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1. 发明授权

US06872753B2 Managing hydrogen and carbon monoxide in a gas to liquid plant to control the H2/CO ratio in the Fischer-Tropsch reactor feed 失效
标题翻译：管理气体到液体设备中的氢气和一氧化碳，以控制费 - 托反应堆进料中的H2 / CO比
公开(公告)号：US06872753B2
公开(公告)日：2005-03-29
申请号：US10388843
申请日：2003-03-15
申请人： Stephen R. Landis , Rafael L. Espinoza , Sergio R. Mohedas , Barbara A. Belt , Vincent H. Melquist , Ralph T. Goodwin, III
发明人： Stephen R. Landis , Rafael L. Espinoza , Sergio R. Mohedas , Barbara A. Belt , Vincent H. Melquist , Ralph T. Goodwin, III
IPC分类号： C01B3/38 , C01B3/48 , C07C27/00
CPC分类号： C01B3/48 , C01B3/386 , C01B2203/0261 , C01B2203/0283 , C01B2203/0288 , C01B2203/0475 , C01B2203/061 , C01B2203/062
摘要： The present invention provides a process for controlling the ratio of hydrogen to carbon monoxide in feed streams to reactors that convert syngas to hydrocarbon liquids. The process includes primary syngas production process for converting hydrocarbon gas to syngas comprising hydrogen and carbon monoxide. The process further includes introducing a hydrogen rich stream, a carbon monoxide rich stream, or both produced by an auxiliary source to a feed stream being passed to a reactor for converting the syngas to hydrocarbon liquid, thereby adjusting the H2/CO ratio in the feed stream. Examples of reactors that may be used to convert syngas to hydrocarbon liquids are FT reactors staged in series and oxygenate producing reactors staged in series.
摘要翻译：本发明提供了一种控制进料流中的氢气与一氧化碳与将合成气转化为烃液体的反应器的比例的方法。该方法包括用于将烃气转化成包含氢气和一氧化碳的合成气的初级合成气生产方法。该方法还包括将富氢流，一氧化碳浓缩物流或由辅助源产生的二者引入进料流中，将其转化为反应器以将合成气转化为烃液体，由此调节进料中的H 2 / CO比流。可用于将合成气转化为烃类液体的反应器的实例是分级式的FT反应器和串联的含氧化合物反应器。

2. 发明授权

US07354507B2 Hydroprocessing methods and apparatus for use in the preparation of liquid hydrocarbons 有权
标题翻译：用于制备液体烃的加氢处理方法和装置
公开(公告)号：US07354507B2
公开(公告)日：2008-04-08
申请号：US10802974
申请日：2004-03-17
申请人： Sridhar Gopalakrishnan , Vincent H. Melquist , Rafael L. Espinoza , Doug S. Jack , Keith Henry Lawson
发明人： Sridhar Gopalakrishnan , Vincent H. Melquist , Rafael L. Espinoza , Doug S. Jack , Keith Henry Lawson
IPC分类号： C10G65/00
CPC分类号： C10G65/00 , C10G2400/04
摘要： The present invention is generally related towards enhancing the yield and/or cold-flow properties of certain hydrocarbon products, increasing the degree of isomerization in a diesel product and/or increasing the production rate of a diesel product. The embodiments generally include reducing the residence time of lighter hydrocarbon fractions during hydrocracking, thereby decreasing secondary cracking, by various configurations of introducing at least two hydrocarbon feedstreams of different boiling ranges at different entry points in a hydrocracking unit. A method further includes forming a hydrocarbons stream comprising primarily C5+ Fischer-Tropsch hydrocarbon products; fractionating hydrocarbons stream to form at least a wax fraction and an intermediate fraction which serve as separate feedstreams to a hydrocracking unit comprising at least two hydroconversion zones. One embodiment comprises the use of a bifunctional catalyst in one of the hydrocracking zones so as to favor hydroisomerization of hydrocarbons to favor the formation of branched paraffins boiling in the diesel range.
摘要翻译：本发明通常涉及提高某些烃产品的产率和/或冷流性质，增加柴油产品中的异构化程度和/或提高柴油产品的生产率。实施方案通常包括通过在加氢裂化装置的不同入口处引入不同沸程的至少两种烃进料流的各种构型，减少加氢裂化期间较轻烃馏分的停留时间，从而减少二次裂化。一种方法还包括形成主要包含C 5+费 - 托烃产物的烃物流; 分馏烃流以形成至少蜡馏分和中间馏分，其用作分离的进料流至包含至少两个加氢转化区的加氢裂化单元。一个实施方案包括在一个加氢裂化区中使用双官能催化剂，以有利于烃的加氢异构化，有利于在柴油范围内沸腾的支链烷烃的形成。

