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11. 发明授权

US4742092A Organopolysiloxane composition 失效
标题翻译：有机聚硅氧烷组合物
公开(公告)号：US4742092A
公开(公告)日：1988-05-03
申请号：US918775
申请日：1986-10-14
申请人： Yoshio Inoue , Masatoshi Arai
发明人： Yoshio Inoue , Masatoshi Arai
IPC分类号： C08L83/06 , C08F2/46 , C08K5/5425 , C08K5/548 , C08L83/04 , C09J183/00 , C09K3/10
CPC分类号： C08K5/5425 , C08L83/04 , C08G77/16 , C08G77/28 , Y10S528/901
摘要： The curable organopolysiloxane composition of the invention is formulated with two kinds of crosslinking agents including an organosilane compound having 2 or 3 isopropenyloxy groups in a molecule and an organopolysiloxane having at least 2 mercapto groups in a molecule added to the base ingredient of a hydroxy-terminated diorganopolysiloxane together with a curing catalyst and a photosensitizer. The composition has two-way curability by the condensation reaction in the presence of atmospheric moisture between the silanolic hydroxy groups and the isopropenyloxy groups and by the ultraviolet-induced addition reaction between the isopropenyloxy groups and the mercapto groups to exhibit very reliable curing behavior giving a cured rubbery elastomer having excellent properties.
摘要翻译：本发明的可固化的有机基聚硅氧烷组合物用两种交联剂配制，所述交联剂包括在分子中具有2或3个异丙烯氧基的有机硅烷化合物和在分子中具有至少2个巯基的有机聚硅氧烷加入至羟基封端的基础成分二有机聚硅氧烷以及固化催化剂和光敏剂。该组合物在硅烷醇羟基和异丙烯氧基之间的大气湿度存在下通过缩合反应和异丙烯氧基与巯基之间的紫外线诱导的加成反应具有双向固化性，表现出非常可靠的固化行为，得到固化橡胶弹性体具有优异的性能。

12. 发明授权

US4735971A Room temperature-curable organopolysiloxane composition 失效
标题翻译：室温可固化的有机聚硅氧烷组合物
公开(公告)号：US4735971A
公开(公告)日：1988-04-05
申请号：US12021
申请日：1987-02-09
申请人： Yoshio Inoue , Masatoshi Arai , Shinichi Sato
发明人： Yoshio Inoue , Masatoshi Arai , Shinichi Sato
IPC分类号： C08L83/06 , C08L83/04 , C08L83/14 , C09J183/00 , C09K3/10 , C08L1/00
CPC分类号： C08L83/14
摘要： The inventive organopolysiloxane composition is curable in two ways, firstly, by the irradiation with ultraviolet light and, secondly, by exposure to a moisture-containing atmospheric air. The principal ingredient of the composition is a diorganopolysiloxane having, in a molecule, at least one isopropenyloxysilyl-substituted ethyl or propyl group bonded to the silicon atom of the polysiloxane chain, which is compounded with a mercaptoalkyl-containing organopolysiloxane, a photosensitizer and, optionally, a curing catalyst for the dealcoholation condensation reaction of the silicon-bonded alkoxy groups under the influence of atmospheric moisture. The composition is advantageous in the improved workability by virtue of the adequate tack-free time or the time taken for surface filming.
摘要翻译：本发明的有机聚硅氧烷组合物可以以两种方式固化，首先是通过用紫外线照射，其次，通过暴露于含湿气氛的空气中。组合物的主要成分是二有机聚硅氧烷，其在分子中具有至少一个与聚硅氧烷链的硅原子键合的异丙烯氧基甲硅烷基取代的乙基或丙基，其与含巯基烷基的有机聚硅氧烷，光敏剂和任选地，在大气湿度的影响下，硅键合的烷氧基的脱醇缩合反应的固化催化剂。该组合物由于适当的无粘性时间或表面成膜所需的时间在改进的可加工性方面是有利的。

