US5990203A
公开(公告)日：1999-11-23
申请号：US72636
申请日：1998-05-04
申请人： John Tze-Chiang Cheng , Heinz Plaumann , Koichi Takamura , Arthur Barry Baughmann , Wai-chun Richard Liu
发明人： John Tze-Chiang Cheng , Heinz Plaumann , Koichi Takamura , Arthur Barry Baughmann , Wai-chun Richard Liu
IPC分类号： C08L95/00 , C08L9/06 , C08L33/06 , C08L63/00 , C08L79/02
CPC分类号： C08L95/00
摘要： The present invention relates to a method for improving the compatibility of random vinyl substituted aromatic/C.sub.4 -C.sub.6 conjugated diolefin polymer/asphalt mixtures comprising adding a modifier to said random vinyl substituted aromatic/C.sub.4 -C.sub.6 conjugated diolefin polymer/asphalt mixture selected from the group consisting of:(a) polymers containing an epoxy functionality(b) polymers containing a carboxyl functionality(c) monomers, oligomers, and polymers containing an amine functionality;(d) monomers, oligomers, and polymers containing an ester functionality; or mixtures thereof.
摘要翻译：本发明涉及一种改进无规乙烯基取代的芳族化合物/ C4-C6共轭二烯烃聚合物/沥青混合物的相容性的方法，包括向所述无规乙烯基取代的芳族/ C4-C6共轭二烯烃聚合物/沥青混合物中加入改性剂包括：（a）含有环氧官能团的聚合物（b）含有羧基官能团的聚合物（c）单体，低聚物和含有胺官能团的聚合物; （d）单体，低聚物和含有酯官能团的聚合物; 或其混合物。

8. 发明申请

US20060051593A1 Urethane acrylate composite structure 审中-公开
标题翻译：聚氨酯丙烯酸酯复合结构
公开(公告)号：US20060051593A1
公开(公告)日：2006-03-09
申请号：US11239892
申请日：2005-09-30
申请人： Calvin Peeler , David Peters , David Kielbasa , Heinz Plaumann
发明人： Calvin Peeler , David Peters , David Kielbasa , Heinz Plaumann
IPC分类号： B32B27/40
CPC分类号： C08G18/672 , C08F290/06 , C08F290/067 , C08G18/7607 , C08G18/7621 , C08G18/7664 , C08G18/7671 , C09D175/16 , Y10T428/31551
摘要： A urethane acrylate composite structure includes a first layer that is a show surface of the urethane acrylate composite structure and a support layer. The support layer includes a urethane acrylate composition that includes a urethane acrylate adduct. The urethane acrylate adduct is the reaction product of an isocyanate component and a stoichiometric excess of a functionalized acrylate component. The isocyanate component includes toluene diisocyanate and polymeric polyphenylmethane polyisocyanate. The functionalized acrylate component is reactive with the isocyanate component. The urethane acrylate composition exhibits improved viscosity due to the isocyanate component. The combination of the toluene diisocyanate and the polymeric polyphenylmethane polyisocyanate results in the improved viscosity of the urethane acrylate composition while maintaining excellent resin curing and finished composite structure properties.
摘要翻译：氨基甲酸酯丙烯酸酯复合结构包括作为氨基甲酸酯丙烯酸酯复合结构的显示表面的第一层和支撑层。支撑层包括包含氨基甲酸酯丙烯酸酯加合物的氨基甲酸酯丙烯酸酯组合物。氨基甲酸酯丙烯酸酯加成物是异氰酸酯组分和化学计量过量的官能化丙烯酸酯组分的反应产物。异氰酸酯组分包括甲苯二异氰酸酯和聚合多苯基甲烷多异氰酸酯。官能化丙烯酸酯组分与异氰酸酯组分反应。氨基甲酸酯丙烯酸酯组合物由于异氰酸酯组分而显示改善的粘度。甲苯二异氰酸酯和聚合聚苯甲烷多异氰酸酯的组合导致改善的氨基甲酸酯丙烯酸酯组合物的粘度，同时保持优异的树脂固化和成品复合结构性能。