3. 发明授权

US07230034B2 Prevention of and recovering from a catalyst bed slumping in a gas-agitated multiphase reactor 有权
标题翻译：在气体搅拌的多相反应器中预防和从催化剂床中回收坍落
公开(公告)号：US07230034B2
公开(公告)日：2007-06-12
申请号：US10804521
申请日：2004-03-19
申请人： Sergio R. Mohedas , Rafael L. Espinoza , Jack E. Cnossen , Todd H. Harkins , Vincent H. Melquist , Larry D. Swinney
发明人： Sergio R. Mohedas , Rafael L. Espinoza , Jack E. Cnossen , Todd H. Harkins , Vincent H. Melquist , Larry D. Swinney
IPC分类号： C07C27/00
CPC分类号： B01J8/22 , B01J8/1809 , B01J8/1827 , B01J2208/00088 , B01J2208/00132 , B01J2208/00548 , C10G2/344
摘要： The invention relates to methods for prevention of and recovery from a catalyst bed slumping in a gas-agitated multiphase hydrocarbon synthesis reactor, while the reactor is either under non-reactive conditions or under reaction promoting conditions when syngas is converted to products. The reactor contains a catalyst bed comprising catalyst particles and a gas injection zone suitable for injecting a reactor gas feed. A method for preventing bed slumping comprises supplying a supplemental gas to the gas-agitated multiphase reactor to prevent the catalyst bed from slumping due to insufficient reactor gas feed flow. The method may include recycling some or all of the supplemental gas to the reactor. The method may further comprise separating the gas injection zone from the catalyst bed with a porous plate so as to prevent migration of catalyst particles into the gas injection zone and to minimize plugging of gas distributor(s) present in said zone.
摘要翻译：本发明涉及用于在气体搅拌的多相烃合成反应器中预防和从催化剂床坍落的方法，同时当合成气转化成产物时，反应器处于非反应性条件或反应促进条件下。反应器包含催化剂床，催化剂床包含催化剂颗粒和适于注入反应器气体进料的气体注入区。防止床塌陷的方法包括向气体搅拌的多相反应器供应补充气体，以防止催化剂床由于反应器气体进料流量不足而塌陷。该方法可以包括将一些或全部补充气体再循环到反应器中。该方法可以进一步包括用多孔板将气体注入区与催化剂床分离，以防止催化剂颗粒迁移到气体注入区中并且使存在于所述区中的气体分配器的堵塞最小化。