13. 发明授权

US4769412A Room temperature-curable silicone rubber composition 失效
标题翻译：室温固化硅橡胶组合物
公开(公告)号：US4769412A
公开(公告)日：1988-09-06
申请号：US929999
申请日：1986-11-12
申请人： Yoshio Inoue , Masatoshi Arai , Kazuyuki Suzuki
发明人： Yoshio Inoue , Masatoshi Arai , Kazuyuki Suzuki
IPC分类号： C08L83/06 , C08K3/04 , C08K13/02 , C08L83/04 , C08K3/22
CPC分类号： C08K3/04
摘要： A room temperature-curable silicone rubber composition having improved heat-resistance is disclosed. The composition is formulated without any siliceous fillers as a reinforcing inorganic filler conventionally used in silicone compositions and, instead, comprises carbon black as a reinforcing filler. Namely, the composition comrises a major amount of a hydroxy-containing organopolysiloxane admixed with a minor amount of an organosilicon compound having at least two hydrolyzable groups per molecule, a curing catalyst, carbon black and iron oxide.
摘要翻译：公开了具有改进的耐热性的室温可固化的硅橡胶组合物。将组合物配制成没有任何硅质填料作为常规用于有机硅组合物的增强无机填料，代替地包括作为增强填料的炭黑。也就是说，该组合物含有大量含有少量含有每分子具有至少两个可水解基团的有机硅化合物，固化催化剂，炭黑和氧化铁的含羟基的有机聚硅氧烷。

14. 发明授权

US4764577A Curable polymeric composition 失效
标题翻译：可固化聚合物组合物
公开(公告)号：US4764577A
公开(公告)日：1988-08-16
申请号：US079063
申请日：1987-07-29
申请人： Yoshio Inoue , Masatoshi Arai
发明人： Yoshio Inoue , Masatoshi Arai
IPC分类号： C08L83/05 , C08K3/00 , C08K5/54 , C08K5/549 , C08L43/00 , C08L43/04 , C08L71/02 , C08L83/06 , C08L83/07 , C08L101/10 , C08G65/32
CPC分类号： C08L101/10 , C08K5/54
摘要： The curable polymeric composition comprises: (A) an organic polymer having at least two alkenyloxysilyl groups; (B) an organosilicon compound having at least two hydrosilyl groups; and (C) a catalytic amount of a platinum compound. When heated, the composition is curable by the hydrosilation reaction between the alkenyloxy groups in the component (A) and the silicon-bonded hydrogen atoms in the component (B) as promoted by the platinum compound to give a rubbery elastomer.
摘要翻译：可固化聚合物组合物包含：（A）具有至少两个烯氧基甲硅烷基的有机聚合物; （B）具有至少两个氢化甲硅烷基的有机硅化合物; 和（C）催化量的铂化合物。当加热时，通过铂化合物促进的化合物（A）中的链烯氧基与化合物（B）中的与硅键合的氢原子之间的氢硅化反应可以固化组合物，得到橡胶状弹性体。

15. 发明授权

US5180771A Room temperature curable organopolysiloxane composition 失效
公开(公告)号：US5180771A
公开(公告)日：1993-01-19
申请号：US508700
申请日：1990-04-13
申请人： Masatoshi Arai , Yoshifumi Inoue , Yoshio Inoue
发明人： Masatoshi Arai , Yoshifumi Inoue , Yoshio Inoue
IPC分类号： C08K3/00 , C08K5/5419 , C08K5/5465 , C08K5/57 , C08L83/04 , C08L83/06
CPC分类号： C08K5/5465 , C08L83/04 , C08G77/16 , C08G77/18 , Y10S528/901
摘要： A room temperature curable organopolysiloxane composition comprising a diorganopolysiloxane having a hydroxyl group or alkoxy groups, a filler, a particular alkoxysilane, an organosilicon compound having a particular guanidinyl group, and an organic tin compound, and further comprising an organosilicon compound having at least one group represented by the general formula: ##STR1## where R.sup.4 is a substituted or unsubstituted monovalent hydrocarbon group, or a substituted or unsubstituted phenyl group, R.sup.5 and R.sup.6 are each a hydrogen atom, methyl or ethyl group, and n is an integer of 0, 1 or 2. By virtue of the last component, the composition exhibits markedly good storage stability.

