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11. 发明申请

US20090253876A1 Fluorene Derivative, Transition Metal Compound, Catalyst for Olefin Polymerization, and Process for Producing Olefin Polymer 有权
标题翻译：芴衍生物，过渡金属化合物，用于烯烃聚合的催化剂，以及生产烯烃聚合物的方法
公开(公告)号：US20090253876A1
公开(公告)日：2009-10-08
申请号：US11920767
申请日：2006-05-24
申请人： Munehito Funaya , Koji Endo , Naritoshi Hirota , Yuichi Yamamura , Koji Kawai
发明人： Munehito Funaya , Koji Endo , Naritoshi Hirota , Yuichi Yamamura , Koji Kawai
IPC分类号： C08F2/00 , C07F7/02 , B01J31/12 , C08F4/42 , C07F7/00 , C07C25/24
CPC分类号： C07C13/567 , C07F7/081 , C07F17/00 , C08F4/65912 , C08F4/65916 , C08F10/00 , C08F110/02 , C08F110/06 , C08F210/16 , C08F4/65927 , C08F2500/17 , C08F2500/03 , C08F2500/15 , C08F210/06 , C08F210/14
摘要： Provided is a novel fluorene derivative which is useful as a catalyst component for olefin polymerization, a transition metal compound containing the fluorene derivative as a part of ligand, a catalyst for olefin polymerization containing the transition metal compound, and a process for producing olefin polymer. The fluorene derivative is characterized by being represented by the following general formula [I]: wherein R1, R2, R3, R5, R6, R7, R8, R9, R10, R11, R12, and R14 are each selected from hydrogen, a hydrocarbon group, and a silicon-containing group, and may be the same as or different from each other, R4 and R13 are each selected from hydrogen, a hydrocarbon group, a silicon-containing group, a sulfur-containing group, an oxygen-containing group, a nitrogen-containing group, and a halogen-containing group, and may be the same as or different from each other, and adjacent substituents of R1 to R14 may be bonded to each other to form a ring, except that the case where R4 and R5, and R12 and R13 are each bonded to each other to form a vinylene group. Also provided is a bridged metallocene compound having both of the skeleton and a cyclopentadiene skeleton.
摘要翻译：提供了可用作烯烃聚合的催化剂组分的新型芴衍生物，含有芴衍生物作为配体的一部分的过渡金属化合物，含有过渡金属化合物的烯烃聚合用催化剂和烯烃聚合物的制造方法。芴衍生物的特征在于由以下通式[I]表示：其中R1，R2，R3，R5，R6，R7，R8，R9，R10，R11，R12和R14各自选自氢，烃基团和含硅基团，并且可以彼此相同或不同，R4和R13各自选自氢，烃基，含硅基团，含硫基团，含氧基团基团，含氮基团和含卤素基团，可以相同或不同，R1〜R14的相邻取代基可以相互键合形成环，除了以下情况 R4和R5以及R12和R13各自彼此键合形成亚乙烯基。还提供了具有骨架和环戊二烯骨架两者的桥连金属茂化合物。

