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1. 发明授权

US5672796A Catalyst and process for hydrocarbon aromatization 失效
标题翻译：用于烃芳构化的催化剂和方法
公开(公告)号：US5672796A
公开(公告)日：1997-09-30
申请号：US574120
申请日：1995-12-18
申请人： Gilbert Fernand Alphonse Froment , Wilfried Jozef Hippolyte Dehertog
发明人： Gilbert Fernand Alphonse Froment , Wilfried Jozef Hippolyte Dehertog
IPC分类号： B01J29/44 , B01J29/48 , C07C2/00 , C07C15/00 , B01J29/06
CPC分类号： B01J29/48 , C07C2/00 , C07C2521/04 , C07C2521/08 , C07C2529/74
摘要： A catalyst and process is described for aromatizing one or more C.sub.3 to C.sub.6 saturated hydrocarbon to a product low in methane and essentially containing ethane or ethane and propane and aromatic hydrocarbons. A partially sulfided, Pt/Re loaded, essentially hydrogen-form, crystalline aluminosilicate molecular sieve exhibiting the MFI structure and having a Si/Al ratio between about 40 and about 600 is shown to have an excellent catalyst lifetime and favor low methane production, high conversion and high selectivity to benzene, toluene and xylenes and ethane or ethane and propane.
摘要翻译：描述了一种催化剂和方法，用于将一种或多种C 3至C 6饱和烃芳族化为低甲烷和基本上含有乙烷，乙烷和丙烷和芳族烃的产物。表现出MFI结构并具有约40至约600的Si / Al比的部分硫化的Pt / Re负载的基本氢形态的结晶硅铝酸盐分子筛显示具有优异的催化剂寿命并有利于低甲烷生产，高对苯，甲苯和二甲苯以及乙烷或乙烷和丙烷的转化率和选择性高。

2. 发明授权

US06548725B2 Process for manufacturing olefins 失效
标题翻译：制造烯烃的方法
公开(公告)号：US06548725B2
公开(公告)日：2003-04-15
申请号：US09918925
申请日：2001-07-31
申请人： Gilbert Fernand Alphonse Froment , Wilfried Jozef Hippolyte Dehertog , Mark P. Kaminsky
发明人： Gilbert Fernand Alphonse Froment , Wilfried Jozef Hippolyte Dehertog , Mark P. Kaminsky
IPC分类号： C07C406
CPC分类号： C07C4/06 , B01J29/061 , B01J29/405 , B01J29/82 , B01J2229/26 , B01J2229/42 , C07C2529/40 , C10G2400/20 , Y02P30/40
摘要： A catalyst and an improved process for producing olefins by catalytic naphtha cracking are described. The process provides relatively higher yields over a commercially important range of naphtha conversion, while providing about the same or lower yields of aromatics and methane over the range. In the process, a hydrocarbon naphtha feedstock including a hydrocarbon having about three to about twenty carbon atoms per molecule is passed into a reactor containing a pentasil zeolite catalyst. The catalyst includes about 0.1 to about 10 weight percent phosphorus and about 0.1 to about 10 weight percent of a promoter metal selected from the group consisting of gallium, germanium, tin and mixtures thereof. The hydrocarbon may be passed into the reactor together with a diluent selected from the group consisting of steam, nitrogen, methane, and ethane and mixtures thereof. Alternatively, the hydrocarbon may be passed into the reactor together with additional propane.
摘要翻译：描述了通过催化石脑油裂解生产烯烃的催化剂和改进方法。该方法在商业上重要的石脑油转化范围上提供相对较高的产率，同时在该范围内提供大约相同或更低的芳族化合物和甲烷的产率。在此过程中，将包含每分子约3至约20个碳原子的烃类石脑油原料进入含有pentasil沸石催化剂的反应器中。催化剂包括约0.1至约10重量％的磷和约0.1至约10重量％的选自镓，锗，锡及其混合物的助催化剂金属。烃可以与选自蒸汽，氮气，甲烷和乙烷的稀释剂及其混合物一起进入反应器。或者，烃可以与另外的丙烷一起进入反应器。

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