16. 发明授权

US5086107A Room temperature-curable organopolysiloxane composition 失效
标题翻译：室温可固化的有机聚硅氧烷组合物
公开(公告)号：US5086107A
公开(公告)日：1992-02-04
申请号：US634998
申请日：1990-12-27
申请人： Masatoshi Arai , Tsuneo Kimura , Yoshio Inoue
发明人： Masatoshi Arai , Tsuneo Kimura , Yoshio Inoue
IPC分类号： C08K3/26 , C08K5/5465 , C08K5/57 , C08L83/04 , C08L83/06 , C09K3/10 , C09K3/12
CPC分类号： C08K5/5465
摘要： A room temperature-curable organopolysiloxane composition capable of giving a highly oil-resistant cured silicone rubber is disclosed. The composition comprises, as the essential ingredients, a hydroxy-terminated diorganopolysiloxane, an iminoxysilane compound as a crosslinking agent, an organotin compound as a catalyst and, as an oil-resistance improver, a combination of zinc carbonate and zinc hydroxide in a powdery form of which the content of zinc hydroxide is, different from conventional basic zinc carbonate, 5 to 50% by weight. By virtue of this unique ingredient, the composition is also advantageous in respect of the high storage stability.
摘要翻译：公开了能够提供高耐油性固化硅橡胶的室温可固化的有机基聚硅氧烷组合物。作为必需成分的组合物含有羟基封端的二有机聚硅氧烷，作为交联剂的亚氨基硅烷化合物，作为催化剂的有机锡化合物，作为耐油改进剂，以粉末状形式的碳酸锌和氢氧化锌的组合其中氢氧化锌的含量与常规的碱式碳酸锌不同，为5至50重量％。凭借这种独特的成分，组合物在高储存稳定性方面也是有利的。

17. 发明授权

US4689363A Oil-resistant room temperature-curable silicone rubber composition 失效
标题翻译：耐油室温固化硅橡胶组合物
公开(公告)号：US4689363A
公开(公告)日：1987-08-25
申请号：US883064
申请日：1986-07-08
申请人： Yoshio Inoue , Masatoshi Arai , Shinichi Sato
发明人： Yoshio Inoue , Masatoshi Arai , Shinichi Sato
IPC分类号： C08L83/00 , C08K5/098 , C08K13/02 , C08L83/04 , C08L83/06 , C08K5/04
CPC分类号： C08K5/098
摘要： The room-temperature curable silicone rubber composition is formulated, in addition to the conventional ingredients of a hydroxy-terminated diorganopolysiloxane and an organosilicon compound having at least two hydrolyzable groups in a molecule, a substantial amount of an alkali metal salt of a weak acid having an acid dissociation constant as expressed by pK.sub.a in the range from 2.0 to 12.0 at 25.degree. C. such as acrylic, methacrylic, benzoic and acetic acids. By virtue of this unique ingredient compounded therein, the composition of the invention can give a vulcanized rubber having outstandingly high resistance against oils used in automobiles even at elevated temperatures.
摘要翻译：除了在分子中具有至少两个可水解基团的羟基封端的二有机聚硅氧烷和有机硅化合物的常规成分之外，配制室温可固化硅橡胶组合物，大量的弱酸碱金属盐具有在25℃，如丙烯酸，甲基丙烯酸，苯甲酸和乙酸，由pKa在2.0至12.0范围内表示的酸解离常数。由于其中混合的这种独特的成分，本发明的组合物可以得到即使在升高的温度下也对汽车中使用的油具有优异的高抗性的硫化橡胶。