12. 发明申请

US20090043057A1 Transition Metal Compound, Catalyst for Olefin Polymerization, and Process for Producing Olefin Polymer 审中-公开
标题翻译：过渡金属化合物，用于烯烃聚合的催化剂，以及生产烯烃聚合物的方法
公开(公告)号：US20090043057A1
公开(公告)日：2009-02-12
申请号：US11920779
申请日：2006-05-24
申请人： Munehito Funaya , Naritoshi Hirota , Yuichi Yamamura , Koji Kawai
发明人： Munehito Funaya , Naritoshi Hirota , Yuichi Yamamura , Koji Kawai
IPC分类号： C08F4/78 , C07F7/08 , C07F11/00 , C08F2/00 , B01J31/12
CPC分类号： C07F17/00 , C08F4/65912 , C08F4/65916 , C08F10/00 , C08F110/06 , C08F210/16 , C08F2500/15 , C08F2500/03 , C08F210/06 , C08F2500/17 , C08F4/65927
摘要： Provided is a transition metal compound novel and useful as a catalyst component for olefin polymerization, a catalyst for olefin polymerization containing the transition metal compound, and a process for producing an olefin polymer using the catalyst for polymerization. The transition metal is characterized by being represented by the following general formula [I]: wherein, R3 is hydrogen, R2 is selected from a hydrocarbon group or a silicon-containing group, R1 and R4 are selected from a hydrocarbon group having 2 to 20 carbon atoms and a silicon-containing group, each of R5, R6, R7, R8, R9, R10, R11, R12, R13 and R14, which is selected from hydrogen, a hydrocarbon group and a silicon-containing group, may be same or different from each other, and adjacent groups from R5 to R14 may be bonded to each other to form a ring. M is a Group 4 transition metal, Y is a carbon atom, Q may be selected from halogen, a hydrocarbon group, an anionic ligand and a neutral ligand capable of coordinating with a lone electron pair, which may be selected in the same combination or different combination, and j is an integer of 1 to 4.
摘要翻译：提供了一种新颖可用作烯烃聚合催化剂组分的过渡金属化合物，含有过渡金属化合物的烯烃聚合催化剂，以及使用聚合催化剂生产烯烃聚合物的方法。过渡金属的特征在于由以下通式[I]表示：其中，R3是氢，R2选自烃基或含硅基团，R1和R4选自具有2〜20个碳原子的烃基碳原子和含硅基团，选自氢，烃基和含硅基团的R5，R6，R7，R8，R9，R10，R11，R12，R13和R14各自可以相同或彼此不同，并且R 5至R 14的相邻基团可以彼此键合形成环。 M是第4族过渡金属，Y是碳原子，Q可以选自卤素，烃基，阴离子配体和能够与单个电子对配位的中性配体，其可以以相同的组合或不同的组合，j为1〜4的整数。

13. 发明授权

US07834204B2 Fluorene derivative, transition metal compound, catalyst for olefin polymerization, and process for producing olefin polymer 有权
标题翻译：芴衍生物，过渡金属化合物，烯烃聚合用催化剂和烯烃聚合物的制造方法
公开(公告)号：US07834204B2
公开(公告)日：2010-11-16
申请号：US11920767
申请日：2006-05-24
申请人： Munehito Funaya , Koji Endo , Naritoshi Hirota , Yuichi Yamamura , Koji Kawai
发明人： Munehito Funaya , Koji Endo , Naritoshi Hirota , Yuichi Yamamura , Koji Kawai
IPC分类号： C07F17/00 , B01J31/22 , C08F4/6592
CPC分类号： C07C13/567 , C07F7/081 , C07F17/00 , C08F4/65912 , C08F4/65916 , C08F10/00 , C08F110/02 , C08F110/06 , C08F210/16 , C08F4/65927 , C08F2500/17 , C08F2500/03 , C08F2500/15 , C08F210/06 , C08F210/14
摘要： Provided is a transition metal compound represented by the general formula [III]: wherein R23, R24, R25, R26, R27, and R28 are each independently selected from hydrogen, a hydrocarbon group, a silicon-containing group, a sulfur-containing group, an oxygen-containing group, a nitrogen-containing group, and a halogen-containing group, adjacent substituents of R23 to R28 are optionally bonded to each other to form a ring, M is a Group 4 transition metal, Y is carbon atom, Q is selected from halogen, a hydrocarbon group, an anionic ligand and a neutral ligand capable of coordinating with a lone electron pair, which is selected in the same combination or different combination, j is an integer of 1 to 4, and Z is a fluorenylidene group comprising a fluorene derivative formula [I] or formula [II]
摘要翻译：提供由通式[III]表示的过渡金属化合物：其中R 23，R 24，R 25，R 26，R 27和R 28各自独立地选自氢，烃基，含硅基团，含硫基团，含氧基团，含氮基团和含卤素基团，R 23〜R 28的相邻取代基可以相互键合形成环，M为4族过渡金属，Y为碳原子， Q选自卤素，烃基，阴离子配体和能够与单电子对配位的中性配体，其以相同的组合或不同的组合选择，j为1〜4的整数，Z为包含芴衍生物式[I]或式[II]的亚芴基

