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1. 发明申请

US20110028644A1 NOVEL COMPOSITIONS, METHODS AND POLYMERS 有权
标题翻译：新型组合物，方法和聚合物
公开(公告)号：US20110028644A1
公开(公告)日：2011-02-03
申请号：US12828121
申请日：2010-06-30
申请人： Christopher T. Brown , Chad Landis , Elena E. Sheina
发明人： Christopher T. Brown , Chad Landis , Elena E. Sheina
IPC分类号： C08L81/02 , C08G75/06 , C08G65/38 , C08G73/10 , C08L79/08
CPC分类号： H01B1/127 , C07D495/04 , C07D495/14 , C07D513/14 , C08G61/12 , C08G61/123 , C08G61/126 , C08G2261/124 , C08G2261/141 , C08G2261/3162 , C08G2261/3243 , C08G2261/334 , C08G2261/344 , C08G2261/364 , C08G2261/414 , C08G2261/91 , C09B57/004 , C09B57/007 , C09B57/08 , C09B69/008 , C09B69/109 , H01L51/0003 , H01L51/0015 , H01L51/0043 , H01L51/0051 , Y02P20/582
摘要： A composition comprising a homopolymer or a copolymer comprising bithiophene units for use in, for example, low band gap materials including uses in organic photovoltaic active layers. The band gap and other properties can be engineered by polymerization methods including selection of monomer structure and ratio of monomer components. In addition, a dimer adapted for making alternating copolymers further comprising one first monomer moiety comprising at least one bithiophene moiety compound covalently linked to one second monomer moiety comprising a different bithiophene moiety or at least one moiety that is not a bithiophene. The composition can be copolymerized to form an alternating copolymer that can be further processed to form a polymeric film used in a printed organic electronic device. A series of novel copolymers are designed that would allow fabrication of materials with tailor made electronic and/or mechanical properties that can be easily manipulated through molecules chemical structure and potentially result in long term stability under ambient conditions that can be advantageous for use in organic electronics (e.g., OPVs, OLEDs, OFETs). Improved methods are disclosed for making monomers comprising a benzo[2,1-b:3,4-b′]dithiophene moiety that are useful as electronics materials.
摘要翻译：包含均聚物或包含双噻吩单元的共聚物的组合物，其用于例如用于有机光伏活性层中的低带隙材料。可以通过包括选择单体结构和单体组分的比例的聚合方法来设计带隙和其它性质。此外，适于制备交替共聚物的二聚体还包含一个第一单体部分，其包含至少一个共价连接到包含不同双噻吩部分的一个第二单体部分或至少一个不是二噻吩的部分的双噻吩部分化合物。该组合物可以共聚以形成可进一步加工以形成印刷有机电子器件中使用的聚合物膜的交替共聚物。一系列新型共聚物被设计成允许制造具有定制的电子和/或机械性质的材料，其可以通过分子化学结构容易地操作，并且潜在地在环境条件下导致长期稳定性，这对于用于有机电子（例如，OPV，OLED，OFET）。公开了用于制备包含可用作电子材料的苯并[2,1-b：3,4-b']二噻吩部分的单体的改进方法。

