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51. 发明授权

US09359334B2 Ligands for sensitizing dyes of dye-sensitized solar cells 有权
标题翻译：染料敏化太阳能电池敏化染料的配体
公开(公告)号：US09359334B2
公开(公告)日：2016-06-07
申请号：US13499012
申请日：2010-09-29
申请人： Mohammad Khaja Nazeeruddin , Michael Graetzel , Alessandro Abbotto , Chiara Marinzi , Norberto Manfredi , Filippo De Angelis
发明人： Mohammad Khaja Nazeeruddin , Michael Graetzel , Alessandro Abbotto , Chiara Marinzi , Norberto Manfredi , Filippo De Angelis
IPC分类号： C07D401/00 , C07D405/00 , C07D409/00 , C07D411/00 , C07D413/00 , C07D417/00 , C07D419/00 , C07D421/00 , C07D409/04 , C07D405/04 , C07D495/04 , C07D495/14 , H01L51/00 , H01G9/20
CPC分类号： C07D409/04 , C07D405/04 , C07D495/04 , C07D495/14 , H01G9/2031 , H01G9/2059 , H01L51/0086 , Y02E10/542 , Y02E10/549
摘要： The present invention provides new bi- and polypyridine ligands of ruthenium dyes. The invention also provides solar cells, in particular dye-sensitized solar cells comprising the dyes. Formula(I):
摘要翻译：本发明提供钌染料的新的双和多吡啶配体。本发明还提供太阳能电池，特别是包含染料的染料敏化太阳能电池。式（I）：

52. 发明授权

US08980440B2 Light-emitting material 有权
标题翻译：发光材料
公开(公告)号：US08980440B2
公开(公告)日：2015-03-17
申请号：US12295933
申请日：2007-04-03
申请人： Mohammad Khaja Nazeeruddin , Cedric Klein , Michael Graetzel
发明人： Mohammad Khaja Nazeeruddin , Cedric Klein , Michael Graetzel
IPC分类号： H01L51/50 , C07F15/00
CPC分类号： C07F15/0046 , Y10S428/917 , Y10T428/265 , Y10T428/31504
摘要： This invention pertains to light emitting materials comprising novel ortho-metalated transition metal complexes [C^N]2M(T)(L), comprising chelate dialkylamino-substituted C^N ligands, monodentate neutral ligand (L) having sp2 hybridized N atom and a monodentate anionic ligand (T) chosen among CN−, CNO−, CNS−. It has been surprisingly found that when the metal has bound thereto in addition to substituted orthometalated ligands, both an anion chosen among cyanide, thiocyanate, cyanate, possessing strong C donor and π acceptor properties, and a monodentate neutral ligand L, as above defined, said ligands advantageously participate in the emission process, significantly shifting emission towards higher energies (blue-shift) and enabling appreciable improvement of the emission efficiency of complexes [C^N]2M(T)(L).Still objects of the invention are the use of said light emitting materials and organic light emitting device comprising said light emitting material.
摘要翻译：本发明涉及包含新型邻位金属过渡金属络合物[C 1 N] 2M（T）（L））的发光材料，其包含螯合二烷基氨基取代的C 1 N配体，具有sp2杂化的N原子的单齿中性配体（L）和选自CN-，CNO-，CNS-的单齿阴离子配位体（T）。已经令人惊奇地发现，当金属除了取代的正极金属化配体之外还结合有金属时，选自氰化物，硫氰酸盐，氰酸盐，具有强C供体和阴离子的阴离子; 受体特性和如上所定义的单齿中性配体L，所述配体有利地参与发射过程，将发射显着地偏移到更高的能量（蓝移）并且使复合物的发射效率明显提高[C ^ N] 2M （T）（L）。本发明的另一个目的是使用所述发光材料和包括所述发光材料的有机发光器件。

53. 发明申请

US20140005397A1 METAL COMPLEX COMPRISING A LIGAND HAVING A COMBINATION OF DONOR-ACCEPTOR SUBSTITUENTS 有权
标题翻译：包含配对接收器替代物的组合的金属复合物
公开(公告)号：US20140005397A1
公开(公告)日：2014-01-02
申请号：US13988267
申请日：2011-11-21
申请人： Michael Graetzel , Etienne David Baranoff , Mohammad Khaja Nazeeruddin
发明人： Michael Graetzel , Etienne David Baranoff , Mohammad Khaja Nazeeruddin
IPC分类号： H01L51/00
CPC分类号： H01L51/0085 , C07F15/0033 , H01L51/009
摘要： Disclosed is a metal complex having a partial structure represented by the following Formula (I-0) or a tautomer thereof: formula (I-0) Cy is a 5 to 7 membered heterocyclic ring, preferably a 6-membered ring, which may be aromatic, non aromatic or partially aromatic and which coordinates to the metal atom through a carbon atom; A is a nitrogen atom a is an integer equal or superior to 1; D is an electron donor group; and b is an integer equal or superior to 1.
摘要翻译：公开了具有由下式（I-0）表示的部分结构或其互变异构体的金属络合物：式（I-0）Cy是5至7元杂环，优选6元环，其可以是芳族，非芳族或部分芳族，并通过碳原子与金属原子配位; A是氮原子，a是等于或高于1的整数; D是电子给体基团; b是等于或高于1的整数。

