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1. 发明授权

US08697016B2 Reactor for carrying out autothermal gas-phase dehydrogenations 有权
标题翻译：用于进行自热气相脱氢反应器
公开(公告)号：US08697016B2
公开(公告)日：2014-04-15
申请号：US12957618
申请日：2010-12-01
申请人： Grigorios Kolios , Wilhelm Ruppel , Ulrike Wegerle , Jasmina Kessel , Wolfgang Gerlinger , Godwind Tafara Peter Mabande , Goetz-Peter Schindler , Albena Kostova , Gerhard Olbert , Peter Pfab
发明人： Grigorios Kolios , Wilhelm Ruppel , Ulrike Wegerle , Jasmina Kessel , Wolfgang Gerlinger , Godwind Tafara Peter Mabande , Goetz-Peter Schindler , Albena Kostova , Gerhard Olbert , Peter Pfab
IPC分类号： B01J8/04 , C07C5/333
CPC分类号： B01J19/2485 , B01J2219/182
摘要： A reactor in the form of an essentially horizontal cylinder for carrying out an autothermal gas-phase dehydrogenation of a hydrocarbon-comprising gas stream by means of an oxygen-comprising gas stream to give a reaction gas mixture over a heterogeneous catalyst configured as monolith is disclosed herein. The interior of the reactor is divided by a detachable, cylindrical or prismatic housing which is arranged in the longitudinal direction of the reactor, gastight in the circumferential direction and open at two end faces of the housing into an inner region, having one or more catalytically active zones. In each case, a packing composed of monoliths may be stacked on top of one another, next to one another, and above one another and before each catalytically active zone. Also in each case, a mixing zone having solid internals and an outer region arranged coaxially to the inner region are provided.
摘要翻译：公开了一种基本上水平的圆筒形式的反应器，用于通过含氧气流进行含烃气流的自热气相脱氢，得到构成为整料的多相催化剂上的反应气体混合物这里。反应器的内部被可拆卸的圆柱形或棱柱形壳体分隔开，该壳体沿反应器的纵向方向布置，在圆周方向上气密并且在壳体的两个端面处开放到具有一个或多个催化剂的内部区域活动区。在每种情况下，由整料组成的包装可以彼此重叠，彼此重叠，并且在每个催化活性区之前堆叠。在每种情况下，还提供了具有固体内部和与内部区域同轴配置的外部区域的混合区域。

2. 发明授权

US07863468B2 Process for producing propylene oxide 有权
标题翻译：生产环氧丙烷的方法
公开(公告)号：US07863468B2
公开(公告)日：2011-01-04
申请号：US11994129
申请日：2006-06-20
申请人： Goetz-Peter Schindler , Christian Walsdorff , Reinhard Koerner , Hans-Georg Goebbel
发明人： Goetz-Peter Schindler , Christian Walsdorff , Reinhard Koerner , Hans-Georg Goebbel
IPC分类号： C07D301/12
CPC分类号： C07D301/12
摘要： The present invention relates to a process for producing propylene oxide comprising (I) reacting propene with hydrogen peroxide in the presence of a catalyst to give a mixture (GI) comprising propylene oxide, unreacted propene, and oxygen; (II) separating propylene oxide from mixture (GI) to give a mixture (GII) comprising propene and oxygen; (III) reducing the oxygen comprised in mixture (GII) at least partially by reaction with hydrogen in the presence of a catalyst comprising Sn and at least one noble metal.
摘要翻译：本发明涉及一种生产环氧丙烷的方法，其包括（I）在催化剂存在下使丙烯与过氧化氢反应，得到包含环氧丙烷，未反应的丙烯和氧的混合物（GI）（II）将环氧丙烷与混合物（GI）分离，得到包含丙烯和氧的混合物（GII）; （III）在包含Sn和至少一种贵金属的催化剂的存在下至少部分地通过与氢反应来还原混合物（GII）中包含的氧。

