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1. 发明授权

US07915378B2 Material for solid polymer electrolyte, and polyether polymer and process for producing same 有权
标题翻译：固体高分子电解质材料和聚醚聚合物及其制备方法
公开(公告)号：US07915378B2
公开(公告)日：2011-03-29
申请号：US11907685
申请日：2007-10-16
申请人： Hideyuki Nishio , Hidenori Onishi , Paul-Andre Lavoie , Richard Laliberte
发明人： Hideyuki Nishio , Hidenori Onishi , Paul-Andre Lavoie , Richard Laliberte
IPC分类号： C08G65/08 , C08G65/14 , C08G65/22
CPC分类号： H01M10/0565 , C08G65/12 , C08L71/02 , C08L2205/05 , H01B1/122 , H01M10/052 , H01M2300/0082
摘要： A material for solid polymer electrolyte, made of a polyether polymer having a moisture content in the range of 400 to 5,000 ppm by weight. A formed solid polymer electrolyte, which is made by mixing the material for solid polymer electrolyte together with an electrolyte salt compound soluble in the polyether polymer, has good ionic conductivity and high mechanical strength. A polyether polymer having a moisture content not larger than 0.04% by weight and a toluene-insoluble content not larger than 5% by weight. This polyether polymer gives a formed solid polymer electrolyte having a smooth surface.
摘要翻译：一种固体聚合物电解质材料，其由水分含量在400至5,000重量ppm范围内的聚醚聚合物制成。通过将固体聚合物电解质材料与可溶于聚醚聚合物的电解质盐化合物混合而形成的固体高分子电解质具有良好的离子导电性和高的机械强度。水分含量不大于0.04重量％，甲苯不溶成分不大于5重量％的聚醚聚合物。该聚醚聚合物得到具有光滑表面的形成的固体聚合物电解质。

2. 发明申请

US20050059798A1 Polyether polymer and process for producing the same 审中-公开
标题翻译：聚醚聚合物及其制备方法
公开(公告)号：US20050059798A1
公开(公告)日：2005-03-17
申请号：US10494693
申请日：2002-11-05
申请人： Hidenori Onishi , Hideyuki Nishio
发明人： Hidenori Onishi , Hideyuki Nishio
IPC分类号： C08G65/04 , C08G65/10 , C08G65/12 , C08G65/14 , C08G65/26
CPC分类号： C08G65/2672 , C08G65/12 , C08G65/14 , C08G65/2669
摘要： A process for producing a polyether polymer by polymerizing a monomer having an oxirane group in the presence of a Lewis base having no active hydrogen such as, for example, a nitrile compound, a cyclic ether compound or an ester compound; and a polyether polymer produced by this process. Thus, a polyether polymer having a minimized amount of undesirable crosslinked product can be produced without reduction of polymerization activity.
摘要翻译：在具有例如腈化合物，环醚化合物或酯化合物的无活性氢的路易斯碱的存在下聚合具有环氧乙烷基团的单体的聚醚聚合物的制造方法; 和通过该方法制备的聚醚聚合物。因此，可以在不降低聚合活性的情况下制备具有最小量的不需要的交联产物的聚醚聚合物。