18. 发明授权

US5357023A Organopolysiloxanes having silethylene linkages and a curable composition comprising the same 失效
标题翻译：具有亚乙烯基键的有机聚硅氧烷和包含它们的可固化组合物
公开(公告)号：US5357023A
公开(公告)日：1994-10-18
申请号：US83387
申请日：1993-06-29
申请人： Yoshio Inoue , Masatoshi Arai , Kazutoshi Fujioka , Tsuneo Kimura
发明人： Yoshio Inoue , Masatoshi Arai , Kazutoshi Fujioka , Tsuneo Kimura
IPC分类号： C08G77/50 , C08L83/14 , C08G77/20
CPC分类号： C08L83/14 , C08G77/50
摘要： A novel organopolysiloxane compound having, in a molecule, at least one silyl-substituted ethyl group of the general formula ##STR1## in which R.sup.1 is a hydrogen atom or a methyl group, R is a monovalent hydrocarbon group and the subscripts a is 2 or and b is 1, 2 or 3, or a linear organopolysiloxane having, at each molecular chain end, at least one of such a group, can be prepared by first reacting a vinyl-containing organopolysiloxane with a hydrogen chlorosilane compound to effect the hydrosilation reaction between the silicon-bonded vinyl groups and the silicon-bonded hydrogen atoms and then the silicon-bonded chlorine atoms are subjected to a dehydrochlorination reaction with a silanol compound of the general formula ##STR2## A composition comprising the organopolysiloxane and a photopolymerization initiator is highly sensitive to light and readily cured into a rubbery elastomer by irradiation with ultraviolet light.
摘要翻译：一种新的有机聚硅氧烷化合物，其在分子中具有至少一个通式为“IMAGE”的甲硅烷基取代的乙基，其中R 1为氢原子或甲基，R为单价烃基，下标a为2或并且b为1,2或3，或者在各分子链末端具有这种基团中的至少一个的线性有机聚硅氧烷可以通过首先使含乙烯基的有机聚硅氧烷与氢氯硅烷化合物反应来进行氢化硅烷化反应硅键合的乙烯基和与硅键合的氢原子之间，然后与硅键合的氯原子与通式为的硅烷醇化合物进行脱氯化氢反应。包含有机聚硅氧烷和光聚合引发剂的组合物是高度的对光敏感，并通过紫外线照射容易地固化成橡胶状弹性体。

19. 发明授权

US5244938A Room temperature curable organopolysiloxane composition 失效
标题翻译：室温可固化有机硅氧烷组合物
公开(公告)号：US5244938A
公开(公告)日：1993-09-14
申请号：US806342
申请日：1991-12-13
申请人： Masatoshi Arai , Yoshifumi Inoue , Yoshio Inoue
发明人： Masatoshi Arai , Yoshifumi Inoue , Yoshio Inoue
IPC分类号： C08K3/00 , C08K5/5419 , C08K5/57 , C08L83/04 , C08L83/06 , C08L83/08
CPC分类号： C08K5/5419 , C08L83/04 , C08L83/08 , C08G77/16 , C08G77/18 , C08G77/24 , Y10S528/901
摘要： The present invention is characterized by adding and mixing an organosilicon compound having alkoxy, groups and an ester linkage in the molecule represented by the following formula: ##STR1## in an amount of 1 to 20 parts by weight per 100 parts by weight of a trifluoropropylalkylpolysiloxane. Said organosilicon compound has a function as a storage stabilizer as well as a curing agent and, according to the present invention, an RTV fluorosilicone composition that has hitherto been difficult to be applied as an adhesive for electric and electronic parts has been made possible to be used in the particular field.

20. 发明授权

US4721766A Room temperature-curable organopolysiloxane composition 失效
标题翻译：室温可固化的有机聚硅氧烷组合物
公开(公告)号：US4721766A
公开(公告)日：1988-01-26
申请号：US894857
申请日：1986-08-08
申请人： Yoshio Inoue , Masatoshi Arai , Koji Yokoo
发明人： Yoshio Inoue , Masatoshi Arai , Koji Yokoo
IPC分类号： C08L83/00 , C08K5/5419 , C08K5/5425 , C08K5/5465 , C08L1/00 , C08L23/00 , C08L27/00 , C08L83/04 , C08L83/06 , C08L101/00 , C08G77/06
CPC分类号： C08K5/5465 , C08L83/04 , C08G77/16 , C08G77/18 , Y10S528/901
摘要： The room temperature-curable organopolysiloxane composition of the invention is imparted with greatly improved stability in prolonged storage without being affected in respect of the curability. The composition is formulated, in addition to the base ingredients of a silanol- or alkoxy-terminated diorganopolysiloxane and a filler, with an alkenyloxy-containing silane compound in an amount of at least equimolar to the silanol groups and water in the base ingredients and a guanidino-containing organosilane compound in a limited amount.
摘要翻译：本发明的室温可固化的有机基聚硅氧烷组合物在长期保存中赋予了极大的改进的稳定性，而不会影响固化性。除了硅烷醇或烷氧基封端的二有机聚硅氧烷和填料的基础成分之外，配合含有至少等摩尔量的含烯氧基的硅烷化合物与基础成分中的硅烷醇基和水，以及含胍基的有机硅烷化合物。

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