2. 发明授权

US08691931B2 Organic electronic devices and polymers, including photovoltaic cells and diketone-based and diketopyrrolopyrrole-based polymers 失效
标题翻译：有机电子器件和聚合物，包括光伏电池和基于二酮和二酮吡咯并吡咯的聚合物
公开(公告)号：US08691931B2
公开(公告)日：2014-04-08
申请号：US12874137
申请日：2010-09-01
申请人： Christopher T. Brown , Christophe René Gaston Grenier , Chad Landis , Elena E. Sheina , Ting Xu
发明人： Christopher T. Brown , Christophe René Gaston Grenier , Chad Landis , Elena E. Sheina , Ting Xu
IPC分类号： C08G14/10
CPC分类号： C08L65/00 , C07D487/04 , C07D495/04 , C07D519/00 , C07F7/0816 , C08G61/12 , C08G61/126 , C08G2261/124 , C08G2261/18 , C08G2261/226 , C08G2261/228 , C08G2261/3223 , C08G2261/334 , C08G2261/344 , C08G2261/364 , C08G2261/414 , C09B57/004 , C09B69/008 , C09B69/109 , C09D165/00 , H01L51/0036 , H01L51/0043 , H01L51/0069 , H01L51/0077 , H01L51/4253 , Y02E10/549 , Y10S428/917
摘要： Polymers which can be used in p-type materials for organic electronic devices and photovoltaic cells. Compounds, monomers, dimers, trimers, and polymers comprising: wherein A1 and A2 each independently comprise a fused ring system comprising at least two fused rings directly covalently linked to the pyrrole rings. Good photovoltaic efficiency and lifetime can be achieved. The R group can provide solubility, environmental stability, and fine tuning of spectroscopic and/or electronic properties. Different polymer microstructures can be prepared which encourage multiple band gaps and broad and strong absorptions. The carbonyl can interact with adjacent thiophene rings to provide backbone with rigidity, induce planarity, and reduce and/or eliminate intramolecular chain twisting defects.
摘要翻译：可用于有机电子器件和光伏电池的p型材料的聚合物。化合物，单体，二聚体，三聚体和聚合物，其包含：其中A1和A2各自独立地包含稠环系统，其包含直接共价连接到吡咯环上的至少两个稠合环。可以实现良好的光伏效率和寿命。 R基团可以提供光谱和/或电子性质的溶解度，环境稳定性和微调。可以制备不同的聚合物微结构，其可以鼓励多个带隙和宽而强的吸收。羰基可以与相邻的噻吩环相互作用以提供具有刚性，诱导平面性的主链，并减少和/或消除分子内链扭曲缺陷。

3. 发明申请

US20110114184A1 ORGANIC ELECTRONIC DEVICES AND POLYMERS, INCLUDING PHOTOVOLTAIC CELLS AND DIKETONE-BASED AND DIKETOPYRROLOPYRROLE-BASED POLYMERS 失效
标题翻译：有机电子器件和聚合物，包括光伏电池和基于二酮和基于二烯丙基的聚合物
公开(公告)号：US20110114184A1
公开(公告)日：2011-05-19
申请号：US12874137
申请日：2010-09-01
申请人： Christopher T. Brown , Christophe René Gaston Grenier , Chad Landis , Elena E. Sheina , Ting Xu
发明人： Christopher T. Brown , Christophe René Gaston Grenier , Chad Landis , Elena E. Sheina , Ting Xu
IPC分类号： H01L31/0256 , C08F28/06 , C07D497/22
CPC分类号： C08L65/00 , C07D487/04 , C07D495/04 , C07D519/00 , C07F7/0816 , C08G61/12 , C08G61/126 , C08G2261/124 , C08G2261/18 , C08G2261/226 , C08G2261/228 , C08G2261/3223 , C08G2261/334 , C08G2261/344 , C08G2261/364 , C08G2261/414 , C09B57/004 , C09B69/008 , C09B69/109 , C09D165/00 , H01L51/0036 , H01L51/0043 , H01L51/0069 , H01L51/0077 , H01L51/4253 , Y02E10/549 , Y10S428/917
摘要： Polymers which can be used in p-type materials for organic electronic devices and photovoltaic cells. Compounds, monomers, dimers, trimers, and polymers comprising: wherein A1 and A2 each independently comprise a fused ring system comprising at least two fused rings directly covalently linked to the pyrrole rings. Good photovoltaic efficiency and lifetime can be achieved. The R group can provide solubility, environmental stability, and fine tuning of spectroscopic and/or electronic properties. Different polymer microstructures can be prepared which encourage multiple band gaps and broad and strong absorptions. The carbonyl can interact with adjacent thiophene rings to provide backbone with rigidity, induce planarity, and reduce and/or eliminate intramolecular chain twisting defects.
摘要翻译：可用于有机电子器件和光伏电池的p型材料的聚合物。化合物，单体，二聚体，三聚体和聚合物，其包含：其中A1和A2各自独立地包含稠环系统，其包含直接共价连接到吡咯环上的至少两个稠合环。可以实现良好的光伏效率和寿命。 R基团可以提供光谱和/或电子性质的溶解度，环境稳定性和微调。可以制备不同的聚合物微结构，其可以鼓励多个带隙和宽而强的吸收。羰基可以与相邻的噻吩环相互作用以提供具有刚性，诱导平面性的主链，并减少和/或消除分子内链扭曲缺陷。

