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61. 发明授权

US5019637A Organopolysiloxane urea derivatives and organopolysiloxane thiourea derivatives, methods of their preparation and use 失效
标题翻译：有机聚硅氧烷脲衍生物和有机聚硅氧烷硫脲衍生物，其制备方法及用途
公开(公告)号：US5019637A
公开(公告)日：1991-05-28
申请号：US431219
申请日：1989-11-03
申请人： Peter Panster , Ulrich Deschler
发明人： Peter Panster , Ulrich Deschler
IPC分类号： B01J20/26 , B01J20/22 , C08G77/42 , C08G77/44 , C08G77/48 , C08G77/54 , C08G77/58
CPC分类号： B01J20/22 , C08G77/54 , C08G77/58
摘要： The invention is relative to optionally cross-linked organopolysiloxane urea derivatives and thiourea derivatives consisting of: ##STR1## wherein X stands for 0 or S andR.sup.1 is a group of the formula: ##STR2## in which R.sup.5 is alkylene with 1 to 10 C atoms or cycloalkylene with 5 to 8 C atoms or a group of the formula: ##STR3## with n=1-6 (on the nitrogen)m=0-6 (on the silicon), wherein R.sup.2 has the same meaning as R.sup.1 or stands for H, R.sup.3 and R.sup.4 have the same meaning as R.sup.1 or stands for H or alkyl with 1 to 5 C atoms. At least two but at the most three groups according to formula (2) are bound to the units according to formula (1). The free valances of the oxygen atoms bound to the silicon atom are saturated by silicon atoms of further groups of formula (2) with the optional inclusion of cross-linking agents. In addition, preparative methods for the products and a use for the removal of dissolved metals from liquid phases are indicated.
摘要翻译：本发明相对于任选的交联的有机聚硅氧烷脲衍生物和硫脲衍生物，其由以下组成：其中X代表0或S，R1是下式的基团：其中R5是具有1至10个C原子的亚烷基或具有5至8个碳原子的亚环烷基或具有n = 1-6（在氮上）m = 0-6（在硅上的下式的基团：），其中R2具有与R 1相同的含义或代表H，R 3和R 4具有与R 1相同的含义或代表H或具有1至5个C原子的烷基。根据式（2），至少两个但最多三个基团与根据式（1）的单元结合。与硅原子结合的氧原子的自由价数由另外的式（2）基团的硅原子饱和，任选地包含交联剂。此外，还指出了产品的制备方法和用于从液相中除去溶解的金属的用途。

62. 发明授权

US5003024A Organosiloxane amine copolycondensates, method of their preparation and use (I) 失效
标题翻译：有机硅氧烷胺共缩聚物，其制备方法和用途（I）
公开(公告)号：US5003024A
公开(公告)日：1991-03-26
申请号：US431218
申请日：1989-11-03
申请人： Peter Panster , Robert Gradl , Peter Kleinschmit
发明人： Peter Panster , Robert Gradl , Peter Kleinschmit
IPC分类号： B01J20/26 , B01J20/22 , C08G77/26 , C08G77/42 , C08G77/44 , C08G77/48 , C08G77/50 , C08G77/54 , C08G77/58
CPC分类号： B01J20/22 , C08G77/26 , C08G77/54 , C08G77/58
摘要： Organosiloxane amine copolycondensates as statistic or block copolycondensates or mixtures thereof consisting of the units ##STR1## in which R.sup.1 to R.sup.5 is ##STR2## and R.sup.6 is bound directly to the nitrogen atom or the double-bonding X group and is alkylene, cycloalkylene or ##STR3## in which n is 1 to 6 and m 0 to 6. The free valences of the oxygen atoms bound to the silicon atom are saturated by silicon atoms of further groups of formula III, optionally with the inclusion of cross-linking agents, X stands for ##STR4## in which R" is H or alkyl. In addition, preparation methods and the use of the products for the removal of dissolved metals from liquid phase or for the adsorption of gaseous compounds.
摘要翻译：有机硅氧烷胺共缩聚物作为统计或嵌段共缩合物或其混合物，其由其中R 1至R 5为（III）且R 6直接键合到氮原子上的单元（I）和（VI）双键X基并且是亚烷基，亚环烷基或者其中n为1至6且m 0至6的亚环烷基或亚环烷基或者其中n为0至6的键。硅原子结合的氧原子的游离价数被硅原子饱和的另外的式III基团，任选地含有交联剂，X代表其中R“是H或烷基的 + TR 。另外，制备方法和产品用于从液相中除去溶解的金属或用于气态化合物的吸附。