54. 发明申请

US20130330632A1 METAL COMPLEXES FOR USE AS DOPANTS AND OTHER USES 有权
标题翻译：金属复合材料用作多晶硅和其他用途
公开(公告)号：US20130330632A1
公开(公告)日：2013-12-12
申请号：US14001307
申请日：2012-02-24
申请人： Julian Burschka , Florian Kessler , Etienne Baranoff , Mohammad Khaja Nazeeruddin , Michael Graetzel
发明人： Julian Burschka , Florian Kessler , Etienne Baranoff , Mohammad Khaja Nazeeruddin , Michael Graetzel
IPC分类号： H01L51/00 , H01L51/42 , H01M10/42 , H01L51/50
CPC分类号： H01L51/42 , C09K9/02 , C09K11/06 , C09K2211/1029 , C09K2211/1044 , C09K2211/187 , H01G9/2018 , H01G9/2031 , H01G9/2059 , H01G9/2095 , H01L51/002 , H01L51/0083 , H01L51/4226 , H01L51/50 , H01L51/5032 , H01L51/5056 , H01L51/5072 , H01M4/60 , H01M4/624 , H01M6/14 , H01M10/05 , H01M10/4235 , Y02E10/549
摘要： The invention relates to electrochemical devices comprising complexes of cobalt comprising at least one ligand with a 5- or six membered, N-containing heteroring. The complex are useful as p- and n-dopants, as over of electrochemical devices, in particular in organic semiconductors. The complexes are further useful as over-discharge prevention and overvoltage protection agents.
摘要翻译：本发明涉及包含钴的复合物的电化学装置，其包含至少一种具有5-或六元N型杂环的配位体。该复合物可用作p-和n-掺杂剂，如电化学装置，特别是在有机半导体中。该配合物可用作过放电防止和过电压保护剂。

55. 发明授权

US08518557B2 Light emitting materials comprising novel ortho-metalated transition metal complexes 失效
标题翻译：发光材料包含新的正金属化的过渡金属络合物
公开(公告)号：US08518557B2
公开(公告)日：2013-08-27
申请号：US12444793
申请日：2007-10-11
申请人： Mohammad Khaja Nazeeruddin , Cedric Klein , Michael Graetzel
发明人： Mohammad Khaja Nazeeruddin , Cedric Klein , Michael Graetzel
IPC分类号： H01L51/54 , C09K11/06
CPC分类号： C09K11/06 , C09K2211/1029 , C09K2211/185 , C09K2211/186 , H01L51/0085 , H01L51/5016 , H05B33/14
摘要： This invention pertains to light emitting materials comprising novel ortho-metalated transition metal complexes [C^N]2ML comprising two orthometalated ligands having imidazole moieties and an ancillary ligand of β-diketonate type. The ortho-metalated transition metal complexes are represented by formula (I): It has been surprisingly found that when the metal has bound thereto both orthometalated ligands comprising imidazole moieties and an ancillary ligand of β-diketonate type, the ligands advantageously participate in the emission process, significantly broadening emission in the visible region and enabling appreciable improvement of the white emission efficiency of complexes [C^N]2ML. Additional objects of the invention are the use of the light emitting materials and organic light emitting device comprising the light emitting material.
摘要翻译：本发明涉及包含新型邻位金属过渡金属络合物[C 2 N] 2ML的发光材料，其包含两个具有咪唑部分的原位金属配体和β-二酮类型的辅助配体。正金属化的过渡金属络合物由式（I）表示：已经令人惊讶地发现，当金属与其结合的是包含咪唑部分的正金属化配体和β-二酮类型的辅助配体时，配体有利地参与发射过程中显着扩大了可见光区域的发射，并使复合物[C ^ N] 2ML的白光发射效率明显提高。本发明的另外的目的是使用包含发光材料的发光材料和有机发光器件。