3. 发明授权

US07847118B2 Process for continuous heterogeneously catalyzed partial dehydrogenation of at least one hydrocarbon to be dehydrogenated 有权
标题翻译：至少一种待脱氢烃的连续不均匀催化部分脱氢的方法
公开(公告)号：US07847118B2
公开(公告)日：2010-12-07
申请号：US11767782
申请日：2007-06-25
申请人： Claus Hechler , Wilhelm Ruppel , Martin Dieterle , Karl-Heinrich Klappert , Klaus Joachim Mueller-Engel , Goetz-Peter Schindler , Catharina Klanner , Hans-Juergen Bassler
发明人： Claus Hechler , Wilhelm Ruppel , Martin Dieterle , Karl-Heinrich Klappert , Klaus Joachim Mueller-Engel , Goetz-Peter Schindler , Catharina Klanner , Hans-Juergen Bassler
IPC分类号： C07C5/327 , C07C61/317 , C07C5/373
CPC分类号： C07C5/333 , B01J8/067 , B01J19/02 , B01J2219/0236 , C07C51/215 , C22C30/00 , C22C38/40 , Y02P20/52 , C07C11/06 , C07C11/02 , C07C57/04
摘要： A process for continuous heterogeneously catalyzed partial dehydrogenation of at least one hydrocarbon to be dehydrogenated in a reactor which is manufactured from a composite material which consists, on its side in contact with the reaction chamber, of a steel B with specific elemental composition which, on its side facing away from the reaction chamber, either directly or via an intermediate layer of copper, or of nickel, or of copper and nickel, is plated onto a steel A with specific elemental composition, and also partial oxidations of the dehydrogenated hydrocarbon and the reactor itself.
摘要翻译：在反应器中连续不均匀催化的待脱氢烃的部分脱氢的方法，该反应器由复合材料制成，该复合材料在其与反应室接触的一侧由具有特定元素组成的钢B组成，其直接或经由铜或镍或铜和镍的中间层离开反应室的一侧被镀在具有特定元素组成的钢A上，并且还将脱氢烃和反应堆本身。

4. 发明申请

US20100048960A1 PROCESS FOR PREPARING ISOPROPANOL AND 2-BUTANOL FROM THE CORRESPONDING ALKANES 失效
标题翻译：从相应的碱中制备异丙醇和2-丁醇的方法
公开(公告)号：US20100048960A1
公开(公告)日：2010-02-25
申请号：US12374351
申请日：2007-07-16
申请人： Georg Degen , Sven Crone , Ralf Boehling , Ansgar Gereon Altenhoff , Wolfgang Rohde , Jochen Buerkle , Goetz-Peter Schindler , Thomas Holtmann , Markus Schmitt
发明人： Georg Degen , Sven Crone , Ralf Boehling , Ansgar Gereon Altenhoff , Wolfgang Rohde , Jochen Buerkle , Goetz-Peter Schindler , Thomas Holtmann , Markus Schmitt
IPC分类号： C07C29/04
CPC分类号： C07C67/04 , C07C29/095 , Y02P20/127 , C07C31/10 , C07C31/12 , C07C69/06 , C07C69/14
摘要： A process for preparing alkanols (I) selected from the group consisting of isopropanol and 2-butanol from the corresponding alkanes (II) selected from the group consisting of propane and n-butane, comprising the steps of: A) providing a starting gas stream a comprising the alkane (II); B) feeding the starting gas stream a comprising the alkane (II) into a dehydrogenation zone and subjecting the alkane (II) to a dehydrogenation to the alkene (III) to obtain a product gas stream b comprising the alkene (III) and unconverted alkane (II), with or without high boilers, steam, hydrogen and low boilers; C) at least compressing product gas stream b, optionally separating product gas stream b into an aqueous phase c1, a phase c2 comprising the alkene (III) and the alkane (II), with or without high boilers, and a gas phase c3 comprising hydrogen and low boilers; D) reacting product gas stream b or the phase c2 comprising alkene (III) and alkane (II) with an organic acid (IV) in an esterification zone to obtain a product mixture d comprising the corresponding alkyl ester (V) of the organic acid and the unconverted alkane (II); E) removing from product mixture d a gas stream e1 which comprises an alkane (II) and is recycled into the dehydrogenation zone if appropriate, and a product mixture e2 comprising the alkyl ester; F) reacting the product mixture e2 comprising the alkyl ester with water in an ester hydrolysis zone to give a product mixture f comprising the alkanol (I) and the organic acid (IV); G) removing the alkanol (I) and the organic acid (IV) from product mixture f and, if appropriate, recycling the organic acid into the esterification zone.
摘要翻译：从选自丙烷和正丁烷的相应的烷烃（II）制备选自异丙醇和2-丁醇的链烷醇（I）的方法，包括以下步骤：A）提供起始气流 a包含烷烃（II）; B）将包含烷烃（II）的起始气体流（a）进料到脱氢区中并使烷烃（II）脱氢至烯烃（III），得到包含烯烃（III）和未转化烷烃的产物气流b （II），有或没有高锅炉，蒸汽，氢气和低锅炉; C）至少压缩产物气流b，任选地将产物气流b分离成水相c1，包含烯烃（III）和烷烃（II）的阶段c2，具有或不具有高锅炉，以及气相c3，其包含氢和低锅炉; D）使产物气流b或包含烯烃（III）和烷烃（II）的相c与酯化区中的有机酸（IV）反应，得到包含相应的有机酸烷基酯（V）的产物混合物d 和未转化的烷烃（II）; E）从产物混合物d除去包含烷烃（II）的气流e1，并且如果合适的话再循环到脱氢区中，以及包含烷基酯的产物混合物e2; F）在酯水解区中使包含烷基酯的产物混合物e2与水反应，得到包含链烷醇（I）和有机酸（IV）的产物混合物f; G）从产物混合物f中除去链烷醇（I）和有机酸（IV），如果合适，将有机酸再循环到酯化区。