14. 发明申请

US20100190941A1 TRANSITION METAL COMPOUND, CATALYST FOR OLEFIN POLYMERIZATION, AND PROCESS FOR PRODUCING OLEFIN POLYMER 审中-公开
标题翻译：过渡金属化合物，烯烃聚合催化剂和生产烯烃聚合物的方法
公开(公告)号：US20100190941A1
公开(公告)日：2010-07-29
申请号：US12753647
申请日：2010-04-02
申请人： Munehito Funaya , Naritoshi Hirota , Yuichi Yamamura , Koji Kawai
发明人： Munehito Funaya , Naritoshi Hirota , Yuichi Yamamura , Koji Kawai
IPC分类号： C08F2/00
CPC分类号： C07F17/00 , C08F4/65912 , C08F4/65916 , C08F10/00 , C08F110/06 , C08F210/16 , C08F2500/15 , C08F2500/03 , C08F210/06 , C08F2500/17 , C08F4/65927
摘要： Provided is a transition metal compound novel and useful as a catalyst component for olefin polymerization, a catalyst for olefin polymerization containing the transition metal compound, and a process for producing an olefin polymer using the catalyst for polymerization. The transition metal is characterized by being represented by the following general formula [I]: wherein, R3 is hydrogen, R2 is selected from a hydrocarbon group or a silicon-containing group, R1 and R4 are selected from a hydrocarbon group having 2 to 20 carbon atoms and a silicon-containing group, each of R5, R6, R7, R8, R9, R10, R11, R12, R13 and R14, which is selected from hydrogen, a hydrocarbon group and a silicon-containing group, may be same or different from each other, and adjacent groups from R5 to R14 may be bonded to each other to form a ring. M is a Group 4 transition metal, Y is a carbon atom, Q may be selected from halogen, a hydrocarbon group, an anionic ligand and a neutral ligand capable of coordinating with a lone electron pair, which may be selected in the same combination or different combination, and j is an integer of 1 to 4.
摘要翻译：提供了一种新颖可用作烯烃聚合催化剂组分的过渡金属化合物，含有过渡金属化合物的烯烃聚合催化剂，以及使用聚合催化剂生产烯烃聚合物的方法。过渡金属的特征在于由以下通式[I]表示：其中，R3是氢，R2选自烃基或含硅基团，R1和R4选自具有2〜20个碳原子的烃基碳原子和含硅基团，选自氢，烃基和含硅基团的R5，R6，R7，R8，R9，R10，R11，R12，R13和R14各自可以相同或彼此不同，并且R 5至R 14的相邻基团可以彼此键合形成环。 M是第4族过渡金属，Y是碳原子，Q可以选自卤素，烃基，阴离子配体和能够与单个电子对配位的中性配体，其可以以相同的组合或不同的组合，j为1〜4的整数。

15. 发明申请

US20080097055A1 Process for Producing Propylene Polymer 有权
标题翻译：生产丙烯聚合物的方法
公开(公告)号：US20080097055A1
公开(公告)日：2008-04-24
申请号：US11661504
申请日：2005-08-29
申请人： Munehito Funaya , Naritoshi Hirota , Mayumi Hiwara , Yasushi Tohi , Koji Kawai , Ryoji Mori , Masahiko Okamoto , Shigenobu Ikenaga , Hiromasa Marubayashi
发明人： Munehito Funaya , Naritoshi Hirota , Mayumi Hiwara , Yasushi Tohi , Koji Kawai , Ryoji Mori , Masahiko Okamoto , Shigenobu Ikenaga , Hiromasa Marubayashi
IPC分类号： C08F4/52 , C08F10/06
CPC分类号： C08F10/00 , C08F4/65912 , C08F4/65916 , C08F10/06 , C08F110/06 , C08F210/06 , Y10S526/943 , C08F4/65927 , C08F2/02 , C08F2500/17 , C08F2500/03 , C08F210/16 , C08F210/08
摘要： A high molecular weight propylene polymer exhibiting high stereoregularity (isotactic) and high position selectivity can be effectively produced by polymerizing at least one monomer selected from propylene, α-olefins and polyenes in the presence of a catalyst for olefin polymerization comprising: (A) a bridged metallocene compound represented by the General Formula [I] given in claims (diphenylmethylene(3-tert-butyl-5-ethyl-cyclopentadienyl)(fluorenyl)zirconium dichloride, etc.); and (B) one or more compound(s) selected from (b-1) an organoaluminumoxy compound (b-2) a compound which reacts with the bridged metallocene compound (A) to form an ion pair, and (b-3) an organoaluminum compound.
摘要翻译：通过在用于烯烃聚合的催化剂的存在下聚合至少一种选自丙烯，α-烯烃和多烯的单体，可以有效地制备显示出高立构规整性（全同立构）和高位置选择性的高分子量丙烯聚合物，其包括：（A）由权利要求中给出的通式[I]表示的桥连金属茂化合物（二苯基亚甲基（3-叔丁基-5-乙基 - 环戊二烯基）（芴基）二氯化锆等）; 和（B）选自（b-1）有机铝氧化合物（b-2）的一种或多种化合物与桥连金属茂化合物（A）反应形成离子对的化合物，和（b-3）有机铝化合物。