3. 发明授权

US07585934B2 Process for producing polyether polymer composition, polyether polymer composition, and solid electrolyte film 有权
标题翻译：制备聚醚聚合物组合物，聚醚聚合物组合物和固体电解质膜的方法
公开(公告)号：US07585934B2
公开(公告)日：2009-09-08
申请号：US10536986
申请日：2003-11-28
申请人： Hideyuki Nishio , Hidenori Onishi
发明人： Hideyuki Nishio , Hidenori Onishi
IPC分类号： C08G65/34
CPC分类号： C08J3/21 , C08G65/30 , C08J3/215 , C08J2371/02 , C08L71/02 , H01M6/181 , H01M10/052 , H01M10/0565 , H01M2300/0082
摘要： A process for producing a polyether polymer composition, comprising incorporating an antioxidant insoluble in an organic solvent and/or a stabilizer soluble in the organic solvent, in a slurry containing a polyether polymer and the organic solvent to disperse or dissolve the antioxidant and/or stabilizer; and then, removing the organic solvent. Also provided a polyether polymer composition comprising a polyether polymer particle, and an antioxidant insoluble in an organic solvent incapable of dissolving the polymer particle, and/or a stabilizer soluble in the organic solvent; and satisfying at least one of the following requirements: (1) most of the antioxidant is deposited on the surface of polymer particle; (2) the polymer has a gel content of not larger than 5% by weight; and (3) most of the stabilizer exists within the polymer particle. The polymer composition produced by the above-mentioned process and the polymer composition satisfying the requirements (1), (2) and (3) give a solid electrolyte film having good mechanical properties.
摘要翻译：一种制备聚醚聚合物组合物的方法，包括将不溶于有机溶剂的抗氧化剂和/或可溶于有机溶剂的稳定剂掺入包含聚醚聚合物和有机溶剂的浆料中以分散或溶解抗氧化剂和/或稳定剂 ; 然后除去有机溶剂。还提供了包含聚醚聚合物颗粒和不溶于不溶于聚合物颗粒的有机溶剂中的抗氧化剂和/或可溶于有机溶剂的稳定剂的聚醚聚合物组合物; 并满足以下要求中的至少一个：（1）大部分抗氧化剂沉积在聚合物颗粒的表面上; （2）聚合物的凝胶含量不大于5重量％; 和（3）大多数稳定剂存在于聚合物颗粒内。通过上述方法制备的聚合物组合物和满足要求（1），（2）和（3）的聚合物组合物得到具有良好机械性能的固体电解质膜。

4. 发明申请

US20060199939A1 Process for producing polyether polymer composition, polyether polymer composition, and solid electrolyte film 有权
公开(公告)号：US20060199939A1
公开(公告)日：2006-09-07
申请号：US10536986
申请日：2003-11-28
申请人： Hideyuki Nishio , Hidenori Onishi
发明人： Hideyuki Nishio , Hidenori Onishi
IPC分类号： C08G8/02
CPC分类号： C08J3/21 , C08G65/30 , C08J3/215 , C08J2371/02 , C08L71/02 , H01M6/181 , H01M10/052 , H01M10/0565 , H01M2300/0082
摘要： A process for producing a polyether polymer composition, comprising incorporating an antioxidant insoluble in an organic solvent and/or a stabilizer soluble in the organic solvent, in a slurry containing a polyether polymer and the organic solvent to disperse or dissolve the antioxidant and/or stabilizer; and then, removing the organic solvent. Also provided a polyether polymer composition comprising a polyether polymer particle, and an antioxidant insoluble in an organic solvent incapable of dissolving the polymer particle, and/or a stabilizer soluble in the organic solvent; and satisfying at least one of the following requirements: (1) most of the antioxidant is deposited on the surface of polymer particle; (2) the polymer has a gel content of not larger than 5% by weight; and (3) most of the stabilizer exists within the polymer particle. The polymer composition produced by the above-mentioned process and the polymer composition satisfying the requirements (1), (2) and (3) give a solid electrolyte film having good mechanical properties.

5. 发明授权

US06894143B2 Polyether polymer, process for producing the same, composition for solid polymer electrolyte, and use thereof 有权
标题翻译：聚醚聚合物，其制造方法，固体高分子电解质用组合物及其用途
公开(公告)号：US06894143B2
公开(公告)日：2005-05-17
申请号：US10482052
申请日：2002-06-28
申请人： Hideyuki Nishio , Hidenori Onishi , Yoshinori Fujii
发明人： Hideyuki Nishio , Hidenori Onishi , Yoshinori Fujii
IPC分类号： C08G65/14 , C08L71/02 , H01M10/052 , H01M10/0565 , C08G65/02
CPC分类号： H01M10/052 , C08G65/14 , C08L71/02 , C08L2205/05 , H01M10/0565 , H01M2300/0082 , C08L2666/22 , C08L71/00
摘要： A composition for solid polymer electrolyte which comprises a polyether polymer and an electrolyte salt compound soluble in the polyether polymer; wherein said polyether polymer is either (1) a polyether polymer having a toluene insoluble content of not larger than 5 weight %, or (2) a polyether polymer having a Mooney viscosity of 3 to 190, which has been prepared by applying a shearing force under heated conditions using an extruder to a polyether polymer having a Mooney viscosity of 10 to 200 so that the Mooney viscosity is reduced by 5 or more. This composition exhibits good film-forming property, and gives a solid polymer electrolyte exhibiting good and uniform ionic conductivity, and having high mechanical strength and surface smoothness. The solid polymer electrolyte is suitable for batteries and capacitors, especially for a lithium ion secondary battery.
摘要翻译：一种固体聚合物电解质组合物，其包含聚醚聚合物和可溶于所述聚醚聚合物的电解质盐化合物; 其中所述聚醚聚合物是（1）甲苯不溶物含量不大于5重量％的聚醚聚合物，或（2）门尼粘度为3至190的聚醚聚合物，其通过施加剪切力在加热条件下使用挤出机至门尼粘度为10〜200的聚醚聚合物，使得门尼粘度降低5以上。该组合物显示出良好的成膜性，并且得到具有良好且均匀的离子导电性并且具有高机械强度和表面光滑度的固体聚合物电解质。固体聚合物电解质适用于电池和电容器，尤其适用于锂离子二次电池。