5. 发明授权

US07592483B2 Preparation of acrolein or acrylic acid or a mixture thereof by heterogeneously catalyzed partial gas phase oxidation of propylene 有权
标题翻译：通过非均相催化的丙烯部分气相氧化制备丙烯醛或丙烯酸或其混合物
公开(公告)号：US07592483B2
公开(公告)日：2009-09-22
申请号：US11131261
申请日：2005-05-18
申请人： Martin Dieterle , Armin Diefenbacher , Goetz-Peter Schindler , Catharina Klanner , Klaus Joachim Mueller-Engel , Christoph Adami
发明人： Martin Dieterle , Armin Diefenbacher , Goetz-Peter Schindler , Catharina Klanner , Klaus Joachim Mueller-Engel , Christoph Adami
IPC分类号： C07C229/00 , C07C53/00 , C07C45/00
CPC分类号： C07C51/252 , C07C45/35 , C07C57/04 , C07C47/22
摘要： A process for preparing acrolein or acrylic acid or a mixture thereof by heterogeneously catalyzed partial gas oxidation of propylene, in which the starting reaction gas mixture has the following contents: from 6 to 9% by volume of propylene, from 8 to 18% by volume of molecular oxygen, from 6 to 30% by volume of propane and from 32 to 72% by volume of molecular nitrogen.
摘要翻译：丙烯醛或丙烯酸或其混合物通过丙烯的非均相催化部分气体氧化制备的方法，其中起始反应气体混合物具有以下含量：6至9体积％的丙烯，8至18体积％的分子氧，6至30体积％的丙烷和32至72体积％的分子氮。

6. 发明授权

US07566799B2 Process for the preparation of alkylaryl compounds and sulfonates thereof 失效
标题翻译：烷基芳基化合物及其磺酸盐的制备方法
公开(公告)号：US07566799B2
公开(公告)日：2009-07-28
申请号：US10490218
申请日：2002-10-01
申请人： Ulrich Steinbrenner , Thomas Heidemann , Goetz-Peter Schindler , Juergen Stephan , Heiko Maas
发明人： Ulrich Steinbrenner , Thomas Heidemann , Goetz-Peter Schindler , Juergen Stephan , Heiko Maas
IPC分类号： C07C15/107 , C07C2/66 , C07C309/31
CPC分类号： C11D1/22 , C07C15/00 , C07C309/31
摘要： The preparation of alkylaryl compounds takes place, inter alia, by a1) preparation of a C4 -olefin mixture from LPG, LNG or MTO streams, b 1) reaction of the C4-olefin mixture obtained in this way over a metathesis catalyst for the preparation of an olefin mixture comprising 2-pentene and/or 3-hexene, and optional removal of 2-pentene and/or 3-hexene, c1) dimerization of the 2-pentane and/or 3-hexene obtained in stage b1) over a dimerization catalyst to give a mixture comprising C10-12-olefins, and optional removal of the C10-12- olefins, d1) reaction of the C10-12-olefin mixtures obtained in stage a1) with an aromatic hydrocarbon in the presence of an alkylation catalyst to form alkylaromatic compounds, it being possible to add additional linear olefins prior to the reaction.
摘要翻译：烷基芳基化合物的制备尤其通过a1）由LPG，LNG或MTO流体制备C4-烯烃混合物，b 1）以这种方式获得的C 4 - 烯烃混合物与复分解催化剂的反应，用于制备的包含2-戊烯和/或3-己烯的烯烃混合物，并任选地除去2-戊烯和/或3-己烯，c1）在步骤b1）中获得的2-戊烷和/或3-己烯的二聚化，二聚催化剂，得到包含C10-12-烯烃的混合物，任选地除去C10-12-烯烃，d1）在烷基化存在下，在步骤a1）中获得的C10-12-烯烃混合物与芳族烃反应催化剂形成烷基芳族化合物，可以在反应之前加入另外的直链烯烃。