56. 发明申请

US20110215276A1 Phosphorescent light-emitting material 审中-公开
标题翻译：磷光发光材料
公开(公告)号：US20110215276A1
公开(公告)日：2011-09-08
申请号：US13128391
申请日：2009-11-10
申请人： Mohammad Khaja Nazeeruddin , Etienne David Baranoff , Michael Graetzel
发明人： Mohammad Khaja Nazeeruddin , Etienne David Baranoff , Michael Graetzel
IPC分类号： C09K11/06 , C07F15/00
CPC分类号： C07F15/0033 , C09K11/06 , C09K2211/1007 , C09K2211/1029 , C09K2211/185 , H01L51/0085 , H01L51/5016
摘要： The present invention relates to light emitting materials including a novel Ir complex, where the Ir is provided with a primary ligand selected from phenyl pyridine ligands substituted with at least one Cl atom. Such light emitting materials have been found to have a significantly enhanced photoluminescence quantum yield over other Ir complexes with a phenyl pyridine ligand having no Cl atom, or even over those with a phenyl pyridine ligand having a halogen atom other than Cl, such as a Br or F atom, and as a result specifically improve the efficiency of a light emitting device. The present invention further relates to the use of such light emitting materials and an organic light emitting device including such light emitting materials.
摘要翻译：本发明涉及包括新型Ir配合物的发光材料，其中Ir具有选自被至少一个Cl原子取代的苯基吡啶配体的主配体。已经发现这种发光材料与具有不具有Cl原子的苯基吡啶配体相比，甚至比具有不是Cl的卤素原子的苯基吡啶配体的那些具有比其它Ir配合物具有显着提高的光致发光量子产率，例如Br 或F原子，并且因此具体地提高了发光器件的效率。本发明还涉及使用这种发光材料和包括这种发光材料的有机发光器件。

57. 发明申请

US20110062541A1 HIGH MOLECULAR EXTINCTION COEFFICIENT METAL DYES 有权
标题翻译：高分子量放射性系数金属染料
公开(公告)号：US20110062541A1
公开(公告)日：2011-03-17
申请号：US12735942
申请日：2009-02-27
申请人： Feifei Gao , Yuan Wang , Jing Zhang , Peng Wang , shaik Mohammad Zakeeruddin , Michael Graetzel
发明人： Feifei Gao , Yuan Wang , Jing Zhang , Peng Wang , shaik Mohammad Zakeeruddin , Michael Graetzel
IPC分类号： H01L31/02 , C07F15/00
CPC分类号： H01L51/0086 , C07F15/0053 , C09B57/10 , H01G9/2013 , H01G9/2031 , H01G9/2059 , Y02E10/542 , Y02E10/549
摘要： The present invention relates to novel compounds that are useful as ligands in organometallic dyes. More particularly, the invention relates to dyes comprising the compounds, said dyes being sensitizing dyes useful in solar cell technology. According to an embodiment, the present invention discloses new ruthenium dyes and their application in dye-sensitized solar cells (DSC). The referred ruthenium dyes with new structural features can be easily synthesized, show more than 85% light-to-electricity conversion efficiency and a higher than 9% cell efficiency.
摘要翻译：本发明涉及可用作有机金属染料中配体的新化合物。更具体地说，本发明涉及包含该化合物的染料，所述染料是用于太阳能电池技术的敏化染料。根据一个实施方案，本发明公开了新的钌染料及其在染料敏化太阳能电池（DSC）中的应用。具有新结构特征的引用钌染料可以容易地合成，显示出超过85％的光电转换效率和高于9％的电池效率。

58. 发明申请

US20100051908A1 Liquid Charge Transporting Material 有权
标题翻译：液体电荷输送材料
公开(公告)号：US20100051908A1
公开(公告)日：2010-03-04
申请号：US12225322
申请日：2007-03-21
申请人： Henry J. Snaith , Shaik Mohammad Zakeeruddin , Michael Graetzel
发明人： Henry J. Snaith , Shaik Mohammad Zakeeruddin , Michael Graetzel
IPC分类号： H01L51/44 , H01B1/12 , C07D265/34 , H01L51/48
CPC分类号： H01L51/0067 , H01L51/002 , H01L51/0059 , H01L51/0076 , H01L51/4226 , Y02E10/549 , Y02P70/521
摘要： The present invention relates to optoelectronic and/or electrochemical devices comprising an organic charge transporting material which is liquid at a temperature of ≦180° C. In particular in dye-sensitised solar cells, quantum efficiency higher than with prior art solid organic hole-transporters is reported. The melting point of a large quantity of organic charge transporting materials may be adjusted to a desired value by selecting suitable substituents. Accordingly, general advantages of the liquid state may be associated with the properties of organic charge transporting materials.
摘要翻译：本发明涉及包含有机电荷输送材料的光电子和/或电化学装置，该有机电荷输送材料在温度为180℃时是液态的。特别是在染料敏化太阳能电池中，量子效率高于现有技术固体有机空穴 - 报道了运输商。可以通过选择合适的取代基将大量有机电荷输送材料的熔点调节到所希望的值。因此，液体状态的一般优点可能与有机电荷输送材料的性质有关。