6. 发明申请

US20080044731A1 Material for solid polymer electrolyte, and polyether polymer and process for producing same 有权
标题翻译：固体高分子电解质材料和聚醚聚合物及其制备方法
公开(公告)号：US20080044731A1
公开(公告)日：2008-02-21
申请号：US11907685
申请日：2007-10-16
申请人： Hideyuki Nishio , Hidenori Onishi , Paul-Andre Lavoie , Richard Laliberte
发明人： Hideyuki Nishio , Hidenori Onishi , Paul-Andre Lavoie , Richard Laliberte
IPC分类号： H01M6/18
CPC分类号： H01M10/0565 , C08G65/12 , C08L71/02 , C08L2205/05 , H01B1/122 , H01M10/052 , H01M2300/0082
摘要： A material for solid polymer electrolyte, made of a polyether polymer having a moisture content in the range of 400 to 5,000 ppm by weight. A formed solid polymer electrolyte, which is made by mixing the material for solid polymer electrolyte together with an electrolyte salt compound soluble in the polyether polymer, has good ionic conductivity and high mechanical strength. A polyether polymer having a moisture content not larger than 0.04% by weight and a toluene-insoluble content not larger than 5% by weight. This polyether polymer gives a formed solid polymer electrolyte having a smooth surface.
摘要翻译：一种固体聚合物电解质材料，其由水分含量在400至5,000重量ppm范围内的聚醚聚合物制成。通过将固体聚合物电解质材料与可溶于聚醚聚合物的电解质盐化合物混合而形成的固体高分子电解质具有良好的离子导电性和高的机械强度。水分含量不大于0.04重量％，甲苯不溶成分不大于5重量％的聚醚聚合物。该聚醚聚合物得到具有光滑表面的形成的固体聚合物电解质。

7. 发明申请

US20060205922A1 Molding material for high-molecular solid electrolytes, moldings of high-molecular solid electrolytes and process for production thereof, and polyether polymer and process for production thereof 审中-公开
标题翻译：高分子固体电解质的成型材料，高分子固体电解质的成型品及其制造方法以及聚醚聚合物及其制造方法
公开(公告)号：US20060205922A1
公开(公告)日：2006-09-14
申请号：US10512432
申请日：2003-04-25
申请人： Hideyuki Nishio , Hidenori Onishi , Paul-Andre Lavoie , Richard Laliberte
发明人： Hideyuki Nishio , Hidenori Onishi , Paul-Andre Lavoie , Richard Laliberte
IPC分类号： C08G65/34
CPC分类号： H01M10/0565 , C08L71/02 , H01M10/052 , H01M2300/0082
摘要： A material for solid polymer electrolyte, comprised of a polyether polymer having a moisture content in the range of 400 to 5,000 ppm by weight. A formed solid polymer electrolyte, which is made by mixing the material for solid polymer electrolyte together with an electrolyte salt compound soluble in the polyether polymer, has good ionic conductivity and high mechanical strength. A polyether polymer having a moisture content not larger than 0.04% by weight and a toluene-insoluble content not larger than 5% by weight. This polyether polymer gives a formed solid polymer electrolyte having a smooth surface.
摘要翻译：一种固体聚合物电解质的材料，其含水分含量为400-5000ppm重量的聚醚聚合物。通过将固体聚合物电解质材料与可溶于聚醚聚合物的电解质盐化合物混合而形成的固体高分子电解质具有良好的离子导电性和高的机械强度。水分含量不大于0.04重量％，甲苯不溶成分不大于5重量％的聚醚聚合物。该聚醚聚合物得到具有光滑表面的形成的固体聚合物电解质。

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