4. 发明授权

US08968885B2 Organic electronic devices and polymers, including photovoltaic cells and diketone-based polymers 有权
标题翻译：有机电子器件和聚合物，包括光伏电池和基于二酮的聚合物
公开(公告)号：US08968885B2
公开(公告)日：2015-03-03
申请号：US12874163
申请日：2010-09-01
申请人： Christopher T. Brown , Christophe René Gaston Grenier , Chad Landis , Elena E. Sheina , Atta Gueye
发明人： Christopher T. Brown , Christophe René Gaston Grenier , Chad Landis , Elena E. Sheina , Atta Gueye
IPC分类号： H01L51/54 , H01L51/46 , C08F228/06 , C08L41/00 , C08L65/00 , C07D487/04 , C07D495/04 , C07D519/00 , C07F7/08 , C08G61/12 , C09D165/00 , H01L51/00 , C09B57/00 , C09B69/00 , C09B69/10 , H01L51/42
CPC分类号： C08L65/00 , C07D487/04 , C07D495/04 , C07D519/00 , C07F7/0816 , C08G61/12 , C08G61/126 , C08G2261/124 , C08G2261/18 , C08G2261/226 , C08G2261/228 , C08G2261/3223 , C08G2261/334 , C08G2261/344 , C08G2261/364 , C08G2261/414 , C09B57/004 , C09B69/008 , C09B69/109 , C09D165/00 , H01L51/0036 , H01L51/0043 , H01L51/0069 , H01L51/0077 , H01L51/4253 , Y02E10/549 , Y10S428/917
摘要： Polymers which can be used in p-type materials for organic electronic devices and photovoltaic cells. Compounds, monomers, dimers, trimers, and polymers comprising: Good photovoltaic efficiency and lifetime can be achieved. The R group can provide solubility, environmental stability, and fine tuning of spectroscopic and/or electronic properties. Different polymer microstructures can be prepared which encourage multiple band gaps and broad and strong absorptions. The carbonyl can interact with adjacent thiophene rings to provide backbone with rigidity, induce planarity, and reduce and/or eliminate intramolecular chain twisting defects. Polymers comprising benzodithiophene and/or benzothiadiazole structures can show particularly high performance.
摘要翻译：可用于有机电子器件和光伏电池的p型材料的聚合物。化合物，单体，二聚体，三聚体和聚合物包括：可以实现良好的光电效率和寿命。 R基团可以提供光谱和/或电子性质的溶解度，环境稳定性和微调。可以制备不同的聚合物微结构，其可以鼓励多个带隙和宽而强的吸收。羰基可以与相邻的噻吩环相互作用以提供具有刚性，诱导平面性的主链，并减少和/或消除分子内链扭曲缺陷。包含苯并二噻吩和/或苯并噻二唑结构的聚合物可表现出特别高的性能。