16. 发明申请

US20080038498A1 Propylene Polymer, Composition Comprising the Polymer, and Molded Product Obtained Therefrom 审中-公开
标题翻译：丙烯聚合物，包含聚合物的组合物和从其获得的成型产品
公开(公告)号：US20080038498A1
公开(公告)日：2008-02-14
申请号：US11793719
申请日：2005-12-22
申请人： Keita Itakura , Munehito Funaya , Ayako Kadosaka , Naritoshi Hirota , Hiroshi Nishikawa , Yuichi Yamamura , Shuji Matsumura , Satoshi Hashizume , Yoshio Sasaki
发明人： Keita Itakura , Munehito Funaya , Ayako Kadosaka , Naritoshi Hirota , Hiroshi Nishikawa , Yuichi Yamamura , Shuji Matsumura , Satoshi Hashizume , Yoshio Sasaki
IPC分类号： C08L23/12
CPC分类号： C08F10/00 , C08F4/65912 , C08F4/65916 , C08F210/06 , C08F210/16 , C08F255/00 , C08F255/02 , C08F297/08 , C08F297/083 , C08L23/083 , C08L23/10 , C08L23/142 , C08L23/16 , C08L51/06 , C08L53/00 , C08L2314/06 , Y10T428/1352 , C08F4/6492 , C08F4/65927 , C08L2666/24 , C08L2666/06 , C08L2666/08 , C08L2666/02 , C08F2500/03 , C08F2500/12 , C08F2500/17 , C08F2500/18
摘要： A propylene polymer which is constituted of 10 to 40 wt % room-temperature n-decane soluble part (Dsol) and 60 to 90 wt % room-temperature n-decane insoluble part (Dinsol), comprises skeletons derived from propylene (MP) and at least one kind of olefin (MX) selected from ethylene and C4 or more α-olefins, and satisfies all of the following requirements [1] to [5]. The polymer is characterized by having a high melting point and a high molecular weight and is suitable for use in producing various moldings therefrom. [1] the molecular weight distribution (Mw/Mn) of both Dsol and Dinsol as determined by GPC is 4.0 or less; [2] the melting point (Tm) of Dinsol is 156° C. or more; [3] the sum of the 2,1-bond content and the 1,3-bond content in Dinsol is 0.05 mol % or less; [4] the intrinsic viscosity [η] (dl/g) of Dsol satisfies the relationship 2.2
摘要翻译：丙烯聚合物由10〜40重量％的室温正癸烷可溶部分（D> sol）和60〜90重量％的室温正癸烷不溶部分（D＆lt; 包括衍生自丙烯（MP）的骨架和选自乙烯和C 4或更多α-烯烃的至少一种烯烃（MX），并且满足以下所有要求[1]至[5] 。聚合物的特征在于具有高熔点和高分子量，并且适用于从其生产各种模制品。 [1]通过GPC测定的D＆amp; S＆gt;和D＆amp; S＆gt;两者的分子量分布（Mw / Mn）为4.0以下; [2] D 的熔点（Tm）为156℃以上; [3] D insol中的2,1-键含量和1,3-键含量的总和为0.05摩尔％以下; [4] D 的特性粘度η（dl / g）满足关系式2.2 <η<6.0; 和[5]衍生自D insol中的烯烃（MX）的骨架的浓度为3.0重量％以下。