9. 发明申请

US20050244653A1 Composite structure, a resin composition for use in the composite structure, and a process for making the same 有权
标题翻译：复合结构体，用于复合结构体的树脂组合物及其制造方法
公开(公告)号：US20050244653A1
公开(公告)日：2005-11-03
申请号：US10834652
申请日：2004-04-29
申请人： Calvin Peeler , Aaron Rath , Heinz Plaumann , James Turnbach
发明人： Calvin Peeler , Aaron Rath , Heinz Plaumann , James Turnbach
IPC分类号： D04H1/00 , D04H13/00
CPC分类号： B32B27/36 , B32B5/08 , B32B27/08 , B32B27/18 , B32B27/20 , B32B27/40 , B32B2250/24 , B32B2262/0261 , B32B2262/0269 , B32B2262/067 , B32B2262/101 , B32B2262/106 , B32B2262/14 , B32B2307/306 , B32B2605/00 , B32B2605/08 , B32B2605/12 , Y10T428/31551 , Y10T428/31565
摘要： The subject invention discloses a composite structure and a resin component for use in the composite structure. The composite structure includes a first layer, comprising a styrenated unsaturated polyester, and a second layer. The first layer is a show surface of the composite structure. The second layer includes the reaction product of the resin component and an isocyanate component. The resin component includes an isocyanate-reactive component, an amine-based catalyst, and a temperature-activated catalyst that is different from the amine-based catalyst. The amine-based catalyst is active at ambient temperature for initiating an exothermic reaction between the isocyanate component and the resin component thereby establishing a reaction temperature greater than the ambient temperature. The temperature-activated catalyst is active at the reaction temperature for completing a cure of the isocyanate component with the resin component.
摘要翻译：本发明公开了一种用于复合结构的复合结构和树脂组分。复合结构包括第一层，其包含苯乙烯化的不饱和聚酯和第二层。第一层是复合结构的显示表面。第二层包括树脂组分和异氰酸酯组分的反应产物。树脂组分包括与胺类催化剂不同的异氰酸酯反应性组分，胺类催化剂和温度活化催化剂。胺类催化剂在环境温度下是有活性的，以引发异氰酸酯组分和树脂组分之间的放热反应，从而建立大于环境温度的反应温度。温度活化的催化剂在反应温度下是有活性的，以完成用树脂组分固化异氰酸酯组分。

10. 发明申请

US20050194713A1 Method of making a molded article 审中-公开
标题翻译：制造模制品的方法
公开(公告)号：US20050194713A1
公开(公告)日：2005-09-08
申请号：US10747639
申请日：2003-12-29
申请人： John Erickson , Dan Wilson , Heinz Plaumann
发明人： John Erickson , Dan Wilson , Heinz Plaumann
IPC分类号： B28B7/22
CPC分类号： B29C44/06 , B29C2037/0035 , B29K2075/00
摘要： The subject invention provides a method of making a molded article (10). The molded article (10) includes a paint layer (12) formed from a paint composition and a polyurethane layer (14) formed from an isocyanate component and an isocyanate-reactive component. The paint composition is applied to a surface (22) of a mold (18, 20) to form the paint layer (12). The paint layer (12) is infused with a base. The polyurethane layer (14) is then adhered to the paint layer (12) in the mold (18, 20) to make the molded article (10). The base promotes adhesion between the paint layer and polyurethane layer of the article by catalyzing a reaction between the isocyanate component in the polyurethane layer (14) and the paint component
摘要翻译：本发明提供了制造模制品（10）的方法。模制品（10）包括由涂料组合物形成的漆层（12）和由异氰酸酯组分和异氰酸酯反应性组分形成的聚氨酯层（14）。将涂料组合物施加到模具（18,20）的表面（22）上以形成涂料层（12）。油漆层（12）注入底座。然后将聚氨酯层（14）粘附到模具（18,20）中的涂料层（12）上以制成模塑制品（10）。基体通过催化聚氨酯层（14）中的异氰酸酯组分与涂料组分（14）之间的反应促进涂料层与制品的聚氨酯层之间的粘附，

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