59. 发明授权

US07420117B2 Photovoltaic cell 有权
标题翻译：光伏电池
公开(公告)号：US07420117B2
公开(公告)日：2008-09-02
申请号：US10417659
申请日：2003-04-17
申请人： Tsuguo Koyanagi , Michael Graetzel
发明人： Tsuguo Koyanagi , Michael Graetzel
IPC分类号： H01L31/00
CPC分类号： H01L51/4226 , H01G9/2031 , H01G9/2036 , H01L51/0086 , Y02E10/542 , Y02E10/549
摘要： A photovoltaic cell includes a substrate having an electrode layer on the surface and having a porous metal oxide semiconductor film which is formed on the electrode layer and on which a photosensitizer is adsorbed, a substrate having an electrode layer on the surface, both of said substrates being arranged in such a manner that the electrode layer and the electrode layer face each other, and an electrolyte layer provided between the semiconductor film and the electrode layer, wherein the semiconductor film contains an inhibitor of back current, and at least one pair of substrate and electrode layer thereon have transparency. The photovoltaic cell is capable of inhibiting back current and decomposition of a spectrosensitizing dye caused by the ultraviolet rays, has high photoelectric conversion efficiency and is capable of generating high electromotive force.
摘要翻译：光伏电池包括在表面上具有电极层的基板，并且具有多孔金属氧化物半导体膜，该多孔金属氧化物半导体膜形成在电极层上，并且其上吸附有光敏剂，具有表面上的电极层的基板，两个基板以使得电极层和电极层彼此面对的方式布置，以及设置在半导体膜和电极层之间的电解质层，其中半导体膜包含反向电流抑制剂，以及至少一对基板其上的电极层具有透明性。光电池能够抑制由紫外线引起的光敏染料的回流和分解，具有高的光电转换效率并且能够产生高电动势。

60. 发明授权

US06936143B1 Tandem cell for water cleavage by visible light 失效
标题翻译：用可见光水分解的串联电池
公开(公告)号：US06936143B1
公开(公告)日：2005-08-30
申请号：US10030036
申请日：2000-04-07
申请人： Michael Graetzel , Jan Augustynski
发明人： Michael Graetzel , Jan Augustynski
IPC分类号： H01L31/04 , C25B1/00 , H01M14/00 , C25B9/00 , C25B11/00
CPC分类号： C25B1/003 , Y02E10/542 , Y02E60/368 , Y02P20/135 , Y02P70/521
摘要： A tandem cell or photoelectrochemical system for the cleavage of water to hydrogen and oxygen by visible light has two superimposed photocells, both cells being connected electrically. The photoactive material in the top cell is a semiconducting oxide placed in contact with an aqueous solution. This semiconducting oxide absorbs the blue and green part of the solar emission spectrum of a light source or light sources and generates with the energy collected oxygen and protons from water. The not absorbed yellow and red light transmits the top cell and enters a second photocell, the bottom cell, which is mounted, in the direction of the light behind, preferably directly behind the top cell. The bottom cell includes a dye-sensitized mesoporous photovoltaic film. The bottom cell converts the yellow, red and near infrared portion of the sunlight to drive the reduction of the protons, which are produced in the top cell during the photo catalytic water oxidation process, to hydrogen.
摘要翻译：用于通过可见光将水切割成氢和氧的串联电池或光电化学系统具有两个叠加的光电池，两个电池均电连接。顶部电池中的光活性材料是与水溶液接触放置的半导体氧化物。该半导体氧化物吸收光源或光源的太阳辐射光谱的蓝色和绿色部分，并产生能量从水中收集的氧和质子。未被吸收的黄色和红色光透射顶部单元并且进入安装在后面的光的方向上的第二光电池，优选地直接位于顶部单元的后面。底部电池包括染料敏化介孔光伏膜。底部电池转换太阳光的黄色，红色和近红外部分以驱动在光催化水氧化过程中在顶部电池中产生的质子的还原为氢。

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