4. 发明授权

US07097787B2 Utilization of micro-channel gas distributor to distribute unreacted feed gas into reactors 有权
标题翻译：利用微通道气体分配器将未反应的进料气体分配到反应器中
公开(公告)号：US07097787B2
公开(公告)日：2006-08-29
申请号：US10619698
申请日：2003-07-15
申请人： Guy H. Lewis , Chien-Ping Pan , Harold A. Wright , David H. Anderson , David M. Minahan , Vincent H. Melquist , Cemal Ercan , Gloria I. Straguzzi , Stephen R. Landis , Phillipp R. Ellison
发明人： Guy H. Lewis , Chien-Ping Pan , Harold A. Wright , David H. Anderson , David M. Minahan , Vincent H. Melquist , Cemal Ercan , Gloria I. Straguzzi , Stephen R. Landis , Phillipp R. Ellison
IPC分类号： C01B3/36 , C01B3/38
CPC分类号： B01J4/001 , B01F3/02 , B01F13/0059 , B01J19/0093 , B01J2219/00783 , B01J2219/00835 , B01J2219/00889 , B01J2219/00891 , B01J2219/00984 , C01B3/386 , C01B2203/0261 , C01B2203/12 , C01B2203/1241 , C01B2203/1276 , C01B2203/1282 , Y02P20/52
摘要： A method of partially oxidizing a feed gas comprises providing a reactor containing a catalyst, providing a gas distributor comprising a body having a plurality of channels therethrough and a plurality of outlets from said channels for distributing gas across the catalyst, feeding the feed gas and the oxygen-containing gas into the gas distributor and allowing the feed gas and the oxygen-containing gas to flow through the gas distributor and out through the outlets into contact with the catalyst. The gas distributor preferably comprises a micro-channel gas distributor, which can be assembled by providing a plurality of etched plates defining flow channels, and stacking and fusing the plates. The reactant gases can be mixed within the gas distributor or maintained separately until they have exited the gas distributor.
摘要翻译：一种部分氧化进料气体的方法包括提供一种含有催化剂的反应器，提供一种气体分配器，其包括具有多个通道的主体和从所述通道的多个出口，用于分配气体穿过催化剂，供给进料气体和含氧气体进入气体分配器并允许进料气体和含氧气体通过气体分配器流出并通过出口与催化剂接触。气体分配器优选地包括微通道气体分配器，其可以通过提供限定流动通道的多个蚀刻板并且堆叠和熔合板来组装。反应物气体可以在气体分配器内混合或分开维护，直到它们离开气体分配器。

5. 发明授权

US07001927B2 Water removal in Fischer-Tropsch processes 有权
公开(公告)号：US07001927B2
公开(公告)日：2006-02-21
申请号：US10320311
申请日：2002-12-16
申请人： Jianping Zhang , Harold A. Wright , Yi Jiang , Joe D. Allison , Kenneth M. York , Sergio R. Mohedas , Vincent H. Melquist
发明人： Jianping Zhang , Harold A. Wright , Yi Jiang , Joe D. Allison , Kenneth M. York , Sergio R. Mohedas , Vincent H. Melquist
IPC分类号： C07C27/00 , B01D12/00 , B01D21/00 , B01D17/12
CPC分类号： B01D21/00 , B01D37/00 , C07C27/00 , C07C27/06 , C07C27/26
摘要： A method for water removal in hydrocarbon product reactors operating at Fischer-Tropsch conditions. The water removal decreases the concentration of water in the reactor. In one embodiment, a method of reducing the concentration of water in a Fischer-Tropsch reactor containing a water-rich hydrocarbon product includes removing water from the water-rich hydrocarbon product of the reactor by a water removal means so as to form a water-reduced hydrocarbon product and returning that product to the reactor.

6. 发明授权

US06797252B2 Hydrocarbon gas to liquid conversion process 失效
公开(公告)号：US06797252B2
公开(公告)日：2004-09-28
申请号：US10303606
申请日：2002-11-25
申请人： Daxiang Wang , Barbara A. Belt , Vincent H. Melquist , Steve R. Landis
发明人： Daxiang Wang , Barbara A. Belt , Vincent H. Melquist , Steve R. Landis
IPC分类号： C01B326
CPC分类号： C01B3/386 , C01B3/48 , C01B2203/0261 , C01B2203/0283 , C01B2203/0288 , C01B2203/0475 , C01B2203/061 , C01B2203/062
摘要： The present invention is directed towards a process that allows for the adjustment of hydrogen concentration in a syngas product or Fischer-Tropsch feedstock stream. In particular, the invention is identified as an improved process for producing syngas comprising a secondary chemical reaction, preferably a water gas shift reaction, that allows for the adjustment of the hydrogen concentration in a syngas product stream. Ultimately, the present invention is for an improved process for converting hydrocarbon-containing gas to liquid hydrocarbons.

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