7. 发明授权

US07388109B2 Preparation of acrolein or acrylic acid or a mixture thereof from propane 有权
标题翻译：从丙烷制备丙烯醛或丙烯酸或其混合物
公开(公告)号：US07388109B2
公开(公告)日：2008-06-17
申请号：US11131248
申请日：2005-05-18
申请人： Otto Machhammer , Goetz-Peter Schindler , Christoph Adami , Claus Hechler , Martin Dieterle
发明人： Otto Machhammer , Goetz-Peter Schindler , Christoph Adami , Claus Hechler , Martin Dieterle
IPC分类号： C07C51/16
CPC分类号： C07C45/33 , B01J8/0453 , B01J8/0457 , B41J2/17513 , C07C45/35 , C07C51/215 , C07C51/252 , C07C47/22 , C07C57/04
摘要： A process for preparing acrolein or acrylic acid or a mixture thereof from propane, in which the propane is initially dehydrogenated under heterogeneous catalysis to give propene, secondary components are removed and the remaining gas mixture, comprising propane and propene, is subjected to the heterogeneously catalyzed partial oxidation to acrolein or acrylic acid or a mixture thereof as the target product, target product is removed from the product gas mixture and the remaining residual gas, comprising excess oxygen and unconverted propane, is recycled into the propane dehydrogenation in such a way that the other propane fed to the dehydrogenation is at least partly converted under dehydrogenating conditions at the recycle point.
摘要翻译：从丙烷制备丙烯醛或丙烯酸或其混合物的方法，其中丙烷最初在非均相催化下脱氢以得到丙烯，次要组分被除去，剩余的包含丙烷和丙烯的气体混合物经历非均相催化部分氧化成丙烯醛或丙烯酸或其混合物作为目标产物，将目标产物从产物气体混合物中除去，剩余的包含过量氧气和未转化的丙烷的残余气体以这样的方式循环到丙烷脱氢中：进料到脱氢的其它丙烷在再循环点的脱氢条件下至少部分转化。

8. 发明授权

US5681973A Microporous heteropolyoxometallates and method of their production and use as catalysts 失效
标题翻译：微孔杂多金属氧酸盐及其生产和使用方法作为催化剂
公开(公告)号：US5681973A
公开(公告)日：1997-10-28
申请号：US502261
申请日：1995-07-13
申请人： Wolfgang Hoelderich , Markus Hoelscher , Goetz-Peter Schindler , Ulli Englert , Bodo Zibrowius , Dietrich Arntz
发明人： Wolfgang Hoelderich , Markus Hoelscher , Goetz-Peter Schindler , Ulli Englert , Bodo Zibrowius , Dietrich Arntz
IPC分类号： B01J27/188 , B01J27/19 , B01J27/198 , B01J31/02 , B01J31/16 , B01J31/34 , B01J31/36 , C07F11/00 , C07F19/00 , C07F9/02 , C07F6/00
CPC分类号： B01J31/1691 , B01J23/002 , B01J27/188 , B01J27/198 , B01J31/0237 , C07F11/005 , B01J2231/70 , B01J2231/72 , B01J2523/00 , B01J2531/56 , B01J2531/64 , B01J2531/66
摘要： Heteropolyoxometallates of tungsten, molybdenum and vanadium with a structurally defined micropore volume, a method of production by means of the hydrothermal reaction of the appropriate metal with an associated oxide, a diamine, phosphoric acid and water, and the use of the novel compounds as catalysts.
摘要翻译：具有结构限定的微孔体积的钨，钼和钒的多金属氧酸盐，通过适当金属与相关氧化物，二胺，磷酸和水的水热反应的生产方法，以及新型化合物作为催化剂的用途。