63. 发明授权

US4954599A Formed, polymeric, tertiary or secondary organosiloxane amine compounds, methods of their preparation and use 失效
标题翻译：形成的聚合物，三级或次级有机硅氧烷胺化合物，其制备和使用方法
公开(公告)号：US4954599A
公开(公告)日：1990-09-04
申请号：US295886
申请日：1989-01-11
申请人： Peter Panster , Peter Kleinschmit
发明人： Peter Panster , Peter Kleinschmit
IPC分类号： B01D53/02 , B01J20/00 , B01J20/26 , B01J31/08 , B01J31/12 , C08G77/48 , C08G77/50 , C08G77/54 , C08G77/56 , C08G77/58 , C08J3/12 , C08J7/00 , C08L83/14
CPC分类号： C08G77/58 , B01J20/26 , B01J31/124 , C08G77/54
摘要： Spherical, polymeric, tertiary or secondary organosiloxane amine compounds comprising: ##STR1## units in which R.sup.1 and R.sup.2 stand for a group: ##STR2## R.sup.4 is an alkylene grouping and the oxygen atoms are saturated by silicon atoms of other groups (II), with the optional inclusion of cross-linking agents, R.sup.3 is equal to R.sup.1 and R.sup.2 or stands for hydrogen, an alkyl, cycloalkyl or the benzyl group. Also disclosed is a method for the preparation of the compounds in spherical form and the use of these products for removing acids from liquids and gases as well as for the adsorption of gaseous organic compounds.
摘要翻译：包括：其中R 1和R 2表示一个基团的单元：（II）R 4是亚烷基，氧原子被硅原子饱和，其它基团（II），任选地含有交联剂，R 3等于R 1和R 2，或代表氢，烷基，环烷基或苄基。还公开了制备球形化合物的方法以及这些产物用于从液体和气体中除去酸以及吸附气态有机化合物的用途。

64. 发明授权

US4758277A Additive for friction coating mixtures 失效
标题翻译：摩擦涂料混合物用添加剂
公开(公告)号：US4758277A
公开(公告)日：1988-07-19
申请号：US938349
申请日：1986-12-04
申请人： Friedrich Spruegel , Peter Panster
发明人： Friedrich Spruegel , Peter Panster
IPC分类号： C09K3/14 , C08J5/14 , C08K3/00 , C08K3/28 , C08K3/30 , F16D69/02
CPC分类号： F16D69/02 , B29L2031/16
摘要： A friction and abrasion controlling additive for friction coating mixtures, especially for the formation of brake pad materials is provided which utilizes TiS.sub.2 as the additive.
摘要翻译：提供了用于摩擦涂层混合物的摩擦和磨损控制添加剂，特别是用于形成制动衬块材料，其利用TiS 2作为添加剂。

65. 发明授权

US4647679A Platinum and/or palladium containing organopolysiloxane-ammonium compounds, method for their preparation and uses 失效
标题翻译：铂和/或钯的有机聚硅氧烷 - 铵化合物，其制备方法和用途
公开(公告)号：US4647679A
公开(公告)日：1987-03-03
申请号：US699968
申请日：1985-02-08
申请人： Peter Panster , Marlies Englisch , Peter Kleinschmit
发明人： Peter Panster , Marlies Englisch , Peter Kleinschmit
IPC分类号： C08G77/00 , B01J23/42 , B01J23/44 , B01J31/02 , B01J31/12 , B01J31/16 , B01J31/30 , C07F7/14 , C08G77/08 , C08G77/26 , C08G77/28 , C08G77/32 , C08G77/38 , C08G77/388 , C08G77/54 , C08G77/58 , C07F15/00
CPC分类号： C08G77/58 , B01J31/0239 , B01J31/124 , B01J31/30 , C07F7/14 , C08G77/54 , B01J2231/323 , Y02P20/582
摘要： Platinum and/or palladium containing organopolysiloxane-ammonium compounds containing units represented by the structural formula: ##STR1## in which R.sup.1, R.sup.2 and R.sup.3 represent:R.sup.5 --SiO.sub.3/2 (2)wherein R.sup.5 is an alkylene group and the free valences of oxygen are satisfied by silicon atom and additional groups of the structural formula (2), optionally with the introduction of a crosslinking agent,R.sup.4 can be R.sup.1, R.sup.2, R.sup.3 or hydrogen, alkyl, cycloalkyl or benzyl,Y.sup.x- is MeX.sub.4.sup.2- or MeX.sub.6.sup.2-, wherein Me is platinum or palladium andX is chlorine or bromine, and can further denote a 1 to 3 valent anion of a protonic acid capable of forming a stable salt with an amine, or the hydroxy group, andx is a number from 1 to 3. Methods for the obtaining the polymeric organosiloxane-ammonium-noble metal complexes and as well as the use thereof as catalysts for hydrosilylation and hydrogenation reactions are disclosed.
摘要翻译：含有以下结构式表示的单元的铂和/或钯的有机聚硅氧烷 - 铵化合物：其中R1，R2和R3表示：R5-SiO3 / 2（2），其中R5是亚烷基，通过硅原子和结构式（2）的另外的基团，任选地引入交联剂，R4可以是R1，R2，R3或氢，烷基，环烷基或苄基，Yx-是MeX42- 或MeX62-，其中Me是铂或钯，X是氯或溴，并且还可以表示能够与胺或羟基形成稳定盐的质子酸的1至3价阴离子，x是公开了获得聚合物有机硅氧烷 - 铵 - 贵金属络合物的方法及其作为氢化硅烷化和氢化反应的催化剂的用途。