17. 发明申请

US20090317615A1 PACKAGING PROPYLENE RESIN COMPOSITION 审中-公开
标题翻译：包装丙烯树脂组合物
公开(公告)号：US20090317615A1
公开(公告)日：2009-12-24
申请号：US12310065
申请日：2007-08-06
申请人： Keita Itakura , Tokutaro Kimura , Mitsuo Kawata , Satoshi Hashizume , Masashi Higuchi , Munehito Funaya
发明人： Keita Itakura , Tokutaro Kimura , Mitsuo Kawata , Satoshi Hashizume , Masashi Higuchi , Munehito Funaya
IPC分类号： B32B27/32 , C08L23/04
CPC分类号： C08F10/00 , C08F4/65912 , C08F4/65916 , C08F4/65925 , C08F4/65927 , C08F110/06 , C08F210/06 , C08F297/08 , C08J5/18 , C08J2323/10 , C08L23/10 , C08L23/12 , C08L23/142 , C08L53/00 , C08L2205/02 , C08L2314/06 , C08F4/6492 , C08F4/6494 , C08L2666/06 , C08L2666/02 , C08F2500/12 , C08F210/16 , C08F2500/17 , C08F2500/03
摘要： Packaging propylene resin compositions are excellent in balance in high transparency, rigidity, low-temperature impact resistance and blocking resistance. Retort films, protective films, medical container packaging films and freshness-keeping films, and sheets for similar purposes are obtained from the compositions. A packaging propylene resin composition includes a propylene polymer (A) satisfying specific requirements and a propylene/ethylene copolymer (B) satisfying specific requirements. In another packaging propylene resin composition, Dinsol and Dsol satisfy specific requirements.
摘要翻译：包装丙烯树脂组合物在高透明度，刚性，耐低温冲击性和耐粘连性方面的平衡优异。从组合物中获得蒸煮膜，保护膜，医疗容器包装膜和保鲜膜，以及类似目的的片材。包装丙烯树脂组合物包括满足特定要求的丙烯聚合物（A）和满足特定要求的丙烯/乙烯共聚物（B）。在另一种包装丙烯树脂组合物中，Dinsol和Dsol满足特定要求。

18. 发明申请

US20090069523A1 Propylene Random Block Copolymer, Resin Composition Containing the Copolymer and Molded Article Made Thereof 审中-公开
标题翻译：丙烯无规嵌段共聚物，含有共聚物的树脂组合物及其制成的模制品
公开(公告)号：US20090069523A1
公开(公告)日：2009-03-12
申请号：US12225689
申请日：2007-03-27
申请人： Keita Itakura , Satoshi Hashizume , Kunihiko Takesue , Munehito Funaya
发明人： Keita Itakura , Satoshi Hashizume , Kunihiko Takesue , Munehito Funaya
IPC分类号： C08F210/00
CPC分类号： C08F297/083 , C08L23/142 , C08L2207/02 , C08L23/16
摘要： The invention provides a propylene random block copolymer (A) that has a melt flow rate from 0.1 to 100 g/10 min and a melting point from 100 to 155° C. and includes 90 to 60% by weight of a portion insoluble (Dinsol) in n-decane at room temperature and 10 to 40% by weight of a portion soluble (Dsol) in n-decane at room temperature, wherein the Dinsol satisfies the following requirements (1) through (3) and the Dsol satisfies the following requirements (4) through (6). The invention further provides molded articles such as sheets, films, injection molded articles, hollow molded articles, injection blow molded articles and fibers, which are formed of the propylene random block copolymer (A) or a propylene resin composition containing the propylene random block copolymer (A). (1) The molecular weight distribution (Mw/Mn) obtained by GPC of the Dinsol is from 1.0 to 3.5, (2) the content of skeletons derived from ethylene in the Dinsol is from 0.5 to 13% by mole, (3) the total amount of 2,1- and 1,3-propylene units in the Dinsol is 0.2% by mole or less, (4) the molecular weight distribution (Mw/Mn) obtained by GPC of the Dsol is from 1.0 to 3.5, (5) the intrinsic viscosity [η] in decalin at 135° C. of the Dsol is from 1.5 to 4 dl/g and (6) the content of skeletons derived from ethylene in the Dsol is from 15 to 35% by mole.
摘要翻译：本发明提供一种丙烯无规嵌段共聚物（A），其熔体流动速率为0.1-100g / 10min，熔点为100-155℃，包括90-60wt％的不溶物（Dinsol ）和室温下正癸烷中可溶解部分（Dsol）的10〜40重量％，其中，D insol为（1）〜（3），Dsol满足下述式要求（4）至（6）。本发明还提供了由丙烯无规嵌段共聚物（A）形成的成型制品，例如片材，薄膜，注塑制品，中空成型制品，注塑吹塑制品和纤维，或含丙烯无规嵌段共聚物（一个）。（1）由Dinsol得到的分子量分布（Mw / Mn）为1.0〜3.5，（2）由Dinsol得到的乙烯的骨架含量为0.5〜13摩尔％，（3） D insol中的2,1-和1,3-丙烯单元的总量为0.2摩尔％以下，（4）通过Dsol的GPC得到的分子量分布（Mw / Mn）为1.0〜3.5（ 5）Dsol的135℃萘烷中的特性粘度η为1.5〜4dl / g，（6）Dsol中衍生自乙烯的骨架含量为15〜35摩尔％。