9. 发明授权

US09091433B2 Monolith catalyst and use thereof 有权
标题翻译：单片催化剂及其用途
公开(公告)号：US09091433B2
公开(公告)日：2015-07-28
申请号：US13321388
申请日：2010-05-18
申请人： Godwind Tafara Peter Mabande , Soo Yin Chin , Goetz-Peter Schindler , Gerald Koermer , Dieter Harms , Burkhard Rabe , Howard Furbeck , Oliver Seel
发明人： Godwind Tafara Peter Mabande , Soo Yin Chin , Goetz-Peter Schindler , Gerald Koermer , Dieter Harms , Burkhard Rabe , Howard Furbeck , Oliver Seel
IPC分类号： F23C13/08 , B01J19/24 , B01J23/40 , B01J23/42 , B01J23/58 , B01J23/62 , B01J23/63 , B01J23/656 , B01J23/96 , B01J35/00 , B01J35/02 , B01J35/04 , B01J37/00 , B01J37/02 , C07C5/333 , C07C5/393 , B01J21/04 , B01J21/06 , B01J38/10 , B01J38/12
CPC分类号： F23C13/08 , B01J19/2485 , B01J21/04 , B01J21/06 , B01J21/066 , B01J23/40 , B01J23/42 , B01J23/58 , B01J23/624 , B01J23/63 , B01J23/6567 , B01J23/96 , B01J35/002 , B01J35/0026 , B01J35/023 , B01J35/04 , B01J37/0036 , B01J37/0045 , B01J37/0205 , B01J37/0228 , B01J37/0242 , B01J37/0248 , B01J38/10 , B01J38/12 , C07C5/3337 , C07C5/393 , C07C2523/42 , C07C2523/62 , F23C2900/9901 , Y02P20/52 , Y02P20/584 , C07C11/06 , C07C11/08 , C07C15/08
摘要： The invention relates to a catalyst comprising a monolith composed of a catalytically inert material with low BET surface area and a catalyst layer which has been applied to the monolith and comprises, on an oxidic support material, at least one noble metal selected from the group consisting of the noble metals of group VIII of the Periodic Table of the Elements, optionally tin and/or rhenium, and optionally further metals, wherein the thickness of the catalyst layer is 5 to 500 micrometers.
摘要翻译：本发明涉及一种催化剂，其包含由具有低BET表面积的催化惰性材料构成的整料和已经施加到整料上的催化剂层，并且在氧化载体材料上包含至少一种选自以下的贵金属：的元素周期表第Ⅷ族的贵金属，任选的锡和/或铼，以及任选的另外的金属，其中催化剂层的厚度为5至500微米。

10. 发明申请

US20120065443A1 MONOLITH CATALYST AND USE THEREOF 有权
标题翻译：单体催化剂及其用途
公开(公告)号：US20120065443A1
公开(公告)日：2012-03-15
申请号：US13321388
申请日：2010-05-18
申请人： Godwind Tafara Peter Mabande , Soo Yin Chin , Goetz-Peter Schindler , Gerald Koermer , Dieter Harms , Burkhard Rabe , Howard Furbeck , Oliver Seel
发明人： Godwind Tafara Peter Mabande , Soo Yin Chin , Goetz-Peter Schindler , Gerald Koermer , Dieter Harms , Burkhard Rabe , Howard Furbeck , Oliver Seel
IPC分类号： C07C5/367 , C07C5/333
CPC分类号： F23C13/08 , B01J19/2485 , B01J21/04 , B01J21/06 , B01J21/066 , B01J23/40 , B01J23/42 , B01J23/58 , B01J23/624 , B01J23/63 , B01J23/6567 , B01J23/96 , B01J35/002 , B01J35/0026 , B01J35/023 , B01J35/04 , B01J37/0036 , B01J37/0045 , B01J37/0205 , B01J37/0228 , B01J37/0242 , B01J37/0248 , B01J38/10 , B01J38/12 , C07C5/3337 , C07C5/393 , C07C2523/42 , C07C2523/62 , F23C2900/9901 , Y02P20/52 , Y02P20/584 , C07C11/06 , C07C11/08 , C07C15/08
摘要： The invention relates to a catalyst comprising a monolith composed of a catalytically inert material with low BET surface area and a catalyst layer which has been applied to the monolith and comprises, on an oxidic support material, at least one noble metal selected from the group consisting of the noble metals of group VIII of the Periodic Table of the Elements, optionally tin and/or rhenium, and optionally further metals, wherein the thickness of the catalyst layer is 5 to 500 micrometers.
摘要翻译：本发明涉及一种催化剂，其包含由具有低BET表面积的催化惰性材料构成的整料和已经施加到整料上的催化剂层，并且在氧化载体材料上包含至少一种选自以下的贵金属：的元素周期表第Ⅷ族的贵金属，任选的锡和/或铼，以及任选的另外的金属，其中催化剂层的厚度为5至500微米。

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