66. 发明授权

US4578496A Polymeric metal-amine complex compounds, processes for their preparation and use 失效
标题翻译：聚合金属 - 胺络合物，其制备和使用方法
公开(公告)号：US4578496A
公开(公告)日：1986-03-25
申请号：US543720
申请日：1983-10-20
申请人： Peter Panster , Peter Kleinschmit
发明人： Peter Panster , Peter Kleinschmit
IPC分类号： C07F7/02 , B01J27/00 , B01J31/16 , B01J31/18 , B01J31/22 , C07B61/00 , C07C29/44 , C07C45/50 , C07C47/02 , C07F1/10 , C07F1/12 , C07F7/12 , C07F7/14 , C07F11/00 , C07F13/00 , C07F15/00 , C07F15/02 , C07F15/04 , C07F15/06 , C08G77/398 , C08G77/58 , C07F7/08 , C07C5/02 , C07C45/00 , C07C69/02
CPC分类号： C08G77/58 , B01J31/1675 , B01J31/1805 , C07C29/16 , C07C45/50 , C07C67/303 , C07F7/14 , C08G77/398 , B01J2231/20 , B01J2231/321 , B01J2231/323 , B01J2231/52 , B01J2231/543 , B01J2231/645 , B01J2531/64 , B01J2531/66 , B01J2531/72 , B01J2531/74
摘要： Polymeric complex compounds of molybdenum, tungsten, manganese, rhenium and of the metals of the sub-groups VIII and I of the Periodic Table of Elements, which complex compounds have a silica-type structure are disclosed. At least one amine ##STR1## is bonded coordinately to the central metal atom. The atomic ratio of metal to nitrogen is from 1:1 to 1:10.sup.6. The required charge compensation is effected by means of an anion. In (1), R.sup.1 and R.sup.2 represent a group ##STR2## and R.sup.4 is an alkylene grouping. The oxygen atoms are saturated by silicon atoms of further groups (2), if appropriate with incorporation of crosslinking agents. R.sup.3 may have the meaning of R.sup.1 and R.sup.2, or represents hydrogen, an alkyl group, a cycloalkyl group or the benzyl group. The polymers can contain several metals. The invention also relates to processes for their preparation, and uses in catalysis.
摘要翻译：公开了复合化合物具有二氧化硅型结构的钼，钨，锰，铼和元素周期表第VIII族和第Ⅰ族的金属的高分子复合化合物。至少一个胺（1）与中心金属原子配位结合。金属与氮的原子比为1:1至1:106。所需的电荷补偿通过阴离子进行。在（1）中，R1和R2表示基团（2），R4是亚烷基。氧原子被其他基团（2）的硅原子饱和，如果合适的话，加入交联剂。 R3可以具有R 1和R 2的含义，或表示氢，烷基，环烷基或苄基。聚合物可以含有几种金属。本发明还涉及其制备方法和催化剂中的用途。

67. 发明授权

US4442040A Polymeric rhodium, iridium and ruthenium phosphine complex compounds, processes for their production and use 失效
标题翻译：聚合铑，铱和钌膦络合物，其生产和使用的方法
公开(公告)号：US4442040A
公开(公告)日：1984-04-10
申请号：US283868
申请日：1981-07-16
申请人： Peter Panster , Peter Kleinschmit
发明人： Peter Panster , Peter Kleinschmit
IPC分类号： C08G77/42 , B01J31/16 , B01J31/24 , B01J31/28 , C07F15/00 , C08G79/00
CPC分类号： C07F15/0013 , B01J31/1675 , B01J31/24 , B01J31/2404 , B01J2231/20 , B01J2231/321 , B01J2231/323 , B01J2231/52 , B01J2231/645 , B01J2531/821 , B01J2531/822 , B01J2531/827
摘要： The invention relates to complex compounds of rhodium, iridium or ruthenium with a silicic acid-like structure with a least one phosphine ligand, the trivalent phosphorus of which is bonded to silicon via at least one divalent organic residue, the remaining three valences of the silicon building, via oxygen bridges arising from the hydrolysis of functional substituents originally bound there, a inter- or intra-molecularly crosslinked polycondensate. The required charge equalization is effected by an anion. Also disclosed are processes for recovery of the polymeric complexes and their use in heterogeneous catalysis of various chemical reactions.
摘要翻译：本发明涉及具有硅酸结构的铑，铱或钌与具有至少一个膦配体的络合物，其三价磷通过至少一个二价有机残基与硅键合，剩余的三价硅通过由原来结合在其上的官能性取代基的水解产生的氧桥构建分子间或分子内交联的缩聚物。所需的电荷均衡由阴离子实现。还公开了回收聚合物络合物的方法及其在各种化学反应的多相催化中的用途。

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