19. 发明申请

US20070149822A1 Thiourethane-based optical material 有权
公开(公告)号：US20070149822A1
公开(公告)日：2007-06-28
申请号：US11707919
申请日：2007-02-20
申请人： Mamoru Tanaka , Shigetoshi Kuma , Munehito Funaya , Seiichi Kobayashi
发明人： Mamoru Tanaka , Shigetoshi Kuma , Munehito Funaya , Seiichi Kobayashi
IPC分类号： C07C321/12
CPC分类号： C08G18/7642 , C08G18/3876 , G02B1/04 , C08L75/04 , C08L81/00
摘要： A composition for making a high-refractive-index resin contains a polythiol compound and a compound containing at least two iso(thio)cyanato groups, the polythiol compound having a dithioacetal, dithioketal, orthotrithioformic ester, or orthotetrathiocarbonic ester skeleton. The molar ratio of the mercapto group to the iso(thio)cyanato group in the composition is greater than 1.0 but not more than 3.0. A method for making a resin by curing the composition, a resin prepared by curing the composition, an optical element made from the resin, and a lens made from the optical element are also provided.

20. 发明申请

US20050131203A1 Thiourethane-based optical material 有权
标题翻译：硫代氨基甲酸酯类光学材料
公开(公告)号：US20050131203A1
公开(公告)日：2005-06-16
申请号：US10509765
申请日：2003-12-12
申请人： Mamoru Tanaka , Shigetoshi Kuma , Munehito Funaya , Seiichi Kobayashi
发明人： Mamoru Tanaka , Shigetoshi Kuma , Munehito Funaya , Seiichi Kobayashi
IPC分类号： C08G18/38 , C08G18/76 , G02B1/04 , C08G75/00
CPC分类号： C08G18/7642 , C08G18/3876 , G02B1/04 , C08L75/04 , C08L81/00
摘要： A composition for making a high-refractive-index resin contains a polythiol compound and a compound containing at least two iso(thio)cyanato groups, the polythiol compound having a dithioacetal, dithioketal, orthotrithioformic ester, or orthotetrathiocarbonic ester skeleton. The molar ratio of the mercapto group to the iso(thio)cyanato group in the composition is greater than 1.0 but not more than 3.0. A method for making a resin by curing the composition, a resin prepared by curing the composition, an optical element made from the resin, and a lens made from the optical element are also provided.
摘要翻译：用于制备高折射率树脂的组合物含有多硫醇化合物和含有至少两个异（硫）氰酸基的化合物，多硫醇化合物具有二硫缩醛，二硫缩酮，邻二硫代甲酸酯或邻四硫代碳酸酯骨架。组合物中巯基与异（硫）氰酸基的摩尔比大于1.0但不大于3.0。通过固化组合物制备树脂的方法，通过固化组合物制备的树脂，由树脂制成的光学元件和由光学元件制成的透镜也被提供。

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