5. 发明授权

US08440785B2 Compositions, methods and polymers 有权
标题翻译：组合物，方法和聚合物
公开(公告)号：US08440785B2
公开(公告)日：2013-05-14
申请号：US12828121
申请日：2010-06-30
申请人： Christopher T. Brown , Chad Landis , Elena E. Sheina
发明人： Christopher T. Brown , Chad Landis , Elena E. Sheina
IPC分类号： C08G75/00
CPC分类号： H01B1/127 , C07D495/04 , C07D495/14 , C07D513/14 , C08G61/12 , C08G61/123 , C08G61/126 , C08G2261/124 , C08G2261/141 , C08G2261/3162 , C08G2261/3243 , C08G2261/334 , C08G2261/344 , C08G2261/364 , C08G2261/414 , C08G2261/91 , C09B57/004 , C09B57/007 , C09B57/08 , C09B69/008 , C09B69/109 , H01L51/0003 , H01L51/0015 , H01L51/0043 , H01L51/0051 , Y02P20/582
摘要： A composition comprising a homopolymer or a copolymer comprising bithiophene units for use in, for example, low band gap materials including uses in organic photovoltaic active layers. The band gap and other properties can be engineered by polymerization methods including selection of monomer structure and ratio of monomer components. In addition, a dimer adapted for making alternating copolymers further comprising one first monomer moiety comprising at least one bithiophene moiety compound covalently linked to one second monomer moiety comprising a different bithiophene moiety or at least one moiety that is not a bithiophene. The composition can be copolymerized to form an alternating copolymer that can be further processed to form a polymeric film used in a printed organic electronic device. A series of novel copolymers are designed that would allow fabrication of materials with tailor made electronic and/or mechanical properties that can be easily manipulated through molecules chemical structure and potentially result in long term stability under ambient conditions that can be advantageous for use in organic electronics (e.g., OPVs, OLEDs, OFETs). Improved methods are disclosed for making monomers comprising a benzo[2,1-b:3,4-b′]dithiophene moiety that are useful as electronics materials.
摘要翻译：包含均聚物或包含双噻吩单元的共聚物的组合物，其用于例如用于有机光伏活性层中的低带隙材料。可以通过包括选择单体结构和单体组分的比例的聚合方法来设计带隙和其它性质。此外，适于制备交替共聚物的二聚体还包含一个第一单体部分，其包含至少一个共价连接到包含不同双噻吩部分的一个第二单体部分或至少一个不是二噻吩的部分的双噻吩部分化合物。该组合物可以共聚以形成可进一步加工以形成印刷有机电子器件中使用的聚合物膜的交替共聚物。一系列新型共聚物被设计成允许制造具有定制的电子和/或机械性质的材料，其可以通过分子化学结构容易地操作，并且潜在地在环境条件下导致长期稳定性，这对于用于有机电子（例如，OPV，OLED，OFET）。公开了用于制备包含可用作电子材料的苯并[2,1-b：3,4-b']二噻吩部分的单体的改进方法。

6. 发明申请

US20110204341A1 ORGANIC ELECTRONIC DEVICES AND POLYMERS, INCLUDING PHOTOVOLTAIC CELLS AND DIKETONE-BASED POLYMERS 有权
标题翻译：有机电子器件和聚合物，包括光伏电池和基于酮酮的聚合物
公开(公告)号：US20110204341A1
公开(公告)日：2011-08-25
申请号：US12874163
申请日：2010-09-01
申请人： Christopher T. Brown , Christophe René Gaston Grenier , Chad Landis , Elena E. Sheina
发明人： Christopher T. Brown , Christophe René Gaston Grenier , Chad Landis , Elena E. Sheina
IPC分类号： H01L51/46 , C08F228/06 , C08L41/00
CPC分类号： C08L65/00 , C07D487/04 , C07D495/04 , C07D519/00 , C07F7/0816 , C08G61/12 , C08G61/126 , C08G2261/124 , C08G2261/18 , C08G2261/226 , C08G2261/228 , C08G2261/3223 , C08G2261/334 , C08G2261/344 , C08G2261/364 , C08G2261/414 , C09B57/004 , C09B69/008 , C09B69/109 , C09D165/00 , H01L51/0036 , H01L51/0043 , H01L51/0069 , H01L51/0077 , H01L51/4253 , Y02E10/549 , Y10S428/917
摘要： Polymers which can be used in p-type materials for organic electronic devices and photovoltaic cells. Compounds, monomers, dimers, trimers, and polymers comprising: Good photovoltaic efficiency and lifetime can be achieved. The R group can provide solubility, environmental stability, and fine tuning of spectroscopic and/or electronic properties. Different polymer microstructures can be prepared which encourage multiple band gaps and broad and strong absorptions. The carbonyl can interact with adjacent thiophene rings to provide backbone with rigidity, induce planarity, and reduce and/or eliminate intramolecular chain twisting defects. Polymers comprising benzodithiophene and/or benzothiadiazole structures can show particularly high performance.
摘要翻译：可用于有机电子器件和光伏电池的p型材料的聚合物。化合物，单体，二聚体，三聚体和聚合物包括：可以实现良好的光电效率和寿命。 R基团可以提供光谱和/或电子性质的溶解度，环境稳定性和微调。可以制备不同的聚合物微结构，其可以鼓励多个带隙和宽而强的吸收。羰基可以与相邻的噻吩环相互作用以提供具有刚性，诱导平面性的主链，并减少和/或消除分子内链扭曲缺陷。包含苯并二噻吩和/或苯并噻二唑结构的聚合物可表现出特别高的性能。

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